arXiv subjects

Marcus Reindl

Publications and source records attributed to Marcus Reindl.

At least 19 recordsLinked to original sources

arXiv2023

Hyperfine-interaction limits polarization entanglement of photons from semiconductor quantum dots

Excitons in quantum dots are excellent sources of polarization-entangled photon pairs, but a quantitative understanding of their interaction with the nuclear spin bath is still missing. Here we investigate the role of hyperfine energy shifts using experimentally accessible parameters and derive an upper limit to the achievable entanglement fidelity. Our results are consistent with all available literature, indicate that spin-noise is often the dominant process limiting the entanglement in InGaAs quantum dots, and suggest routes to alleviate its effect.

quant-ph↗

arXiv2023

Coherent Quantum Interconnection between On-Demand Quantum Dot Single Photons and a Resonant Atomic Quantum Memory

Long-range quantum communication requires the development of in-out light-matter interfaces to achieve a quantum advantage in entanglement distribution. Ideally, these quantum interconnections should be as fast as possible to achieve high-rate entangled qubits distribution. Here, we demonstrate the coherent quanta exchange between single photons generated on-demand from a GaAs quantum dot and atomic ensemble in a $^{87}$Rb vapor quantum memory. Through an open quantum system analysis, we demonstrate the mapping between the quantized electric field of photons and the coherence of the atomic ensemble. Our results play a pivotal role in understanding quantum light-matter interactions at the short time scales required to build fast hybrid quantum networks.

quant-ph↗

arXiv2022

GaAs quantum dots under quasi-uniaxial stress: experiment and theory

The optical properties of excitons confined in initially-unstrained GaAs/AlGaAs quantum dots are studied as a function of a variable quasi-uniaxial stress. To allow the validation of state-of-the-art computational tools for describing the optical properties of nanostructures, we determine the quantum dot morphology and the in-plane components of externally induced strain tensor at the quantum dot positions. Based on these \textsl{experimental} parameters, we calculate the strain-dependent excitonic emission energy, degree of linear polarization, and fine-structure splitting using a combination of eight-band ${\bf k}\cdot{\bf p}$ formalism with multiparticle corrections using the configuration interaction method. The experimental observations are quantitatively well reproduced by our calculations and deviations are discussed.

cond-mat.mes-hall↗

arXiv2022

Surface passivation and oxide encapsulation to improve optical properties of a single GaAs quantum dot close to the surface

Epitaxial GaAs quantum dots grown by droplet etching have recently shown excellent properties as sources of single photons as well as entangled photon pairs. Integration in some nanophotonic structures requires surface-to-dot distances of less than 100 nm. This demands a surface passivation scheme, which could be useful to lower the density of surface states. To address this issue, sulphur passivation with dielectric overlayer as an encapsulation is used for surface to QD distances of 40 nm, which results in the partial recovery of emission linewidths to bulk values as well as in the increase of the photoluminescence intensity.

physics.app-ph↗

arXiv2021

GaAs quantum dots grown by droplet etching epitaxy as quantum light sources

This paper presents an overview and perspectives on the epitaxial growth and optical properties of GaAs quantum dots obtained with the droplet etching method as high-quality sources of quantum light. We illustrate the recent achievements regarding the generation of single photons and polarization entangled photon pairs and the use of these sources in applications of central importance in quantum communication, such as entanglement swapping and quantum key distribution.

quant-ph↗

arXiv2020

Quantum dots as potential sources of strongly entangled photons for quantum networks

The generation and long-haul transmission of highly entangled photon pairs is a cornerstone of emerging photonic quantum technologies, with key applications such as quantum key distribution and distributed quantum computing. However, a natural limit for the maximum transmission distance is inevitably set by attenuation in the medium. A network of quantum repeaters containing multiple sources of entangled photons would allow to overcome this limit. For this purpose, the requirements on the source's brightness and the photon pairs' degree of entanglement and indistinguishability are stringent. Despite the impressive progress made so far, a definitive scalable photon source fulfilling such requirements is still being sought for. Semiconductor quantum dots excel in this context as sub-poissonian sources of polarization entangled photon pairs. In this work we present the state-of-the-art set by GaAs based quantum dots and use them as a benchmark to discuss the challenges to overcome towards the realization of practical quantum networks.

