arXiv subjects

Mark J. H. Ku

Publications and source records attributed to Mark J. H. Ku.

17 recordsLinked to original sources

arXiv2025

Machine Learning for Improved Current Density Reconstruction from 2D Vector Magnetic Images

The reconstruction of electrical current densities from magnetic field measurements is an important technique with applications in materials science, circuit design, quality control, plasma physics, and biology. Analytic reconstruction methods exist for planar currents, but break down in the presence of high spatial frequency noise or large standoff distance, restricting the types of systems that can be studied. Here, we demonstrate the use of a deep convolutional neural network for current density reconstruction from two-dimensional (2D) images of vector magnetic fields acquired by a quantum diamond microscope (QDM) utilizing a surface layer of Nitrogen Vacancy (NV) centers in diamond. Trained network performance significantly exceeds analytic reconstruction for data with high noise or large standoff distances. This machine learning technique can perform quality inversions on lower SNR data, reducing the data collection time by a factor of about 400 and permitting reconstructions of weaker and three-dimensional current sources.

physics.comp-ph↗

arXiv2024

Diamond Micro-Chip for Quantum Microscopy

The nitrogen vacancy (NV) center in diamond is an increasingly popular quantum sensor for microscopy of electrical current, magnetization, and spins. However, efficient NV-sample integration with a robust, high-quality interface remains an outstanding challenge to realize scalable, high-throughput microscopy. In this work, we characterize a diamond micro-chip (DMC) containing a (111)-oriented NV ensemble; and demonstrate its utility for high-resolution quantum microscopy. We perform strain imaging of the DMC and find minimal detrimental strain variation across a field-of-view of tens of micrometer. We find good ensemble NV spin coherence and optical properties in the DMC, suitable for sensitive magnetometry. We then use the DMC to demonstrate wide-field microscopy of electrical current, and show that diffraction-limited quantum microscopy can be achieved. We also demonstrate the deterministic transfer of DMCs with multiple materials of interest for next-generation electronics and spintronics. Lastly, we develop a polymer-based technique for DMC placement. This work establishes the DMC's potential to expand the application of NV quantum microscopy in materials, device, geological, biomedical, and chemical sciences.

physics.app-ph↗

arXiv2023

Dressed-state control of effective dipolar interaction between strongly-coupled solid-state spins

Strong interactions between spins in many-body solid-state quantum system is a crucial resource for exploring and applying non-classical states. In particular, electronic spins associated with defects in diamond system are a leading platform for the study of collective quantum phenomena and for quantum technology applications. While such solid-state quantum defect systems have the advantage of scalability and operation under ambient conditions, they face the key challenge of controlling interactions between the defects spins, since the defects are spatially fixed inside the host lattice with relative positions that cannot be well controlled during fabrication. In this work, we present a dressed-state approach to control the effective dipolar coupling between solid-state spins; and then demonstrate this scheme experimentally using two strongly-coupled nitrogen vacancy (NV) centers in diamond. Including Rabi driving terms between the m$_s$ = 0 and $\pm$1 states in the NV spin Hamiltonian allows us to turn on and off or tune the effective dipolar coupling between two NV spins. Through Ramsey spectroscopy, we detect the change of the effective dipolar field generated by the control NV spin prepared in different dressed states. To observe the change of interaction dynamics, we then deploy spin-lock-based polarization transfer measurements via a Hartmann-Hahn matching condition between two NV spins in different dressed states. We perform simulations that indicate the promise for this robust scheme to control the distribution of interaction strengths in strongly-interacting spin systems, including interaction strength homogenization in a spin ensemble, which can be a valuable tool for studying non-equilibrium quantum phases and generating high fidelity multi-spin correlated states for quantum-enhanced sensing.

quant-ph↗

arXiv2022

Phonon-mediated strong coupling between a three-dimensional topological insulator and a two-dimensional antiferromagnetic material

