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Maycon Motta

Publications and source records attributed to Maycon Motta.

6 recordsLinked to original sources

Electrical manipulation of oxygen stoichiometry in multiterminal YBa$_2$Cu$_3$O$_{7-\delta}$ junctions

Local manipulation of oxygen stoichiometry offers a route to control the electronic properties of complex oxides, yet the selective modification of individual current-carrying branches through oxygen redistribution remains unexplored in multiterminal high-temperature superconducting junctions. In a YBa$_2$Cu$_3$O$_{7-\delta}$ Y-shaped three-terminal device, we demonstrate the possibility to electrically control oxygen vacancy migration on a hand-picked terminal while largely preserving the other two. Oxygen-depleted propagating fronts are directly visualized by the resulting change in optical reflectivity and they are linked to the evolution of the electrical response. The process is highly directional and determined by the polarity of the applied current, allowing for the creation of either a converging or a diverging propagating front from the central node of the Y-shaped device. The associated changes in resistance exhibit relaxation on a timescale of minutes, driven by the vacancy concentration gradient. Effects of oxygen migration are also mapped by Kelvin Probe Force Microscopy and Scanning Laser Microscopy, which probe work-function changes and spatially resolved variations in the superconducting transition, respectively. Notably, the Tc contrast revealed by the latter provides a quantitative handle on the underlying oxygen content, enabling direct visualization of oxygen redistribution. Finite-element modeling and nanoprobe X-ray diffraction qualitatively reproduce the observed vacancy redistribution. These results establish a post-fabrication route to locally tune properties of superconducting multiterminal devices such as nanocryotrons, yTron, and tunable weak links.

cond-mat.supr-con

Probing Electromigration of Oxygen Vacancies in YBa$_2$Cu$_3$O$_{7-\delta}$ Devices by Multimodal X-ray Techniques

Control of oxygen vacancies by electrical currents in complex oxides such as YBa$_2$Cu$_3$O$_{7-\delta}$ (YBCO) has attracted considerable interest due to the relative simplicity of its implementation and its potential for both fundamental studies and the tuning of superconducting device properties. However, the structural evolution and depth-dependent effects associated with current-based techniques remain largely unexplored, particularly with respect to the connection between optical signatures and the spatial distribution of oxygen vacancies. Here, we combine nanoprobe X-ray Diffraction (NanoXRD), Cu K-edge X-ray Absorption Near-Edge Structure (XANES), X-ray Photoelectron Spectroscopy (XPS), electrical transport, and optical measurements to reveal modifications induced in YBCO microbridges by pulsed electromigration. We observe a c-axis expansion correlated with spectroscopic features of oxygen depletion in the Cu-O chains, and we confirm that oxygen redistribution, crystallographic changes, and copper coordination evolve consistently across techniques. Notably, the spatial profile of unit-cell expansion closely follows the optical contrast observed after electromigration, demonstrating that the different signatures capture the same underlying oxygen reordering. We further show that optical microscopy cannot reliably capture bipolar electromigration involving strong resistance modifications, as surface deoxygenation appears largely irreversible. Taken together, our findings provide a significant step toward a microscopic understanding of current-assisted oxygen migration in YBCO and establish a framework for effectively exploiting vacancy control in high-temperature superconducting devices.

cond-mat.supr-con

Nanobridge SQUIDs as multilevel memory elements

With the development of novel computing schemes working at cryogenic temperatures, superconducting memory elements have become essential. In this context, superconducting quantum interference devices (SQUIDs) are promising candidates, as they may trap different discrete amounts of magnetic flux. We demonstrate that a field-assisted writing scheme allows such a device to operate as a multilevel memory by the readout of eight distinct vorticity states at zero magnetic field. We present an alternative mechanism based on single phase slips which allows to switch the vorticity state while preserving superconductivity. This mechanism provides a possibly deterministic channel for flux control in SQUID-based memories, under the condition that the field-dependent energy of different vorticity states are nearby.

cond-mat.supr-con

Influence of pinning centers of different natures onsurrounding vortices

Studies involving vortex dynamics and their interaction with pinning centers are an important ingredient to reach higher critical currents in superconducting materials. The vortex distribution around arrays of engineered defects, such as blind and through holes, may help to improve the superconducting properties. Thus, in this work, we used the time-dependent Ginzburg-Landau theory to investigate the vortex dynamics in superconductors of mesoscopic dimensions with a large central square defect with three different configurations: (i) a hole which passes through the sample (interface with the vacuum); (ii) a superconducting region with lower critical temperature (Tc); and (iii) a region with a more robust superconductivity, i.e., with a higherTc. Such systems can be envisaged as elementary building blocks of a macroscopic decorated specimen. Therefore, we evaluated the influence of different interfaces on the vortex dynamics and their effects in the field-dependent magnetization and time-dependent induced electric potential variation. The results show that the lower critical field is independent from the nature of the defect. However, the currents crowd at the vertices of the through hole producing a lower degradation of the local superconductivity, which may increase the upper critical field. On the other hand, the last type of defect can be used to control the vortex dynamics in the main superconducting region around the defect with more accuracy. Whereas the first two defects are attractive for the vortices, the third type is repulsive for them, being needed several vortices penetrated in the superconducting matrix to have vortices penetrated into it.

cond-mat.supr-con

Optimum heat treatment to enhance the weak-linkresponse of Y123 nanowires prepared by SolutionBlow Spinning

Although the production of YBa$_{2}$Cu$_{3}$O$_{7-\delta}$ (Y123) has been extensively reported, there is still a lack of information on the ideal heat treatment to produce this material in the form of one dimension nanostructures. Thus, by means of the Solution Blow Spinning technique, metals embedded in polymer fibers were prepared. These polymer composite fibers were fired and then investigated by thermogravimetric analysis. The maximum sintering temperatures of heat treatment were chosen in the interval \SI{850}{\celsius}-\SI{925}{\celsius} for one hour under oxygen flux. SEM images allowed us to determine the wire diameter as approximately 350~nm for all samples, as well as to map the evolution of the entangled wire morphology with the sintering temperature. XRD analysis indicated the presence of Y123 and secondary phases in all samples. Ac magnetic susceptibility and dc magnetization measurements demonstrated that the sample sintered at \SI{925}{\celsius}/1h is the one with the highest weak-link critical temperature and the largest diamagnetic response.

cond-mat.mtrl-sci

One-pot synthesis: a simple and fast method to obtain ceramic superconducting materials

The one-pot method focuses on the reduction of the number of steps or chemical reactions in the synthesis of materials, and it is very appealing in terms of sustainability. In addition to this point of view, superconductors are desired materials due to their unusual properties, such as the zero resistivity and the perfect diamagnetism. One-pot, Thus, in this work, we described the one-pot synthesis of YBa2Cu3O7-{\delta} superconducting ceramic. In just two steps and a few hours, a polymer composite solution was prepared, which originates a powder after burning the polymer out with pure phase and with superconducting properties better than those produced by other techniques.

cond-mat.mtrl-sci