arXiv subjects

Matthias Krüger

Publications and source records attributed to Matthias Krüger.

At least 37 records · Page 2Linked to original sources

arXiv2024

Mobility-induced kinetic effects in multicomponent mixtures

We give an overview exploring the role of kinetics in multicomponent mixtures. Compared to the most commonly studied binary (single species plus solvent) case, multicomponent fluids show a rich interplay between kinetics and thermodynamics due to the possibility of fractionation, interdiffusion of mixture components and collective motion. This leads to a competition between multiple timescales that change depending on the underlying kinetics. At high densities, crowding effects are relevant and non-equilibrium structures can become long-lived. We present the main approaches for the study of kinetic effects in multicomponents mixtures, including the role of crowding, and explore their consequences for equilibrium and non-equilibrium scenarios. We conclude by identifying the main challenges in the field.

cond-mat.soft↗

arXiv2024

Heat radiation and transfer for nanoparticles in the presence of a cylinder

We study heat radiation and radiative heat transfer for nanoparticles in the presence of an infinitely long cylinder in different geometrical configurations, based on its electromagnetic Green's tensor. The heat radiation of a single particle can be enhanced by placing it close to a nanowire, and this enhancement can be much larger as compared to placing it close to a plate of the same material. The heat transfer along a cylinder decays much slower than through empty vacuum, being especially long-ranged in the case of a perfectly conducting nanowire, and showing nonmonotonic behavior in the case of a SiC cylinder. Exploring the dependence on the relative azimuthal angle of the nanoparticles, we find that the results are insensitive to small angles, but they can be drastically different when the angle is large, depending on the material. Finally, we demonstrate that a cylinder can either enhance or block the heat flux when placed perpendicular to the interparticle distance line, where the blocking in particular is strongly enhanced compared to the geometry of a sphere of same radius.

quant-ph↗

arXiv2024

Magnetization fluctuations and magnetic aftereffect probed via the anomalous Hall effect

Taking advantage of the anomalous Hall effect, we electrically probe low-frequency magnetization fluctuations at room temperature in a thin ferromagnetic Pt/Co/AlO$_x$ layer stack with perpendicular magnetic anisotropy. We observe a strong enhancement of the Hall voltage fluctuations within the hysteretic region of the magnetization loop. Analyzing both the temporal evolution of the anomalous Hall voltage and its frequency-dependent noise power density, we identify two types of magnetic noise: abrupt changes in the magnetic domain configuration, evident as Barkhausen-like steps in the Hall voltage time trace, yield a noise power density spectrum scaling with frequency as $1/f^β$ with $β\approx 1.9$. In contrast, quasi-stationary magnetization configurations are connected with a magnetic noise power density with an exponent $β\approx 0.9$. The observation of Barkausen steps and relaxation effects shows that the magnetic system is in a non-stationary state in the hysteresis region, such that the fluctuation-dissipation theorem cannot be expected to hold. However, the time-dependent change in the Hall voltage for constant magnetic field strength resembles the integrated noise power.

cond-mat.mes-hall↗

arXiv2024

Scale-dependent heat transport in dissipative media via electromagnetic fluctuations

We develop a theory for heat transport via electromagnetic waves inside media, and use it to derive a spatially nonlocal thermal conductivity tensor, in terms of the electromagnetic Green's function and potential, for any given system. While typically negligible for optically dense bulk media, the electromagnetic component of conductivity can be significant for optically dilute media, and shows regimes of Fourier transport as well as unhindered transport. Moreover, the electromagnetic contribution is relevant even for dense media, when in presence of interfaces, as exemplified for the in-plane conductivity of a nanosheet, which shows a variety of phenomena, including absence of a Fourier regime.

physics.class-ph↗

arXiv2023

Friction of a driven chain: Role of momentum conservation, Goldstone and radiation modes

