arXiv subjects

Maria Teresa Mercaldo

Publications and source records attributed to Maria Teresa Mercaldo.

At least 37 records · Page 2Linked to original sources

arXiv2023

High orbital-moment Cooper pairs by crystalline symmetry breaking

The pairing structure of superconducting materials is regulated by the point group symmetries of the crystal. Here, we study spin-singlet multiorbital superconductivity in materials with unusually low crystalline symmetry content and unveil the the appearance of even-parity (s-wave) Cooper pairs with high orbital moment. We show that the lack of mirror and rotation symmetries makes pairing states with quintet orbital angular momentum symmetry-allowed. A remarkable fingerprint of this type of pairing state is provided by a nontrivial superconducting phase texture in momentum space with $π$-shifted domains and walls with anomalous phase winding. The pattern of the quintet pairing texture is shown to depend on the orientation of the orbital polarization and the strength of the mirror and/or rotation symmetry breaking terms. Such momentum dependent phase makes Cooper pairs with net orbital component suited to design orbitronic Josephson effects. We discuss how an intrinsic orbital dependent phase can set out anomalous Josephson couplings by employing superconducting leads with nonequivalent breaking of crystalline symmetry.

cond-mat.supr-con↗

arXiv2023

Designing spin and orbital sources of Berry curvature at oxide interfaces

Quantum materials can display physical phenomena rooted in the geometry of electronic wavefunctions. The corresponding geometric tensor is characterized by an emergent field known as Berry curvature (BC). Large BCs typically arise when electronic states with different spin, orbital or sublattice quantum numbers hybridize at finite crystal momentum. In all materials known to date, the BC is triggered by the hybridization of a single type of quantum number. Here, we report the discovery of the first material system having both spin and orbital-sourced BC: LaAlO$_3$/SrTiO$_3$ interfaces grown along the [111] direction. We detect independently these two sources and directly probe the BC associated to the spin quantum number through measurements of an anomalous planar Hall effect. The observation of a nonlinear Hall effect with time-reversal symmetry signals large orbital-mediated BC dipoles. The coexistence of different forms of BC enables the combination of spintronic and optoelectronic functionalities in a single material.

cond-mat.mes-hall↗

arXiv2023

Orbital design of Berry curvature: pinch points and giant dipoles induced by crystal fields

The Berry curvature (BC) - a quantity encoding the geometric properties of the electronic wavefunctions in a solid - is at the heart of different Hall-like transport phenomena, including the anomalous Hall and the non-linear Hall and Nernst effects. In non-magnetic quantum materials with acentric crystalline arrangements, local concentrations of BC are generally linked to single-particle wavefunctions that are a quantum superposition of electron and hole excitations. BC-mediated effects are consequently observed in two-dimensional systems with pairs of massive Dirac cones and three-dimensional bulk crystals with quartets of Weyl cones. Here, we demonstrate that in materials equipped with orbital degrees of freedom local BC concentrations can arise even in the complete absence of hole excitations. In these solids, the crystals fields appearing in very low-symmetric structures trigger BCs characterized by hot-spots and singular pinch points. These characteristics naturally yield giant BC dipoles and large non-linear transport responses in time-reversal symmetric conditions.

cond-mat.mes-hall↗

arXiv2022

Odd-frequency pairing in a nonunitary p-wave superconductor with multiple Majorana fermions

Odd-frequency Cooper pairs are gathering attention for the convenience of investigating the edge state of topological superconductors including Majorana fermions. Although a spinless p-wave superconductor has only one Majorana fermion in a topological phase, the system with magnetic fields can reach the topological phases with multiple Majorana fermions. To distinguish these multiple Majorana fermion phases, we correlate the energy spectrum with the odd-frequency pair amplitude as increasing the system size. The system size dependence tells us three pieces of information: the parity of the number of the Majorana fermions at the edge, the number of low-energy modes corresponding to the Majorana fermions with different localization lengths, and the fingerprints of the Majorana fermions. Also, we present the spatial dependence of the odd-frequency f vector that is created from odd-frequency pair amplitude and the spin structure of odd-frequency Cooper pairs. We find that the odd-frequency f vector is fixed in the same direction in any topological phase. Also, we show that the spin state of odd-frequency Cooper pairs tends to be oriented toward the direction of the magnetic fields. Our results highlight the odd-frequency Cooper pairs can be a good indicator for the detection of the multiple Majorana fermions and the distinction among the topological phases.

