arXiv subjects

Mark R. Hirsbrunner

Publications and source records attributed to Mark R. Hirsbrunner.

At least 19 recordsLinked to original sources

arXiv2026

The influence of quantum geometry on the phase boundary and collective excitations of electron liquids and crystals

Recent experiments on multilayer graphene systems have reinvigorated the study of electron crystallization, now with the inclusion of quantum geometry. In this work, we apply time-dependent Hartree-Fock (TDHF) to the $λ$-jellium model to analyze the impact that quantum geometry has on the electronic liquid--crystal phase diagram and how it modifies the collective modes and responses of the liquid and crystal phases. In agreement with recent results utilizing neural quantum states, we find that quantum geometry favours electron crystallization, shifting the transition to higher densities. We also study the instabilities revealed by TDHF in the Fermi liquid ground state at low densities, providing insight into the fluctuations driving the crystallization transition. We further find that quantum geometry reduces the dispersion of the plasmon mode and suppresses Friedel oscillations deep in the liquid phase. Resolving the density response in terms of individual orbitals, we find that this suppression is caused by spectral weight transfer to an out-of-phase inter-orbital mode. Finally, we show that an analogous mode that emerges in the crystal phase corresponds to the breathing mode of an emergent real-space pseudospin skyrmion lattice.

cond-mat.mes-hall↗

arXiv2026

Quantum criticality and nonequilibrium dynamics on a Lieb lattice of Rydberg atoms

Neutral-atom quantum simulators offer a promising approach to the exploration of strongly interacting many-body systems, with applications spanning condensed matter, statistical mechanics, and high-energy physics. Through a combination of quantum experiments, numerical calculations, and analytical methods, we demonstrate a rich set of phenomena accessible on such quantum simulators by studying an array of Rydberg atoms placed on the Lieb lattice. First, we map out the ground states and phase diagram of the system, identifying a range of density-wave-ordered phases -- including a collinear phase stabilized purely by quantum fluctuations -- and find good agreement between theory and experiment. Allowing for local control of the detuning field thereafter, we discover a quantum analog of the classical liquid-vapor transition between two density-wave phases distinguished by sublattice occupation, and probe its underlying hysteretic dynamics. Furthermore, we study out-of-equilibrium quantum quenches and observe anomalously slow relaxation dynamics consistent with the kinetic constraints of an emergent string phase. These results highlight how geometric control offered by neutral-atom simulators can extend the frontiers of programmable quantum matter, enabling access to complex phases, metastability, and thermalization dynamics in many-body quantum systems.

cond-mat.quant-gas↗

arXiv2026

Elastic Response and Instabilities of Anomalous Hall Crystals

Anomalous Hall crystals (AHCs) are exotic phases of matter that simultaneously break continuous translation symmetry and exhibit the quantum anomalous Hall effect. AHCs have recently been proposed to explain the observation of an integer quantum anomalous Hall phase in a multilayer graphene system. Despite intense theoretical and experimental interest, little is known about the mechanical properties of AHCs. We study the elastic properties of AHCs first by using a continuum model with quadratic dispersion and uniform Berry curvature. We find using time-dependent Hartree-Fock that the stiffness of the AHC is an order of magnitude smaller than that of the WC, which we attribute to the finite Chern number of the AHC preventing exponential localization of the charge density. By modifying the dispersion relation to include a local minimum modeled after that of rhombohedral pentalayer graphene (R5G), we find that deformations away from the triangular lattice minimize the AHC's kinetic energy, which overwhelms the small stiffness and triggers a mechanical instability. Using a microscopic model of R5G, we observe a similar mechanical instability over an experimentally relevant parameter regime. We conclude that the topologically limited stiffness of AHCs makes them susceptible to mechanical instabilities, an important consideration when interpreting experiments in terms of AHCs.

cond-mat.str-el↗

arXiv2026

Topological phonons in anomalous Hall crystals

Recent experiments on few-layer graphene structures have reported indirect signatures of anomalous Hall crystals (AHCs), but the need for a top gate to stabilize the phase precludes direct imaging of the emergent electronic lattice. This situation necessitates the investigation of alternative signatures of AHCs. The gapless phonons of the emergent electronic lattice provide a clear distinction from conventional quantum Hall states, but it may be difficult to disentangle these phonons from the plethora of other possible low-lying modes. Intriguingly, the quantum geometry of the underlying electronic ground state can imprint on the collective modes, possibly leading the phonons themselves to be topological. Were this the case, the resulting neutral chiral edge modes would provide a further signature of an AHC. Using time-dependent Hartree-Fock, we compute the spectra of collective modes of Wigner crystals (WCs) and AHCs arising in minimal models and study the topology of the phonons and low-lying excitons. Across the WC to AHC transition, we observe a series of band inversions among collective modes, producing topological phonons and excitons, and a sharp sign change in the phonon Chern number upon entering the AHC phase. We conclude by discussing the relevance of collective mode topology to experiments on candidate systems for AHCs.

