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Maziyar Jalaal

Publications and source records attributed to Maziyar Jalaal.

At least 19 recordsLinked to original sources

Droplet Deformation and Emulsion Rheology in Two-Dimensional Odd Stokes Flow

We study the deformation of a two-dimensional viscous droplet in simple shear in the presence of odd viscosity. We derive an analytical solution for the droplet shape and surrounding flow field within the framework of odd Stokes flow, allowing for differences in both even and odd viscosity between the droplet and the surrounding fluid. This solution yields closed-form expressions for the macroscopic apparent even and odd viscosities of a dilute emulsion. We show that, provided all viscosity differences remain moderate, the steady-state Taylor deformation parameter satisfies $D_T^\infty = \text{Ca} + \mathcal{O}(\text{Ca}^2)$ so that the leading-order droplet deformation is unchanged from the classical (even-viscous) result. Nevertheless, pronounced effects emerges beyond leading order, where our direct numerical simulations reveal odd-viscous differences to the droplet deformation. In addition, we show that the flow is influenced only by the difference in odd viscosity between the droplet and the medium and not on their individual values. Our analysis clarifies how odd viscosity might modify the effective rheology of dilute emulsions and provides a framework for interpreting droplet-based measurements of odd-viscous response. Key words: odd viscosity $|$ droplets $|$ emulsions $|$ surface tension $|$ chiral fluids

cond-mat.soft

On Linear and Non-Linear Mechanics of Cyanobacterial Colonies

Toxic cyanobacterial blooms are a growing environmental concern that affects freshwater ecosystems, drinking water supplies, and public health. The cyanobacterium Microcystis is among the most important bloom forming species. It often grows in large colonies, which enhances its flotation, reduces grazing, and improves nutrient regulation. Microcystis cells are held together by a matrix of extracellular polymeric substances (EPS), making colony mechanics crucial for bloom formation. However, an analysis of the biomechanical properties of cyanobacterial colonies, and how these properties relate to environmental conditions like nutrient availability, remains largely missing. Here, we use micropipette force sensors to quantify the linear and non-linear mechanical properties of individual colonies at single-cell resolution. Bulk shear rheology complements these measurements by probing macroscopic properties. The measured tensile strength and yield stress are broadly comparable to those of bacterial biofilms and are far greater than the hydrodynamic stresses typically found in wind-mixed lakes. This implies that cyanobacterial colonies are highly resistant to fragmentation by natural mixing processes. We also show that low nutrient availability, particularly low phosphorus, produced stronger colonies, suggesting structural changes in the EPS. Overall, our results establish mechanical testing as a tool for a more complete and physically grounded understanding of cyanobacterial colony formation.

cond-mat.soft

Biogenic bubbles enable microbial escape from physical confinement

Immotile microbes inhabit nearly every environment on Earth, from soils and sediments to food matrices -- yet how they disperse through these physically confining environments is poorly understood. Here, we show that immotile microbial colonies confined in a model transparent yield-stress matrix can achieve long-range dispersal by harnessing their own metabolism. Using yeast as a model organism, we find that fermentation drives dissolved CO$_2$ to supersaturation, nucleating biogenic bubbles that grow, yield the matrix, and rise, hydrodynamically entraining cells vertically in their wake. Sequential bubble nucleation sculpts persistent columnar colonies extending far beyond what growth alone permits. Multiple colonies interact via their fermentation byproducts, merging and mixing genetically as they collectively sculpt self-sustaining conduit networks. Our findings reveal a third mode of microbial dispersal, distinct from the canonical mechanisms of motility and growth, with implications for ecology, environmental science, and biotechnology. More broadly, they exemplify a previously unrecognized class of active behavior -- Metabolically Driven Active Matter -- in which metabolic byproducts reshape the physical landscape of confinement to drive population-scale motion.