cond-mat.supr-con↗

arXiv2022

Frustration driven Josephson phase dynamics

The Josephson equations predict remarkable effects concerning the phase state of a superconducting junction with an oscillating current induced by a static voltage. Whether the paradigm can be twisted by yielding an oscillating voltage without making use of harmonic drives is a fundamentally relevant problem yet not fully settled. Here, we demonstrate that a dynamical regime with an oscillating phase evolution is a general hallmark of driven Josephson systems exhibiting sign competition in the Josephson couplings. We show that in frustrated Josephson systems an oscillating phase dynamics gets switched on by driving the changeover among different ground states, which can be induced by varying the parameters that set the phase state. Remarkably, the character of the transitions in the Josephson phase space allows different types of dynamics, with few or several harmonics. This result sets out a characteristic mark of any superconducting system with frustrated Josephson couplings and can be exploited to disentangle the complexity of the underlying phases.

cond-mat.supr-con↗

arXiv2021

Zero magnetic-field orbital vortices in s-wave spin-singlet superconductors

Breaking of time-reversal and point-group spatial symmetries can have a profound impact on superconductivity. One of the most extraordinary effects, due to the application of a magnetic field, is represented by the Abrikosov vortices with charged supercurrents circulating around their cores. Whether a similar phenomenon can be obtained by exploiting spatial symmetry breaking, e.g. through electric fields or mechanical strain, is a fundamentally relevant but not yet fully settled problem. Here, we show that in two-dimensional spin-singlet superconductors with unusually low degree of spatial symmetry content, vortices with supercurrents carrying angular momentum around the core can form and be energetically stable. The vortex has zero net magnetic flux since it is made up of counter-propagating Cooper pairs with opposite orbital moments. By solving self-consistently the Bogoliubov - de Gennes equations in real space, we demonstrate that the orbital vortex is stable and we unveil the spatial distribution of the superconducting order parameter around its core. The resulting amplitude has a characteristic pattern with a pronounced angular anisotropy that deviates from the profile of conventional magnetic vortices. These hallmarks guide predictions and proposals for the experimental detection.

cond-mat.supr-con↗

arXiv2021

Spectroscopic Signatures of Gate-Controlled Superconducting Phases

We investigate the tunneling conductance of superconductor-insulator-normal metal (SIN) and superconductor-insulator-superconductor (SIS) heterostructures with one superconducting side of the junction that is electrically driven and can exhibit $π$-pairing through a modification of the surface inversion asymmetric couplings. In SIN tunneling we find that the variation of the electrically driven interactions generally brings an increase of quasi-particles in the gap due to orbitally polarized depaired states, irrespective of the inter-band phase rearrangement. The peak of SIN conductance at the gap edge varies with a trend that depends both on the strength of the surface interactions as well as on the character of the gate-induced superconducting state. While this shift can be also associated with thermal effects in the SIN configuration, for the SIS geometry at low temperature the electric field does not yield the characteristic matching peak at voltages related with the difference between the gaps of the superconducting electrodes. This observation sets out a distinctive mark for spectroscopically distinguishing the thermal population effects from the quantum gate-driven signatures. In SIS the electrostatic gating yields a variety of features with asymmetric peaks and broadening of the conductance spectral weight. These findings indicate general qualitative trends for both SIN and SIS tunneling spectroscopy which could serve to evaluate the impact of gate-control on superconductors and the occurrence of non-centrosymmetric orbital antiphase pairing.

cond-mat.supr-con↗

arXiv2021

Gate-control of the current-flux relation of a Josephson quantum interferometer based on proximitized metallic nanojuntions

