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Marcus Reindl

Publications and source records attributed to Marcus Reindl.

28 records · Page 2Linked to original sources

Semiconductor quantum dots as an ideal source of polarization entangled photon pairs on-demand: a review

More than 80 years passed since the first publication on entangled quantum states. In this period of time the concept of spookily interacting quantum states became an emerging field of science. After various experiments proving the existence of such non-classical states, visionary ideas were put forward to exploit entanglement in quantum information science and technology. These novel concepts have not yet come out of the experimental stage, mostly because of the lack of suitable, deterministic sources of entangled quantum states. Among many systems under investigation, semiconductor quantum dots are particularly appealing emitters of on-demand, single polarization-entangled photon-pairs. Although, it was originally believed that quantum dots must exhibit a limited degree of entanglement related to numerous decoherence effects present in the solid-state. Recent studies invalidated the premise of unavoidable entanglement degrading effects. We review the relevant experiments which have led to these important discoveries and discuss the remaining challenges for the anticipated quantum technologies.

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Strain-Tunable GaAs Quantum dot: A Nearly Dephasing-Free Source of Entangled Photon Pairs on Demand

Entangled photon generation from semiconductor quantum dots via the biexciton-exciton cascade underlies various decoherence mechanisms related to the solid-state nature of the quantum emitters. So far, this has prevented the demonstration of nearly-maximally entangled photons without the aid of inefficient and complex post-selection techniques that are hardly suitable for quantum communication technologies. Here, we tackle this challenge using strain-tunable GaAs quantum dots driven under two-photon resonant excitation and with strictly-degenerate exciton states. We demonstrate experimentally that our on-demand source generates polarization-entangled photons with fidelity of 0.978(5) and concurrence of 0.97(1) without resorting to post-selection techniques. Moreover, we show that the remaining decoherence mechanisms can be overcome using a modest Purcell enhancement so as to achieve a degree of entanglement >0.99. Our results highlight that GaAs quantum dots can be readily used in advanced communication protocols relying on the non-local properties of quantum entanglement.

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Electromagnetically Induced Transparency of On-demand Single Photons in a Hybrid Quantum Network

Long range quantum communication and quantum information processing require the development of light-matter interfaces for distributed quantum networks. Even though photons are ideal candidates for network links to transfer quantum information, the system of choice for the realization of quantum nodes has not been identified yet. Ideally, one strives for a hybrid network architecture, which will consist of different quantum systems, combining the strengths of each system. However, interfacing different quantum systems via photonic channels remains a major challenge because a detailed understanding of the underlying light-matter interaction is missing. Here, we show the coherent manipulation of single photons generated on-demand from a semiconductor quantum dot using a rubidium vapor quantum memory, forming a hybrid quantum network. We demonstrate the engineering of the photons' temporal wave function using four-level atoms and the creation of a new type of electromagnetic induced transparency for quantum dot photons on resonance with rubidium transitions. Given the short lifetime of our quantum dot transition the observed dynamics cannot be explained in the established steady-state picture. Our results play a pivotal role in understanding quantum light-matter interactions at short time scales. These findings demonstrate a fundamental active node to construct future large-scale hybrid quantum networks.

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On-demand semiconductor source of 780 nm single photons with controlled temporal wave packets

We report on a fast, bandwidth-tunable single-photon source based on an epitaxial GaAs quantum dot. Exploiting spontaneous spin-flip Raman transitions, single photons at $780\,$nm are generated on-demand with tailored temporal profiles of durations exceeding the intrinsic quantum dot lifetime by up to three orders of magnitude. Second-order correlation measurements show a low multi-photon emission probability ($g^{2}(0)\sim\,0.10-0.15$) at a generation rate up to $10\,$MHz. We observe Raman photons with linewidths as low as $200\,$MHz, narrow compared to the $1.1\,$GHz linewidth measured in resonance fluorescence. The generation of such narrow-band single photons with controlled temporal shapes at the rubidium wavelength is a crucial step towards the development of an optimized hybrid semiconductor-atom interface.

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Two-photon interference from two blinking quantum emitters

We investigate the effect of blinking on the two-photon interference measurement from two independent quantum emitters. We find that blinking significantly alters the statistics in the second-order intensity correlation function g$^{(2)}(τ)$ and the outcome of two-photon interference measurements performed with independent quantum emitters. We theoretically demonstrate that the presence of blinking can be experimentally recognized by a deviation from the g$^{(2)}_{D}(0)=0.5$ value when distinguishable photons impinge on a beam splitter. Our results show that blinking imposes a mandatory cross-check measurement to correctly estimate the degree of indistinguishablility of photons emitted by independent quantum emitters.

