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Marco Polini

Publications and source records attributed to Marco Polini.

At least 91 records · Page 5Linked to original sources

Adiabatic perturbation theory of nonequilibrium light-controlled superconductivity

Recent experiments, in which Terahertz (THz) light has been used to induce nonequilibrium superconducting states, have raised a number of intriguing fundamental questions. Theoretically, these experiments are most often described within the Floquet formalism, which suffers a number of well-known limitations (e.g. Floquet heating). Alternative approaches rely on heavy numerical methods. In this Article we develop an analytical theory of nonequilibrium superconductivity that combines path integrals on the Kostantinov-Perel' time contour with adiabatic perturbation theory [G. Rigolin, G. Ortiz, and V.H. Ponce, Phys. Rev. A~{\bf 78}, 052508 (2008)]. We consider a general system of electrons and Raman phonons coupled by the Fröhlich interaction, in the presence of a time-dependent external field which acts on the phonon subsystem. The latter is supposed to model the THz light-induced excitation of nonlinear interactions between infrared and Raman phonons. Assuming that the external field has a slow dependence on time, we derive equations for the dynamical superconducting gap, calculating the leading adiabatic term and the first non-adiabatic correction. Our nonequilibrium formulas can be solved numerically with a minimal increase of computational complexity with respect to that needed to calculate the superconducting gap at equilibrium.

cond-mat.supr-con↗

Piezoelectricity and valley Chern number in inhomogeneous hexagonal 2D crystals

Conversion of mechanical forces to electric signal is possible in non-centrosymmetric materials due to linear piezoelectricity. The extraordinary mechanical properties of two-dimensional materials and their high crystallinity make them exceptional platforms to study and exploit the piezoelectric effect. Here, the piezoelectric response of non-centrosymmetric hexagonal two-dimensional crystals is studied using the modern theory of polarization and ${\bm k} \cdot {\bm p}$ model Hamiltonians. An analytical expression for the piezoelectric constant is obtained in terms of topological quantities such as the {\it valley Chern number}. The theory is applied to semiconducting transition metal dichalcogenides and hexagonal Boron Nitride. We find good agreement with available experimental measurements for MoS$_2$. We further generalise the theory to study the polarization of samples subjected to inhomogeneous strain (e.g.~nanobubbles). We obtain a simple expression in terms of the strain tensor, and show that charge densities $\gtrsim 10^{11} {\rm cm}^{-2}$ can be induced by realistic inhomogeneous strains, $ε\approx 0.01 - 0.03$.

cond-mat.mtrl-sci↗

Plasmons in realistic graphene/hexagonal boron nitride moiré patterns

Van der Waals heterostructures employing graphene and hexagonal boron nitride (hBN) crystals have emerged as a promising platform for plasmonics thanks to the tunability of their collective modes with carrier density and record values for plasmonics figures of merit. In this Article we investigate theoretically the role of moiré-pattern superlattices in nearly aligned graphene on hBN by using continuum-model Hamiltonians derived from ab initio calculations. We calculate the system's energy loss function for a variety of chemical potential values that are accessible in gated devices. Our calculations reveal that the electron-hole asymmetry of the moiré bands leads to a remarkable asymmetry of the plasmon dispersion between positive and negative chemical potentials, showcasing the intricate band structure and rich absorption spectrum across the secondary Dirac point gap for the hole bands.

cond-mat.mes-hall↗

Nonlinear anomalous photocurrents in Weyl semimetals

We study the second-order nonlinear optical response of a Weyl semimetal (WSM), i.e. a three-dimensional metal with linear band touchings acting as point-like sources of Berry curvature in momentum space, termed "Weyl-Berry monopoles". We first show that the anomalous second-order photocurrent of WSMs can be elegantly parametrized in terms of Weyl-Berry dipole and quadrupole moments. We then calculate the corresponding charge and node conductivities of WSMs with either broken time-reversal invariance or inversion symmetry. In particular, we predict a universal dissipationless second-order anomalous node conductivity for WSMs belonging to the TaAs family.

