arXiv subjects

Masahito Mochizuki

Publications and source records attributed to Masahito Mochizuki.

At least 55 records · Page 3Linked to original sources

arXiv2023

Controllable Creation of Skyrmion Bags in a Ferromagnetic Nanodisk

Skyrmion bags are composed of an outer skyrmion and arbitrary inner skyrmions, which have recently been observed in bulk chiral magnets, but still remain elusive in magnetic films. Here, we propose a method of creating skyrmion bags in a thin-film nanodisk, which includes three steps. Firstly, the size of outer skyrmion is enlarged by a vertical magnetic field, then inner skyrmions are nucleated at an off-center area by local current injection, and the system is finally reconstructed due to multiple inter-skyrmion potentials. Thus, skyrmion bags with topological charge up to forty can be created. Simulated Lorentz transmission electron microscopy images are given to facilitate the experimental demonstration. Our proposal is expected to inspire relevant experiments in magnetic films, and pave the way for potential spintronic applications based on skyrmion bags.

cond-mat.mes-hall↗

arXiv2023

Theory of magnetic vortex crystals induced by electric dipole interactions

Recent Lorentz transmission electron microscopy experiments have revealed a variety of noncollinear spin textures including topological magnetisms such as skyrmions, biskyrmions and multiple skyrmions in thin-plate magnetic samples of e.g., perovskite manganites and hexaferrites whose crystal structures originally have spatial inversion symmety. Motivated by these experiments, we investigate a spin-lattice coupled model involving both magnetic and electric dipole interactions by the Monte Carlo technique based on the stochastic cut-off method and propose a physical mechanism for realizing topological spin textures in which the electric dipole interaction plays a key role. This mechanism is ubiquitous that stabilizes noncollinear and topological spin textures in thin-plate samples of magnetic materials.

cond-mat.str-el↗

arXiv2023

Thermoelectric effect of skyrmion crystal confined in a magnetic disk

We theoretically propose that an electric voltage can be generated by thermal gradient with a rotating skyrmion crystal confined in a magnetic disk. We find that the rotation of skyrmion crystal induced by diffusive thermal magnon currents in the presence of temperature gradient gives rise to spinmotive forces in the radial direction through coupling to conduction-electron spins. The amplitude of generated spinmotive force is larger for a larger temperature gradient at a lower temperature. The proposed phenomenon can be exploited as spintronics-based thermoelectric devices to realize the conversion of heat to electricity.

cond-mat.mes-hall↗

arXiv2023

Machine-learning detection of the Berezinskii-Kosterlitz-Thouless transition and the second-order phase transition in the XXZ models

We propose two machine-learning methods based on neural networks, which we respectively call the phase-classification method and the temperature-identification method, for detecting different types of phase transitions in the XXZ models without prior knowledge of their critical temperatures. The XXZ models have exchange couplings which are anisotropic in the spin space where the strength is represented by a parameter $Δ(>0)$. The models exhibit the second-order phase transition when $Δ>1$, whereas the Berezinskii-Kosterlitz-Thouless (BKT) phase transition when $Δ<1$. In the phase-classification method, the neural network is trained using spin or vortex configurations of well-known classical spin models other than the XXZ models, e.g., the Ising models and the XY models, to classify those of the XXZ models to corresponding phases. We demonstrate that the trained neural network successfully detects the phase transitions for both $Δ>1$ and $Δ<1$, and the evaluated critical temperatures coincide well with those evaluated by conventional numerical calculations. In the temperature-identification method, on the other hand, the neural network is trained so as to identify temperatures at which the input spin or vortex configurations are generated by the Monte Carlo thermalization. The critical temperatures are evaluated by analyzing the optimized weight matrix, which coincide with the result of numerical calculation for the second-order phase transition in the Ising-like XXZ model with $Δ=1.05$ but cannot be determined uniquely for the BKT transition in the XY-like XXZ model with $Δ=0.95$.