quant-ph↗

arXiv2020

Quantum cryptography with highly entangled photons from semiconductor quantum dots

State-of-the-art quantum key distribution systems are based on the BB84 protocol and single photons generated by lasers. These implementations suffer from range limitations and security loopholes, which require expensive adaptation. The use of polarization entangled photon pairs substantially alleviates the security threads while allowing for basically arbitrary transmission distances when embedded in quantum repeater schemes. Semiconductor quantum dots are capable of emitting highly entangled photon pairs with ultra-low multi-pair emission probability even at maximum brightness. Here we report on the first implementation of the BBM92 protocol using a quantum dot source with an entanglement fidelity as high as 0.97(1). For a proof of principle, the key generation is performed between two buildings, connected by 350 metre long fiber, resulting in an average key rate of 135 bits/s and a qubit error rate of 0.019 over a time span of 13 hours, without resorting to time- or frequency-filtering techniques. Our work demonstrates the viability of quantum dots as light sources for entanglement-based quantum key distribution and quantum networks. By embedding them in state-of-the-art photonic structures, key generation rates in the Gbit/s range are at reach.

quant-ph↗

arXiv2020

The crux of using the cascaded emission of a 3-level quantum ladder system to generate indistinguishable photons

We investigate the degree of indistinguishability of cascaded photons emitted from a 3-level quantum ladder system; in our case the biexciton-exciton cascade of semiconductor quantum dots. For the 3-level quantum ladder system we theoretically demonstrate that the indistinguishability is inherently limited for both emitted photons and determined by the ratio of the lifetimes of the excited and intermediate states. We experimentally confirm this finding by comparing the quantum interference visibility of non-cascaded emission and cascaded emission from the same semiconductor quantum dot. Quantum optical simulations produce very good agreement with the measurements and allow to explore a large parameter space. Based on our model, we propose photonic structures to optimize the lifetime ratio and overcome the limited indistinguishability of cascaded photon emission from a 3-level quantum ladder system.

cond-mat.mes-hall↗

arXiv2020

The Origin of Antibunching in Resonance Fluorescence

Epitaxial quantum dots have emerged as one of the best single-photon sources, not only for applications in photonic quantum technologies but also for testing fundamental properties of quantum optics. One intriguing observation in this area is the scattering of photons with subnatural linewidth from a two-level system under resonant continuous wave excitation. In particular, an open question is whether these subnatural linewidth photons exhibit simultaneously antibunching as an evidence of single-photon emission. Here, we demonstrate that this simultaneous observation of subnatural linewidth and antibunching is not possible with simple resonant excitation. First, we independently confirm single-photon character and subnatural linewidth by demonstrating antibunching in a Hanbury Brown and Twiss type setup and using high-resolution spectroscopy, respectively. However, when filtering the coherently scattered photons with filter bandwidths on the order of the homogeneous linewidth of the excited state of the two-level system, the antibunching dip vanishes in the correlation measurement. Our experimental work is consistent with recent theoretical findings, that explain antibunching from photon-interferences between the coherent scattering and a weak incoherent signal in a skewed squeezed state.

cond-mat.mes-hall↗

arXiv2019

Single-Particle-Picture Breakdown in laterally weakly confining GaAs Quantum Dots

We present a detailed investigation of different excitonic states weakly confined in single GaAs/AlGaAs quantum dots obtained by the Al droplet-etching method. For our analysis we make use of temperature-, polarization- and magnetic field-dependent $\mu$-photoluminescence measurements, which allow us to identify different excited states of the quantum dot system. Besides that, we present a comprehensive analysis of g-factors and diamagnetic coefficients of charged and neutral excitonic states in Voigt and Faraday configuration. Supported by theoretical calculations by the Configuration interaction method, we show that the widely used single-particle Zeeman Hamiltonian cannot be used to extract reliable values of the g-factors of the constituent particles from excitonic transition measurements.