cond-mat.mes-hall↗

arXiv2025

Electronic Crystal Phases in the Presence of Non-Uniform Berry Curvature and Tunable Berry Flux: The $λ_N$-Jellium model

Recent experiments on multilayer graphene systems have rekindled interest in electronic crystal phases in two dimensions -- but now for phases enriched by non-trivial quantum geometry. In this work, we introduce a simple continuum model with tunable Berry curvature distribution and total flux, enabling systematic study of crystallization in geometrically nontrivial bands. In the noninteracting limit, the addition of a C6-symmetric periodic potential yields a rich phase diagram, for which we provide several analytical insights. Notably, we derive a general formula for the Chern number in the weak-potential regime that is broadly applicable to single-band projected models. Removing the periodic potential and treating Coulomb interactions self-consistently at the Hartree-Fock level, the resulting phase diagrams host a variety of crystalline states, including anomalous Hall crystals, halo Wigner crystals in which localized electrons spontaneously acquire orbital angular momentum leading to depleted electron occupation at the zone center, and a novel halo anomalous Hall crystal that combines these properties with a finite Chern number. We identify why these phases are energetically favorable through analytical and energetic considerations. Our results provide insight into the interplay between crystallization and band geometry, while also offering a simple toy model amenable to numerical methods beyond mean-field.

cond-mat.str-el↗

arXiv2025

Probing quantum geometry with two-dimensional nonlinear optical spectroscopy

Recent studies have shown that the nonlinear optical response of crystalline systems is fundamentally a quantum geometric property. In this work, we propose two-dimensional coherent spectroscopy (2DCS), which measures the nonlinear conductivity as a function of two independent frequencies using two time-delayed light pulses, as a probe of quantum geometry. We show how the two-frequency second-order nonlinear conductivity, which is naturally measured by 2DCS, decomposes into distinct quantum geometric contributions. We identify a term arising from the multi-band quantum connection that does not appear in linear response, and show that it can be measured in isolation by considering specific polarizations and enforcing time-reversal symmetry. We explore this finding via model calculations for transition metal dichalcogenides and Sr$_2$RuO$_4$. Through these examples, we demonstrate how 2DCS enables study of the quantum connection, providing a way to compare the quantum geometry of different materials. We also show that one can gain rough momentum-resolved knowledge of the quantum geometry by varying the chemical potential.

cond-mat.mes-hall↗

arXiv2025

Quantized crystalline-electromagnetic responses in insulators

We introduce new classes of gapped topological phases characterized by quantized crystalline-electromagnetic responses, termed "multipolar Chern insulators". These systems are characterized by nonsymmorphic momentum-space symmetries and mirror symmetries, leading to quantization of momentum-weighted Berry curvature multipole moments. We construct lattice models for such phases and confirm their quantized responses through numerical calculations. These systems exhibit bound charge and momentum densities at lattice and magnetic defects, and currents induced by electric or time-varying strain fields. Our work extends the classification of topological matter by uncovering novel symmetry-protected topological phases with quantized responses.

cond-mat.mes-hall↗

arXiv2024

Beyond MP2 initialization for unitary coupled cluster quantum circuits

The unitary coupled cluster (UCC) ansatz is a promising tool for achieving high-precision results using the variational quantum eigensolver (VQE) algorithm in the NISQ era. However, results on quantum hardware are thus far very limited and simulations have only accessed small system sizes. We advance the state of the art of UCC simulations by utilizing an efficient sparse wavefunction circuit solver and studying systems up to 64 qubits. Here we report results obtained using this solver that demonstrate the power of the UCC ansatz and address pressing questions about optimal initial parameterizations and circuit construction, among others. Our approach enables meaningful benchmarking of the UCC ansatz, a crucial step in assessing the utility of VQE for achieving quantum advantage.

quant-ph↗

arXiv2024

A circuit-generated quantum subspace algorithm for the variational quantum eigensolver

Recent research has shown that wavefunction evolution in real- and imaginary-time can generate quantum subspaces with significant utility for obtaining accurate ground state energies. Inspired by these methods, we propose combining quantum subspace techniques with the variational quantum eigensolver (VQE). In our approach, the parameterized quantum circuit is divided into a series of smaller subcircuits. The sequential application of these subcircuits to an initial state generates a set of wavefunctions that we use as a quantum subspace to obtain high-accuracy groundstate energies. We call this technique the circuit subspace variational quantum eigensolver (CSVQE) algorithm. By benchmarking CSVQE on a range of quantum chemistry problems, we show that it can achieve significant error reduction in the best case compared to conventional VQE, particularly for poorly optimized circuits, greatly improving convergence rates. Furthermore, we demonstrate that when applied to circuits trapped at a local minima, CSVQE can produce energies close to the global minimum of the energy landscape, making it a potentially powerful tool for diagnosing local minima.