physics.bio-ph

Cage Breaking Far from Equilibrium

Active matter can flow and yield under conditions where passive matter jams and slows down, as self-propulsion significantly modulates particle escape from local cages. How activity microscopically reshapes the caging environment to produce this effect, however, remains poorly understood. Here we study a minimal active-matter model of cage breaking: three distinguishable self-propelling disks under circular confinement. This simple setting allows us to construct an entropic landscape for rearrangements and to compare it exactly with its equilibrium counterpart. At low activity the landscape is effectively bistable, whereas at high activity it develops additional metastable basins associated with frustrated clusters at the boundary. We quantify the system's departure from equilibrium and show that cage breaking is fastest when the persistence length matches the particle radius, linking a geometric microscopic scale to the enhanced dynamics of active glasses. Extending the landscape to two dimensions reveals circulating probability currents, and a Markov-state description shows that detailed balance is broken both in the continuous landscape dynamics and in the coarse-grained transitions between entropic basins. Our results provide a minimal microscopic framework for understanding how activity reshapes caging, relaxation, and irreversibility in dense nonequilibrium matter.

cond-mat.soft

Non-Reciprocal Capillary Waves

Capillary waves are a classical free-surface phenomenon in fluid mechanics, yet their behavior in chiral fluids remains largely unexplored. We show that odd viscosity breaks the reciprocity of capillary waves. Using linear theory together with fully nonlinear direct numerical simulations, we find that surface tension creates two inequivalent branches of odd capillary waves: a dispersive branch and a quasi-acoustic branch absent in the capillarity-free limit. Their unequal propagation and attenuation transform standing waves into traveling waves and produce an anomalously deep vortical boundary layer. Above a threshold odd viscosity, nonlinear accumulation of vorticity near the surface reverses the induced shear current and drives bulk particles opposite to the wave motion, giving rise to an anti-Stokes drift with no counterpart in conventional fluids. Our results show how combining capillarity with broken parity can be used to control wave propagation and transport at fluid interfaces, opening a route toward one-way fluidic waveguiding and chirality-programmed interfacial flows.

physics.flu-dyn

Coalescence of Printed Yield Stress Filaments in Direct Ink Writing

In direct ink writing (DIW), neighbouring filaments of yield-stress inks are deposited side-by-side and are expected to merge into smooth, mechanically robust structures. Unlike Newtonian filaments, coalescence can arrest in finite time, leaving a permanent, non-flat ridge set by the competition between capillarity and rheology. Here we study the coalescence of two printed yield-stress filaments, combining scaling theory for the arrested state, direct numerical simulations, and DIW experiments on Carbopol gels imaged by optical coherence tomography. In the viscoplastic limit, we predict and observe an approximately linear decrease of the final bridge height with plastocapillary number and a critical yield stress above which coalescence does not initiate. Simulations further show that elasticity becomes important at high plastocapillary number, enabling larger final bridge heights via a crossover from a rigid Herschel--Bulkley solid to a deformable Kelvin--Voigt response. Our findings provide a framework for predicting deposition profiles and, ultimately, for mitigating residual topography in DIW.

cond-mat.soft

Rheology of Two-Dimensional Dilute Emulsions

The single droplet under shear is a foundational problem in fluid mechanics. In computational fluid dynamics, the two-dimensional (2D) formulation offers advantages in both computational efficiency and relevance, yet its theoretical treatment remains relatively underdeveloped. In this brief note, we present an analytical treatment of this problem, beginning with a derivation of the Lamb solution for 2D Stokes flows, which in turn is used to obtain the flow fields around a droplet in a purely extensional flow. Using these flow fields, expressions are obtained for the apparent viscosity, $\mu^*$, of a dilute emulsion as well as a small deformation theory. We show that $\mu^* = \mu( 1 + f(\lambda) \phi) + \mathcal{O}(\phi^2)$ with $f(\lambda) = (2\lambda + 1)/(\lambda + 1)$ where $\lambda$ is the ratio of the droplet viscosity to the matrix viscosity and $\phi$ is the area fraction covered by the suspended phase. Also the steady state value of the Taylor deformation parameter $D_T^\infty$, in the capillarity-dominated regime, obeys $D_T^\infty = g(\lambda)\,\text{Ca}$, where Ca is the capillary number and $g(\lambda) = 1$. This contrasts with the 3D case, where $g(\lambda)$ depends on $\lambda$. These results are then validated through direct numerical simulations across a wide range of viscosity ratios ($0.01 < \lambda < 100$). Our results provide a basic theoretical framework for interpreting 2D droplet simulations and provide clear benchmarks for computational fluid dynamics.