cond-mat.stat-mech↗

arXiv2022

Low-Energy Excitations of Skyrmion Crystals in a Centrosymmetric Kondo-Lattice Magnet: Decoupled Spin-Charge Excitations and Nonreciprocity

We theoretically study spin and charge excitations of skyrmion crystals stabilized by conduction-electron-mediated magnetic interactions via spin-charge coupling in a centrosymmetric Kondo-lattice model by large-scale spin-dynamics simulations combined with the kernel polynomial method. We reveal clear segregation of spin and charge excitation channels and nonreciprocal nature of the spin excitations governed by the Fermi-surface geometry, which are unique to the skyrmion crystals in centrosymmetric itinerant hosts and can be a source of novel physical phenomena.

cond-mat.str-el↗

arXiv2022

Photoinduced 120-degree spin order in the Kondo-lattice model on a triangular lattice

We theoretically predict the emergence of 120-degree spin order as a nonequilibrium steady state in the photodriven Kondo-lattice model on a triangular lattice. In the system away from the half filling with ferromagnetic ground state, the photoexcitation of conduction electrons and the photoinduced renormalization of bandwidth cause reconstruction of band structure and subsequent redistribution of the electrons through relaxations, which result in an electronic structure similar to that in the half-filled system at equilibrium, where the 120-degree spin order is stabilized. In this photoinduced 120-degree spin ordered phase, domains of different spin-ordered planes are formed, and vortices of spin chirality vectors called $Z_2$ vortices appear at points where multiple domains meet. We also discuss favorable conditions and experimental feasibility to observe the predicted photoinduced magnetic phase transition by investigating dependencies on the light parameters (amplitude, frequency, and polarization), the electron filling, the strength of Kondo coupling, and the effects of antiferromagnetic coupling among the localized spins. Photoinduced magnetic structures proposed so far have been limited to simple collinear (anti)ferromagnetic orders or local magnetic defects in magnets. The present work paves a way to optical creation of complex noncollinear magnetisms as global nonequilibrium steady phase in photodriven systems.

cond-mat.str-el↗

arXiv2022

Dynamical phase transitions in the photodriven charge-ordered Dirac-electron system

Photoinduced phase transitions and charge dynamics in the interacting Dirac-electron system with a charge-ordered ground state are theoretically studied by taking an organic salt $α$-(BEDT-TTF)$_2$I$_3$. By analysing the extended Hubbard model for this compound using a combined method of numerical simulations based on the time-dependent Schrödinger equation and the Floquet theory, we observe successive dynamical phase transitions from the charge-ordered insulator to a gapless Dirac semimetal and, eventually, to a Chern insulator phase under irradiation with circularly polarized light. These phase transitions occur as a consequence of two major effects of circularly polarized light, i.e., closing of the charge gap through melting the charge order and opening of the topological gap by breaking the time reversal symmetry at the Dirac points. We demonstrate that these photoinduced phenomena are governed by charge dynamics of driven correlated Dirac electrons.

cond-mat.str-el↗

arXiv2022

Predicted novel type of photoinduced topological phase transition accompanied by collision and collapse of Dirac-cone pair in organic salt $α$-(BEDT-TTF)$_2$I$_3$

Photoinduced topological phase transitions in the Dirac-electron systems have attracted intensive research interest since its theoretical prediction in graphene, where the application of circularly polarized light opens a gap at the Dirac points and renders the system a topologically nontrivial Chern insulator phase through breaking the time-reversal symmetry. However, most of the previously studied phenomena in two-dimensional Dirac systems are basically based on the same physicical mechanism, i.e., the gap opening in the Dirac electron bands with circularly polarized light, and it is lacking in variety of the physics. In this paper, we theoretically predict a novel type of photoinduced topological phase transition accompanied by collision and collapse of gapped Dirac points in the organic salt $α$-(BEDT-TTF)$_2$I$_3$. By constructing the Floquet theory for this compound, we demonstrate that the irradiation of elliptically polarized light causes collision of the Dirac points through the photoinduced band deformation and their collapse, which eventually results in the topological phase transition from a topological semimetal with gapped Dirac cones to a normal insulator when the elliptical axis is oriented at a specfic angle with respect to the crystallographic axes. We argue that this novel photoinduced phase transition can be experimentally detected by the measurement of Hall conductivity. The present work enriches the fundamental physics of photoinduced topological phase transitions and thus contribute to development of this rapidly growing research field.