Van der Waals antiferromagnetic and topological insulator materials provide powerful platforms for modern optical, electronic, and spintronic devices applications. The interaction between an antiferromagnet (AFM) and a topological insulator (TI), if sufficiently strong, could offer emergent hybrid material properties that enable new functionality exceeding what is possible in any individual material constituent. In this work, we study strong coupling between THz excitations in a three dimensional (3D) topological insulator and a quasi-two dimensional (2D) antiferromagnetic material resulting in a new hybridized mode, namely a surface Dirac plasmon-phonon-magnon polariton. We find that the interaction between a surface Dirac plasmon polariton in the 3D TI and a magnon polariton in the 2D AFM is mediated by the phonon coupling in the 3D TI material. The coupling of phonons with an electromagnetic wave propagating in the 3D TI enhances the permittivity of the TI thin film in a way that results in a strong correlation between the dispersion of Dirac plasmon polaritons on the surfaces of the TI with the thickness of the TI. As a result, the dispersion of surface Dirac plasmon polaritons in the TI can be tuned toward resonance with the magnon polariton in the AFM material by varying the TI's thickness, thereby enhancing the strength of the coupling between the excitations in the two materials. The strength of this coupling, which results in the surface Dirac plasmon-phonon-magnon polariton, can be parameterized by the amplitude of the avoided-crossing splitting between the two polariton branches at the magnon resonance frequency...

cond-mat.mes-hall↗

arXiv2022

Controllable tunability of a Chern number within the electronic-nuclear spin system in diamond

Chern numbers are gaining traction as they characterize topological phases in various physical systems. However, the resilience of the system topology to external perturbations makes it challenging to experimentally investigate transitions between different phases. In this study, we demonstrate the transitions of Chern number from 0 to 3, synthesized in an electronic-nuclear spin system associated with the nitrogen-vacancy (NV) centre in diamond. The Chern number is characterized by the number of degeneracies enclosed in a control Hamiltonian parameter sphere. The topological transitions between different phases are depicted by varying the radius and offset of the sphere. We show that the measured topological phase diagram is not only consistent with the numerical calculations but can also be mapped onto an interacting three-qubit system. The NV system may also allow access to even higher Chern numbers, which can be applied to exploring exotic topology or topological quantum information.

quant-ph↗

arXiv2022

Scanning X-ray Diffraction Microscopy for Diamond Quantum Sensing

Understanding nano- and micro-scale crystal strain in CVD diamond is crucial to the advancement of diamond quantum technologies. In particular, the presence of such strain and its characterization present a challenge to diamond-based quantum sensing and information applications -- as well as for future dark matter detectors where directional information of incoming particles is encoded in crystal strain. Here, we exploit nanofocused scanning X-ray diffraction microscopy to quantitatively measure crystal deformation from defects in diamond with high spatial and strain resolution. Combining information from multiple Bragg angles allows stereoscopic three-dimensional modeling of strain feature geometry; the diffraction results are validated via comparison to optical measurements of the strain tensor based on spin-state-dependent spectroscopy of ensembles of nitrogen vacancy (NV) centers in the diamond. Our results demonstrate both strain and spatial resolution sufficient for directional detection of dark matter via X-ray measurement of crystal strain, and provide a promising tool for diamond growth analysis and improvement of defect-based sensing.

physics.app-ph↗

arXiv2022

High-precision mapping of diamond crystal strain using quantum interferometry

Crystal strain variation imposes significant limitations on many quantum sensing and information applications for solid-state defect qubits in diamond. Thus, precision measurement and control of diamond crystal strain is a key challenge. Here, we report diamond strain measurements with a unique set of capabilities, including micron-scale spatial resolution, millimeter-scale field-of-view, and a two order-of-magnitude improvement in volume-normalized sensitivity over previous work [1], reaching $5(2) \times 10^{-8}/\sqrt{\rm{Hz}\cdot\rm{μm}^3}$ (with spin-strain coupling coefficients representing the dominant systematic uncertainty). We use strain-sensitive spin-state interferometry on ensembles of nitrogen vacancy (NV) color centers in single-crystal CVD bulk diamond with low strain gradients. This quantum interferometry technique provides insensitivity to magnetic-field inhomogeneity from the electronic and nuclear spin bath, thereby enabling long NV ensemble electronic spin dephasing times and enhanced strain sensitivity. We demonstrate the strain-sensitive measurement protocol first on a scanning confocal laser microscope, providing quantitative measurement of sensitivity as well as three-dimensional strain mapping; and second on a wide-field imaging quantum diamond microscope (QDM). Our strain microscopy technique enables fast, sensitive characterization for diamond material engineering and nanofabrication; as well as diamond-based sensing of strains applied externally, as in diamond anvil cells or embedded diamond stress sensors, or internally, as by crystal damage due to particle-induced nuclear recoils.