physics.flu-dyn

Spreading droplets of yield-stress fluids with and without gravity

We investigate the effect of gravity on the spreading of droplets of yield stress fluids, by performing both microgravity experiments (in a drop tower) and experiments under terrestrial gravity. We investigate the dependence of the final droplet shape on yield stress and gravity. Droplets are deposited on a thin film of the same material, allowing to directly test scaling laws derived from the thin-film equation for viscoplastic fluids. Microgravity conditions allow to vary independently the two relevant dimensionless numbers, the Bond number, B, and the plastocapillary number, J, and thus to disentangle the influence of surface tension from that of the yield stress on the droplet shapes. Simulations using a visco-elastic model with shear thinning complement the experiments and show good agreement regarding the droplet shapes. Possible deviations arising in the regime of non-negligible elastic effects and large plastocapillary numbers (large yield stress) are discussed.

physics.flu-dyn

Bouncing microdroplets on hydrophobic surfaces

Intuitively, slow droplets stick to a surface and faster droplets splash or bounce. However, recent work suggests that on non-wetting surfaces, whether microdroplets stick or bounce depends only on their size and fluid properties, but not on the incoming velocity. Here, we show using theory and experiments that even poorly wetting surfaces have a velocity-dependent criterion for bouncing of aqueous droplets, which is as high as 6 m/s for diameters of 30-50 microns on hydrophobic surfaces such as Teflon. We quantify this criterion by analyzing the interplay of dissipation, surface adhesion, and incoming kinetic energy, and describe a wealth of associated phenomena, including air bubbles and satellite droplets. Our results on inertial microdroplets elucidate fundamental processes crucial to aerosol science and technology.

physics.flu-dyn

Odd Droplets: Fluids with Odd Viscosity and Highly Deformable Interfaces

Flows with deformable interfaces are commonly controlled by applying an external field or modifying the boundaries that interact with the fluid, but realizing such solutions can be demanding or impractical in various scenarios. Here, we demonstrate that fluids with broken symmetries can self-control their mechanics. We present a continuum model of a viscous fluid with highly deformable interfaces subject to capillary stresses. Our model features odd viscosity, a parity-violating property that emerges in chiral fluids. Using direct numerical simulations, we focus on the impact of an odd droplet on a superhydrophobic surface. We demonstrate that odd viscosity dramatically disrupts conventional symmetric spreading by inducing asymmetric deformations and chiral flow patterns. Our analysis reveals a variety of dynamic regimes, including leftward and rightward bouncing, as well as rolling, depending on the relative strength of the odd viscosity. Our work illustrates that regulating odd viscosity provides a promising framework for controlling multiphase flows and designing functional metamaterials with tailored fluidic properties.

cond-mat.soft

Laser-induced droplet deformation: curvature inversion explained from instantaneous pressure impulse

We investigate the shape of a tin sheet formed from a droplet struck by a nanosecond laser pulse. Specifically, we examine the dynamics of the process as a function of laser beam properties, focusing on the outstanding riddle of curvature inversion: tin sheets produced in experiments and state-of-the-art extreme ultraviolet (EUV) nanolithography light sources curve in a direction opposite to previous theoretical predictions. We resolve this discrepancy by combining direct numerical simulations with experimental data, demonstrating that curvature inversion can be explained by an instantaneous pressure impulse with low kurtosis. Specifically, we parametrize a dimensionless pressure width, $W$, using a raised cosine function and successfully reproduce the experimentally observed curvature over a wide range of laser-to-droplet diameter ratios, $0.3 < d/D_0 < 0.8$. The simulation process described in this work has applications in the EUV nanolithography industry, where a laser pulse deforms a droplet into a sheet, which is subsequently ionized by a second pulse to produce EUV-emitting plasma.