quant-ph↗

arXiv2024

False vacuum decay and nucleation dynamics in neutral atom systems

Metastable states of quantum many-body systems with confinement offer a means to simulate false vacuum phenomenology, including non-equilibrium dynamical processes like decay by nucleation, in truncated limits. Recent work has examined the decay process in 1D ferromagnetic Ising spins and superfluids. In this paper, we study nucleation dynamics in 1D antiferromagnetic neutral atom chains with Rydberg interactions, using both numerical simulations and analytic modeling. We apply a staggered local detuning field to generate the metastable and ground states. Our efforts focus on two dynamical regimes: decay and annealing. In the first, we corroborate the phenomenological decay rate scaling and determine the associated parameter range for the decay process; in the second, we uncover and elucidate a procedure to anneal the metastable state from the initial to the final system, with intermediate nucleation events. We further propose experimental protocols to prepare the required states and perform quenches on near-term neutral atom quantum simulators, examining the experimental feasibility of our proposed setup and parameter regime.

quant-ph↗

arXiv2024

Long-lived oscillations of metastable states in neutral atom systems

Metastable states arise in a range of quantum systems and can be observed in various dynamical scenarios, including decay, bubble nucleation, and long-lived oscillations. The phenomenology of metastable states has been examined in quantum many-body systems, notably in 1D ferromagnetic Ising spin systems and superfluids. In this paper, we study long-lived oscillations of metastable and ground states in 1D antiferromagnetic neutral atom chains with long-range Rydberg interactions. We use a staggered local detuning field to achieve confinement. Using theoretical and numerical models, we identify novel spectral signatures of quasiparticle oscillations distinct to antiferromagnetic neutral atom systems and interpret them using a classical energy model of short-range meson repulsion. Finally, we evaluate the experimental accessibility of our proposed setup on current neutral-atom platforms and discuss experimental feasibility and constraints.

quant-ph↗

arXiv2024

Engineering quantum states with neutral atoms

Aquila, an analog quantum simulation platform developed by QuEra Computing, supports control of the position and coherent evolution of up to 256 neutral atoms. This study details novel experimental protocols designed for analog quantum simulators that generate Bell state entanglement far away from the blockade regime, construct a $Z_2$ state with a defect induced by an ancilla, and optimize the driving fields schedule to prepare excited states with enhanced fidelity. We additionally evaluate the effectiveness of readout error mitigation techniques in improving the fidelity of measurement results. All experiments were executed on Aquila from QuEra and facilitated by the AWS Braket interface. Our experimental results closely align with theoretical predictions and numerical simulations. The insights gained from this study showcase Aquila's capabilities in handling complex quantum simulations and computations, and also pave the way for new avenues of research in quantum information processing and physics that employ programmable analog hardware platforms.

quant-ph↗

arXiv2024

Crystalline axion electrodynamics in charge-ordered Dirac semimetals

Three-dimensional Dirac semimetals can be driven into an insulating state by coupling to a charge density wave (CDW) order. Here, we consider the quantized crystalline responses of such charge-ordered Dirac semimetals, which we dub Dirac-CDW insulators, in which charge is bound to disclination defects of the lattice. Using analytic and numeric methods we show the following. First, when the CDW is lattice-commensurate, disclination-line defects of the lattice have a quantized charge per length. Second, when the CDW is inversion-symmetric, disclinations of the lattice have a quantized electric polarization. Third, when the CDW is lattice-commensurate and inversion-symmetric, disclinations are characterized by a "disclination filling anomaly" -- a quantized difference in the total charge bound to disclination-lines of Dirac-CDW with open and periodic boundaries. We construct an effective response theory that captures the topological responses of the Dirac-CDW insulators in terms of a total derivative term, denoted the $R\wedge F$ term. The $R\wedge F$ term describes the crystalline analog of the axion electrodynamics that are found in Weyl semimetal-CDW insulators. We also use the crystalline responses and corresponding response theories to classify the strongly correlated topological phases of three-dimensions Dirac-semimetals.

cond-mat.str-el↗

arXiv2023

Competing Higher Order Topological Superconducting Phases in Triangular Lattice Magnet-Superconductor Hybrid Systems

We demonstrate that a plethora of higher order topological phases emerge in magnet-superconductor hybrid (MSH) systems through the interplay of a stacked magnetic structure and an underlying triangular surface lattice; the latter being of great current experimental interest. Such lattices offer the ability to create three main types of edge terminations -- called x-, y- and y'-edges -- of MSH islands that, in turn, give rise to a complex phase diagrams exhibiting various regions of HOTSC phases. We identify the single adatom chain, as well as a pair of adjacent adatom chains (called a double-chain), as the basic building blocks for the emergence of HOTSC phases. Of particular interest are those HOTSC phase which arise from a competition between the topology of single and double-chain blocks, which are absent for square latices.