quant-ph↗

arXiv2022

Above-room-temperature ferromagnetism in ultrathin van der Waals magnet

Two-dimensional (2D) magnetic van der Waals materials provide a powerful platform for studying fundamental physics of low-dimensional magnetism, engineering novel magnetic phases, and enabling ultrathin and highly tunable spintronic devices. To realize high quality and practical devices for such applications, there is a critical need for robust 2D magnets with ordering temperatures above room temperature that can be created via exfoliation. Here the study of exfoliated flakes of cobalt substituted Fe5GeTe2 (CFGT) exhibiting magnetism above room temperature is reported. Via quantum magnetic imaging with nitrogen-vacancy centers in diamond, ferromagnetism at room temperature was observed in CFGT flakes as thin as 16 nm. This corresponds to one of the thinnest room-temperature 2D magnet flakes exfoliated from robust single crystals, reaching a thickness relevant to practical spintronic applications. The Curie temperature Tc of CFGT ranges from 310 K in the thinnest flake studied to 328 K in the bulk. To investigate the prospect of high-temperature monolayer ferromagnetism, Monte Carlo calculations were performed which predicted a high value of Tc ~270 K in CFGT monolayers. Pathways towards further enhancing monolayer Tc are discussed. These results support CFGT as a promising platform to realize high-quality room-temperature 2D magnet devices.

cond-mat.mtrl-sci↗

arXiv2022

Revealing room temperature ferromagnetism in exfoliated Fe$_5$GeTe$_2$ flakes with quantum magnetic imaging

Van der Waals material Fe$_5$GeTe$_2$, with its long-range ferromagnetic ordering near room temperature, has significant potential to become an enabling platform for implementing novel spintronic and quantum devices. To pave the way for applications, it is crucial to determine the magnetic properties when the thickness of Fe5GeTe2 reaches the few-layers regime. However, this is highly challenging due to the need for a characterization technique that is local, highly sensitive, artifact-free, and operational with minimal fabrication. Prior studies have indicated that Curie temperature TC can reach up to close to room temperature for exfoliated Fe$_5$GeTe$_2$ flakes, as measured via electrical transport; there is a need to validate these results with a measurement that reveals magnetism more directly. In this work, we investigate the magnetic properties of exfoliated thin flakes of van der Waals magnet Fe$_5$GeTe$_2$ via a quantum magnetic imaging technique based on nitrogen vacancy diamond. Through imaging the stray fields, we confirm room-temperature magnetic order in Fe$_5$GeTe$_2$ thin flakes with thickness down to 7 units cell. The stray field patterns and their response to magnetizing fields with different polarities point to a perpendicular easy-axis anisotropy. Furthermore, we perform imaging at different temperatures and determine the Curie temperature of the flakes at Tc~300 K. These results provide the basis for realizing a room-temperature monolayer ferromagnet with Fe$_5$GeTe$_2$. This work also demonstrates that the imaging technique enables a rapid screening of multiple flakes simultaneously, thereby paving the way towards high throughput characterization of potential 2D magnets near room temperature.

cond-mat.mes-hall↗

arXiv2021

Directional detection of dark matter with diamond

Searches for WIMP dark matter will in the near future be sensitive to solar neutrinos. Directional detection offers a method to reject solar neutrinos and improve WIMP searches, but reaching that sensitivity with existing directional detectors poses challenges. We propose a combined atomic/particle physics approach using a large-volume diamond detector. WIMP candidate events trigger a particle detector, after which spectroscopy of nitrogen vacancy centers reads out the direction of the incoming particle. We discuss the current state of technologies required to realize directional detection in diamond and present a path towards a detector with sensitivity below the neutrino floor.

