arXiv subjects

Mark F. Gyure

Publications and source records attributed to Mark F. Gyure.

15 recordsLinked to original sources

arXiv2026

Rapid Charge Stability Diagram Generation from Device-level Modeling of Semiconductor Quantum Dots

Self-consistent Schr\"odinger-Poisson calculations are a powerful tool for predicting the behavior of layered semiconductor quantum dot devices. However, characterization of charge stability diagrams through fully simulated gate-voltage sweeps is computationally expensive. Combining a Multi-Domain Multi-Model (MDMM) approach with an automated tuning routine, we identify gate voltages associated with selected charge configurations. This small set of self-consistent simulations can be augmented with Full Configuration Interaction (FCI) energy calculations to extract charging energies, lever arms, and interdot Coulomb interactions to directly parameterize a Hubbard model for rapid charge stability diagram generation. For an Intel Tunnel Falls Si/SiGe device, we demonstrate the Hubbard model's ability to reproduce charge stability diagrams at a fraction of the computational cost in comparison to voltage bias sweeps. We further compare the simulated diagrams to experimental data and demonstrate qualitative agreement. Our result represents a step towards predictive digital twin models for semiconductor quantum dot devices. Finally, we apply this workflow towards lever arm engineering in a second device, demonstrating that the method extends to multiple architectures.

cond-mat.mes-hall↗

arXiv2026

Silicon-Germanium Heterostructures with Enhanced Valley Splitting for Spin Qubits

Achieving valley splittings well in excess of the thermal energy of electrons and avoiding valley excitations is essential for the consistent initialization, operation and readout of gate-defined Si spin qubits. In this work, we present a device-level optimization strategy for pushing valley splittings to between 1 and 5 meV, well beyond values reported in nearly all previous theoretical studies. Using device-scale simulations that incorporate atomistic alloy disorder through a 1D tight-binding theory, we demonstrate that our proposed approach yields large valley splittings with a tight distribution across disorder realizations, a key requirement for reproducible qubit performance at scale. The approach rests on an unorthodox Si/SiGe heterostructure design combining a narrow quantum well, a small Ge spike, and a pure-Ge cap. We corroborate these predictions with targeted atomistic density functional theory calculations. These results offer a clear path forward for scalable Si/SiGe spin qubit devices and, if realized experimentally, effectively eliminate valley splitting as an existential problem for large scale SiGe-based quantum processors.

cond-mat.mes-hall↗

arXiv2025

Fast charge noise sensing using a spectator valley state in a singlet-triplet qubit

Semiconductor spin qubits are a promising platform for quantum computing but remain vulnerable to charge noise. Accurate, in situ measurement of charge noise could enable closed-loop control and improve qubit performance. Here, we propose a method for real-time detection of charge noise using a silicon singlet-triplet qubit with one electron initialized in an excited valley state. This valley excitation acts as a spectator degree of freedom, coupled to a high-quality resonator via the exchange interaction, which is sensitive to charge-noise-induced voltage fluctuations. Dispersive readout of the resonator enables a continuous, classical measurement of exchange fluctuations during qubit operation. Signal-to-noise analysis shows that, under realistic device parameters, sub-millisecond measurement times are possible using a quantum-limited amplifier. Even without such an amplifier, similar performance is achievable with appropriately engineered resonator parameters. This approach allows the probe to monitor slow drift in exchange in real time, opening the door to feedback and feedforward strategies for maintaining high-fidelity quantum operations. Importantly, the protocol preserves spin coherence and can be run concurrently with qubit logic gates.

cond-mat.mes-hall↗

arXiv2024

Towards Utilizing Scanning Gate Microscopy as a High-Resolution Probe of Valley Splitting in Si/SiGe Heterostructures

A detailed understanding of the material properties that affect the splitting between the two low-lying valley states in Si/SiGe heterostructures will be increasingly important as the number of spin qubits is increased. Scanning gate microscopy has been proposed as a method to measure the spatial variation of the valley splitting as a tip-induced dot is moved around in the plane of the Si quantum well. We develop a simulation using an electrostatic model of the scanning gate microscope tip and the overlapping gate structure combined with an approximate solution to the three-dimensional Schr\"odinger-Poisson equation in the device stack. Using this simulation, we show that a tip-induced quantum dot formed near source and drain electrodes can be adiabatically moved to a region far from the gate electrodes. We argue that by spatially translating the tip-induced dot across a defect in the Si/SiGe interface, changes in valley splitting can be detected.