physics.flu-dyn

Optimal disk packing of chloroplasts in plant cells

Photosynthesis is vital for the survival of entire ecosystems on Earth. While light is fundamental to this process, excessive exposure can be detrimental to plant cells. Chloroplasts, the photosynthetic organelles, actively move in response to light and self-organize within the cell to tune light absorption. These disk-shaped motile organelles must balance dense packing for enhanced light absorption under dim conditions with spatial rearrangements to avoid damage from excessive light exposure. Here, we reveal that the packing characteristics of chloroplasts within plant cells show signatures of optimality. Combining measurements of chloroplast densities and three-dimensional cell shape in the water plant Elodea densa, we construct an argument for optimal cell shape versus chloroplast size to achieve two targets: dense packing into a two-dimensional monolayer for optimal absorption under dim light conditions and packing at the sidewalls for optimal light avoidance. We formalize these constraints using a model for random close packing matched with packing simulations of polydisperse hard disks confined within rectangular boxes. The optimal cell shape resulting from these models corresponds closely to that measured in the box-like plant cells, highlighting the importance of particle packing in the light adaptation of plants. Understanding the interplay between structure and function sheds light on how plants achieve efficient photo adaptation. It also highlights a broader principle: how cell shape relates to the optimization of packing finite and relatively small numbers of organelles under confinement. This universal challenge in biological systems shares fundamental features with the mechanics of confined granular media and the jamming transitions in dense active and passive systems across various scales and contexts.

cond-mat.soft

Glandular Trichome Rupture in Tomato Plants is an Ultra-Fast & Sensitive Defense Mechanism Against Insects

Trichomes, specialized hair-like structures on the surfaces of many plants, play a crucial role in defense against herbivorous insects. We investigated the biomechanics of type VI glandular trichomes in cultivated tomato (Solanum lycopersicum) and its wild relative (Solanum habrochaites). Using micropipette force sensors and high-speed imaging, we uncovered the rupture mechanics underlying gland bursting, highlighting the small forces and short time-scales involved in this process. Additionally, we observed larvae of the Western flower thrips (Frankliniella occidentalis), a major pest in tomato cultivation, inadvertently triggering trichome rupture and accumulating glandular secretions on their bodies. These findings demonstrate how rapid gland bursting and the fluid dynamics of glandular secretions act as an efficient and swift plant defense mechanism against insect herbivory.

physics.bio-ph

ActiveCheerios: 3D-Printed Marangoni-Driven Active Particles at an Interface

Marangoni surfers are simple, cost-effective tabletop experiments that, despite their simplicity, exhibit rich dynamics and collective behaviors driven by physicochemical mechanisms, hydrodynamic interactions, and inertial motion. This work introduces self-propelled particles designed and manufactured through 3D printing to move on the air-water interface. We develop particles with tunable motility and controlled particle-particle interactions by leveraging surface tension-mediated forces, such as the Marangoni effect for propulsion and the Cheerios effect for interactions. Rapid prototyping through 3D printing facilitates the exploration of a wide design space, enabling precise control over particle shape and function. We exemplify this by creating translational and chiral particles. Additionally, we investigate self-assembly in this system and highlight its potential for modular designs where mechanically linked particles with varying characteristics follow outlined trajectories. This research offers a flexible, low-cost approach to designing active interfacial systems and opens new possibilities for further advancements of adaptive, multifunctional devices.