physics.ins-det↗

arXiv2020

Robustness of quantized transport through edge states of finite length: Imaging current density in Floquet topological vs. quantum spin and anomalous Hall insulators

The theoretical analysis of topological insulators (TIs) has been traditionally focused on infinite homogeneous crystals with band gap in the bulk and nontrivial topology of their wavefunctions, or infinite wires whose boundaries host surface or edge metallic states. However, experimental devices contain finite-size topological region attached to normal metal (NM) leads, which poses a question about how precise is quantization of longitudinal conductance and how electrons transition from topologically trivial NM leads into the edge states. This is particularly pressing issues for recently conjectured two-dimensional (2D) Floquet TI where electrons flow from time-independent NM leads into time-dependent edge states---the very recent experimental realization of Floquet TI using graphene irradiated by circularly polarized light did not exhibit either quantized longitudinal or Hall conductance. Here we employ charge conserving solution for Floquet-nonequlibrium Green functions (NEGFs) of irradiated graphene nanoribbon to compute longitudinal two-terminal conductance, as well as spatial profiles of local current density as electrons propagate from NM leads into the Floquet TI. In the case of Floquet TI both bulk and edge local current densities contribute equally to total current, which leads to longitudinal conductance below the expected quantized plateau that is slightly reduced by edge vacancies. We propose two experimental schemes to detect coexistence of bulk and edge current densities within Floquet TI: (i) drilling a nanopore in the interior of irradiated region of graphene will induce backscattering of bulk current density, thereby reducing longitudinal conductance by $\sim 28$%; (ii) imaging of magnetic field produced by local current density using diamond NV centers.

cond-mat.mes-hall↗

arXiv2020

Imaging viscous flow of the Dirac fluid in graphene

The electron-hole plasma in charge-neutral graphene is predicted to realize a quantum critical system whose transport features a universal hydrodynamic description, even at room temperature. This quantum critical "Dirac fluid" is expected to have a shear viscosity close to a minimum bound, with an inter-particle scattering rate saturating at the Planckian time $\hbar/(k_B T)$. While electrical transport measurements at finite carrier density are consistent with hydrodynamic electron flow in graphene, a "smoking gun" of viscous behavior remains elusive. In this work, we directly image viscous Dirac fluid flow in graphene at room temperature via measurement of the associated stray magnetic field. Nanoscale magnetic imaging is performed using quantum spin magnetometers realized with nitrogen vacancy (NV) centers in diamond. Scanning single-spin and wide-field magnetometry reveals a parabolic Poiseuille profile for electron flow in a graphene channel near the charge neutrality point, establishing the viscous transport of the Dirac fluid. This measurement is in contrast to the conventional uniform flow profile imaged in an Ohmic conductor. Via combined imaging-transport measurements, we obtain viscosity and scattering rates, and observe that these quantities are comparable to the universal values expected at quantum criticality. This finding establishes a nearly-ideal electron fluid in neutral graphene at room temperature. Our results pave the way to study hydrodynamic transport in quantum critical fluids relevant to strongly-correlated electrons in high-$T_c$ superconductors. This work also highlights the capability of quantum spin magnetometers to probe correlated-electronic phenomena at the nanoscale.

cond-mat.mes-hall↗

arXiv2015

From Planar Solitons to Vortex Rings and Lines: Cascade of Solitonic Excitations in a Superfluid Fermi Gas

We follow the time evolution of a superfluid Fermi gas of resonantly interacting $^6$Li atoms after a phase imprint. Via tomographic imaging, we observe the formation of a planar dark soliton, its subsequent snaking, and its decay into a vortex ring, which in turn breaks to finally leave behind a single solitonic vortex. In intermediate stages we find evidence for an exotic structure resembling the $Φ$-soliton, a combination of a vortex ring and a vortex line. Direct imaging of the nodal surface reveals its undulation dynamics and its decay via the puncture of the initial soliton plane. The observed evolution of the nodal surface represents dynamics beyond superfluid hydrodynamics, calling for a microscopic description of unitary fermionic superfluids out of equilibrium.