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Phonon-assisted two-photon interference from remote quantum emitters

Photonic quantum technologies are on the verge of finding applications in everyday life with quantum cryptography and the quantum internet on the horizon. Extensive research has been carried out to determine suitable quantum emitters and single epitaxial quantum dots are emerging as near-optimal sources of bright, on-demand, highly indistinguishable single photons and entangled photon pairs. In order to build up quantum networks, it is now essential to interface remote quantum emitters. However, this is still an outstanding challenge, as the quantum states of dissimilar 'artificial atoms' have to be prepared on-demand with high fidelity, and the generated photons have to be made indistinguishable in all possible degrees of freedom. Here, we overcome this major obstacle and show an unprecedented two-photon interference (visibility of 51+/-5%) from remote strain-tunable GaAs quantum dots, emitting on-demand photon-pairs. We achieve this result by exploiting for the first time the full potential of the novel phonon-assisted two-photon excitation scheme, which allows for the generation of highly indistinguishable (visibility of 71+/-9%) entangled photon-pairs (fidelity of 90+/-2%), it enables push-to button biexciton state preparation (fidelity of 80+/-2%) and it outperforms conventional resonant two-photon excitation schemes in terms of robustness against environmental decoherence. Our results mark an important milestone for the practical realization of quantum repeaters and complex multi-photon entanglement experiments involving dissimilar artificial atoms.

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Electrically-Pumped Wavelength-Tunable GaAs Quantum Dots Interfaced with Rubidium Atoms

We demonstrate the first wavelength-tunable electrically-pumped source of non-classical light that can emit photons with wavelength in resonance with the D2 transitions of 87Rb atoms. The device is fabricated by integrating a novel GaAs single-quantum-dot light-emitting-diode (LED) onto a piezoelectric actuator. By feeding the emitted photons into a 75-mm-long cell containing warm 87Rb atom vapor, we observe slow-light with a temporal delay of up to 3.4 ns. In view of the possibility of using 87Rb atomic vapors as quantum memories, this work makes an important step towards the realization of hybrid-quantum systems for future quantum networks.

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Highly indistinguishable and strongly entangled photons from symmetric GaAs quantum dots

The development of scalable sources of non-classical light is fundamental to unlock the technological potential of quantum photonics\cite{Kimble:Nat2008}. Among the systems under investigation, semiconductor quantum dots are currently emerging as near-optimal sources of indistinguishable single photons. However, their performances as sources of entangled-photon pairs are in comparison still modest. Experiments on conventional Stranski-Krastanow InGaAs quantum dots have reported non-optimal levels of entanglement and indistinguishability of the emitted photons. For applications such as entanglement teleportation and quantum repeaters, both criteria have to be met simultaneously. In this work, we show that this is possible focusing on a system that has received limited attention so far: GaAs quantum dots grown via droplet etching. Using a two-photon resonant excitation scheme, we demonstrate that these quantum dots can emit triggered polarization-entangled photons with high purity (g^(2)(0)=0.002 +/-0.002), high indistinguishability (0.93 +/-0.07) and high entanglement fidelity (0.94 +/-0.01). Such unprecedented degree of entanglement, which in contrast to InGaAs can theoretically reach near-unity values, allows Bell's inequality (2.64 +/-0.01) to be violated without the aid of temporal or spectral filtering. Our results show that if quantum-dot entanglement resources are to be used for future quantum technologies, GaAs might be the system of choice.

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An artificial Rb atom in a semiconductor with lifetime-limited linewidth

We report results important for the creation of a best-of-both-worlds quantum hybrid system consisting of a solid-state source of single photons and an atomic ensemble as quantum memory. We generate single photons from a GaAs quantum dot (QD) frequency-matched to the Rb D2-transitions and then use the Rb transitions to analyze spectrally the quantum dot photons. We demonstrate lifetime-limited QD linewidths (1.48 GHz) with both resonant and non-resonant excitation. The QD resonance fluorescence in the low power regime is dominated by Rayleigh scattering, a route to match quantum dot and Rb atom linewidths and to shape the temporal wave packet of the QD photons. Noise in the solid-state environment is relatively benign: there is a blinking of the resonance fluorescence at MHz rates but negligible upper state dephasing of the QD transition. We therefore establish a close-to-ideal solid-state source of single photons at a key wavelength for quantum technologies.

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Scalable Sources of Entangled Photons with Wavelength on Demand

The prospect of using the quantum nature of light for secure communication keeps spurring the search and investigation of suitable sources of entangled-photons. Semiconductor quantum dots are arguably the most attractive. They can generate indistinguishable entangled-photons deterministically, and are compatible with current photonic-integration technologies, a set of properties not shared by any other entanglement resource. However, as no two quantum dots are identical, they emit entangled-photons with random energies. This hinders their exploitation in communication protocols requiring entangled-states with well-defined energies. Here, we introduce scalable quantum-dot-based sources of polarization-entangled-photons whose energy can be controlled via dynamic strain-engineering without degrading the degree of entanglement of the source. As a test-bench, we interface quantum dots with clouds of atomic vapours, and we demonstrate slow-entangled-photons from a single quantum emitter. These results pave the way towards the implementation of hybrid quantum networks where entanglement is distributed among distant parties using scalable optoelectronic devices.

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