cond-mat.str-el↗

arXiv2022

Reservoir Computing with Spin Waves in Skyrmion Crystal

Magnetic skyrmions are nanometric spin textures characterized by a quantized topological invariant in magnets and often emerge in a crystallized form called skyrmion crystal in an external magnetic field. We propose that magnets hosting a skyrmion crystal possess high potential for application to reservoir computing, which is one of the most successful information processing techniques inspired by functions of human brains. Our skyrmion-based reservoir exploits precession dynamics of magnetizations, i.e., spin waves, propagating in the skyrmion crystal. Because of complex interferences and slow relaxations of the spin-wave dynamics, the skyrmion spin-wave reservoir attains several important characteristics required for reservoir computing, e.g., the generalization ability, the nonlinearity, and the short-term memory. We investigate these properties by imposing three standard tasks to test the performances of reservoir, i.e., the duration-estimation task, the short-term memory task, and the parity-check task. Through these investigations, we demonstrate that magnetic skyrmion crystals are promising materials for spintronics reservoir devices. Because magnetic skyrmions emerge spontaneously in magnets via self-organization process under application of a static magnetic field, the proposed skyrmion reservoir requires neither advanced nanofabrication nor complicated manufacturing for production in contrast to other previously proposed magnetic reservoirs constructed with fabricated spintronics devices. Our proposal is expected to realize a breakthrough in the research of spintronics reservoirs of high performance.

cond-mat.mes-hall↗

arXiv2021

Dynamical Switching of Magnetic Topology in Microwave-Driven Itinerant Magnet

We theoretically demonstrate microwave-induced dynamical switching of magnetic topology in centrosymmetric itinerant magnets by taking the Kondo-lattice model on a triangular lattice, which is known to exhibit two types of skyrmion lattices with different magnetic topological charges of |Nsk| = 1 and 2. Our numerical simulations reveal that intense excitation of a resonance mode with circularly polarized microwave field can switch the magnetic topology, i.e., from the skyrmion lattice with |Nsk| = 1 to another skyrmion lattice with |Nsk| = 2 or to a nontopological magnetic order with |Nsk| = 0 depending on the microwave frequency. This magnetic-topology switching shows various distinct behaviors, that is, deterministic irreversible switching, probabilistic irreversible switching, and temporally random fluctuation depending on the microwave frequency and the strength of the external magnetic field, the variety of which is attributable to different energy landscapes in the dynamical regime. The obtained results are also discussed in the light of time-evolution equations based on an effective model derived using perturbation expansions.

cond-mat.str-el↗

arXiv2021

Proposed Negative Thermal Expansion in Honeycomb-Lattice Antiferromagnets

We theoretically propose possible magnetism-induced negative thermal expansion in honeycomb-lattice antiferromagnets with edge-sharing networks of $MX_6$ octahedra where $M$ and $X$ are transition-metal and ligand ions, respectively. In this crystal structure, the nearest-neighbor exchange interaction is composed of two competing contributions, i.e., the antiferromagnetic contribution from a direct 180$^\circ$ $M$-$M$ bond and the ferromagnetic contribution from 90$^\circ$ $M$-$X$-$M$ bonds, amplitudes of which have different bond-length dependence. Numerical analysis of the spin-lattice model of the honeycomb-lattice antiferromagnets demonstrates that the negative thermal expansion can occur when the system enters the antiferromagnetic phase with lowering temperature so as to maximize the energy gain associated with the bond-length dependent antiferromagnetic exchange interaction. The present work provides a guiding principle for searching new materials and eventually contributes to diversify the family of materials that host the negative thermal expansion originating from the spin-lattice coupling on the honeycomb lattices or related crystal structures.