cond-mat.mes-hall↗

arXiv2019

Strain tunable single-photon source based on a quantum dot-micropillar system

Scalable quantum photonic architectures demand highly efficient, high-purity single-photon sources, which can be frequency matched via external tuning. We demonstrate a single-photon source based on an InAs quantum dot embedded in a micropillar resonator, which is frequency tunable via externally-applied stress. Our platform combines the advantages of a Bragg micropillar cavity and the piezo-strain-tuning technique enabling single photon spontaneous emission enhancement via the Purcell effect and quantum dot (QD) with tunable wavelength. Our optomechanical platform has been implemented by integration of semiconductor-based QD-micropillars on a piezoelectric substrate. The fabricated device exhibits spontaneous emission enhancement with a Purcell factor of 4.4$\pm$0.7 and allows for a pure triggered single-photon generation with $g^{(2)}(0)$ < 0.07 under resonant excitation. A quantum dot emission energy tuning range of 0.75 meV for 27 kV/cm applied to the piezo substrate has been achieved. Our results pave the way towards the scalable implementation of single-photon quantum photonic technologies using optoelectronic devices.

cond-mat.mes-hall↗

arXiv2019

Resolving the temporal evolution of line broadening in quantum emitters

Light emission from solid-state quantum emitters is inherently prone to environmental decoherence, which results in an inhomogeneous line broadening and in the deterioration of photon indistinguishability. Here we employ photon correlation Fourier spectroscopy (PCFS) to study the temporal evolution of such a broadening for the biexciton and exciton emission in resonantly driven GaAs quantum dots. Differently from previous experiments, the time scales we probe range from a few nanoseconds to milliseconds and, simultaneously, the spectral resolution we achieve can be as small as 2 $\mu$eV. We find pronounced differences in the temporal evolution of the two lines, which we attribute to differences in their homogeneous linewidth and sensitivity to charge noise. We then analyze the effect of irradiation with additional white light, which reduces blinking at the cost of enhanced charge noise. Due to its robustness against experimental imperfections and its high temporal resolution and bandwidth, PCFS outperforms established spectroscopy techniques, such as Michelson interferometry. We discuss its practical implementation, its limitations, and the possibility to use it to estimate the indistinguishability of consecutively emitted single photons for applications in quantum communication and photonic-based quantum information processing.

cond-mat.mes-hall↗

arXiv2019

Highly indistinguishable single photons from incoherently and coherently excited GaAs quantum dots

Semiconductor quantum dots are converging towards the demanding requirements of photonic quantum technologies. Among different systems, quantum dots with dimensions exceeding the free-exciton Bohr radius are appealing because of their high oscillator strengths. While this property has received much attention in the context of cavity quantum electrodynamics, little is known about the degree of indistinguishability of single photons consecutively emitted by such dots and on the proper excitation schemes to achieve high indistinguishability. A prominent example is represented by GaAs quantum dots obtained by local droplet etching, which recently outperformed other systems as triggered sources of entangled photon pairs. On these dots, we compare different single-photon excitation mechanisms, and we find (i) a "phonon bottleneck" and poor indistinguishability for conventional excitation via excited states and (ii) photon indistinguishablilities above 90% for both strictly resonant and for incoherent acoustic- and optical-phonon-assisted excitation. Among the excitation schemes, optical phonon-assisted excitation enables straightforward laser rejection without a compromise on the source brightness together with a high photon indistinguishability.

cond-mat.mes-hall↗

arXiv2019

Resonance fluorescence of GaAs quantum dots with near-unity photon indistinguishability

Photonic quantum technologies call for scalable quantum light sources that can be integrated, while providing the end user with single and entangled photons on-demand. One promising candidate are strain free GaAs/AlGaAs quantum dots obtained by droplet etching. Such quantum dots exhibit ultra low multi-photon probability and an unprecedented degree of photon pair entanglement. However, different to commonly studied InGaAs/GaAs quantum dots obtained by the Stranski-Krastanow mode, photons with a near-unity indistinguishability from these quantum emitters have proven to be elusive so far. Here, we show on-demand generation of near-unity indistinguishable photons from these quantum emitters by exploring pulsed resonance fluorescence. Given the short intrinsic lifetime of excitons confined in the GaAs quantum dots, we show single photon indistinguishability with a raw visibility of $V_{raw}=(94.2\pm5.2)\,\%$, without the need for Purcell enhancement. Our results represent a milestone in the advance of GaAs quantum dots by demonstrating the final missing property standing in the way of using these emitters as a key component in quantum communication applications, e.g. as an entangled source for quantum repeater architectures.

