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Marin Soljačić

Publications and source records attributed to Marin Soljačić.

At least 127 records · Page 7Linked to original sources

The Quantum Hall Effect with Wilczek's charged magnetic flux tubes instead of electrons

Composites formed from charged particles and magnetic flux tubes, proposed by Wilczek, are one model for anyons - particles obeying fractional statistics. Here we propose a scheme for realizing charged flux tubes, in which a charged object with an intrinsic magnetic dipole moment is placed between two semi-infinite blocks of a high permeability ($μ_r$) material, and the images of the magnetic moment create an effective flux tube. We show that the scheme can lead to a realization of Wilczek's anyons, when a two-dimensional electron system, which exhibits the integer quantum Hall effect (IQHE), is sandwiched between two blocks of the high-$μ_r$ material with a temporally fast response (in the cyclotron and Larmor frequency range). The signature of Wilczek's anyons is a slight shift of the resistivity at the plateau of the IQHE. Thus, the quest for high-$μ_r$ materials at high frequencies, which is underway in the field of metamaterials, and the quest for anyons, are here found to be on the same avenue.

cond-mat.str-el↗

Superlight inverse Doppler effect

There is a century-old tenet [1, 2] that the inverse Doppler frequency shift of light [3-13] is impossible in homogeneous systems with a positive refractive index. Here we break this long-held tenet by predicting a new kind of Doppler effect of light inside the Cherenkov cone. Ever since the classic work of Ginzburg and Frank, it has been known that a superlight (i.e., superluminal) normal Doppler effect [14-18] appears inside the Cherenkov cone when the velocity of the source v is larger than the phase velocity of light v_p. By further developing their theory we discover that an inverse Doppler frequency shift will arise when v>2v_p. We denote this as the superlight inverse Doppler effect. Moreover, we show that the superlight inverse Doppler effect can be spatially separated from the other Doppler effects by using highly squeezed polaritons (such as graphene plasmons), which may facilitate the experimental observation.

physics.optics↗

Quantum plasmons with optical-range frequencies in doped few-layer graphene

Although plasmon modes exist in doped graphene, the limited range of doping achieved by gating restricts the plasmon frequencies to a range that does not include visible and infrared. Here we show, through the use of first-principles calculations, that the high levels of doping achieved by lithium intercalation in bilayer and trilayer graphene shift the plasmon frequencies into the visible range. To obtain physically meaningful results, we introduce a correction of the effect of plasmon interaction across the vacuum separating periodic images of the doped graphene layers, consisting of transparent boundary conditions in the direction perpendicular to the layers; this represents a significant improvement over the Exact Coulomb cutoff technique employed in earlier works. The resulting plasmon modes are due to local field efffects and the non-local response of the material to external electromagnetic fields, requiring a fully quantum mechanical treatment. We describe the features of these quantum plasmons, including the dispersion relation, losses and field localization. Our findings point to a strategy for fine-tuning the plasmon frequencies in graphene and other two dimensional materials.

cond-mat.mes-hall↗

Multifrequency superscattering from subwavelength hyperbolic structures

Superscattering, i.e., a phenomenon of the scattering cross section from a subwavelength object exceeding the single-channel limit, has important prospects in enhanced sensing/spectroscopy, solar cells, and biomedical imaging. Superscattering can be typically constructed only at a single frequency regime, and depends critically on the inescapable material losses. Under such realistic conditions, superscattering has not been predicted nor observed to exist simultaneously at multiple frequency regimes. Here we introduce multifrequency superscattering in a subwavelength hyperbolic structure, which can be made from artificial metamaterials or from naturally-existing materials, such as hexagonal boron nitride (BN), and show the advantage of such hyperbolic materials for reducing structural complexity. The underlying mechanism is revealed to be the multimode resonances at multiple frequency regimes as appear in BN due to the peculiar dispersion of phonon-polaritons. Importantly, the multifrequency superscattering has a high tolerance to material losses and some structural variations, bringing the concept of multifrequency superscattering closer to useful and realistic conditions.

