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Matthias C. Löbl

Publications and source records attributed to Matthias C. Löbl.

At least 19 recordsLinked to original sources

Purification of photonic graph states

Graph states constitute the main building block for quantum computing with photons. Quantum emitters with a hosted spin can deterministically generate photonic graph states, strongly lowering the overhead of multiplexing highly probabilistic linear-optics graph state generation. However, they generally suffer from various noise sources, resulting in reduced fidelities of the produced states. To mitigate this issue, we develop purification schemes for entangled photonic states. We first develop purification schemes to purify arbitrary photonic GHZ and other CSS states, which we generalize to all photonic graph states and stabilizer states. The proposed purification schemes have a high success probability of up to $1/2$ and require only linear optics and photon detectors. We optimize cascaded purification schemes for various graph states, taking into account phenomenological Pauli errors or physical noise in time-bin-encoded graph state generation with quantum emitters.

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The subthreshold issue of fusion-based quantum computing

Fusion-based quantum architectures are the leading approach to photonic quantum computing. However, the sub-threshold regime, where logical error rates must reach the levels required by useful applications, has received little attention. We show that in this regime, fusion failure imposes a noise floor on the logical error rate that prevents all-linear-optics architectures from reaching the required rates at low overhead. For fusion-based architectures using quantum emitter spins, we show that the noise floor is reduced by orders of magnitude at a lower overhead.

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Fusion-based implementation of qLDPC codes with quantum emitters

Quantum low-density parity check (qLDPC) codes offer higher encoding rate than topological codes, e.g. surface codes, making them favourable for practical, fault-tolerant quantum computing with low overhead. These codes are particularly well-suited for fusion-based photonic implementations as this platform readily supports non-local connections. We propose an architecture specifically tailored to quantum emitters which can implement any Calderbank-Shor-Steane (CSS) qLDPC code. In this architecture, the photonic resource states are deterministically produced via quantum emitters and a conditional repeat-until-success strategy is incorporated to achieve high photon loss tolerance. We simulate small exemplary Bivariate Bicycle qLDPC codes and analyse the performance of our constructions under relevant physical noise mechanisms, including erasures due to fusion failure or photon loss, as well as Pauli errors. We obtain performances comparable with topological architectures though with significantly higher encoding rates.

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Transforming graph states via Bell state measurements

Graph states are key resources for measurement-based quantum computing, which is particularly promising for photonic systems. Fusions are probabilistic Bell state measurements, measuring pairs of parity operators of two qubits. Fusions can be used to connect/entangle different graph states, making them a powerful resource for measurement-based and related fusion-based quantum computing. There are several different graph structures and types of Bell state measurements, yet the associated graph transformations have only been analyzed for specific cases. Here, we provide a full set of graph transformation rules and give an intuitive visualization based on Venn diagrams of local neighborhoods of graph nodes. We derive these graph transformations for all types of rotated type-II fusion, showing that there are five different fusion success cases. Finally, we give application examples of the derived graph transformation rules and show that they can be used to construct graph codes or simulate fusion networks.

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Generating graph states with a single quantum emitter and the minimum number of fusions

Graph states are the key resources for measurement- and fusion-based quantum computing with photons, yet their creation is experimentally challenging. We optimize a hybrid graph-state generation scheme using a single quantum emitter and linear optics Bell-state measurements called fusions. We first generate a restricted class of states from a single quantum emitter and then apply fusions to create a target graph state, where we use a dynamic programming approach to find the construction that requires the lowest possible number of fusions. Our analysis yields a lookup table for constructing $\sim 2.8\times 10^7$ non-isomorphic graph states with the minimum number of fusions. The lookup table covers all graph states with up to eight qubits and several other ones with up to 14 qubits. We present construction protocols of selected graph states and provide the lookup table. For large graph states that are not in the lookup table, we derive bounds for the required number of fusions using graph-theoretic properties. Finally, we use the lookup table to search for the best graph codes for loss-tolerant encodings, given a fixed number of fusions for their construction.

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Breadth-first graph traversal union-find decoder

Fast decoding algorithms are decisive for real-time quantum error correction and for analyzing properties of error correction codes. Here, we develop variants of the union-find decoder that simplify its implementation and provide potential decoding speed advantages. Furthermore, we show how these methods can be adapted to decode non-topological quantum low-density-parity-check (qLDPC) codes. All the developed decoders can directly include both qubit erasures and Pauli errors in the decoding step, thus addressing the dominant noise mechanisms for photonic quantum computing. We investigate the strengths and weaknesses of the different decoder variants, benchmark their speed and threshold error rates on several codes, and provide the used source code.

