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Marin Soljačić

Publications and source records attributed to Marin Soljačić.

At least 145 records · Page 8Linked to original sources

Optically Thin Metallic Films for High-radiative-efficiency Plasmonics

Plasmonics enables deep-subwavelength concentration of light and has become important for fundamental studies as well as real-life applications. Two major existing platforms of plasmonics are metallic nanoparticles and metallic films. Metallic nanoparticles allow efficient coupling to far field radiation, yet their synthesis typically leads to poor material quality. Metallic films offer substantially higher quality materials, but their coupling to radiation is typically jeopardized due to the large momentum mismatch with free space. Here, we propose and theoretically investigate optically thin metallic films as an ideal platform for high-radiative-efficiency plasmonics. For far-field scattering, adding a thin high-quality metallic substrate enables a higher quality factor while maintaining the localization and tunability that the nanoparticle provides. For near-field spontaneous emission, a thin metallic substrate, of high quality or not, greatly improves the field overlap between the emitter environment and propagating surface plasmons, enabling high-Purcell (total enhancement > $10^4$), high-quantum-yield (> 50 %) spontaneous emission, even as the gap size vanishes (3$\sim$5 nm). The enhancement has almost spatially independent efficiency and does not suffer from quenching effects that commonly exist in previous structures.

physics.optics↗

Dynamical Mechanism of Two-Dimensional Plasmon Launching by Swift Electrons

Launching of surface plasmons by swift electrons has long been utilized in electron-energy-loss spectroscopy (EELS) to investigate plasmonic properties of ultrathin, or two-dimensional (2D), electron systems. However, its spatio-temporal process has never been revealed. This is because the impact of an electron will generate not only plasmons, but also photons, whose emission cannot be achieved at a single space-time point, as fundamentally determined from the uncertainty principle. Here, we propose that such a space-time limitation also applies to surface plasmon generation in EELS experiment. On the platform of graphene, we demonstrate within the framework of classical electrodynamics that the launching of 2D plasmons by an electron's impact is delayed after a hydrodynamic splashing-like process, which occurs during the plasmonic "formation time" when the electron traverses the "formation zone." Considering this newly revealed process, we show that previous estimates on the yields of graphene plasmons in EELS have been overestimated.

physics.optics↗

Formation Mechanism of Guided Resonances and Bound States in the Continuum in Photonic Crystal Slabs

We develop a formalism, based on the mode expansion method, to describe the guided resonances and bound states in the continuum (BICs) in photonic crystal slabs with one-dimensional periodicity. This approach provides analytic insights to the formation mechanisms of these states: the guided resonances arise from the transverse Fabry-Pérot condition, and the divergence of the resonance lifetimes at the BICs is explained by a destructive interference of radiation from different propagating components inside the slab. We show BICs at the center and on the edge of the Brillouin zone protected by symmetry, as well as BICs at generic wave vectors not protected by symmetry.

physics.optics↗

Fundamental limits to optical response in absorptive systems

At visible and infrared frequencies, metals show tantalizing promise for strong subwavelength resonances, but material loss typically dampens the response. We derive fundamental limits to the optical response of absorptive systems, bounding the largest enhancements possible given intrinsic material losses. Through basic conservation-of-energy principles, we derive geometry-independent limits to per-volume absorption and scattering rates, and to local-density-of-states enhancements that represent the power radiated or expended by a dipole near a material body. We provide examples of structures that approach our absorption and scattering limits at any frequency, by contrast, we find that common "antenna" structures fall far short of our radiative LDOS bounds, suggesting the possibility for significant further improvement. Underlying the limits is a simple metric, $|χ|^2 / \operatorname{Im} χ$ for a material with susceptibility $χ$, that enables broad technological evaluation of lossy materials across optical frequencies.

physics.optics↗

Power--bandwidth limitations of an optical resonance

We present shape-independent upper limits to the power--bandwidth product for a single resonance in an optical scatterer, with the bound depending only on the material susceptibility. We show that quasistatic metallic scatterers can nearly reach the limits, and we apply our approach to the problem of designing $N$ independent, subwavelength scatterers to achieve flat, broadband response even if they individually exhibit narrow resonant peaks.

physics.optics↗

An Invisible Metallic Mesh

We introduce a solid material that is itself invisible, possessing identical electromagnetic properties as air (i.e. not a cloak) at a desired frequency. Such a material could provide improved mechanical stability, electrical conduction and heat dissipation to a system, without disturbing incident electromagnetic radiation. One immediate application would be towards perfect antenna radomes. Unlike cloaks, such a transparent and self-invisible material has yet to be demonstrated. Previous research has shown that a single sphere or cylinder coated with plasmonic or dielectric layers can have a dark-state with considerably suppressed scattering cross-section, due to the destructive interference between two resonances in one of its scattering channels. Nevertheless, a massive collection of these objects will have an accumulated and detectable disturbance to the original field distribution. Here we overcome this bottleneck by lining up the dark-state frequencies in different channels. Specifically, we derive analytically, verify numerically and demonstrate experimentally that deliberately designed corrugated metallic wires can have record-low scattering amplitudes, achieved by aligning the nodal frequencies of the first two scattering channels. This enables an arbitrary assembly of these wires to be omnidirectionally invisible and the effective constitutive parameters nearly identical to air. Measured transmission spectra at microwave frequencies reveal indistinguishable results for all the arrangements of the 3D-printed samples studied.