physics.optics↗

Controlling light emission with electron wave interference

It is a long standing question whether or not one can change the nature of spontaneous emission by a free electron through shaping the electron wavefunction. On one hand, shaping the electron wavefunction changes the respective charge and current densities of the electron. On the other hand, spontaneous emission of an electron is an incoherent process and can often be insensitive to the shape of the electron wavefunction. In this work, we arrive at an affirmative answer examining Bremsstrahlung radiation by free electron superposition states. We find that the radiation can be markedly different from an incoherent sum of the radiations of the two states because of interference of the radiation amplitudes from the two components of the superposition. The ability to control free electron spontaneous emission via interference may eventually result in a new degree of control over radiation over the entire electromagnetic spectrum in addition to the ability to deterministically introduce quantum behavior into normally classical light emission processes.

quant-ph↗

Gated Orthogonal Recurrent Units: On Learning to Forget

We present a novel recurrent neural network (RNN) based model that combines the remembering ability of unitary RNNs with the ability of gated RNNs to effectively forget redundant/irrelevant information in its memory. We achieve this by extending unitary RNNs with a gating mechanism. Our model is able to outperform LSTMs, GRUs and Unitary RNNs on several long-term dependency benchmark tasks. We empirically both show the orthogonal/unitary RNNs lack the ability to forget and also the ability of GORU to simultaneously remember long term dependencies while forgetting irrelevant information. This plays an important role in recurrent neural networks. We provide competitive results along with an analysis of our model on many natural sequential tasks including the bAbI Question Answering, TIMIT speech spectrum prediction, Penn TreeBank, and synthetic tasks that involve long-term dependencies such as algorithmic, parenthesis, denoising and copying tasks.

cs.LG↗

Smith-Purcell Radiation from Low-Energy Electrons

Recent advances in the fabrication of nanostructures and nanoscale features in metasurfaces offer a new prospect for generating visible, light emission from low energy electrons. In this paper, we present the experimental observation of visible light emission from low-energy free electrons interacting with nanoscale periodic surfaces through the Smith-Purcell (SP) effect. SP radiation is emitted when electrons pass in close proximity over a periodic structure, inducing collective charge motion or dipole excitations near the surface, thereby giving rise to electromagnetic radiation. We demonstrate a controlled emission of SP light from nanoscale gold gratings with periodicity as small as 50 nm, enabling the observation of visible SP radiation by low energy electrons (1.5 to 6 keV), an order of magnitude lower than previously reported. We study the emission wavelength and intensity dependence on the grating pitch and electron energy, showing agreement between experiment and theory. Further reduction of structure periodicity should enable the production of SP-based devices that operate with even slower electrons that allow an even smaller footprint and facilitate the investigation of quantum effects for light generation in nanoscale devices. A tunable light source integrated in an electron microscope would enable the development of novel electron-optical correlated spectroscopic techniques, with additional applications ranging from biological imaging to solid-state lighting.

physics.optics↗

Spectral and spatial shaping of Smith Purcell Radiation

The Smith Purcell effect, observed when an electron beam passes in the vicinity of a periodic structure, is a promising platform for the generation of electromagnetic radiation in previously-unreachable spectral ranges. However, most of the studies of this radiation were performed on simple periodic gratings, whose radiation spectrum exhibits a single peak and its higher harmonics predicted by a well-established dispersion relation. Here, we propose a method to shape the spatial and spectral far-field distribution of the radiation using complex periodic and aperiodic gratings. We show, theoretically and experimentally, that engineering multiple peak spectra with controlled widths located at desired wavelengths is achievable using Smith-Purcell radiation. Our method opens the way to free-electron driven sources with tailored angular and spectral response, and gives rise to focusing functionality for spectral ranges where lenses are unavailable or inefficient.

physics.optics↗

Tunable UV-Emitters through Graphene Plasmons

Control over the spontaneous emission of light through tailored optical environments remains a fundamental paradigm in nanophotonics. The use of highly-confined plasmons in materials such as graphene provides a promising platform to enhance transition rates in the IR-THz by many orders of magnitude. However, such enhancements involve near-field plasmon modes or other kinds of near-field coupling like quenching, and it is challenging to use these highly confined modes to harness light in the far-field due to the difficulty of plasmonic outcoupling. Here, we propose that through the use of radiative cascade chains in multi-level emitters, IR plasmons can be used to enhance far field spectra in the visible and UV range, even at energies greater than 10 eV. Combining Purcell-enhancement engineering, graphene plasmonics, and radiative cascade can result in a new type of UV emitter whose properties can be tuned by electrically doping graphene. Varying the distance between the emitter and the graphene surface can change the strength of the far-field emission lines by two orders of magnitude. We also find that the dependence of the far-field emission on the Fermi energy is potentially extremely sharp at the onset of interband transitions, allowing the Fermi energy to effectively serve as a "switch" for turning on and off certain plasmonic and far-field emissions.