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Efficient percolation simulations for lossy photonic fusion networks

The study of percolation phenomena has various applications ranging from social networks or materials science to quantum information. The most common percolation models are bond- or site-percolation for which the Newman-Ziff algorithm enables an efficient simulation. Here, we consider several non-standard percolation models that appear in the context of measurement-based photonic quantum computing with so-called graph states and fusion networks. The associated percolation thresholds determine the tolerance to photon loss in such systems and we develop modifications of the Newman-Ziff algorithm to perform the corresponding percolation simulation efficiently. We demonstrate our algorithms by using them to characterize exemplary fusion networks and graph states. The used source code is provided as an open-source repository.

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Loss-tolerant architecture for quantum computing with quantum emitters

We develop an architecture for measurement-based quantum computing using photonic quantum emitters. The architecture exploits spin-photon entanglement as resource states and standard Bell measurements of photons for fusing them into a large spin-qubit cluster state. The scheme is tailored to emitters with limited memory capabilities since it only uses an initial non-adaptive (ballistic) fusion process to construct a fully percolated graph state of multiple emitters. By exploring various geometrical constructions for fusing entangled photons from deterministic emitters, we improve the photon loss tolerance significantly compared to similar all-photonic schemes.

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Quantum Interference of Identical Photons from Remote GaAs Quantum Dots

Photonic quantum technology provides a viable route to quantum communication, quantum simulation, and quantum information processing. Recent progress has seen the realisation of boson sampling using 20 single-photons and quantum key distribution over hundreds of kilometres. Scaling the complexity requires architectures containing multiple photon-sources, photon-counters, and a large number of indistinguishable single photons. Semiconductor quantum dots are bright and fast sources of coherent single-photons. For applications, a significant roadblock is the poor quantum coherence upon interfering single photons created by independent quantum dots. Here, we demonstrate two-photon interference with near-unity visibility ($93.0\pm0.8$)\% using photons from two completely separate GaAs quantum dots. The experiment retains all the emission into the zero-phonon-line -- only the weak phonon-sideband is rejected -- and temporal post-selection is not employed. Exploiting the quantum interference, we demonstrate a photonic controlled-not circuit and an entanglement with fidelity ($85.0\pm 1.0$)\% between photons of different origins. The two-photon interference visibility is high enough that the entanglement fidelity is well above the classical threshold. The high mutual-coherence of the photons stems from high-quality materials, a diode-structure, and the relatively large quantum dot size. Our results establish a platform, GaAs QDs, for creating coherent single photons in a scalable way.

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Structural symmetry-breaking to explain radiative Auger transitions in self-assembled quantum dots

The optical spectrum of a quantum dot is typically dominated by the fundamental transition between the lowest-energy configurations. However, the radiative Auger process can result in additional red-shifted emission lines. The origin of these lines is a combination of Coulomb interaction and symmetry-breaking in the quantum dot. In this paper, we present measurements of such radiative Auger lines for a range of InGaAs/GaAs self-assembled quantum dots and use a tight-binding model with a configuration interaction approach to explain their appearance. Introducing a composition fluctuation cluster in the dot, our calculations show excellent agreement with measurements. We relate our findings to group theory explaining the origin of the additional emission lines. Our model and results give insight into the interplay between the symmetry breaking in a quantum dot and the position and strength of the radiative Auger lines.

cond-mat.mes-hall↗

Optically driving the radiative Auger transition

In a radiative Auger process, optical decay is accompanied by simultaneous excitation of other carriers. The radiative Auger process gives rise to weak red-shifted satellite peaks in the optical emission spectrum. These satellite peaks have been observed over a large spectral range: in the X-ray emission of atoms; close to visible frequencies on donors in semiconductors and quantum emitters; and at infrared frequencies as shake-up lines in two-dimensional systems. So far, all the work on the radiative Auger process has focussed on detecting the spontaneous emission. However, the fact that the radiative Auger process leads to photon emission suggests that the transition can also be optically excited. In such an inverted radiative Auger process, excitation would correspond to simultaneous photon absorption and electronic de-excitation. Here, we demonstrate optical driving of the radiative Auger transition on a trion in a semiconductor quantum dot. The radiative Auger and the fundamental transition together form a $Λ$-system. On driving both transitions of this $Λ$-system simultaneously, we observe a reduction of the fluorescence signal by up to $70\%$. Our results demonstrate a type of optically addressable transition connecting few-body Coulomb interactions to quantum optics. The results open up the possibility of carrying out THz spectroscopy on single quantum emitters with all the benefits of optics: coherent laser sources, efficient and fast single-photon detectors. In analogy to optical control of an electron spin, the $Λ$-system between the radiative Auger and the fundamental transitions allows optical control of the emitters' orbital degree of freedom.

