arXiv subjects

Masato Takiguchi

Publications and source records attributed to Masato Takiguchi.

11 recordsLinked to original sources

arXiv2026

Non-Centrosymmetric $\gamma$-Phase GaS Nanobelts for On-Chip Nonlinear Photonic Applications

Second-order nonlinear optical processes in van der Waals (vdW) semiconductors offer a compelling route toward compact, integrable photon-conversion platforms. Among III-VI vdW semiconductors, GaS is particularly attractive owing to its wide bandgap suppressing two-photon absorption under near-infrared laser excitation. However, bulk GaS typically crystallizes in the centrosymmetric $\beta$ phase, which eliminates second-order nonlinearity and severely limits its application in nonlinear photonics. Here, we demonstrate that GaS nanobelts synthesized via self-catalyzed vapor-liquid-solid growth predominantly crystallize in non-centrosymmetric $\gamma$-phase stacking. This behavior originates from edge-selective growth kinetics at the Ga catalyst interface, which stabilizes the $\gamma$ phase and enables deterministic in-plane dipole moment alignment. The GaS nanobelts exhibit strong second-harmonic generation (SHG) with intensities comparable to those of GaSe, a widely used nonlinear optical material. Furthermore, we integrate the nanobelts onto SiN waveguides and demonstrate efficient on-chip SHG and sum-frequency generation. These results establish $\gamma$-GaS nanobelts as a transferable one-dimensional nonlinear materials well suited for on-chip photonic integration and indicate their strong potential for nonlinear optical applications.

physics.optics↗

arXiv2025

Inverse-Designed Non-Hermitian Hollow Nanowire Cavity for Generating Optical Orbital Angular Momentum

We designed a gallium nitride hexagonal hollow nanowire whispering gallery mode cavity that generates an |m|=6 topological light with orbital angular momentum (OAM). OAM is generated by breaking the cross-sectional mirror symmetry of the nanowire, which creates a non-Hermitian system. This is achieved by replacing the central airhole of the hollow nanowire with a cluster of 6 overlapping circular air holes with rotational offset relative to the hexagonal cross-sectional profile of the nanowire. The design parameters were then further optimized in Finite Element Method using an inverse design method to maximize the normalized OAM order |l|. We were able to realize of a cavity mode with |l| = 5.7, a mode purity of about 97%, and a Q-factor of ~250. This marks the first OAM generating active photonic device design falling within a sub-micron footprint, with additional novelties of being single component and materialistically homogeneous.

physics.optics↗

arXiv2025

On-chip room-temperature CW lasing from a III-V nanowire integrated with a Si photonic crystal platform

We report the demonstration of continuous-wave (CW) lasing at room temperature from a III-V semiconductor nanowire integrated into a Si photonic crystal (PhC) cavity. Conventional hybrid nanowire lasers [M. Takiguchi. et.al., APL Photonics, 2, 046106 (2017)], which typically feature circular nanowire-cross-sections, suffer from a weak optical confinement, preventing CW lasing under ambient conditions. To overcome this limitation, we fabricated nanowires with rectangular cross-sections via dry etching and integrated them into the air trenches of Si PhC cavities formed using atomic force microscope tips. This configuration forms a hybrid photonic crystal cavity with an improved optical confinement. As a result, we achieved room-temperature CW oscillation from a single nanowire, representing a significant step toward on-chip nanophotonic light sources. This unique in-plane integration of the nanolaser in the same plane as the Si slab rather than on top of the substrate will contribute to the development of compact, scalable, and CMOS-compatible photonic circuits.

physics.optics↗

arXiv2025

Chiral Diffraction from Aperiodic Monotile Lattice

Aperiodic systems such as quasiperiodic systems exhibit unique properties different from periodic structures. In 2023, Smith et al. discovered a new aperiodic structure: a single-shaped tile that can only tile space aperiodically, known as an aperiodic monotile. Although the aperiodic monotile possesses intriguing mathematical properties, its experimental investigation remains unexplored. In this study, we report an experimental investigation of diffraction patterns from a monotile lattice using a nanophotonic platform. We observed clear Bragg peaks, which is evidence of long-range order and a chiral structure of the diffraction patterns. Furthermore, we found exotic behavior in circular polarization dependence, which cannot be observed in conventional quasiperiodic structures. These findings establish the monotile lattice as a novel class of aperiodic systems, expanding the study of nonperiodic structures beyond conventional quasicrystals.

physics.optics↗

arXiv2023

Vector beam generation from standing hollow GaN nanowire lasers on sapphire substrate

We fabricated GaN based hollow nanowires standing upright on a sapphire substrate by the sublimation method and found that they exhibit laser oscillation at room temperature. These very long, hollow, nano-sized structures cannot be fabricated by other means. Furthermore, we determined the condition under which the fundamental mode is azimuthally polarized by investigating the dispersion of the hollow structure. Examination of the measured emission properties indicates that the hollow nanowire operates as a topological, vector-beam, light source.

physics.optics↗

arXiv2020

Emulating the local Kuramoto model with an injection-locked photonic crystal laser array