physics.optics↗

Shaping Polaritons to Reshape Selection Rules

The discovery of orbital angular momentum (OAM) in light established a new degree of freedom by which to control not only its flow but also its interaction with matter. Here, we show that by shaping extremely sub-wavelength polariton modes, for example by imbuing plasmon and phonon polariton with OAM, we engineer which transitions are allowed or forbidden in electronic systems such as atoms, molecules, and artificial atoms. Crucial to the feasibility of these engineered selection rules is the access to conventionally forbidden transitions afforded by sub-wavelength polaritons. We also find that the position of the absorbing atom provides a surprisingly rich parameter for controlling which absorption processes dominate over others. Additional tunability can be achieved by altering the polaritonic properties of the substrate, for example by tuning the carrier density in graphene, potentially enabling electronic control over selection rules. Our findings are best suited to OAM-carrying polaritonic modes that can be created in graphene, monolayer conductors, thin metallic films, and thin films of polar dielectrics such as boron nitride. By building on these findings we foresee the complete engineering of spectroscopic selection rules through the many degrees of freedom in the shape of optical fields.

physics.optics↗

Polarization state of radiation from a photonic crystal slab

We point out that the polarization state of radiation from a photonic crystal slab is strongly constrained by the direct non-resonant scattering process. The phase difference between the two linearly-polarized components in the far field can be predicted analytically and is largely independent of the periodic pattern. We verify the prediction with full-field electromagnetic simulations.

physics.optics↗

Tunable Efficient Unitary Neural Networks (EUNN) and their application to RNNs

Using unitary (instead of general) matrices in artificial neural networks (ANNs) is a promising way to solve the gradient explosion/vanishing problem, as well as to enable ANNs to learn long-term correlations in the data. This approach appears particularly promising for Recurrent Neural Networks (RNNs). In this work, we present a new architecture for implementing an Efficient Unitary Neural Network (EUNNs); its main advantages can be summarized as follows. Firstly, the representation capacity of the unitary space in an EUNN is fully tunable, ranging from a subspace of SU(N) to the entire unitary space. Secondly, the computational complexity for training an EUNN is merely $\mathcal{O}(1)$ per parameter. Finally, we test the performance of EUNNs on the standard copying task, the pixel-permuted MNIST digit recognition benchmark as well as the Speech Prediction Test (TIMIT). We find that our architecture significantly outperforms both other state-of-the-art unitary RNNs and the LSTM architecture, in terms of the final performance and/or the wall-clock training speed. EUNNs are thus promising alternatives to RNNs and LSTMs for a wide variety of applications.

cs.LG↗

Infrared Topological Plasmons in Graphene

We propose a two-dimensional plasmonic platform - periodically patterned monolayer graphene - which hosts topological one-way edge states operable up to infrared frequencies. We classify the band topology of this plasmonic system under time-reversal-symmetry breaking induced by a static magnetic field. At finite doping, the system supports topologically nontrivial bandgaps with mid-gap frequencies up to tens of terahertz. By the bulk-edge correspondence, these bandgaps host topologically protected one-way edge plasmons, which are immune to backscattering from structural defects and subject only to intrinsic material and radiation loss. Our findings reveal a promising approach to engineer topologically robust chiral plasmonic devices and demonstrate a realistic example of high-frequency topological edge state.