cond-mat.soft

Fragmentation and aggregation of cyanobacterial colonies

Fluid flow has a major effect on the aggregation and fragmentation of bacterial colonies. Yet, a generic framework to understand and predict how hydrodynamics affects colony size remains elusive. This study investigates how fluid flow affects the formation and maintenance of large colonial structures in cyanobacteria, using an experimental technique that precisely controls hydrodynamic conditions. We performed experiments on laboratory cultures and lake samples of the cyanobacterium Microcystis, while their colony size distribution was measured simultaneously by direct microscopic imaging. We demonstrate that EPS-embedded cells formed by cell division exhibit significant mechanical resistance to shear forces. However, at elevated hydrodynamic stress levels (exceeding those typically generated by surface wind mixing) these colonies experience fragmentation through an erosion process. We also show that single cells can aggregate into small colonies due to fluid flow. However, the structural integrity of these flow-induced colonies is weaker than that of colonies formed by cell division. We provide a mathematical analysis to support the experiments and demonstrate that a population model with two categories of colonies describes the measured size distributions. Our results shed light on the specific conditions wherein flow-induced fragmentation and aggregation of cyanobacteria are decisive and indicate that colony formation under natural conditions is mainly driven by cell division, although flow-induced aggregation could play a role in dense bloom events. These findings can be used to improve prediction models and mitigation strategies for toxic cyanobacterial blooms and also offer potential applications in other areas such as algal biotechnology or medical settings where the dynamics of biological aggregates play a significant role.

cond-mat.soft

Morphodynamics of chloroplast network control light-avoidance response in the non-motile dinoflagellate Pyrocystis lunula

Photosynthetic algae play a significant role in oceanic carbon capture. Their performance, however, is constantly challenged by fluctuations in environmental light conditions. Here, we show that the non-motile single-celled marine dinoflagellate Pyrocystis lunula can internally contract its chloroplast network in response to light. By exposing the cell to various physiological light conditions and applying temporal illumination sequences, we find that network morphodynamics follows simple rules, as established in a mathematical model. Our analysis of the chloroplast structure reveals that its unusual reticulated morphology constitutes properties similar to auxetic metamaterials, facilitating drastic deformations for light-avoidance, while confined by the cell wall. Our study shows how the topologically complex network of chloroplasts is crucial in supporting the dinoflagellate's adaptation to varying light conditions, thereby facilitating essential life-sustaining processes.

physics.bio-ph

Optimal shape design of printing nozzles for extrusion-based additive manufacturing

The optimal design seeks the best possible solution(s) for a mechanical structure, device, or system, satisfying a series of requirements and leading to the best performance. In this work, optimized nozzle shapes have been designed for a wide range of polymer melts to be used in extrusion-based additive manufacturing, which aims to minimize pressure drop and allow greater flow control at large extrusion velocities. This is achieved with a twofold approach, combining a global optimization algorithm with computational fluid dynamics for optimizing a contraction geometry for viscoelastic fluids and validating these geometries experimentally. In the optimization process, variable coordinates for the nozzle's contraction section are defined, the objective function is selected, and the optimization algorithm is guided within manufacturing constraints. Comparisons of flow-type and streamline plots reveal that the nozzle shape significantly influences flow patterns. Depending on the rheological properties, the optimized solution either promotes shear or extensional flow, enhancing the material flow rate. Finally, experimental validation of the nozzle performance assessed the actual printing flow, the extrusion force and the overall print control. It is shown that optimizing the nozzle can significantly reduce backflow-related pressure drop, positively impacting total pressure drop (up to 41%) and reducing backflow effects. This work has real-world implications for the additive manufacturing industry, offering opportunities for increased printing speeds, enhanced productivity, and improved printing quality and reliability. Our research contributes to advancing extrusion-based printing processes technology, addressing industry demands and enhancing the field of additive manufacturing.

physics.flu-dyn

Ductile-to-brittle transition and yielding in soft amorphous materials: perspectives and open questions

Soft amorphous materials are viscoelastic solids ubiquitously found around us, from clays and cementitious pastes to emulsions and physical gels encountered in food or biomedical engineering. Under an external deformation, these materials undergo a noteworthy transition from a solid to a liquid state that reshapes the material microstructure. This yielding transition was the main theme of a workshop held from January 9 to 13, 2023 at the Lorentz Center in Leiden. The manuscript presented here offers a critical perspective on the subject, synthesizing insights from the various brainstorming sessions and informal discussions that unfolded during this week of vibrant exchange of ideas. The result of these exchanges takes the form of a series of open questions that represent outstanding experimental, numerical, and theoretical challenges to be tackled in the near future.

cond-mat.soft