We demonstrate an Al superconducting quantum interference device in which the Josephson junctions are implemented through gate-controlled proximitized Cu mesoscopic weak-links. The latter behave analogously to genuine superconducting metals in terms of the response to electrostatic gating, and provide a good performance in terms of current-modulation visibility. We show that, through the application of a static gate voltage, we are able to modify the interferometer current-flux relation in a fashion which seems compatible with the introduction of $π$-channels within the gated weak-link. Our results suggest that the microscopic mechanism at the origin of the suppression of the switching current in the interferometer is apparently phase coherent, resulting in an overall damping of the superconducting phase rigidity. We finally tackle the performance of the interferometer in terms of responsivity to magnetic flux variations in the dissipative regime, and discuss the practical relevance of gated proximity-based all-metallic SQUIDs for magnetometry at the nanoscale.

cond-mat.supr-con↗

arXiv2020

Electrically Tunable Superconductivity Through Surface Orbital Polarization

We investigate the physical mechanisms for achieving an electrical control of conventional spin-singlet superconductivity in thin films by focusing on the role of surface orbital polarization. Assuming a multi-orbital description of the metallic state, due to screening effects the electric field acts by modifying the strength of the surface potential and, in turn, yields non-trivial orbital-Rashba couplings. The resulting orbital polarization at the surface and in its close proximity is shown to have a dramatic impact on superconductivity. We demonstrate that, by varying the strength of the electric field, the superconducting phase can be either suppressed, i.e. turned into normal metal, or undergo a $0-π$ transition with the $π$ phase being marked by non-trivial sign change of the superconducting order parameter between different bands. These findings unveil a rich scenario to design heterostructures with superconducting orbitronics effects.

cond-mat.supr-con↗

arXiv2020

Unveiling Mechanisms of Electric Field Effects on Superconductors by Magnetic Field Response

We demonstrate that superconducting aluminium nano-bridges can be driven into a state with complete suppression of the critical supercurrent via electrostatic gating. Probing both in- and out-of-plane magnetic field responses in the presence of electrostatic gating can unveil the mechanisms that primarily cause the superconducting electric field effects. Remarkably, we find that a magnetic field, independently of its orientation, has only a weak influence on the critical electric field that identifies the transition from the superconducting state to a phase with vanishing critical supercurrent. This observation points to the absence of a direct coupling between the electric field and the amplitude of the superconducting order parameter or $2π$-phase slips via vortex generation. The magnetic field effect observed in the presence of electrostatic gating is described within a microscopic model where a spatially uniform inter-band $π$-phase is stabilized by the electric field. Such an intrinsic superconducting phase rearrangement can account for the suppression of the supercurrent, as well as for the weak dependence of the critical magnetic fields on the electric field.

cond-mat.supr-con↗

arXiv2020

Nodal Andreev Spectra in Multi-Majorana Three-Terminal Josephson Junctions

We investigate the Andreev-bound-state (ABS) spectra of three-terminal Josephson junctions which consist of 1D topological superconductors (TSCs) harboring multiple zero-energy edge Majorana bound states (MBSs) protected by chiral symmetry. Our theoretical analysis relies on the exact numerical diagonalization of the Bogoliubov-de Gennes (BdG) Hamiltonian describing the three interfaced TSCs, complemented by an effective low-energy description solely based on the coupling of the interfacial MBSs arising before the leads get contacted. Considering the 2D synthetic space spanned by the two independent superconducting phase differences, we demonstrate that the ABS spectra may contain either point or line nodes, and identify $\mathbb{Z}_2$ topological invariants to classify them. We show that the resulting type of nodes depends on the number of preexisting interfacial MBSs, with nodal lines necessarily appearing when two TSCs harbor an unequal number of MBSs. Specifically, the precise number of interfacial MBSs determines the periodicity of the spectrum under $2π$-slidings of the phase differences and, as a result, also controls the shape of the nodal lines in synthetic space. When chiral symmetry is preserved, the lines are open and coincide with high-symmetry lines of synthetic space, while when it is violated the lines can also transform into loops and chains. The nodal spectra are robust by virtue of the inherent particle-hole symmetry of the BdG Hamiltonian, and give rise to distinctive experimental signatures that we identify.