We analytically study friction and dissipation of a driven bead in a 1D harmonic chain, and analyze the role of internal damping mechanism as well as chain length. Specifically, we investigate Dissipative Particle Dynamics and Langevin Dynamics, as paradigmatic examples that do and do not display translational symmetry, with distinct results: For identical parameters, the friction forces can differ by many orders of magnitude. For slow driving, a Goldstone mode traverses the entire system, resulting in friction of the driven bead that grows arbitrarily large (Langevin) or gets arbitrarily small (Dissipative Particle Dynamics) with system size. For a long chain, the friction for DPD is shown to be bound, while it shows a singularity (i.e. can be arbitrarily large) for Langevin damping. For long underdamped chains, a radiation mode is recovered in either case, with friction independent of damping mechanism. For medium length chains, the chain shows the expected resonant behavior. At the resonance, friction is non-analytic in damping parameter $γ$, depending on it as $γ^{-1}$. Generally, no zero frequency bulk friction coefficient can be determined, as the limits of small frequency and infinite chain length do not commute, and we discuss the regimes where "simple" macroscopic friction occurs.

cond-mat.stat-mech↗

arXiv2023

Entropy bound for time reversal markers

We derive a bound for entropy production in terms of the mean of normalizable path-antisymmetric observables. The optimal observable for this bound is shown to be the signum of entropy production, which is often easier determined or estimated than entropy production itself. It can be preserved under coarse graining by use of a simple path grouping algorithm. We demonstrate this relation and its properties using a driven network on a ring, for which the bound saturates for short times for any driving strength. This work can open a way to systematic coarse graining of entropy production.

cond-mat.stat-mech↗

arXiv2023

Trace expressions and associated limits for equilibrium Casimir torque

We exploit fluctuational electrodynamics to present trace expressions for the torque experienced by arbitrary objects in a passive, nonabsorbing, rotationally invariant background environment. We present trace expressions for equilibrium Casimir torque which complement recently derived nonequilibrium torque expressions and explicate their relation to the Casimir free energy. We then use the derived trace expressions to calculate, via Lagrange duality, semianalytic structure-agnostic bounds on the Casimir torque between an anisotropic (reciprocal or nonreciprocal) dipolar particle and a macroscopic body composed of a local isotropic electric susceptibility, separated by vacuum.

physics.optics↗

arXiv2023

Memory-induced alignment of colloidal dumbbells

When a colloidal probe is forced through a viscoelastic fluid which is characterized by a long stress-relaxation time, the fluid is excited out of equilibrium. This is leading to a number of interesting effects including a non-trivial recoil of the probe when the driving force is removed. Here, we experimentally and theoretically investigate the transient recoil dynamics of non-spherical particles, i.e., colloidal dumbbells. In addition to a translational recoil of the dumbbells, we also find a pronounced angular reorientation which results from the relaxation of the surrounding fluid. Our findings are in good agreement with a Langevin description based on the symmetries of a director (dumbbell) as well as a microscopic bath-rod model. Remarkably, we find a frustrated state with amplified fluctuations when the dumbbell is oriented perpendicular to the direction of driving. Our results demonstrate the complex behavior of non-spherical objects within a relaxing environment which are of immediate interest for the motion of externally but also self-driven asymmetric objects in viscoelastic fluids.

cond-mat.soft↗

arXiv2023

Long-range super-Planckian heat transfer between nanoemitters in a resonant cavity

We study radiative heat transfer between two nanoemitters placed inside different types of closed cavities by means of a fluctuational-electrodynamics approach. We highlight a very sharp dependence of this transfer on cavity width, and connect this to the matching between the material-induced resonance and the resonant modes of the cavity. In resonant configurations, this allows for an energy-flux amplification of several orders of magnitude with respect to the one exchanged between two emitters in vacuum as well as between two black-bodies, even at separation distances much larger than the thermal wavelength. On the other hand, variations of the cavity width by a few percent allow a reduction of the flux by several orders of magnitude and even a transition to inhibition compared to the vacuum scenario. Our results pave the way to the design of thermal waveguides for the long-distance transport of super-Planckian heat flux and selective heat transfer in many-body system.

cond-mat.mes-hall↗

arXiv2023

Friction on layered media: How deep do phonons reach?

