arXiv subjects

Maxime Dupont

Publications and source records attributed to Maxime Dupont.

At least 37 records · Page 2Linked to original sources

arXiv2022

Quantum criticality using a superconducting quantum processor

Quantum criticality emerges from the collective behavior of many interacting quantum particles, often at the transition between different phases of matter. It is one of the cornerstones of condensed matter physics, which we access on noisy intermediate-scale (NISQ) quantum devices by leveraging a dynamically driven phenomenon. We probe the critical properties of the one-dimensional quantum Ising model on a programmable superconducting quantum chip via a Kibble-Zurek process, obtain scaling laws, and estimate critical exponents despite inherent sources of errors on the hardware. In addition, we investigate how the improvement of NISQ computers (more qubits, less noise) will consolidate the computation of those universal physical properties. A one-parameter noise model captures the effect of imperfections and reproduces the experimental data. Its systematic study reveals that the noise, analogously to temperature, induces a new length scale in the system. We introduce and successfully verify modified scaling laws, directly accounting for the noise without any prior knowledge. It makes data analyses for extracting physical properties transparent to noise. By understanding how imperfect quantum hardware modifies the genuine properties of quantum states of matter, we enhance the power of NISQ processors considerably for addressing quantum criticality and potentially other phenomena and algorithms.

quant-ph↗

arXiv2021

Spatiotemporal Crossover between Low- and High-Temperature Dynamical Regimes in the Quantum Heisenberg Magnet

The stranglehold of low temperatures on fascinating quantum phenomena in one-dimensional quantum magnets has been challenged recently by the discovery of anomalous spin transport at high temperatures. Whereas both regimes have been investigated separately, no study has attempted to reconcile them. For instance, the paradigmatic quantum Heisenberg spin-$1/2$ chain falls at low temperature within the Tomonaga-Luttinger liquid framework, while its high-temperature dynamics is superdiffusive and relates to the Kardar-Parisi-Zhang universality class in $1+1$ dimensions. This Letter aims at reconciling the two regimes. Building on large-scale matrix product state simulations, we find that they are connected by a temperature-dependent spatiotemporal crossover. As the temperature $T$ is reduced, we show that the onset of superdiffusion takes place at longer length and timescales $\propto 1/T$. This prediction has direct consequences for experiments including nuclear magnetic resonance: it is consistent with earlier measurements on the nearly ideal Heisenberg $S=1/2$ chain compound Sr$_2$CuO$_3$, yet calls for new and dedicated experiments.

cond-mat.str-el↗

arXiv2021

Monolayer CrCl$_3$ as an ideal Test Bed for the Universality Classes of 2D Magnetism

The monolayer halides CrX$_3$ (X=Cl, Br, I) attract significant attention for realizing 2D magnets with genuine long-range order (LRO), challenging the Mermin-Wagner theorem. Here, we show that monolayer CrCl$_3$ has the unique benefit of exhibiting tunable magnetic anisotropy upon applying a compressive strain. This opens the possibility to use CrCl$_3$ for producing and studying both ferromagnetic and antiferromagnetic 2D Ising-type LRO as well as the Berezinskii-Kosterlitz-Thouless (BKT) regime of 2D magnetism with quasi-LRO. Using state-of-the-art density functional theory, we explain how realistic compressive strain could be used to tune the monolayer's magnetic properties so that it could exhibit any of these phases. Building on large-scale quantum Monte Carlo simulations, we compute the phase diagram of strained CrCl$_3$, as well as the magnon spectrum with spin-wave theory. Our results highlight the eminent suitability of monolayer CrCl$_3$ to achieve very high BKT transition temperatures, around 50 K, due to their singular dependence on the weak easy-plane anisotropy of the material.

cond-mat.str-el↗

arXiv2021

Learning the ground state of a non-stoquastic quantum Hamiltonian in a rugged neural network landscape