cond-mat.supr-con↗

arXiv2023

Anomalous crystalline-electromagnetic responses in semimetals

We present a unifying framework that allows us to study the mixed crystalline-electromagnetic responses of topological semimetals in spatial dimensions up to $D = 3$ through dimensional augmentation and reduction procedures. We show how this framework illuminates relations between the previously known topological semimetals, and use it to identify a new class of quadrupolar nodal line semimetals for which we construct a lattice tight-binding Hamiltonian. We further utilize this framework to quantify a variety of mixed crystalline-electromagnetic responses, including several that have not previously been explored in existing literature, and show that the corresponding coefficients are universally proportional to weighted momentum-energy multipole moments of the nodal points (or lines) of the semimetal. We introduce lattice gauge fields that couple to the crystal momentum and describe how tools including the gradient expansion procedure, dimensional reduction, compactification, and the Kubo formula can be used to systematically derive these responses and their coefficients. We further substantiate these findings through analytical physical arguments, microscopic calculations, and explicit numerical simulations employing tight-binding models.

cond-mat.mes-hall↗

arXiv2023

Crystalline-electromagnetic responses of higher order topological semimetals

Previous work has shown that time-reversal symmetric Weyl semimetals with a quadrupolar arrangement of first-order Weyl nodes exhibit a mixed crystalline-electromagnetic response. For systems with higher order Weyl nodes, which are attached to both surface and hinge Fermi arcs, additional phenomena appear on surfaces of codimension $n>1$, such as electromagnetic responses of the hinges. Here we construct a model possessing a quadrupole of higher order Weyl nodes to study the interplay between higher order topology and mixed crystalline-electromagnetic responses. We show that the higher order nature of the Weyl nodes yields a dipole of Dirac nodes on certain surfaces, leading to a mixed crystalline-electromagnetic \emph{surface} response that binds charge to dislocations and momentum-density to magnetic fields. In addition, we show that the model possesses a bulk quadrupole moment of crystal-momentum that provides a link between the bulk and surface responses of the system.

cond-mat.mes-hall↗

arXiv2022

Higher Order Topological Superconductivity in Magnet-Superconductor Hybrid Systems

Quantum engineering of topological superconductors and of the ensuing Majorana zero modes might hold the key for realizing a new paradigm for the implementation of topological quantum computing and topology-based devices. Magnet-superconductor hybrid (MSH) systems have proven to be experimentally versatile platforms for the creation of topological superconductivity by custom-designing the complex structure of their magnetic layer. Here, we demonstrate that higher order topological superconductivity (HOTSC) can be realized in two-dimensional MSH systems by using stacked magnetic structures. We show that the sensitivity of the HOTSC to the particular magnetic stacking opens an unprecedented ability to tune the system between trivial and topological phases using atomic manipulation techniques. We propose that the realization of HOTSC in MSH systems, and in particular the existence of the characteristic Majorana corner modes, allows for the implementation of a measurement-based protocols for topological quantum computing.

cond-mat.supr-con↗

arXiv2022

Evidence for a robust sign-changing s-wave order parameter in monolayer films of superconducting Fe (Se,Te)/Bi2Te3

The Fe-based superconductor Fe (Se,Te) combines non-trivial topology with unconventional superconductivity and may be an ideal platform to realize exotic states such as high-order topological corner modes and Majorana modes. Thin films of Fe (Se,Te) are important for device fabrication, phase sensitive transport measurements and for realizing proposals to engineer higher-order modes. However, while bulk Fe (Se,Te) has been extensively studied with a variety of techniques, the nature of the superconducting order parameter in the monolayer limit has not yet been explored. In this work, we study monolayer films of Fe (Se,Te) on Bi2Te3 with scanning tunneling spectroscopy and Bogoliubov quasiparticle interference (BQPI). We discover that the monolayer Fe (Se,Te)/Bi2Te3 heterostructures host a robust, multigap superconducting state that strongly resembles the bulk. BQPI maps at the gap energies show a strong spatial modulation, oriented 45 degrees to the Fe-Se bond direction. Analysis of the phase-referenced quasiparticle interference signal reveals a sign-changing s-wave order parameter similar to the bulk. Moreover, we observe a unique pattern of sign changes in the BQPI signal which have not been observed in the bulk. Our work establishes monolayer Fe (Se,Te)/Bi2Te3 as a robust multi-band unconventional superconductor and sets the stage for explorations of non-trivial topology in this highly-tunable system.

cond-mat.supr-con↗