cond-mat.supr-con↗

arXiv2019

Magnetoelectrically-Tunable Andreev-Bound-State Spectra and Spin Polarization in P-Wave Josephson Junctions

We demonstrate how the boundary-driven reconstruction of the superconducting order parameter can be employed to manipulate the zero-energy Majorana bound states (MBSs) occurring in a topological Josephson junction. We focus on an interface of two p-wave superconductors, which are described by a spin-vector order parameter $\bf{d}$. Apart from the sensitivity of $\bf{d}$ to external Zeeman/exchange fields, here, we show that the orientation of $\bf{d}$ throughout the junction can be controlled by electrically gating the weak link. The remarkable local character of this knob is a manifestation of the edge reconstruction of the order parameter, which takes place whenever different $\bf{d}$-vector configurations in each superconductor compete and are close in energy. As a consequence, the spin-dependent superconducting-phase difference across the junction is switchable from $0$ to $π$. Moreover, in the regime where multiple edge MBSs occur for each superconductor, the Andreev-bound-state (ABS) spectra can be twisted by the application of either a charge- or spin-phase difference across the interface, and give rise to a rich diversity of nonstandard ABS dispersions. Interestingly, some of these dispersions show band crossings protected by fermion parity, despite their $2π$-periodic character. These crossings additionally unlock the possibility of nontrivial topology in synthetic spaces, when considering networks of such 1D junctions. Lastly, the interface MBSs induce a distinct elecronic spin polarization near the junction, which possesses a characteristic spatial pattern that allows the detection of MBSs using spin-polarized scanning tunneling microscopy. These findings unveil novel paths to mechanisms for ABS engineering and single-out signatures relevant for the experimental detection and manipulation of MBSs.

cond-mat.supr-con↗

arXiv2019

Synthetic Weyl Points and Chiral Anomaly in Majorana Devices with Nonstandard Andreev-Bound-State Spectra

We demonstrate how to design various nonstandard types of Andreev-bound-state (ABS) dispersions, via a composite construction relying on Majorana bound states (MBSs). Here, the MBSs appear at the interface of a Josephson junction consisting of two topological superconductors (TSCs). Each TSC harbors multiple MBSs per edge by virtue of a chiral or unitary symmetry. We find that, while the ABS dispersions are $2π$-periodic, they still contain multiple crossings which are protected by the conservation of fermion parity. A single junction with four interface MBSs and all MBS couplings fully controllable, or, networks of such coupled junctions with partial coupling tunability, open the door for topological bandstructures with Weyl points or nodes in synthetic dimensions, which in turn allow for fermion-parity (FP) pumping with a cycle set by the ABS-dispersion details. In fact, in the case of nodes, the FP pumping is a manifestation of chiral anomaly in 2D synthetic spacetime. The possible experimental demonstration of ABS engineering in these devices, further promises to unveil new paths for the detection of MBSs and higher-dimensional chiral anomaly.

cond-mat.supr-con↗

arXiv2019

A minimal tight-binding model for the quasi-one-dimensional superconductor K2Cr3As3

We present a systematic derivation of a minimal five-band tight-binding model for the description of the electronic structure of the recently discovered quasi one-dimensional superconductor K2Cr3As3. Taking as a reference the density-functional theory (DFT) calculation, we use the outcome of a Lowdin procedure to refine a Wannier projection and fully exploit the predominant weight at the Fermi level of the states having the same symmetry of the crystal structure. Such states are described in terms of five atomic-like d orbitals: four planar orbitals, two dxy and two dx2-y2, and a single out-of-plane one, dz2 . We show that this minimal model reproduces with great accuracy the DFT band structure in a broad energy window around the Fermi energy. Moreover, we derive an explicit simplified analytical expression of such model, which includes three nearest-neighbor hopping terms along the z direction and one nearest-neighbor term within the xy plane. This model captures very efficiently the energy spectrum of the system and, consequently, can be used to study transport properties, superconductivity and dynamical effects in this novel class of superconductors.

cond-mat.supr-con↗

arXiv2018

Optimizing the tight-binding parametrization of the quasi-one-dimensional superconductor K2Cr3As3