Strongly interacting quantum systems described by non-stoquastic Hamiltonians exhibit rich low-temperature physics. Yet, their study poses a formidable challenge, even for state-of-the-art numerical techniques. Here, we investigate systematically the performance of a class of universal variational wave-functions based on artificial neural networks, by considering the frustrated spin-$1/2$ $J_1-J_2$ Heisenberg model on the square lattice. Focusing on neural network architectures without physics-informed input, we argue in favor of using an ansatz consisting of two decoupled real-valued networks, one for the amplitude and the other for the phase of the variational wavefunction. By introducing concrete mitigation strategies against inherent numerical instabilities in the stochastic reconfiguration algorithm we obtain a variational energy comparable to that reported recently with neural networks that incorporate knowledge about the physical system. Through a detailed analysis of the individual components of the algorithm, we conclude that the rugged nature of the energy landscape constitutes the major obstacle in finding a satisfactory approximation to the ground state wavefunction, and prevents learning the correct sign structure. In particular, we show that in the present setup the neural network expressivity and Monte Carlo sampling are not primary limiting factors.

physics.comp-ph↗

arXiv2021

Quantum magnetism on small-world networks

While classical spin systems in random networks have been intensively studied, much less is known about quantum magnets in random graphs. Here, we investigate interacting quantum spins on small-world networks, building on mean-field theory and extensive quantum Monte Carlo simulations. Starting from one-dimensional (1D) rings, we consider two situations: all-to-all interacting and long-range interactions randomly added. The effective infinite dimension of the lattice leads to a magnetic ordering at finite temperature $T_\mathrm{c}$ with mean-field criticality. Nevertheless, in contrast to the classical case, we find two distinct power-law behaviors for $T_\mathrm{c}$ versus the average strength of the extra couplings. This is controlled by a competition between a characteristic length scale of the random graph and the thermal correlation length of the underlying 1D system, thus challenging mean-field theories. We also investigate the fate of a gapped 1D spin chain against the small-world effect.

cond-mat.str-el↗

arXiv2021

From trivial to topological paramagnets: The case of $\mathbb{Z}_2$ and $\mathbb{Z}_2^3$ symmetries in two dimensions

Using quantum Monte Carlo simulations, we map out the phase diagram of Hamiltonians interpolating between trivial and non-trivial bosonic symmetry-protected topological phases, protected by $\mathbb{Z}_2$ and $\mathbb{Z}_2^3$ symmetries, in two dimensions. In all cases, we find that the trivial and the topological phases are separated by an intermediate phase in which the protecting symmetry is spontaneously broken. Depending on the model, we identify a variety of magnetic orders on the triangular lattice, including ferromagnetism, $\sqrt{3}\times\sqrt{3}$ order, and stripe orders (both commensurate and incommensurate). Critical properties are determined through a finite-size scaling analysis. Possible scenarios regarding the nature of the phase transitions are discussed.

cond-mat.str-el↗

arXiv2020

Dirty bosons on the Cayley tree: Bose-Einstein condensation versus ergodicity breaking

Building on large-scale quantum Monte Carlo simulations, we investigate the zero-temperature phase diagram of hard-core bosons in a random potential on site-centered Cayley trees with branching number $K=2$. In order to follow how the Bose-Einstein condensate (BEC) is affected by the disorder, we focus on both the zero-momentum density, probing the quantum coherence, and the one-body density matrix (1BDM) whose largest eigenvalue monitors the off-diagonal long-range order. We further study its associated eigenstate which brings useful information about the real-space properties of this leading eigenmode. Upon increasing randomness, we find that the system undergoes a quantum phase transition at finite disorder strength between a long-range ordered BEC state, fully ergodic at large scale, and a new disordered Bose glass regime showing conventional localization for the coherence fraction while the 1BDM displays a non-trivial algebraic vanishing BEC density together with a non-ergodic occupation in real-space. These peculiar properties can be analytically captured by a simple phenomenological description on the Cayley tree which provides a physical picture of the Bose glass regime.

cond-mat.dis-nn↗

arXiv2020

Universal spin dynamics in infinite-temperature one-dimensional quantum magnets

We address the nature of spin dynamics in various integrable and non-integrable, isotropic and anisotropic quantum spin-$S$ chains, beyond the paradigmatic $S=1/2$ Heisenberg model. In particular, we investigate the algebraic long-time decay $\propto t^{-1/z}$ of the spin-spin correlation function at infinite temperature, using state-of-the-art simulations based on tensor network methods. We identify three universal regimes for the spin transport, independent of the exact microscopic model: (i) superdiffusive with $z=3/2$, as in the Kardar-Parisi-Zhang universality class, when the model is integrable with extra symmetries such as spin isotropy that drive the Drude weight to zero, (ii) ballistic with $z=1$ when the model is integrable with a finite Drude weight, and (iii) diffusive with $z=2$ with easy-axis anisotropy or without integrability, at variance with previous observations.