physics.optics↗

Quantum Čerenkov Radiation: Spectral Cutoffs and the Role of Spin and Orbital Angular Momentum

We show that the well-known Čerenkov Effect contains new phenomena arising from the quantum nature of charged particles. The Čerenkov transition amplitudes allow coupling between the charged particle and the emitted photon through their orbital angular momentum (OAM) and spin, by scattering into preferred angles and polarizations. Importantly, the spectral response reveals a discontinuity immediately below a frequency cutoff that can occur in the optical region. Specifically, with proper shaping of electron beams (ebeams), we predict that the traditional Čerenkov radiation angle splits into two distinctive cones of photonic shockwaves. One of the shockwaves can move along a backward cone, otherwise considered impossible for Čerenkov radiation in ordinary matter. Our findings are observable for ebeams with realistic parameters, offering new applications including novel quantum optics sources, and open a new realm for Čerenkov detectors involving the spin and orbital angular momentum of charged particles.

quant-ph↗

Controlling Directionality and Dimensionality of Wave Propagation through Separable Bound States in the Continuum

A bound state in the continuum (BIC) is an unusual localized state that is embedded in a continuum of extended states. Here, we present the general condition for BICs to arise from wave equation separability and show that the directionality and dimensionality of their resonant radiation can be controlled by exploiting perturbations of certain symmetry. Using this general framework, we construct new examples of separable BICs in realistic models of optical potentials for ultracold atoms, photonic systems, and systems described by tight binding. Such BICs with easily reconfigurable radiation patterns allow for applications such as the storage and release of waves at a controllable rate and direction, systems that switch between different dimensions of confinement, and experimental realizations in atomic, optical, and electronic systems.

quant-ph↗

Three-dimensional topological photonic crystal with a single surface Dirac cone

A single Dirac cone on the surface is the hallmark of three-dimensional (3D) topological insulators, where the double degeneracy at the Dirac point is protected by time-reversal symmetry and the spin-splitting away from the point is provided by the spin-orbital coupling. Here we predict a single Dirac-cone surface state in a 3D photonic crystal, where the degeneracy at the Dirac point is protected by a nonsymmorphic glide reflection and the linear splitting away from it is enabled by breaking time-reversal symmetry. Such a gapless surface state is fully robust against random disorder of any type. This bosonic topological band structure is achieved by applying alternating magnetization to gap out the 3D "generalized Dirac points" discovered in the bulk of our crystal. The $Z_2$ bulk invariant is characterized through the evolution of Wannier centers. Our proposal--readily realizable using ferrimagnetic materials at microwave frequencies--can also be regarded as the photonic analog of topological crystalline insulators, providing the first 3D bosonic symmetry-protected topological system.

cond-mat.mes-hall↗

The Harper-Hofstadter Hamiltonian and conical diffraction in photonic lattices with grating assisted tunneling

We introduce a grating assisted tunneling scheme for tunable synthetic magnetic fields in photonic lattices, which can be implemented at optical frequencies in optically induced one- and two-dimensional dielectric photonic lattices. We demonstrate a conical diffraction pattern in particular realization of these lattices which possess Dirac points in $k$-space, as a signature of the synthetic magnetic fields. The two-dimensional photonic lattice with grating assisted tunneling constitutes the realization of the Harper-Hofstadter Hamiltonian.

physics.optics↗

Spawning rings of exceptional points out of Dirac cones

The Dirac cone underlies many unique electronic properties of graphene and topological insulators, and its band structure--two conical bands touching at a single point--has also been realized for photons in waveguide arrays, atoms in optical lattices, and through accidental degeneracy. Deformations of the Dirac cone often reveal intriguing properties; an example is the quantum Hall effect, where a constant magnetic field breaks the Dirac cone into isolated Landau levels. A seemingly unrelated phenomenon is the exceptional point, also known as the parity-time symmetry breaking point, where two resonances coincide in both their positions and widths. Exceptional points lead to counter-intuitive phenomena such as loss-induced transparency, unidirectional transmission or reflection, and lasers with reversed pump dependence or single-mode operation. These two fields of research are in fact connected: here we discover the ability of a Dirac cone to evolve into a ring of exceptional points, which we call an "exceptional ring." We experimentally demonstrate this concept in a photonic crystal slab. Angle-resolved reflection measurements of the photonic crystal slab reveal that the peaks of reflectivity follow the conical band structure of a Dirac cone from accidental degeneracy, whereas the complex eigenvalues of the system are deformed into a two-dimensional flat band enclosed by an exceptional ring. This deformation arises from the dissimilar radiation rates of dipole and quadrupole resonances, which play a role analogous to the loss and gain in parity-time symmetric systems. Our results indicate that the radiation that exists in any open system can fundamentally alter its physical properties in ways previously expected only in the presence of material loss and gain.