We theoretically study the frictional damping of a small probe object on a coated planar surface, analyzing the resulting phonon modes via a theory of viscoelasticity. Three different types of excitations are found to contribute to friction in distinct ways: traveling (3D) spherical waves, traveling (2D) surface waves, and evanescent waves. While traveling waves transport energy away from the probe, determined by long range elastic properties (wavelength), evanescent waves transform energy into heat in a near-field range, characterized by the size of the probe. Thus, fundamentally different behaviors are predicted, depending on coating thickness and material properties.

cond-mat.stat-mech↗

arXiv2023

Memory induced Magnus effect

Spinning objects which move through air or liquids experience a Magnus force. This effect is commonly exploited in ball sports but also of considerable importance for applications and fundamental science. Opposed to large objects where Magnus forces are strong, they are only weak at small scales and eventually vanish for overdamped micron-sized particles in simple liquids. Here we demonstrate an about one-million-fold enhanced Magnus force of spinning colloids in viscoelastic fluids. Such fluids are characterized by a time-delayed response to external perturbations which causes a deformation of the fluidic network around the moving particle. When the particle additionally spins, the deformation field becomes misaligned relative to the particle's moving direction, leading to a force perpendicular to the direction of travel and the spinning axis. The presence of strongly enhanced memory-induced Magnus forces at microscales opens novel applications for particle sorting and steering, the creation and visualization of anomalous flows and more.

cond-mat.soft↗

arXiv2023

Nonequilibrium mixture dynamics: A model for mobilities and its consequences

Extending the famous Model B for the time evolution of a liquid mixture, we derive an approximate expression for the mobility matrix that couples the different mixture components. This approach is based on a single component fluid with particles that are artificially grouped into separate species labelled by ``colors''. The resulting mobility matrix depends on a single dimensionless parameter, which can be determined efficiently from experimental data or numerical simulations, and includes existing standard forms as special cases. We identify two distinct mobility regimes, corresponding to collective motion and interdiffusion, respectively, and show how they emerge from the microscopic properties of the fluid. As a test scenario, we study the dynamics after a thermal quench, providing a number of general relations and analytical insights from a Gaussian theory. Specifically, for systems with two or three components, analytical results for the time evolution of the equal time correlation function compare well to results of Monte Carlo simulations of a lattice gas. A rich behavior is observed, including the possibility of transient fractionation.

cond-mat.stat-mech↗

arXiv2022

Composition Dependent Instabilities in Mixtures With Many Components

Understanding the phase behavior of mixtures with many components is important in many contexts, including as a key step toward a physics-based description of intracellular compartmentalization. Here, we study the instabilities of a mixture model where the second virial coefficients are taken as random Gaussian variables. Using tools from free probability theory we obtain the exact spinodal curve and the nature of instabilities for a mixture with an arbitrary composition, thus lifting the assumption of uniform mixture component densities pervading previous studies. We show that, by controlling the volume fraction of only a few components, one can systematically change the nature of the spinodal instability and achieve demixing for realistic scenarios by a strong {\em composition imbalance amplification}. This results from a non-trivial interplay of entropic effects due to non-uniform composition and complexity in the interactions. Our approach allows for the inclusion of any finite number of structured interactions, leading to a competition between different forms of demixing as density is varied.

cond-mat.stat-mech↗

arXiv2022

Radiative heat transfer with a cylindrical waveguide decays logarithmically slow

Radiative heat transfer between two far-field-separated nanoparticles placed close to a perfectly conducting nanowire decays logarithmically slow with the interparticle distance. This makes a cylinder an excellent waveguide which can transfer thermal electromagnetic energy to arbitrary large distances with almost no loss. It leads to a dramatic increase of the heat transfer, so that, for almost any (large) separation, the transferred energy can be as large as for isolated particles separated by a few hundred nanometers. A phenomenologically found analytical formula accurately describes the numerical results over a wide range of parameters.