cond-mat.str-el↗

arXiv2019

From eigenstate to Hamiltonian: Prospects for ergodicity and localization

This paper addresses the so-called inverse problem which consists in searching for (possibly multiple) parent target Hamiltonian(s), given a single quantum state as input. Starting from $Ψ_0$, an eigenstate of a given local Hamiltonian $\mathcal{H}_0$, we ask whether or not there exists another parent Hamiltonian $\mathcal{H}_\mathrm{P}$ for $Ψ_0$, with the same local form as $\mathcal{H}_0$. Focusing on one-dimensional quantum disordered systems, we extend the recent results obtained for Bose-glass ground states [M. Dupont and N. Laflorencie, Phys. Rev. B 99, 020202(R) (2019)] to Anderson localization, and the many-body localization (MBL) physics occurring at high energy. We generically find that any localized eigenstate is a very good approximation for an eigenstate of a distinct parent Hamiltonian, with an energy variance $σ_\mathrm{P}^2(L)=\langle\mathcal{H}_\mathrm{P}^2\rangle_{Ψ_0}-\langle\mathcal{H}_\mathrm{P}\rangle_{Ψ_0}^2$ vanishing as a power law of system size $L$. This decay is microscopically related to a chain-breaking mechanism, also signalled by bottlenecks of vanishing entanglement entropy. A similar phenomenology is observed for both Anderson and MBL. In contrast, delocalized ergodic many-body eigenstates uniquely encode the Hamiltonian in the sense that $σ_\mathrm{P}^2(L)$ remains finite at the thermodynamic limit, i.e., $L\to+\infty$. As a direct consequence, the ergodic-MBL transition can be very well captured from the scaling of $σ_\mathrm{P}^2(L)$.

cond-mat.dis-nn↗

arXiv2019

NMR relaxation in the spin-1 Heisenberg chain

We consider the isotropic $S=1$ Heisenberg chain with a finite Haldane gap $Δ$ and use state-of-the-art numerical techniques to investigate its dynamical properties at finite temperature, focusing on the nuclear spin-lattice relaxation rate $1/T_1$ measured in nuclear magnetic resonance (NMR) experiments for instance. In particular, we analyze the contributions from modes with momenta close to $q\approx 0$ and $q\approx π$ as a function of temperature. At high-temperature, we observe spin diffusion with a non-trivial exponent. At low-temperature, we argue that a simple activated behavior $1/T_1 \propto\exp(-Δ/T)$ can only be observed at temperatures much smaller than the gap $Δ$.

cond-mat.str-el↗

arXiv2019

Numerical study of the temperature dependence of the NMR relaxation rate across the superfluid-Bose glass transition in one dimension

We study the nuclear magnetic resonance (NMR) spin-lattice relaxation rate $1/T_1$ in random one-dimensional spin chains as function of the temperature and disorder strength. In the zero temperature limit, the system displays a disorder-induced quantum phase transition between a critical Tomonaga-Luttinger liquid (TLL) phase and a localized Bose glass phase. The $1/T_1$ is investigated across this transition using large-scale simulations based on matrix product state techniques. We find that this quantity can detect the transition and probe the value of the dimensionless TLL parameter $K$. We also compute the NMR relaxation rate distributions for each temperature and disorder strength considered. In particular we discuss the applicability of the stretched exponential fit to the return-to-equilibrium function in order to extract the $1/T_1$ experimentally. The results presented here should provide valuable insights in regards of future NMR experiments in realistic disordered spin compounds.

cond-mat.str-el↗

arXiv2019

Many-body localization as a large family of localized ground states

Many-body localization (MBL) addresses the absence of thermalization in interacting quantum systems, with non-ergodic high-energy eigenstates behaving as ground states, only area-law entangled. However, computing highly excited many-body eigenstates using exact methods is very challenging. Instead, we show that one can address high-energy MBL physics using ground-state methods, which are much more amenable to many efficient algorithms. We find that a localized many-body ground state of a given interacting disordered Hamiltonian $\mathcal{H}_0$ is a very good approximation for a high-energy eigenstate of a parent Hamiltonian, close to $\mathcal{H}_0$ but more disordered. This construction relies on computing the covariance matrix, easily achieved using density-matrix renormalization group for disordered Heisenberg chains up to $L=256$ sites.