cond-mat.mes-hall↗

arXiv2024

Proposed real-time charge noise measurement via valley state reflectometry

We theoretically propose a method to perform in situ measurements of charge noise during logical operations in silicon quantum dot spin qubits. Our method does not require ancillary spectator qubits but makes use of the valley degree of freedom in silicon. Sharp interface steps or alloy disorder in the well provide a valley transition dipole element that couples to the field of an on-chip microwave resonator, allowing rapid reflectometry of valley splitting fluctuations caused by charge noise. We derive analytic expressions for the signal-to-noise ratio that can be expected and use tight binding simulations to extract the key parameters (valley splitting and valley dipole elements) under realistic disorder. We find that unity signal-to-noise ratio can often be obtained with measurement times below 1ms, faster than typical decoherence times, opening the potential for closed-loop control, real-time recalibration, and feedforward circuits

cond-mat.mes-hall↗

arXiv2023

Multielectron dots provide faster Rabi oscillations when the core electrons are strongly confined

Increasing the number of electrons in electrostatically confined quantum dots can enable faster qubit gates. Although this has been experimentally demonstrated, a detailed quantitative understanding has been missing. Here we study one- and three-electron quantum dots in silicon/silicon-germanium heterostructures within the context of electrically-driven spin resonance (EDSR) using full configuration interaction and tight binding approaches. Our calculations show that anharmonicity of the confinement potential plays an important role: while the EDSR Rabi frequency of electrons in a harmonic potential is indifferent to the electron number, soft anharmonic confinements lead to larger and hard anharmonic confinements lead to smaller Rabi frequencies. We also confirm that double dots allow fast Rabi oscillations, and further suggest that purposefully engineered confinements can also yield similarly fast Rabi oscillations in a single dot. Finally, we discuss the role of interface steps. These findings have important implications for the design of multielectron Si/SiGe quantum dot qubits.

cond-mat.mes-hall↗

arXiv2022

Microwave-frequency scanning gate microscopy of a Si/SiGe double quantum dot

Conventional quantum transport methods can provide quantitative information on spin, orbital, and valley states in quantum dots, but often lack spatial resolution. Scanning tunneling microscopy, on the other hand, provides exquisite spatial resolution of the local electronic density of states, but often at the expense of speed. Working to combine the spatial resolution and energy sensitivity of scanning probe microscopy with the speed of microwave measurements, we couple a metallic probe tip to a Si/SiGe double quantum dot that is integrated with a local charge detector. We first demonstrate that a dc-biased tip can be used to change the charge occupancy of the double dot. We then apply microwave excitation through the scanning tip to drive photon-assisted tunneling transitions in the double dot. We infer the double dot energy level diagram from the frequency and detuning dependence of the photon-assisted tunneling resonance condition. These measurements allow us to resolve $\sim$65 $μ$eV excited states, an energy scale consistent with typical valley splittings in Si/SiGe. Future extensions of this approach may allow spatial mapping of the valley splitting in Si devices, which is of fundamental importance for spin-based quantum processors.

cond-mat.mes-hall↗

arXiv2022

High-precision real-space simulation of electrostatically-confined few-electron states

In this paper we present a computational procedure that utilizes real-space grids to obtain high precision approximations of electrostatically confined few-electron states such as those that arise in gated semiconductor quantum dots. We use the Full Configuration Interaction (FCI) method with a continuously adapted orthonormal orbital basis to approximate the ground and excited states of such systems. We also introduce a benchmark problem based on a realistic analytical electrostatic potential for quantum dot devices. We show that our approach leads to highly precise computed energies and energy differences over a wide range of model parameters. The analytic definition of the benchmark allows for a collection of tests that are easily replicated, thus facilitating comparisons with other computational approaches.

cond-mat.mes-hall↗

arXiv2020

Resonant Exchange Operation in Triple-Quantum-Dot Qubits for Spin-Photon Transduction

Triple quantum dots (TQDs) are promising semiconductor spin qubits because of their all-electrical control via fast, tunable exchange interactions and immunity to global magnetic fluctuations. These qubits can experience strong transverse interaction with photons in the resonant exchange (RX) regime, when exchange is simultaneously active on both qubit axes. However, most theoretical work has been based on phenomenological Fermi-Hubbard models, which may not fully capture the complexity of the qubit spin-charge states in this regime. Here we investigate exchange in Si/SiGe and GaAs TQDs using full configuration interaction (FCI) calculations which better describe practical device operation. We show that high exchange operation in general, and the RX regime in particular, can differ significantly from simple models, presenting new challenges and opportunities for spin-photon coupling. We highlight the impact of device electrostatics and effective mass on exchange and identify a new operating point (XRX) where strong spin-photon coupling is most likely to occur in Si/SiGe TQDs. Based on our numerical results, we analyze the feasibility of a remote entanglement cavity iSWAP protocol and discuss design pathways for improving fidelity. Our analysis provides insight into the requirements for TQD spin-photon transduction and demonstrates more generally the necessity of accurate modeling of exchange in spin qubits.