cond-mat.mtrl-sci↗

Gate-tunable spatial modulation of localized plasmon resonances

Nanoplasmonics exploits the coupling between light and collective electron density oscillations (plasmons) to bypass the stringent limits imposed by diffraction. This coupling enables confinement of light to sub-wavelength volumes and is usually exploited in nanostructured metals. Substantial efforts are being made at the current frontier of the field to employ electron systems in semiconducting and semimetallic materials since these add the exciting possibility of realizing electrically tunable and/or active nanoplasmonic devices. Here we demonstrate that a suitable design of the doping profile in a semiconductor nanowire (NW) can be used to tailor the plasmonic response and induce localization effects akin to those observed in metal nanoparticles. Moreover, by field-effect carrier modulation, we demonstrate that these localized plasmon resonances can be spatially displaced along the nanostructure body, thereby paving the way for the implementation of spatially tunable plasmonic circuits.

cond-mat.mes-hall↗

High-yield production of 2D crystals by wet-jet milling

Efficient and scalable production of two-dimensional (2D) materials is required to overcome technological hurdles towards the creation of a 2D-materials-based industry. Here, we present a novel approach developed for the exfoliation of layered crystals, i.e., graphite, hexagonal boron nitride and transition metal dichalcogenides. The process is based on high-pressure wet-jet-milling (WJM), resulting in 2 L/hr production of 10 g/L of single- and few-layer 2D crystal flakes in dispersion making the scaling-up more affordable. The WJM process enables the production of defect-free and high-quality 2D-crystal dispersions on a large scale, opening the way for the full exploitation in different commercial applications, e.g., anodes active material in lithium ion batteries, reinforcement in polymer-graphene composites, and transparent conductors as we demonstrate in this report.

cond-mat.mtrl-sci↗

Multiband Plasmonic Sierpinski Carpet Fractal Antennas

Deterministic fractal antennas are employed to realize multimodal plasmonic devices. Such structures show strongly enhanced localized electromagnetic fields typically in the infrared range with a hierarchical spatial distribution. Realization of engineered fractal antennas operating in the optical regime would enable nanoplasmonic platforms for applications, such as energy harvesting, light sensing, and bio/chemical detection. Here, we introduce a novel plasmonic multiband metamaterial based on the Sierpinski carpet (SC) space-filling fractal, having a tunable and polarization-independent optical response, which exhibits multiple resonances from the visible to mid-infrared range. We investigate gold SCs fabricated by electron-beam lithography on CaF$_{2}$ and Si/SiO$_{2}$ substrates. Furthermore, we demonstrate that such resonances originate from diffraction-mediated localized surface plasmons, which can be tailored in deterministic fashion by tuning the shape, size, and position of the fractal elements. Moreover, our findings illustrate that SCs with high order of complexity present a strong and hierarchically distributed electromagnetic near-field of the plasmonic modes. Therefore, engineered plasmonic SCs provide an efficient strategy for the realization of compact active devices with a strong and broadband spectral response in the visible/mid-infrared range. We take advantage of such a technology by carrying out surface enhanced Raman spectroscopy (SERS) on Brilliant Cresyl Blue molecules deposited onto plasmonic SCs. We achieve a broadband SERS enhancement factor up to $10^{4}$, thereby providing a proof-of-concept application for chemical diagnostics.

physics.optics↗

Quantum non-local theory of topological Fermi arc plasmons in Weyl semimetals

The surface of a Weyl semimetal (WSM) displays Fermi arcs, i.e. disjoint segments of a two-dimensional Fermi contour. We present a quantum-mechanical non-local theory of chiral Fermi arc plasmons in WSMs with broken time-reversal symmetry. These are collective excitations constructed from topological Fermi arc and bulk electron states and arising from electron-electron interactions, which are treated in the realm of the random phase approximation. Our theory includes quantum effects associated with the penetration of the Fermi arc surface states into the bulk and dissipation, which is intrinsically non-local in nature and arises from decay processes mainly involving bulk electron-hole pair excitations.