cond-mat.dis-nn↗

arXiv2018

Dynamical response and dimensional crossover for spatially anisotropic antiferromagnets

Theoretically challenging, the understanding of the dynamical response in quantum antiferromagnets is of great interest, in particular for both inelastic neutron scattering (INS) and nuclear magnetic resonance (NMR) experiments. In such a context, we theoretically address this question for quasi-one-dimensional quantum magnets, e.g. weakly coupled spin chains for which many compounds are available in Nature. In this class of systems, the dimensional crossover between a three-dimensional ordered regime at low temperature towards one-dimensional physics at higher temperature is a non-trivial issue, notably difficult concerning dynamical properties. Here we present a comprehensive theoretical study based on both analytical calculations (bosonization + random phase and self-consistent harmonic approximations) and numerical simulations (quantum Monte Carlo + stochastic analytic continuation) which allows us to describe the full temperature crossover for the NMR relaxation rate $1/T_1$, from one-dimensional Tomonaga-Luttinger liquid physics to the three-dimensional ordered regime, as a function of inter-chain couplings. The dynamical structure factor, directly probing the INS intensity, is also computed in the different regimes.

cond-mat.str-el↗

arXiv2018

Dynamical properties of the $S=\frac{1}{2}$ random Heisenberg chain

We use numerical techniques to study dynamical properties at finite temperature ($T$) of the Heisenberg spin chain with random exchange couplings, which realizes the random singlet (RS) fixed point in the low-energy limit. Specifically, we study the dynamic spin structure factor $S(q,ω)$, which can be probed directly by inelastic neutron scattering experiments and, in the limit of small $ω$, in nuclear magnetic resonance (NMR) experiments through the spin-lattice relaxation rate $1/T_1$. Our work combines three complementary methods: exact diagonalization, matrix-product-state algorithms, and stochastic analytic continuation of quantum Monte Carlo results in imaginary time. Unlike the uniform system, whose low-energy excitations at low $T$ are restricted to $q$ close to $0$ and $π$, our study reveals a continuous narrow band of low-energy excitations in $S(q,ω)$, extending throughout the Brillouin zone. Close to $q=π$, the scaling properties of these excitations are well captured by the RS theory, but we also see disagreements with some aspects of the predicted $q$-dependence further away from $q=π$. Furthermore we find spin diffusion effects close to $q=0$ that are not contained within the RS theory but give non-negligible contributions to the mean $1/T_1$. To compare with NMR experiments, we consider the distribution of the local $1/T_1$ values, which is broad, approximately described by a stretched exponential. The mean value first decreases with $T$, but starts to increase and diverge below a crossover temperature. Although a similar divergent behavior has been found for the static uniform susceptibility, this divergent behavior of $1/T_1$ has never been seen in experiments. Our results show that the divergence of the mean $1/T_1$ is due to rare events in the disordered chains and is concealed in experiments, where the typical $1/T_1$ value is accessed.

cond-mat.str-el↗

arXiv2017

Competing Bose-Glass physics with disorder-induced Bose-Einstein condensation in the doped $S=1$ antiferromagnet Ni(Cl$_{1-x}$Br$_x$)$_2$-4SC(NH$_2$)$_2$ at high magnetic fields