cond-mat.mes-hall↗

arXiv2017

A logical qubit in a linear array of semiconductor quantum dots

We design and analyze a logical qubit composed of a linear array of electron spins in semiconductor quantum dots. To avoid the difficulty of fully controlling a two-dimensional array of dots, we adapt spin control and error correction to a one-dimensional line of silicon quantum dots. Control speed and efficiency are maintained via a scheme in which electron spin states are controlled globally using broadband microwave pulses for magnetic resonance while two-qubit gates are provided by local electrical control of the exchange interaction between neighboring dots. Error correction with two-, three-, and four-qubit codes is adapted to a linear chain of qubits with nearest-neighbor gates. We estimate an error correction threshold of 1e-4. Furthermore, we describe a sequence of experiments to validate the methods on near-term devices starting from four coupled dots.

quant-ph↗

arXiv2014

Undoped accumulation-mode Si/SiGe quantum dots

We report on a quantum dot device design that combines the low disorder properties of undoped SiGe heterostructure materials with an overlapping gate stack in which each electrostatic gate has a dominant and unique function -- control of individual quantum dot occupancies and of lateral tunneling into and between dots. Control of the tunneling rate between a dot and an electron bath is demonstrated over more than nine orders of magnitude and independently confirmed by direct measurement within the bandwidth of our amplifiers. The inter-dot tunnel coupling at the (0,2)<-->(1,1) charge configuration anti-crossing is directly measured to quantify the control of a single inter-dot tunnel barrier gate. A simple exponential dependence is sufficient to describe each of these tunneling processes as a function of the controlling gate voltage.

cond-mat.mes-hall↗

arXiv2011

Pauli spin blockade in undoped Si/SiGe two-electron double quantum dots

We demonstrate double quantum dots fabricated in undoped Si/SiGe heterostructures relying on a double top-gated design. Charge sensing shows that we can reliably deplete these devices to zero charge occupancy. Measurements and simulations confirm that the energetics are determined by the gate-induced electrostatic potentials. Pauli spin blockade has been observed via transport through the double dot in the two electron configuration, a critical step in performing coherent spin manipulations in Si.

cond-mat.mes-hall↗

arXiv2011

Measurement of valley splitting in high-symmetry Si/SiGe quantum dots

We have demonstrated few-electron quantum dots in Si/SiGe and InGaAs, with occupation number controllable from N = 0. These display a high degree of spatial symmetry and identifiable shell structure. Magnetospectroscopy measurements show that two Si-based devices possess a singlet N =2 ground state at low magnetic field and therefore the two-fold valley degeneracy is lifted. The valley splittings in these two devices were 120 and 270 μeV, suggesting the presence of atomically sharp interfaces in our heterostructures.

cond-mat.mes-hall↗

arXiv2010

High fidelity quantum gates via dynamical decoupling

Realizing the theoretical promise of quantum computers will require overcoming decoherence. Here we demonstrate numerically that high fidelity quantum gates are possible within a framework of quantum dynamical decoupling. Orders of magnitude improvement in the fidelities of a universal set of quantum gates, relative to unprotected evolution, is achieved over a broad range of system-environment coupling strengths, using recursively constructed (concatenated) dynamical decoupling pulse sequences.

quant-ph↗

arXiv2009

Lifetime measurements (T1) of electron spins in Si/SiGe quantum dots

We have observed the Zeeman-split excited state of a spin-1/2 multi-electron Si/SiGe depletion quantum dot and measured its spin relaxation time T1 in magnetic fields up to 2 T. Using a new step-and-reach technique, we have experimentally verified the g-value of 2.0 +/- 0.1 for the observed Zeeman doublet. We have also measured T1 of single- and multi-electron spins in InGaAs quantum dots. The lifetimes of the Si/SiGe system are appreciably longer than those for InGaAs dots for comparable magnetic field strengths, but both approach one second at sufficiently low fields (< 1 T for Si, and < 0.2 T for InGaAs).

cond-mat.mes-hall↗