cond-mat.str-el↗

arXiv2021

Predicted photoinduced pair annihilation of emergent magnetic charges in the organic salt $α$-(BEDT-TTF)$_2$I$_3$ irradiated by linearly polarized light

Prolonged experimental attempts to find magnetic monopoles (i.e., elementary particles with an isolated magnetic charge in three dimensions) have not yet been successful despite intensive efforts made since Dirac's proposal in 1931. Particle physicists have predicted the possible collision and pair annihilation of two magnetic charges with opposite signs. However, if such annihilation exists, its experimental observation would be difficult because its energy scale is predicted to be tremendously high ($\sim$10$^{16}$ GeV). In the present work, we theoretically predict using the Floquet theory that a pair of slightly gapped Dirac-cone bands in a weakly-charge-ordered organic conductor $α$-(BEDT-TTF)$_2$I$_3$, which behave as magnetic charges with opposite signs in the momentum space, exhibit pair annihilation under irradiation with linearly polarized light. This photoinduced pair annihilation is accompanied by a non-topological phase transition to the Floquet normal insulator phase in contrast to the well-known circularly-polarized-light-induced topological phase transition to the Floquet Chern insulator phase. We discuss that $α$-(BEDT-TTF)$_2$I$_3$ has a peculiar band structure capable of realizing a suitable experimental condition (i.e., off-resonant condition) and a charge ordered state providing a required staggered site potential and thereby provides a rare example of materials that can be used to observe the predicted pair annihilation phenomenon. The feasibility of experimental observation is also discussed.

cond-mat.str-el↗

arXiv2021

Machine-learning detection of the Berezinskii-Kosterlitz-Thouless transitions in the q-state clock models

We demonstrate that a machine learning technique with a simple feedforward neural network can sensitively detect two successive phase transitions associated with the Berezinskii-Kosterlitz-Thouless (BKT) phase in q-state clock models simultaneously by analyzing the weight matrix components connecting the hidden and output layers. We find that the method requires only a data set of the raw spatial spin configurations for the learning procedure. This data set is generated by Monte-Carlo thermalizations at selected temperatures. Neither prior knowledge of, for example, the transition temperatures, number of phases, and order parameters nor processed data sets of, for example, the vortex configurations, histograms of spin orientations, and correlation functions produced from the original spin-configuration data are needed, in contrast with most of previously proposed machine learning methods based on supervised learning. Our neural network evaluates the transition temperatures as T_2/J=0.921 and T_1/J=0.410 for the paramagnetic-to-BKT transition and BKT-to-ferromagnetic transition in the eight-state clock model on a square lattice. Both critical temperatures agree well with those evaluated in the previous numerical studies.

cond-mat.stat-mech↗

arXiv2021

Floquet theory of photoinduced topological phase transitions in the organic salt $α$-(BEDT-TTF)$_2$I$_3$ irradiated with elliptically polarized light

We theoretically investigate possible photoinduced topological phase transitions in the organic salt $α$-(BEDT-TTF)$_2$I$_3$, which possesses a pair of inclined massless Dirac-cone bands between the conduction and valence bands under uniaxial pressure. The Floquet analyses of a driven tight-binding model for this material reveal rich photoinduced variations of band structures, Chern numbers, and Hall conductivities under irradiation with elliptically polarized light. The obtained phase diagrams contain a variety of nonequilibrium steady phases, e.g., the Floquet Chern insulator, Floquet semimetal, and Floquet normal insulator phases. This work widens a scope of target materials for research on photoinduced topological phase transitions and contributes to development of research on the optical manipulations of electronic states in matters.

cond-mat.str-el↗

arXiv2021

Real-time dynamics of the photoinduced topological state in organic conductor $α$-(BEDT-TTF)$_2$I$_3$ under continuous-wave and pulse excitations

