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Markku Vainio

Publications and source records attributed to Markku Vainio.

23 records · Page 2Linked to original sources

Diode-laser-pumped continuous-wave mid-infrared optical parametric oscillator

We report a singly resonant continuous-wave optical parametric oscillator (SRO), which is pumped by a semiconductor laser system and operates in the mid-infrared region (2.9 to 3.6 μm). Fast tuning of the mid-infrared output wavelength by more than 200 nm is demonstrated by scanning the pump laser wavelength through only 1.25 nm, without any need to adjust the SRO settings. The exceptionally large tuning range is obtained by choosing a pump wavelength (780 nm) that corresponds to a turning point of the group velocity mismatch between the phase-matched signal and idler waves of the SRO.

physics.optics↗

Sub-part-per-trillion level detection of hydrogen fluoride by cantilever-enhanced photo-acoustic spectroscopy

We present a highly sensitive hydrogen fluoride detector based on simple cantilever-enhanced photo-acoustic spectroscopy. A noise equivalent concentration of 5 parts-per-trillion was achieved in 1 s and 650 parts-per-quadrillion in 32 min. The limits were reached with an average optical power of 950 mW using a new continuous-wave optical parametric oscillator at 2.476 μm. The achieved normalized noise equivalent absorption coefficient was 2.7$\times$10$^{-10}$ Wcm$^{-1}$ Hz$^{-1/2}$.

physics.ins-det↗

Fully Stabilized Mid-Infrared Frequency Comb for High-Precision Molecular Spectroscopy

A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a fully stabilized near-infrared Er-doped fiber laser comb to the mid-infrared region. The method is simple, as no phase-locked loops or reference lasers are needed. Precise locking of optical frequencies of the mid-infrared comb to the pump comb is experimentally verified at sub-20 mHz level, which corresponds to a fractional statistical uncertainty of 2x10-16 at the center frequency of the mid-infrared comb. The fully stabilized mid-infrared comb is an ideal tool for high-precision molecular spectroscopy, as well as for optical frequency metrology in the mid-infrared region, which is difficult to access with other stabilized frequency comb techniques.

physics.optics↗

Spectral characterization of a frequency comb based on cascaded quadratic nonlinearities inside an optical parametric oscillator

We present an experimental study of optical frequency comb generation based on cascaded quadratic nonlinearities inside a continuous-wave-pumped optical parametric oscillator. We demonstrate comb states which produce narrow-linewidth intermode beat note signals, and we verify the mode spacing uniformity of the comb at the Hz level. We also show that spectral quality of the comb can be improved by modulating the parametric gain at a frequency that corresponds to the comb mode spacing. We have reached a high average output power of over 4 W in the near-infrared region, at ~2 μm.

physics.optics↗

Radiocarbon Dioxide detection based on Cavity Ring-Down Spectroscopy and a Quantum Cascade Laser

Monitoring of radiocarbon ($^{14}$C) in carbon dioxide is demonstrated using mid-infrared spectroscopy and a quantum cascade laser. The measurement is based on cavity ring-down spectroscopy, and a high sensitivity is achieved with a simple setup. The instrument was tested using a standardised sample containing elevated levels of radiocarbon. Radiocarbon dioxide could be detected from samples with an isotopic ratio $^{14}$C/C as low as 50 parts-per-trillion, corresponding to an activity of 5 kBq/m$^3$ in pure CO$_2$, or 2 Bq/m$^3$ in air after extraction of the CO$_2$ from an air sample. The instrument is simple, compact and robust, making it the ideal tool for on-site measurements. It is aimed for monitoring of radioactive gaseous emissions in nuclear power environment, during the operation and decommissioning of nuclear power plants. Its high sensitivity also makes it the ideal tool for the detection of leaks in radioactive waste repositories.

physics.optics↗