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Radiative Auger Process in the Single-Photon Limit

In a multi-electron atom, an excited electron can decay by emitting a photon. Typically, the leftover electrons are in their ground state. In a radiative Auger process, the leftover electrons are in an excited state and a redshifted photon is created. In a semiconductor quantum dot, radiative Auger is predicted for charged excitons. Here we report the observation of radiative Auger on trions in single quantum dots. For a trion, a photon is created on electron-hole recombination, leaving behind a single electron. The radiative Auger process promotes this additional (Auger) electron to a higher shell of the quantum dot. We show that the radiative Auger effect is a powerful probe of this single electron: the energy separations between the resonance fluorescence and the radiative Auger emission directly measure the single-particle splittings of the electronic states in the quantum dot with high precision. In semiconductors, these single-particle splittings are otherwise hard to access by optical means as particles are excited typically in pairs, as excitons. After the radiative Auger emission, the Auger carrier relaxes back to the lowest shell. Going beyond the original theoretical proposals, we show how applying quantum optics techniques to the radiative Auger photons gives access to the single-electron dynamics, notably relaxation and tunneling. This is also hard to access by optical means: even for quasi-resonant $p$-shell excitation, electron relaxation takes place in the presence of a hole, complicating the relaxation dynamics. The radiative Auger effect can be exploited in other semiconductor nanostructures and quantum emitters in the solid state to determine the energy levels and the dynamics of a single carrier.

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Narrow optical linewidths and spin pumping on charge-tunable, close-to-surface self-assembled quantum dots in an ultra-thin diode

We demonstrate full charge control, narrow optical linewidths, and optical spin pumping on single self-assembled InGaAs quantum dots embedded in a $162.5\,\text{nm}$ thin diode structure. The quantum dots are just $88\,\text{nm}$ from the top GaAs surface. We design and realize a p-i-n-i-n diode that allows single-electron charging of the quantum dots at close-to-zero applied bias. In operation, the current flow through the device is extremely small resulting in low noise. In resonance fluorescence, we measure optical linewidths below $2\,μ\text{eV}$, just a factor of two above the transform limit. Clear optical spin pumping is observed in a magnetic field of $0.5\,\text{T}$ in the Faraday geometry. We present this design as ideal for securing the advantages of self-assembled quantum dots -- highly coherent single photon generation, ultra-fast optical spin manipulation -- in the thin diodes required in quantum nano-photonics and nano-phononics applications.

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Low-Noise GaAs Quantum Dots for Quantum Photonics

Quantum dots are both excellent single-photon sources and hosts for single spins. This combination enables the deterministic generation of Raman-photons -- bandwidth-matched to an atomic quantum-memory -- and the generation of photon cluster states, a resource in quantum communication and measurement-based quantum computing. GaAs quantum dots in AlGaAs can be matched in frequency to a rubidium-based photon memory, and have potentially improved electron spin coherence compared to the widely used InGaAs quantum dots. However, their charge stability and optical linewidths are typically much worse than for their InGaAs counterparts. Here, we embed GaAs quantum dots into an $n$-$i$-$p$-diode specially designed for low-temperature operation. We demonstrate ultra-low noise behaviour: charge control via Coulomb blockade, close-to lifetime-limited linewidths, and no blinking. We observe high-fidelity optical electron-spin initialisation and long electron-spin lifetimes for these quantum dots. Our work establishes a materials platform for low-noise quantum photonics close to the red part of the spectrum.