We theoretically study the real-time dynamics of the photoinduced topological phase transition to a nonequilibrium Floquet Chern insulator in an organic conductor $α$-(BEDT-TTF)$_2$I$_3$, which was recently predicted using the Floquet theory. By using a tight-binding model of $α$-(BEDT-TTF)$_2$I$_3$ that hosts a pair of tilted Dirac-cone bands at the Fermi level, we solve the time-dependent Schrödinger equation and obtained time evolutions of physical quantities for continuous-wave and pulse excitations with circularly polarized light. We demonstrate that, for the continuous-wave excitations, time profiles of the Chern number and the Hall conductivity show indications of the Floquet topological insulator. We argue that the Hall conductivity exhibits a slow oscillation with its frequency corresponding to a photoinduced direct gap determined by the Floquet band structure. With pulse excitations, transient excitation spectra are obtained, from which we infer the formation of Floquet bands and the gap opening at the Dirac point during the pulse irradiation. This dynamical gap formation is also manifested by the slow oscillation component of the Hall conductivity; that is, its frequency increases with time toward the pulse peak at which it nearly coincides with the photoinduced direct gap. The relevance of the results to experiments is also discussed.

cond-mat.str-el↗

arXiv2020

Theory of the Inverse Faraday Effect due to the Rashba Spin-Oribt Interactions: Roles of Band Dispersions and Fermi Surfaces

We theoretically study the inverse Faraday effect, i.e., the optical induction of spin polarization with circularly polarized light, by particularly focusing on effects of band dispersions and Fermi surfaces in crystal systems with the spin-orbit interaction (SOI). By numerically solving the time-dependent Schrödinger equation of a tight-binding model with the Rashba-type SOI, we reproduce the light-induced spin polarization proportional to $E_0^2/ω^3$ where $E_0$ and $ω$ are the electric-field amplitude and the angular frequency of light, respectively. This optical spin induction is attributed to dynamical magnetoelectric coupling between the light electric field and the electron spins mediated by the SOI. We elucidate that the magnitude and sign of the induced spin polarization sensitively depend on the electron filling. To understand these results, we construct an analytical theory based on the Floquet theorem. The theory successfully explains the dependencies on $E_0$ and $ω$ and ascribes the electron-filling dependence to a momentum-dependent effective magnetic field governed by the Fermi-surface geometry. Several candidate materials and experimental conditions relevant to our theory and model parameters are also discussed. Our findings will enable us to engineer the magneto-optical responses of matters via tuning the material parameters.

cond-mat.str-el↗

arXiv2020

Predicted Photo-Induced Topological Phases in Organic Salt $α$-(BEDT-TTF)$_2$I$_3$

The emergence of photo-induced topological phases and their phase transitions are theoretically predicted in organic salt $α$-(BEDT-TTF)$_2$I$_3$, which possesses inclined Dirac cones in its band structure. By analyzing a photo-driven tight-binding model describing conduction electrons in the BEDT-TTF layer using the Floquet theorem, we demonstrate that irradiation with circularly polarized light opens a gap at the Dirac points, and the system eventually becomes a Chern insulator characterized by a quantized topological invariant. A rich phase diagram is obtained in plane of amplitude and frequency of light, which contains Chern insulator, semimetal, and normal insulator phases. We find that the photo-induced Hall conductivity provides a sensitive means to detect the predicted phase evolutions experimentally. This work contributes towards developing the optical manipulation of electronic states in matter through broadening the range of target materials that manifest photo-induced topological phase transitions.

cond-mat.str-el↗

arXiv2020

Creation of nanometric magnetic skyrmions by global application of circularly polarized microwave magnetic field

From a theoretical perspective, we demonstrate that nanometric magnetic skyrmions are created by application of a circularly polarized microwave magnetic field to a thin-plate Dzyaloshinskii-Moriya ferromagnet with fabricated rectangular holes. This phenomenon is caused by an effective steady magnetic field perpendicular to the microwave-polarization plane induced by the rotating magnetic field and the intense interference of spin waves excited by this magnetic field due to the hole structure, which causes reversals of local magnetizations and results in the formation of skyrmions. Our proposal provides a new option to write or create magnetic textures the sizes of which are much smaller than the spot size of the external stimulus such as magnetic field, light, and microwave.

cond-mat.mes-hall↗