arXiv subjects

Maziyar Jalaal

Publications and source records attributed to Maziyar Jalaal.

32 records · Page 2Linked to original sources

arXiv2023

Ductile-to-brittle transition and yielding in soft amorphous materials: perspectives and open questions

Soft amorphous materials are viscoelastic solids ubiquitously found around us, from clays and cementitious pastes to emulsions and physical gels encountered in food or biomedical engineering. Under an external deformation, these materials undergo a noteworthy transition from a solid to a liquid state that reshapes the material microstructure. This yielding transition was the main theme of a workshop held from January 9 to 13, 2023 at the Lorentz Center in Leiden. The manuscript presented here offers a critical perspective on the subject, synthesizing insights from the various brainstorming sessions and informal discussions that unfolded during this week of vibrant exchange of ideas. The result of these exchanges takes the form of a series of open questions that represent outstanding experimental, numerical, and theoretical challenges to be tackled in the near future.

cond-mat.soft↗

arXiv2023

Billiards with Spatial Memory

Many classes of active matter develop spatial memory by encoding information in space, leading to complex pattern formation. It has been proposed that spatial memory can lead to more efficient navigation and collective behaviour in biological systems and influence the fate of synthetic systems. This raises important questions about the fundamental properties of dynamical systems with spatial memory. We present a framework based on mathematical billiards in which particles remember their past trajectories and react to them. Despite the simplicity of its fundamental deterministic rules, such a system is strongly non-ergodic and exhibits highly-intermittent statistics, manifesting in complex pattern formation. We show how these self-memory-induced complexities emerge from the temporal change of topology and the consequent chaos in the system. We study the fundamental properties of these billiards and particularly the long-time behaviour when the particles are self-trapped in an arrested state. We exploit numerical simulations of several millions of particles to explore pattern formation and the corresponding statistics in polygonal billiards of different geometries. Our work illustrates how the dynamics of a single-body system can dramatically change when particles feature spatial memory and provide a scheme to further explore systems with complex memory kernels.

nlin.CD↗

arXiv2023

Elasto-viscoplastic Spreading: from Plastocapillarity to Elastocapillarity

We study the spreading of elastoviscoplastic (EVP) droplets under surface tension effects. The non- Newtonian material flows like a viscoelastic liquid above the yield stress and behaves like a viscoelastic solid below it. Hence, the droplet initially flows under surface tension forces but eventually reaches a final equilibrium shape when the stress everywhere inside the droplet falls below the resisting rheological stresses. We use numerical simulations and combine Volume-of-Fluid (VOF) method and an EVP constitutive model to systematically study the dynamics of spreading and the final shape of the droplets. The spreading process examined in this study finds applications in coating, droplet-based inkjet printing, and 3D printing, where complex fluids such as paints, thermoplastic filaments, or bio-inks are deposited onto surfaces. Additionally, the computational framework enables the study of a wide range of multiphase interfacial phenomena, from elastocapillarity to plastocapillarity.

cond-mat.soft↗

arXiv2023

Elastocapillary Worthington jets

The retraction of an impacting droplet on a non-wetting substrate is often associated with the formation of a Worthington jet, which is fed by the retracting liquid. A non-Newtonian rheology of the liquid is known to affect the retraction of the impacting droplet. Here we present a novel phenomenon related to the impact of viscoelastic droplets on non-wettable substrates. We reveal that the viscoelasticity of the liquid results in an \emph{elastocapillary} regime in the stretching Worthington jet, distinguished by a pinned contact line and a slender jet that does not detach from the droplet. We identify the impact conditions, in the Weber number -- Deborah number phase space, for observing these \emph{elastocapillary} Worthington jets. Such jets exhibit an effectively nearly linear (in time) variation of the strain rate. Upon further extension, the jet exhibits beads-on-a-string structures, characteristic of the \emph{elastocapillary} thinning of slender viscoelastic liquid filaments. The \emph{elastocapillary} Worthington jet is not only relevant for a droplet impact on a solid substrate scenario, but can also be expected in other configurations where a Worthington jet is observed for viscoelastic liquids, such as drop impact on a liquid pool and bubble bursting at an interface.

physics.flu-dyn↗

arXiv2022

Viscoplastic Lines: Printing a Single Filament of Yield Stress Material on a Surface

This study presents the spreading of a single filament of a yield stress (viscoplastic) fluid extruded onto a pre-wetted solid surface. The filaments spread laterally under surface tension forces until they reach a final equilibrium shape when the yield stress dominates. We use a simple experimental setup to print the filaments on a moving surface and measure their final width using optical coherence tomography. Additionally, we present a scaling law for the final width and determine the corresponding pre-factor using asymptotic analysis. We then analyse the level of agreement between the theory and experiments and discuss the possible origins of discrepancies. The process studied here has applications in extrusion-based thermoplastic and bio-3D printing.

physics.flu-dyn↗

arXiv2022

Interfacial aggregation of self-propelled Janus colloids in sessile droplets

Living microorganisms in confined systems typically experience an affinity to populate boundaries. The reason for such affinity to interfaces can be a combination of their directed motion and hydrodynamic interactions at distances larger than their own size. Here we will show that self-propelled Janus particles (polystyrene particles partially coated with platinum) immersed in droplets of water and hydrogen peroxide tend to accumulate in the vicinity of the liquid/gas interface. Interestingly, the interfacial accumulation occurs despite the presence of an evaporation-driven flow caused by a solutal Marangoni flow, which typically tends to redistribute the particles within the droplet's bulk. By performing additional experiments with passive colloids (flow tracers) and comparing with numerical simulations for both particle active motion and the fluid flow, we disentangle the dominating mechanisms behind the observed interfacial particle accumulation. These results allow us to make an analogy between active Janus particles and some biological microswimmers concerning how they interact with their environment.