cond-mat.mes-hall↗

Low-loss Plasmonic Dielectric Nanoresonators

Material losses in metals are a central bottleneck in plasmonics for many applications. Here we propose and theoretically demonstrate that metal losses can be successfully mitigated with dielectric particles on metallic films, giving rise to hybrid dielectric--metal resonances. In the far field, they yield strong and efficient scattering, beyond even the theoretical limits of all-metal and all-dielectric structures. In the near field, they offer high-Purcell-factor (${>}5000$), high-quantum-efficiency (${>}90\%$), and highly directional emission at visible and infrared wavelengths. Their quality factors can be readily tailored from plasmonic-like (${\sim}10$) to dielectric-like (${\sim}10^3$), with wide control over the individual resonant coupling to photon, plasmon, and dissipative channels. Compared with conventional plasmonic nanostructures, such resonances show robustness against detrimental nonlocal effects and provide higher field enhancement at extreme nanoscopic sizes and spacings. These hybrid resonances equip plasmonics with high efficiency, which has been the predominant goal since the field's inception.

physics.optics↗

Topological magnetoplasmon

Classical wave fields are real-valued, ensuring the wave states at opposite frequencies and momenta to be inherently identical. Such a particle-hole symmetry can open up new possibilities for topological phenomena in classical systems. Here we show that the historically studied two-dimensional (2D) magnetoplasmon, which bears gapped bulk states and gapless one-way edge states near zero frequency, is topologically analogous to the 2D topological $p+\Ii p$ superconductor with chiral Majorana edge states and zero modes. We further predict a new type of one-way edge magnetoplasmon at the interface of opposite magnetic domains, and demonstrate the existence of zero-frequency modes bounded at the peripheries of a hollow disk. These findings can be readily verified in experiment, and can greatly enrich the topological phases in bosonic and classical systems.

cond-mat.mes-hall↗

Laser-Induced Linear Electron Acceleration in Free Space

Linear acceleration in free space is a topic that has been studied for over 20 years, and its ability to eventually produce high-quality, high energy multi-particle bunches has remained a subject of great interest. Arguments can certainly be made that such an ability is very doubtful. Nevertheless, we chose to develop an accurate and truly predictive theoretical formalism to explore this remote possibility in a computational experiment. The formalism includes exact treatment of Maxwell's equations, exact relativistic treatment of the interaction among the multiple individual particles, and exact treatment of the interaction at near and far field. Several surprising results emerged. For example, we find that 30 keV electrons (2.5% energy spread) can be accelerated to 7.7 MeV (2.5% spread) and to 205 MeV (0.25% spread) using 25 mJ and 2.5 J lasers respectively. These findings should hopefully guide and help develop compact, high-quality, ultra-relativistic electron sources, avoiding conventional limits imposed by material breakdown or structural constraints.

physics.acc-ph↗

Tailoring the energy distribution and loss of 2D plasmons

The ability to tailor the energy distribution of plasmons at the nanoscale has many applications in nanophotonics, such as designing plasmon lasers, spasers, and quantum emitters. To this end, we analytically study the energy distribution and the proper field quantization of 2D plasmons with specific examples for graphene plasmons. We find that the portion of the plasmon energy contained inside graphene (energy confinement factor) can exceed 50%, despite graphene being infinitely thin. In fact, this very high energy confinement can make it challenging to tailor the energy distribution of graphene plasmons just by modifying the surrounding dielectric environment or the geometry, such as changing the separation distance between two coupled graphene layers. However, by adopting concepts of parity-time symmetry breaking, we show that tuning the loss in one of the two coupled graphene layers can simultaneously tailor the energy confinement factor and propagation characteristics, causing the phenomenon of loss-induced plasmonic transparency.

physics.optics↗

Quantum corrections in nanoplasmonics: shape, scale, and material

The classical treatment of plasmonics is insufficient at the nanometer-scale due to quantum mechanical surface phenomena. Here, an extension to the classical paradigm is reported which rigorously remedies this deficiency through the incorporation of first-principles surface response functions - the Feibelman d-parameters - in general geometries. Several analytical results for the leading-order plasmonic quantum corrections are obtained in a first-principles setting; particularly, a clear separation of the roles of shape, scale, and material is established. The utility of the formalism is illustrated by the derivation of a modified sum-rule for complementary structures, a rigorous reformulation of Kreibig's phenomenological damping prescription, and an account of the small-scale resonance-shifting of simple and noble metal nanostructures. These insights open the technological design space and deepen our fundamental understanding of nanoplasmonics beyond the classical regime.

cond-mat.mes-hall↗