cond-mat.quant-gas↗

arXiv2014

Motion of a Solitonic Vortex in the BEC-BCS Crossover

We observe a long-lived solitary wave in a superfluid Fermi gas of $^6$Li atoms after phase-imprinting. Tomographic imaging reveals the excitation to be a solitonic vortex, oriented transverse to the long axis of the cigar-shaped atom cloud. The precessional motion of the vortex is directly observed, and its period is measured as a function of the chemical potential in the BEC-BCS crossover. The long period and the correspondingly large ratio of the inertial to the bare mass of the vortex are in good agreement with estimates based on superfluid hydrodynamics that we derive here using the known equation of state in the BEC-BCS crossover.

cond-mat.quant-gas↗

arXiv2013

Heavy Solitons in a Fermionic Superfluid

Topological excitations are found throughout nature, in proteins and DNA, as dislocations in crystals, as vortices and solitons in superfluids and superconductors, and generally in the wake of symmetry-breaking phase transitions. In fermionic systems, topological defects may provide bound states for fermions that often play a crucial role for the system's transport properties. Famous examples are Andreev bound states inside vortex cores, fractionally charged solitons in relativistic quantum field theory, and the spinless charged solitons responsible for the high conductivity of polymers. However, the free motion of topological defects in electronic systems is hindered by pinning at impurities. Here we create long-lived solitons in a strongly interacting fermionic superfluid by imprinting a phase step into the superfluid wavefunction, and directly observe their oscillatory motion in the trapped superfluid. As the interactions are tuned from the regime of Bose-Einstein condensation (BEC) of tightly bound molecules towards the Bardeen-Cooper-Schrieffer (BCS) limit of long-range Cooper pairs, the effective mass of the solitons increases dramatically to more than 200 times their bare mass. This signals their filling with Andreev states and strong quantum fluctuations. For the unitary Fermi gas, the mass enhancement is more than fifty times larger than expectations from mean-field Bogoliubov-de Gennes theory. Our work paves the way towards the experimental study and control of Andreev bound states in ultracold atomic gases. In the presence of spin imbalance, the solitons created here represent one limit of the long sought-after Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state of mobile Cooper pairs.

cond-mat.quant-gas↗

arXiv2013

Collective Modes in a Unitary Fermi Gas across the Superfluid Phase Transition

We provide a joint theoretical and experimental investigation of the temperature dependence of the collective oscillations of first sound nature exhibited by a highly elongated harmonically trapped Fermi gas at unitarity, including the region below the critical temperature for superfluidity. Differently from the lowest axial breathing mode, the hydrodynamic frequencies of the higher nodal excitations show a temperature dependence, which is calculated starting from Landau two-fluid theory and using the available experimental knowledge of the equation of state. The experimental results agree with high accuracy with the predictions of theory and provide the first evidence for the temperature dependence of the collective frequencies near the superfluid phase transition.

cond-mat.quant-gas↗

arXiv2011

Revealing the Superfluid Lambda Transition in the Universal Thermodynamics of a Unitary Fermi Gas

We have observed the superfluid phase transition in a strongly interacting Fermi gas via high-precision measurements of the local compressibility, density and pressure down to near-zero entropy. Our data completely determine the universal thermodynamics of strongly interacting fermions without any fit or external thermometer. The onset of superfluidity is observed in the compressibility, the chemical potential, the entropy, and the heat capacity. In particular, the heat capacity displays a characteristic lambda-like feature at the critical temperature of $T_c/T_F = 0.167(13)$. This is the first clear thermodynamic signature of the superfluid transition in a spin-balanced atomic Fermi gas. Our measurements provide a benchmark for many-body theories on strongly interacting fermions, relevant for problems ranging from high-temperature superconductivity to the equation of state of neutron stars.

cond-mat.quant-gas↗