cond-mat.mes-hall↗

Spin-vorticity coupling in viscous electron fluids

We consider spin-vorticity coupling - the generation of spin polarization by vorticity - in viscous two-dimensional electron systems with spin-orbit coupling. We first derive hydrodynamic equations for spin and momentum densities in which their mutual coupling is determined by the rotational viscosity. We then calculate the rotational viscosity microscopically in the limits of weak and strong spin-orbit coupling. We provide estimates that show that the spin-orbit coupling achieved in recent experiments is strong enough for the spin-vorticity coupling to be observed. On the one hand, this coupling provides a way to image viscous electron flows by imaging spin densities. On the other hand, we show that the spin polarization generated by spin-vorticity coupling in the hydrodynamic regime can, in principle, be much larger than that generated, e.g. by the spin Hall effect, in the diffusive regime.

cond-mat.mes-hall↗

Nonlocal superconducting correlations in graphene in the quantum Hall regime

We study Andreev processes and nonlocal transport in a three-terminal graphene-superconductor hybrid system under a quantizing perpendicular magnetic field [G.-H. Lee et al., Nature Phys. 13, 693 (2017)]. We find that the amplitude of the crossed Andreev reflection (CAR) processes crucially depends on the orientation of the lattice. By employing Landauer-Büttiker scattering theory, we find that CAR is generally very small for a zigzag edge, while for an armchair edge it can be larger than the normal transmission, thereby resulting in a negative nonlocal resistance. In the case of an armchair edge and with a wide superconducting region (as compared to the superconducting coherence length), CAR exhibits large oscillations as a function of the magnetic field due to interference effects. This results in sign changes of the nonlocal resistance.

cond-mat.mes-hall↗

Confining graphene plasmons to the ultimate limit

Graphene plasmons have recently attracted a great deal of attention because of their tunability, long lifetime, and high degree of field confinement in the vertical direction. Nearby metal gates have been shown to modify the graphene plasmon dispersion and further confine their electric field. We study the plasmons of a graphene sheet deposited on a metal, in the regime in which metal bands do not hybridize with massless Dirac fermion bands. We derive exact results for the dispersion and lifetime of the plasmons of such hybrid system, taking into account metal nonlocalities. The graphene plasmon dispersion is found to be acoustic and pushed down in energy towards the upper boundary of the intraband graphene particle-hole continuum, thereby strongly enhancing the vertical confinement of these excitations. Landau damping of such acoustic plasmons due to particle-hole excitations in the metal gate is found to be surprisingly weak, with quality factors exceeding $Q = 10^{2}$.

cond-mat.mes-hall↗

Tuning the Drude weight of Dirac-Weyl fermions in one-dimensional ring traps

We study the response to an applied flux of an interacting system of Dirac-Weyl fermions confined in a one-dimensional (1D) ring. Combining analytical calculations with density-matrix renormalization group results, we show that tuning of interactions leads to a unique many-body system that displays either a suppression or an enhancement of the Drude weight - the zero-frequency peak in the ac conductivity - with respect to the non-interacting value. An asymmetry in the interaction strength between same- and different-pseudospin Dirac-Weyl fermions leads to Drude weight enhancement. Viceversa, symmetric interactions lead to Drude weight suppression. Our predictions can be tested in mixtures of ultracold fermions in 1D ring traps.

cond-mat.quant-gas↗

Optical conductivity of a quantum electron gas in a Sierpinski carpet

Recent advances in nanofabrication methods have made it possible to create complex two-dimensional artificial structures, such as fractals, where electrons can be confined. The optoelectronic and plasmonic properties of these exotic quantum electron systems are largely unexplored. In this article, we calculate the optical conductivity of a two-dimensional electron gas in a Sierpinski carpet (SC). The SC is a paradigmatic fractal that can be fabricated in a planar solid-state matrix by means of an iterative procedure. We show that the optical conductivity as a function of frequency (i.e. the optical spectrum) converges, at finite temperature, as a function of the fractal iteration. The calculated optical spectrum features sharp peaks at frequencies determined by the smallest geometric details at a given fractal iteration. Each peak is due to excitations within sets of electronic state-pairs, whose wave functions are characterized by quantum confinement in the SC at specific length scales, related to the frequency of the peak.