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Large-Range Frequency Tuning of a Narrow-Linewidth Quantum Emitter

A hybrid system of a semiconductor quantum dot single photon source and a rubidium quantum memory represents a promising architecture for future photonic quantum repeaters. One of the key challenges lies in matching the emission frequency of quantum dots with the transition frequency of rubidium atoms while preserving the relevant emission properties. Here, we demonstrate the bidirectional frequency-tuning of the emission from a narrow-linewidth (close-to-transform-limited) quantum dot. The frequency tuning is based on a piezoelectric strain-amplification device, which can apply significant stress to thick bulk samples. The induced strain shifts the emission frequency of the quantum dot over a total range of $1.15\ \text{THz}$, about three orders of magnitude larger than its linewidth. Throughout the whole tuning process, both the spectral properties of the quantum dot and its single-photon emission characteristics are preserved. Our results show that external stress can be used as a promising tool for reversible frequency tuning of high-quality quantum dots and pave the wave towards the realisation of a quantum dot -- rubidium atoms interface for quantum networking.

cond-mat.mes-hall↗

A bright and fast source of coherent single photons

A single photon source is a key enabling technology in device-independent quantum communication, quantum simulation for instance boson sampling, linear optics-based and measurement-based quantum computing. These applications involve many photons and therefore place stringent requirements on the efficiency of single photon creation. The scaling on efficiency is an exponential function of the number of photons. Schemes taking full advantage of quantum superpositions also depend sensitively on the coherence of the photons, i.e. their indistinguishability. It is therefore crucial to maintain the coherence over long strings of photons. Here, we report a single photon source with an especially high system efficiency: a photon is created on-demand at the output of the final optical fibre with a probability of 57%. The coherence of the photons is very high and is maintained over a stream consisting of thousands of photons; the repetition rate is in the GHz regime. We break with the established semiconductor paradigms, such as micropillars, photonic crystal cavities and waveguides. Instead, we employ gated quantum dots in an open, tunable microcavity. The gating ensures low-noise operation; the tunability compensates for the lack of control in quantum dot position and emission frequency; the output is very well-matched to a single-mode fibre. An increase in efficiency over the state-of-the-art by more than a factor of two, as reported here, will result in an enormous decrease in run-times, by a factor of $10^{7}$ for 20 photons.

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Near Transform-limited Quantum Dot Linewidths in a Broadband Photonic Crystal Waveguide

Planar nanophotonic structures enable broadband, near-unity coupling of emission from quantum dots embedded within, thereby realizing ideal singe-photon sources. The efficiency and coherence of the single-photon source is limited by charge noise, which results in the broadening of the emission spectrum.We report suppression of the noise by fabricating photonic crystal waveguides in a gallium arsenide membrane containing quantum dots embedded in a $p$-$i$-$n$ diode. Local electrical contacts in the vicinity of the waveguides minimize the leakage current and allow fast electrical control ($\approx$4 MHz bandwidth) of the quantum dot resonances. Resonant linewidth measurements of $79$ quantum dots coupled to the photonic crystal waveguides exhibit near transform-limited emission over a 6 nm wide range of emission wavelengths. Importantly, the local electrical contacts allow independent tuning of multiple quantum dots on the same chip, which together with the transform-limited emission are key components in realizing multiemitter-based quantum information processing.

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On-chip deterministic operation of quantum dots in dual-mode waveguides for a plug-and-play single-photon source

A deterministic source of coherent single photons is an enabling device of quantum-information processing for quantum simulators, and ultimately a full-fledged quantum internet. Quantum dots (QDs) in nanophotonic structures have been employed as excellent sources of single photons, and planar waveguides are well suited for scaling up to multiple photons and emitters exploring near-unity photon-emitter coupling and advanced active on-chip functionalities. An ideal single-photon source requires suppressing noise and decoherence, which notably has been demonstrated in electrically-contacted heterostructures. It remains a challenge to implement deterministic resonant excitation of the QD required for generating coherent single photons, since residual light from the excitation laser should be suppressed without compromising source efficiency and scalability. Here, we present the design and realization of a novel planar nanophotonic device that enables deterministic pulsed resonant excitation of QDs through the waveguide. Through nanostructure engineering, the excitation light and collected photons are guided in two orthogonal waveguide modes enabling deterministic operation. We demonstrate a coherent single-photon source that simultaneously achieves high-purity ($g^{(2)}(0)$ = 0.020 $\pm$ 0.005), high-indistinguishability ($V$ = 96 $\pm$ 2 %), and $>$80 % coupling efficiency into the waveguide. The novel `plug-and-play' coherent single-photon source could be operated unmanned for several days and will find immediate applications, e.g., for constructing heralded multi-photon entanglement sources for photonic quantum computing or sensing.

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