physics.optics↗

Experimental observation of Weyl points

In 1929, Hermann Weyl derived the massless solutions from the Dirac equation - the relativistic wave equation for electrons. Neutrinos were thought, for decades, to be Weyl fermions until the discovery of the neutrino mass. Moreover, it has been suggested that low energy excitations in condensed matter can be the solutions to the Weyl Hamiltonian. Recently, photons have also been proposed to emerge as Weyl particles inside photonic crystals. In all cases, two linear dispersion bands in the three-dimensional (3D) momentum space intersect at a single degenerate point - the Weyl point. Remarkably, these Weyl points are monopoles of Berry flux with topological charges defined by the Chern numbers. These topological invariants enable materials containing Weyl points to exhibit a wide variety of novel phenomena including surface Fermi arcs, chiral anomaly, negative magnetoresistance, nonlocal transport, quantum anomalous Hall effect, unconventional superconductivity[15] and others [16, 17]. Nevertheless, Weyl points are yet to be experimentally observed in nature. In this work, we report on precisely such an observation in an inversion-breaking 3D double-gyroid photonic crystal without breaking time-reversal symmetry.

cond-mat.mtrl-sci↗

Air-compatible Broadband Angular Selective Material Systems

An optical broadband angular selective filter achieved by stacking of one-dimensional photonic crystals has promising potential in various applications. In this report, we demonstrate the first experimental realization of an optical broadband angular selective filter capable of operation in air, in contrast to our previous demonstration in index matching liquid.

physics.optics↗

Optimization of sharp and viewing-angle-independent structural color

Structural coloration produces some of the most brilliant colors in nature and has many applications. However, the two competing properties of narrow bandwidth and broad viewing angle have not been achieved simultaneously in previous studies. Here, we use numerical optimization to discover geometries where a sharp 7% bandwidth in scattering is achieved, yet the peak wavelength varies less than 1%, and the peak height and peak width vary less than 6% over broad viewing angles (0--90$^\circ$) under a directional illumination. Our model system consists of dipole scatterers arranged into several rings; interference among the scattered waves is optimized to yield the wavelength-selective and angle-insensitive response. Such designs can be useful for the recently proposed transparent displays that are based on wavelength-selective scattering.

physics.optics↗

Weyl points in three-dimensional optical lattices: synthetic magnetic monopoles in momentum space

We show that Hamiltonians with Weyl points can be realized for ultracold atoms using laser-assisted tunneling in three-dimensional optical lattices. Weyl points are synthetic magnetic monopoles that exhibit a robust, three-dimensional linear dispersion. They are associated with many interesting topological states of matter, such as Weyl semimetals and chiral Weyl fermions. However, Weyl points have yet to be experimentally observed in any system. We show that this elusive goal is well-within experimental reach with an extension of the techniques recently used to obtain the Harper Hamiltonian.

cond-mat.quant-gas↗

Topological Photonics

Topology is revolutionizing photonics, bringing with it new theoretical discoveries and a wealth of potential applications. This field was inspired by the discovery of topological insulators, in which interfacial electrons transport without dissipation even in the presence of impurities. Similarly, new optical mirrors of different wave-vector space topologies have been constructed to support new states of light propagating at their interfaces. These novel waveguides allow light to flow around large imperfections without back-reflection. The present review explains the underlying principles and highlights the major findings in photonic crystals, coupled resonators, metamaterials and quasicrystals.

physics.optics↗

Binary matrices of optimal autocorrelations as alignment marks

We define a new class of binary matrices by maximizing the peak-sidelobe distances in the aperiodic autocorrelations. These matrices can be used as robust position marks for in-plane spatial alignment. The optimal square matrices of dimensions up to 7 by 7 and optimal diagonally-symmetric matrices of 8 by 8 and 9 by 9 were found by exhaustive searches.

cs.CV↗

Fundamental limits to nanoparticle extinction

We show that there are shape-independent upper bounds to the extinction cross section per unit volume of randomly oriented nanoparticles, given only material permittivity. Underlying the limits are restrictive sum rules that constrain the distribution of quasistatic eigenvalues. Surprisingly, optimally-designed spheroids, with only a single quasistatic degree of freedom, reach the upper bounds for four permittivity values. Away from these permittivities, we demonstrate computationally-optimized structures that surpass spheroids and approach the fundamental limits.

physics.optics↗