cond-mat.mes-hall↗

High-power collective charging of a solid-state quantum battery

Quantum information theorems state that it is possible to exploit collective quantum resources to greatly enhance the charging power of quantum batteries (QBs) made of many identical elementary units. We here present and solve a model of a QB that can be engineered in solid-state architectures. It consists of $N$ two-level systems coupled to a single photonic mode in a cavity. We contrast this collective model ("Dicke QB"), whereby entanglement is genuinely created by the common photonic mode, to the one in which each two-level system is coupled to its own separate cavity mode ("Rabi QB"). By employing exact diagonalization, we demonstrate the emergence of a quantum advantage in the charging power of Dicke QBs, which scales like $\sqrt{N}$ for $N\gg 1$.

cond-mat.mes-hall↗

Non-local transport and the Hall viscosity of 2D hydrodynamic electron liquids

In a fluid subject to a magnetic field the viscous stress tensor has a dissipationless antisymmetric component controlled by the so-called Hall viscosity. We here propose an all-electrical scheme that allows a determination of the Hall viscosity of a two-dimensional electron liquid in a solid-state device.

cond-mat.mes-hall↗

Lippmann-Schwinger theory for two-dimensional plasmon scattering

Long-lived and ultra-confined plasmons in two-dimensional (2D) electron systems may provide a sub-wavelength diagnostic tool to investigate localized dielectric, electromagnetic, and pseudo-electromagnetic perturbations. In this Article, we present a general theoretical framework to study the scattering of 2D plasmons against such perturbations in the non-retarded limit. We discuss both parabolic-band and massless Dirac fermion 2D electron systems. Our theory starts from a Lippmann-Schwinger equation for the screened potential in an inhomogeneous 2D electron system and utilizes as inputs analytical long-wavelength expressions for the density-density response function, going beyond the local approximation. We present illustrative results for the scattering of 2D plasmons against a point-like charged impurity and a one-dimensional electrostatic barrier due to a line of charges. Exact numerical results obtained from the solution of the Lippmann-Schwinger equation are compared with approximate results based on the Born and eikonal approximations. The importance of nonlocal effects is finally emphasized.

cond-mat.mes-hall↗

Electrical 2π phase control of infrared light in a 350nm footprint using graphene plasmons

Modulating the amplitude and phase of light is at the heart of many applications such as wavefront shaping, transformation optics, phased arrays, modulators and sensors. Performing this task with high efficiency and small footprint is a formidable challenge. Metasurfaces and plasmonics are promising , but metals exhibit weak electro-optic effects. Two-dimensional materials, such as graphene, have shown great performance as modulators with small drive voltages. Here we show a graphene plasmonic phase modulator which is capable of tuning the phase between 0 and 2π in situ. With a footprint of 350nm it is more than 30 times smaller than the 10.6$μ$m free space wavelength. The modulation is achieved by spatially controlling the plasmon phase velocity in a device where the spatial carrier density profile is tunable. We provide a scattering theory for plasmons propagating through spatial density profiles. This work constitutes a first step towards two-dimensional transformation optics for ultra-compact modulators and biosensing.

physics.app-ph↗

Tuning quantum non-local effects in graphene plasmonics

The response of an electron system to electromagnetic fields with sharp spatial variations is strongly dependent on quantum electronic properties, even in ambient conditions, but difficult to access experimentally. We use propagating graphene plasmons, together with an engineered dielectric-metallic environment, to probe the graphene electron liquid and unveil its detailed electronic response at short wavelengths.The near-field imaging experiments reveal a parameter-free match with the full theoretical quantum description of the massless Dirac electron gas, in which we identify three types of quantum effects as keys to understanding the experimental response of graphene to short-ranged terahertz electric fields. The first type is of single-particle nature and is related to shape deformations of the Fermi surface during a plasmon oscillations. The second and third types are a many-body effect controlled by the inertia and compressibility of the interacting electron liquid in graphene. We demonstrate how, in principle, our experimental approach can determine the full spatiotemporal response of an electron system.

cond-mat.mes-hall↗