The Kuramoto model is a mathematical model for describing the collective synchronization phenomena of coupled oscillators. We theoretically demonstrate that an array of coupled photonic crystal lasers emulates the Kuramoto model with non-delayed nearest-neighbor coupling (the local Kuramoto model). Our novel strategy employs indirect coupling between lasers via additional cold cavities. By installing cold cavities between laser cavities, we avoid the strong coupling of lasers and realize ideal mutual injection-locking with effective non-delayed dissipative coupling. First, after discussing the limit cycle interpretation of laser oscillation, we demonstrate the synchronization of two indirectly coupled lasers by numerically simulating coupled-mode equations. Second, by performing a phase reduction analysis, we show that laser dynamics in the proposed device can be mapped to the local Kuramoto model. Finally, we briefly demonstrate that a chain of indirectly coupled photonic crystal lasers actually emulates the one-dimensional local Kuramoto chain. We also argue that our proposed structure, which consists of periodically aligned cold cavities and laser cavities, will best be realized by using state-of-the-art buried multiple quantum well photonic crystals.

physics.optics↗

arXiv2020

Designs toward synchronization of optical limit cycles with coupled silicon photonic crystal microcavities

A driven high-Q Si microcavity is known to exhibit limit cycle oscillation originating from carrier-induced and thermo-optic nonlinearities. We propose a novel nanophotonic device to realize synchronized optical limit cycle oscillations with coupled silicon (Si) photonic crystal (PhC) microcavities. Here, coupled limit cycle oscillators are realized by using coherently coupled Si PhC microcavities. By simulating coupled-mode equations, we theoretically demonstrate mutual synchronization (entrainment) of two limit cycles induced by coherent coupling. Furthermore, we interpret the numerically simulated synchronization in the framework of phase description. Since our proposed design is perfectly compatible with current silicon photonics fabrication processes, the synchronization of optical limit cycle oscillations will be implemented in future silicon photonic circuits.

physics.optics↗

arXiv2019

Probing the Ginzburg-Landau Potential for Lasers Using Higher-order Photon Correlations

Lasing transition is known to be analogous to the second-order phase transition. Furthermore, for some cases, it is possible to define the Ginzburg-Landau (GL) potential, and the GL theory predicts the photon statistical properties of lasers. However, the GL potential for lasers is surprising, because lasers are operating far from equilibrium. In this paper, we theoretically examine the validity of the GL theory for lasers in terms of various parameters, particularly, the ratio between photon and carrier lifetimes. For this purpose, we use stochastic rate equations and higher-order photon correlation functions. With higher-order photon correlation measurements, we can check whether or not laser dynamics are described by the GL theory. We demonstrate that, for low-$\beta$ lasers, the GL theory is applicable even when the photon lifetime is comparable to the carrier lifetime and that photon-carrier relaxation oscillation is the fundamental origin of the breakdown of the GL theory, which can be understood in the framework of center manifold reduction.

cond-mat.mes-hall↗

arXiv2019

Low- and high-$\beta$ lasers in Class-A limit: photon statistics, linewidth, and the laser-phase transition analogy

Nanocavity lasers are commonly characterized by the spontaneous coupling coefficient $\beta$ that represents the fraction of photons emitted into the lasing mode. While $\beta$ is conventionally discussed in semiconductor lasers where the photon lifetime is much shorter than the carrier lifetime (class-B lasers), little is known about $\beta$ in atomic lasers where the photon lifetime is much longer than the other lifetimes and only the photon degree of freedom exists (class-A lasers). We investigate the impact of the spontaneous coupling coefficient $\beta$ on lasing properties in the class-A limit by extending the well-known Scully-Lamb master equation. We demonstrate that, in the class-A limit, all the photon statistics are uniquely characterized by $\beta$ and that the laser phase transition-like analogy becomes transparent. In fact, $\beta$ perfectly represents the "system size" in phase transition. Finally, we investigate the laser-phase transition analogy from the standpoint of a quantum dissipative system. Calculating a Liouvillian gap, we clarify the relation between $\beta$ and the continuous phase symmetry breaking.

cond-mat.mes-hall↗

arXiv2019

All-optical dynamic modulation of spontaneous emission rate in hybrid optomechanical cavity quantum electrodynamics systems

Recent nanofabrication technologies have miniaturized optical and mechanical resonators, and have led to a variety of novel optomechanical systems in which optical and mechanical modes are strongly coupled. Here we hybridize an optomechanical resonator with two-level emitters and successfully demonstrate all-optical dynamic control of optical transition in the two-level system by the mechanical oscillation via the cavity quantum-electrodynamics (CQED) effect. Employing copper-doped silicon nanobeam optomechanical resonators, we have observed that the spontaneous emission rate of excitons bound to copper atoms is dynamically modulated by the optically-driven mechanical oscillation within the time scale much shorter than the emission lifetime. The result is explained very well with an analytical model including the dynamic modulation of the Purcell effect and the exciton population. To the best of our knowledge, this is the first demonstration of a dynamic modulation of the spontaneous emission rate by mechanical oscillations. Our achievement will open up a novel field of hybrid optomechanical CQED systems in which three body--optical transitions, optical resonance modes, and mechanical resonance modes--are strongly coupled and will pave the way for novel hybrid quantum systems.

physics.optics↗

arXiv2016

Continuous-wave operation and 10-Gb/s direct modulation of InAsP/InP sub-wavelength nanowire laser on silicon photonic crystal

We demonstrated sub-wavelength (~111 nm diameter) single nanowire (NW) continuous wave (CW) lasers on silicon photonic crystal in the telecom-band with direct modulation at 10 Gb/s by optical pumping at cryogenic temperatures. To estimate the small signal response and pseudo-random bit sequence (PRBS) modulation of our CW lasers, we employed a new signal detection technique that employs a superconducting single photon detector and a time-correlated single photon counting module. The results showed that our NW laser was unambiguously modulated at above 10 Gb/s and an open eye pattern was obtained. This is the first demonstration of a telecom-band CW NW laser with high-speed PRBS modulation.

physics.optics↗