We study the interplay between disorder and interactions for emergent bosonic degrees of freedom induced by an external magnetic field in the Br-doped spin-gapped antiferromagnetic material Ni(Cl$_{1-x}$Br$_x$)$_2$-4SC(NH$_2$)$_2$ (DTNX). Building on nuclear magnetic resonance experiments at high magnetic field [A. Orlova et al., Phys. Rev. Lett. 118, 067203 (2017)], we describe the localization of isolated impurity states, providing a realistic theoretical modeling for DTNX. Going beyond single impurity localization we use quantum Monte Carlo simulations to explore many-body effects from which pairwise effective interactions lead to a (impurity-induced) BEC revival [M. Dupont, S. Capponi, and N. Laflorencie, Phys. Rev. Lett. 118, 067204 (2017)]. We further address the question of the existence of a many-body localized Bose-glass (BG) phase in DTNX, which is found to compete with a series of a new kind of BEC regimes made out of the multi-impurity states. The global magnetic field-temperature phase diagram of DTNX reveals a very rich structure for low impurity concentration, with consecutive disorder-induced BEC mini-domes separated by intervening many-body localized BG regimes. Upon increasing the impurity level, multiple mini-BEC phases start to overlap, while intermediate BG regions vanish.

cond-mat.str-el↗

arXiv2017

Disorder-induced Revival of the Bose-Einstein Condensation in Ni(Cl$_{1-x}$Br$_x$)$_2$-4SC(NH$_2$)$_2$ at High Magnetic Fields

Building on recent NMR experiments [Phys. Rev. Lett. 118, 067203], we theoretically investigate the high magnetic field regime of the disordered quasi-one-dimensional $S=1$ antiferromagnetic material Ni(Cl$_{1-x}$Br$_x$)$_2$-4SC(NH$_2$)$_2$. The interplay between disorder, chemically controlled by Br-doping, interactions, and the external magnetic field, leads to a very rich phase diagram. Beyond the well-known antiferromagnetically ordered regime, analog of a Bose condensate of magnons, which disappears when $H\ge 12.3$ T, we unveil a resurgence of phase coherence at higher field $H\sim 13.6$ T, induced by the doping. Interchain couplings stabilize finite temperature long-range order whose extension in the field - temperature space is governed by the concentration of impurities $x$. Such a "mini-condensation" contrasts with previously reported Bose-glass physics in the same regime, and should be accessible to experiments.

cond-mat.str-el↗

arXiv2017

Nuclear Magnetic Resonance Reveals Disordered Level-Crossing Physics in the Bose-Glass Regime of the Br-doped Ni(Cl$_{1-x}$Br$_x$)$_2$-4SC(NH$_2$)$_2$ Compound at a High Magnetic Field

By measuring the nuclear magnetic resonance (NMR) 1/T_1 relaxation rate in the Br (bond) doped DTN compound, Ni(Cl(1-x)Br_x)2-4SC(NH2)2 (DTNX), we show that the low-energy spin dynamics of its high magnetic field "Bose-glass" regime is dominated by a strong peak of spin fluctuations found at the nearly doping-independent position H* = 13.6 T. From its temperature and field dependence we conclude that this corresponds to a level crossing of the energy levels related to the doping-induced impurity states. Observation of the local NMR signal from the spin adjacent to the doped Br allowed us to fully characterize this impurity state. We have thus quantified a microscopic theoretical model that paves the way to better understanding of the Bose-glass physics in DTNX, as revealed in the related theoretical study [M. Dupont, S. Capponi, and N. Laflorencie, Phys. Rev. Lett. 118, 067204 (2017), arXiv:1610.05136].

cond-mat.str-el↗

arXiv2017

Nuclear magnetic resonance study of the magnetic-field-induced ordered phase in the NiCl2-4SC(NH2)2 compound

Nuclear magnetic resonance (NMR) study of the high magnetic field (H) part of the Bose-Einstein condensed (BEC) phase of the quasi-onedimensional (quasi-1D) antiferromagnetic quantum spin-chain compound NiCl2-4SC(NH2)2 (DTN) was performed. We precisely determined the phase boundary, Tc(H), down to 40 mK; the critical boson density, n_c(Tc); and the absolute value of the BEC order parameter S_perp at very low temperature (T = 0.12 K). All results are accurately reproduced by numerical quantum Monte Carlo simulations of a realistic three-dimensional (3D) model Hamiltonian. Approximate analytical predictions based on the 1D Tomonaga-Luttinger liquid description are found to be precise for Tc(H), but less so for S_perp(H), which is more sensitive to the strength of 3D couplings, in particular close to the critical field. A mean-field treatment, based on the Hartree-Fock-Popov description, is found to be valid only up to n_c = 4% (T < 0.3 K), while for higher n_c boson interactions appear to modify the density of states.

cond-mat.str-el↗