quant-ph↗

arXiv2022

Nanoscale friction controlled by top layer thickness in [LaMnO$_{3}$]$_{m}$/[SrMnO$_{3}$]$_{n}$ superlattices

We conducted lateral force microscopy measurements on seven [LaMnO$_{3}$]$_{m}$/[SrMnO$_{3}$]$_{n}$ superlattices with varied layer thicknesses. We observe that the friction forces and the friction coefficients initially increase with increasing LaMnO3 top layer thickness, followed by saturation when the top layer thickness exceeds a few nanometers. These observations clearly demonstrate that sliding friction is affected by sub-surface material properties to a depth of several nanometers and is not just determined by dynamics in the contact interface. We argue that the sub-surface dissipated energy is governed by damping in the elastically strained volume below the AFM tip, an effect which we estimate via thermoelasticity. The absence of a correlation between friction and the thermal resistivity of our superlattices shows furthermore that high-frequency phonons and heat conduction do not play a role in determining friction. Our observations thus demonstrate that friction can be tailored by sub-surface material properties.

cond-mat.mtrl-sci↗

arXiv2022

Equilibrium forces on non-reciprocal materials

We discuss and analyze the properties of Casimir forces acting between nonreciprocal objects in thermal equilibrium. By starting from the fluctuation-dissipation theorem and splitting the force into those arising from individual sources, we show that if all temperatures are equal, the resulting force is reciprocal and is derivable as the gradient of a Casimir (free) energy. While the expression for the free energy is identical to the one for reciprocal objects, there are several distinct features: To leading order in reflections, the free energy can be decomposed as the sum of two terms, the first corresponding to two reciprocal objects, and the second corresponding to two anti-reciprocal objects. The first term is negative and typically yields attraction, while the second can have either sign. For the case of two objects that are each other's mirror images, the second term is positive and yields repulsion. The sum of terms can lead to overall repulsive forces, in agreement with previous observations. Stable configurations, ruled out for reciprocal cases, appear possible for nonreciprocal objects. We show that for three objects, a three-body free energy exists, indicating that previously found persistent heat currents in situations of three objects cannot be used to produce persistent torques.

quant-ph↗

arXiv2022

How are mobility and friction related in viscoelastic fluids?

The motion of a colloidal probe in a viscoelastic fluid is described by friction or mobility, depending on whether the probe is moving with a velocity or feeling a force. While the Einstein relation describes an inverse relationship valid for Newtonian solvents, both concepts are generalized to time-dependent memory kernels in viscoelastic fluids. We theoretically and experimentally investigate their relation by considering two observables: the recoil after releasing a probe that was moved through the fluid and the equilibrium mean squared displacement (MSD). Applying concepts of linear response theory, we generalize Einstein's relation and thereby relate recoil and MSD, which both provide access to the mobility kernel. With increasing concentration, however, MSD and recoil show distinct behaviors, rooted in different behaviors of the two kernels. Using two theoretical models, a linear two-bath particle model and hard spheres treated by mode-coupling theory, we find a Volterra relation between the two kernels, explaining differing timescales in friction and mobility kernels under variation of concentration.

cond-mat.soft↗

arXiv2022

Trace Expressions and Associated Limits for Non-Equilibrium Casimir Torque

We exploit fluctuational electrodynamics to present trace expressions for the torque experienced by arbitrary objects in a passive, non-absorbing, rotationally invariant background environment. Specializing to a single object, this formalism, together with recently developed techniques for calculating bounds via Lagrange duality, is then used to derive limits on the maximum Casimir torque that a single object with an isotropic electric susceptibility can experience when out of equilibrium with its surrounding environment. The maximum torque achievable at any wavelength is shown to scale in proportion to body volumes in both subwavelength (quasistatics) and macroscopic (ray optics) settings, and come within an order of magnitude of achievable torques on topology optimized bodies. Finally, we discuss how to extend the formalism to multiple bodies, deriving expressions for the torque experienced by two subwavelength particles in proximity to one another.

physics.optics↗