cond-mat.mes-hall↗

arXiv2019

Entanglement swapping with photons generated on-demand by a quantum dot

Photonic entanglement swapping, the procedure of entangling photons without any direct interaction, is a fundamental test of quantum mechanics and an essential resource to the realization of quantum networks. Probabilistic sources of non-classical light can be used for entanglement swapping, but quantum communication technologies with device-independent functionalities demand for push-button operation that, in principle, can be implemented using single quantum emitters. This, however, turned out to be an extraordinary challenge due to the stringent requirements on the efficiency and purity of generation of entangled states. Here we tackle this challenge and show that pairs of polarization-entangled photons generated on-demand by a GaAs quantum dot can be used to successfully demonstrate all-photonic entanglement swapping. Moreover, we develop a theoretical model that provides quantitative insight on the critical figures of merit for the performance of the swapping procedure. This work shows that solid-state quantum emitters are mature for quantum networking and indicates a path for scaling up.

quant-ph↗

arXiv2018

On-demand generation of background--free single photons from a solid-state source

True on--demand high--repetition--rate single--photon sources are highly sought after for quantum information processing applications. However, any coherently driven two-level quantum system suffers from a finite re-excitation probability under pulsed excitation, causing undesirable multi--photon emission. Here, we present a solid--state source of on--demand single photons yielding a raw second--order coherence of $g^{(2)}(0)=(7.5\pm1.6)\times10^{-5}$ without any background subtraction nor data processing. To this date, this is the lowest value of $g^{(2)}(0)$ reported for any single--photon source even compared to the previously best background subtracted values. We achieve this result on GaAs/AlGaAs quantum dots embedded in a low--Q planar cavity by employing (i) a two--photon excitation process and (ii) a filtering and detection setup featuring two superconducting single--photon detectors with ultralow dark-count rates of $(0.0056\pm0.0007) s^{-1}$ and $(0.017\pm0.001) s^{-1}$, respectively. Re--excitation processes are dramatically suppressed by (i), while (ii) removes false coincidences resulting in a negligibly low noise floor.

cond-mat.mes-hall↗

arXiv2018

High-yield fabrication of entangled photon emitters for hybrid quantum networking using high-temperature droplet epitaxy

Several semiconductor quantum dot techniques have been investigated for the generation of entangled photon pairs. Among the other techniques, droplet epitaxy enables the control of the shape, size, density, and emission wavelength of the quantum emitters. However, the fraction of the entanglement-ready quantum dots that can be fabricated with this method is still limited to around 5%, and matching the energy of the entangled photons to atomic transitions (a promising route towards quantum networking) remains an outstanding challenge. Here, we overcome these obstacles by introducing a modified approach to droplet epitaxy on a high symmetry (111)A substrate, where the fundamental crystallization step is performed at a significantly higher temperature as compared to previous reports. Our method drastically improves the yield of entanglement-ready photon sources near the emission wavelength of interest, which can be as high as 95% due to the low values of fine structure splitting and radiative lifetime, together with the reduced exciton dephasing offered by the choice of GaAs/AlGaAs materials. The quantum dots are designed to emit in the operating spectral region of Rb-based slow-light media, providing a viable technology for quantum repeater stations.

cond-mat.mes-hall↗

arXiv2018

Semiconductor quantum dots as an ideal source of polarization entangled photon pairs on-demand: a review

More than 80 years passed since the first publication on entangled quantum states. In this period of time the concept of spookily interacting quantum states became an emerging field of science. After various experiments proving the existence of such non-classical states, visionary ideas were put forward to exploit entanglement in quantum information science and technology. These novel concepts have not yet come out of the experimental stage, mostly because of the lack of suitable, deterministic sources of entangled quantum states. Among many systems under investigation, semiconductor quantum dots are particularly appealing emitters of on-demand, single polarization-entangled photon-pairs. Although, it was originally believed that quantum dots must exhibit a limited degree of entanglement related to numerous decoherence effects present in the solid-state. Recent studies invalidated the premise of unavoidable entanglement degrading effects. We review the relevant experiments which have led to these important discoveries and discuss the remaining challenges for the anticipated quantum technologies.

quant-ph↗