Searcharxiv⌕ Search

arXiv subjects

Matthew J. Olszta

Publications and source records attributed to Matthew J. Olszta.

4 recordsLinked to original sources

Voltage-tunable Josephson Junctions on Germanium Quantum Wells with in-situ Aluminum Contacts

Voltage-tunable Josephson junctions (VT-JJs) are an emerging element in superconducting quantum electronics with potential to expand the functionality of conventional designs. While VT-JJs are largely compatible with wafer-scale semiconductor processing, their integration into quantum circuits remains a challenge due to unmitigated semiconductor microwave loss. Here, a deep mesa etch process, wherein the epitaxial material is removed except the VT-JJ device, will facilitate the integration of VT-JJs with low-microwave-loss circuit elements by allowing these circuit elements to be placed directly on a low-loss substrate. A Germanium quantum well is grown by Molecular Beam Epitaxy (MBE) on a float zone silicon substrate with in-situ deposited aluminum contacts. This combination allows the formation of an oxide-free superconductor-semiconductor interface. The deep mesa etch process is optimized to produce a sidewall taper sufficient for continuous metal deposition from the substrate to the top of the mesa for electrostatic gate electrodes and interconnects. The fabricated Josephson junctions demonstrate gate-tunable supercurrents with a maximum critical current over 100 nA and critical-current normal-resistance product of $8.63~μV$. These results demonstrate a pathway toward improved integration of voltage-tunable superconducting circuit elements with quantum electronic building blocks such as couplers and qubits.

cond-mat.mes-hall↗

Born-Qualified: An Autonomous Framework for Deploying Advanced Energy and Electronic Materials

Autonomous science is transforming how we discover materials and chemical systems for advanced energy technologies. However, many initially promising systems never reach deployment. This "valley of death" stems from optimization that prioritizes laboratory metrics over industrial viability. We propose a new strategy: "born-qualified" autonomous development, which embeds manufacturability, cost, and durability constraints from the outset. This approach is enabled by four pillars, including the development of multi-objective metrics, causal models, a modular infrastructure, and embedding manufacturing in the discovery loop. Realizing this vision will require sustained, community-wide commitment, but the potential return on that investment is commensurate with the scale of the challenge.

cond-mat.mtrl-sci↗

Mind the Gap: Bridging the Divide Between AI Aspirations and the Reality of Autonomous Characterization

What does materials science look like in the "Age of Artificial Intelligence?" Each materials domain-synthesis, characterization, and modeling-has a different answer to this question, motivated by unique challenges and constraints. This work focuses on the tremendous potential of autonomous characterization within electron microscopy. We present our recent advancements in developing domain-aware, multimodal models for microscopy analysis capable of describing complex atomic systems. We then address the critical gap between the theoretical promise of autonomous microscopy and its current practical limitations, showcasing recent successes while highlighting the necessary developments to achieve robust, real-world autonomy.

cond-mat.mtrl-sci↗

One Dimensional Wormhole Corrosion in Metals

Corrosion is a ubiquitous failure mode of materials in extreme environments. The more localized it is, the more difficult it is to detect and more deleterious its effects. Often, the progression of localized corrosion is accompanied by the evolution of porosity in materials, creating internal void-structures that facilitate the ingress of the external environment into the interior of the material, further accelerating the internal corrosion. Previously, the dominant morphology of such void-structures has been reported to be either three-dimensional (3D) or two-dimensional (2D). Here, we report a more localized form of corrosion, which we call 1D wormhole corrosion. Using electron tomography, we show multiple examples of this 1D and percolating morphology that manifests a significantly high aspect ratio differentiable from 2D and 3D corrosion. To understand the origin of this mechanism in a Ni-Cr alloy corroded by molten salt, we combined energy-filtered four-dimensional scanning transmission electron microscopy (EF-4D-STEM) and ab initio density functional theory (DFT) calculations to develop a vacancy mapping method with nanometer-resolution, identifying a remarkably high vacancy concentration in the diffusion-induced grain boundary migration (DIGM) zone, up to 100 times the equilibrium value at the melting point. These vacancy supersaturation regions act as the precursors of wormholes, and lead to the asymmetrical growth of voids along GBs. We show that similar 1D penetrating corrosion morphologies could also occur in other materials or corrosion conditions, implying the broad impact of this extremely localized corrosion mechanism. Deciphering the origins of 1D corrosion is an important step towards designing structural materials with enhanced corrosion resistance, and also offers new pathways to create ordered-porous materials for functional applications.

cond-mat.mtrl-sci↗