We study the tight-binding dispersion of the recently discovered superconductor K2Cr3As3, obtained from Wannier projection of Density Functional Theory (DFT) results. In order to establish quantitatively the actual degree of quasi-one dimensionality of this compound, we analyze the electronic band structure for two reduced sets of hopping parameters: one restricted to the Cr-As tubes and another one retaining a minimal number of in-plane hoppings. The corresponding total and local density of states of the compound are also computed with the aim of assessing the tight-binding results with respect to the DFT ones. We find a quite good agreement with the DFT results for the more extended set of hopping parameters, especially for what concerns the orbitals that dominate at the Fermi level. Accordingly, we conclude that one cannot avoid taking into account in-plane hoppings up to the next-nearest-neighbors cells even only to describe correctly the Fermi surface cuts and the populations along the kz direction. Such a choice of a minimal number of hopping parameters directly reflects in the possibility of correctly describing correlations and magnetic interactions.

cond-mat.supr-con↗

arXiv2018

Topological signatures of the coexistence of antiferromagnetism and odd-parity spin-triplet superconductivity

Strongly correlated systems exhibit a rich phenomenology due to the antagonism of a diversity of ordered phases. The aftermath of this interplay can lead to a coexistence which takes place at a microscopic level, or, a phase separation in which non-overlapping single-order domains extend throughout the material. In most cases it appears experimentally challenging to disentangle the two scenarios, unless, there exist robust and measurable properties particular to only one of the two types of coexistence. This is for instance the case when the type of coexistence decides on the appearance of topologically protected excitations, such as, Majorana fermions. In this work, we explore a concrete example falling into this category of systems, and specifically, we investigate one-dimensional odd-parity spin-triplet superconductors in the presence of antiferromagnetism. We determine the symmetry conditions for the occurrence of Majorana edge states and explore their response to variations of the strength and orientation of the antiferromagnetic field $\boldsymbol{M}$, as well as, the spin structure of the Cooper pairs controlled by the so-called $\boldsymbol{d}$-vector.

cond-mat.supr-con↗

arXiv2017

Magnetic manipulation of topological states in p-wave superconductors

Substantial experimental investigation has provided evidence for spin-triplet pairing in diverse classes of materials and in a variety of artificial heterostructures. A fundamental challenge in actual experiments is how to manipulate the topological behavior of $p$-wave superconductors (PSCs) that could open perspectives for applications. Such a control knob is naturally provided by the spin-triplet character of the PSC order parameter, described by the spin d-vector. Therefore, in this work we investigate the magnetic field response of one-dimensional (1d) PSCs and demonstrate that the structure of the Cooper pair spin-configuration is crucial to set topological phases with an enhanced number of Majorana fermions per edge, N, ranging from N=0 to 4. The topological phase diagram, consisting of phases with Majorana modes at the edge, becomes significantly modified when one tunes the strength of the applied field and allows for long range hopping amplitudes in the 1d PSC. We find transitions between phases with different number of Majorana fermions per edge that can be both induced by a variation of the hopping strength and a spin rotation of the d-vector. Hence, the interplay of the applied magnetic field and the internal spin degree of freedom of the PSC opens a new promising route for engineering topological phases with large number of Majorana modes.

cond-mat.supr-con↗

arXiv2016

Magnetic-Field-Induced Topological Reorganization of a P-wave Superconductor

In this work we illustrate the detrimental impact of the Cooper pair's spin-structure on the thermodynamic and topological properties of a spin-triplet superconductor in an applied Zeeman field. We particularly focus on the paradigmatic one-dimensional case (Kitaev chain) for which we self-consistently retrieve the energetically preferred Cooper pair spin-state in terms of the corresponding spin d-vector. The latter undergoes a substantial angular and amplitude reorganization upon the variation of the strength and the orientation of the field and results to a modification of the bulk topological phase diagram. Markedly, when addressing the open chain we find that the orientation of the d-vector varies spatially near the boundary, affecting in this manner the appearance of Majorana fermions at the edge or even altering the properties of the bulk region. Our analysis reveals the limitations and breakdown of the bulk-boundary correspondence in interacting topological systems.

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