physics.flu-dyn↗

arXiv2022

Spreading of droplets under various gravitational accelerations

We describe a setup to perform systematic studies on the spreading of droplets of complex fluids under microgravity conditions. Tweaking the gravitational acceleration under which droplets are deposited provides access to different regimes of the spreading dynamics, quantified through the Bond number. In particular, microgravity allows to form large droplets while remaining in the regime where surface tension effects and internal driving stresses are predominant over hydrostatic forces. The VIP-DROP2 experimental module provides a versatile platform to study a wide range of complex fluids through the deposition of axisymmetric droplets. The module offers the possibility to deposit droplets on a precursor layer, which can be composed of the same or of a different fluid. Besides, it allows to deposit four droplets simultaneously, while conducting shadowgraphy on all of them, and observing either the flow field (through particle image velocimetry), or the stress distribution inside the droplet in the case of stress birefringent fluids. Developed for a drop tower catapult system, it is designed to withstand a vertical acceleration of up to 30 times Earth's gravitational acceleration in the downwards direction, and can operate remotely, under microgravity conditions. We provide a detailed description of the module, and exemplary data analysis for droplets spreading on-ground and in microgravity.

physics.flu-dyn↗

arXiv2022

Chloroplasts in plant cells show active glassy behavior under low light conditions

Plants have developed intricate mechanisms to adapt to changing light conditions. Besides photo- and helio- tropism -- the differential growth towards light and the diurnal motion with respect to sunlight -- chloroplast motion acts as a fast mechanism to change the intracellular structure of leaf cells. While chloroplasts move towards the sides of the plant cell to avoid strong light, they accumulate and spread out into a layer on the bottom of the cell at low light to increase the light absorption efficiency. Although the motion of chloroplasts has been studied for over a century, the collective organelle-motion leading to light adapting self-organized structures remains elusive. Here we study the active motion of chloroplasts under dim light conditions, leading to an accumulation in a densely packed quasi-2D layer. We observe burst-like re-arrangements and show that these dynamics resemble colloidal systems close to the glass transition by tracking individual chloroplasts. Furthermore, we provide a minimal mathematical model to uncover relevant system parameters controlling the stability of the dense configuration of chloroplasts. Our study suggests that the meta-stable caging close to the glass-transition in the chloroplast mono-layer serves a physiological relevance. Chloroplasts remain in a spread-out configuration to increase the light uptake, but can easily fluidize when the activity is increased to efficiently re-arrange the structure towards an avoidance state. Our research opens new questions about the role that dynamical phase transitions could play in self-organized intracellular responses of plant cells towards environmental cues.

cond-mat.soft↗

arXiv2021

Crown formation from a cavitating bubble close to a free surface

A rapidly growing bubble close to a free surface induces jetting: a central jet protruding outwards and a crown surrounding it at later stages. While the formation mechanism of the central jet is known and documented, that of the crown remains unsettled. We perform axisymmetric simulations of the problem using the free software program basilisk, where a finite-volume compressible solver has been implemented, that uses a geometric Volume-of-Fluid method (VoF) for the tracking of the interface. We show that the mechanism of crown formation is a combination of a pressure distortion over the curved interface, inducing flow focusing, and of a flow reversal, caused by the second expansion of the toroidal bubble that drives the crown. The work culminates in a parametric study with the Weber number, the Reynolds number, the pressure ratio and the dimensionless bubble distance to the free surface as control parameters. Their effects on both the central jet and the crown are explored. For high Weber numbers, we observe the formation of weaker "secondary crowns", highly correlated with the third oscillation cycle of the bubble.

physics.flu-dyn↗

arXiv2021

Bursting Bubble in a Viscoplastic Medium

When a rising bubble in a Newtonian liquid reaches the liquid-air interface, it can burst, leading to the formation of capillary waves and a jet on the surface. Here, we numerically study this phenomenon in a yield stress fluid. We show how viscoplasticity controls the fate of these capillary waves and their interaction at the bottom of the cavity. Unlike Newtonian liquids, the free surface converges to a non-flat final equilibrium shape once the driving stresses inside the pool fall below the yield stress. Details of the dynamics, including the flow's energy budgets, are discussed. The work culminates in a regime map with four main regimes with different characteristic behaviours.

physics.flu-dyn↗

arXiv2021

Emergence of bimodal motility in active droplets

To explore and react to their environment, living micro-swimmers have developed sophisticated strategies for locomotion - in particular, motility with multiple gaits. To understand the physical principles associated with such a behavioural variability,synthetic model systems capable of mimicking it are needed. Here, we demonstrate bimodal gait switching in autophoretic droplet swimmers. This minimal experimental system is isotropic at rest, a symmetry that can be spontaneously broken due to the nonlinear coupling between hydrodynamic and chemical fields, inducing a variety of flow patterns that lead to different propulsive modes. We report a dynamical transition from quasi-ballistic to bimodal chaotic motion, controlled by the viscosity of the swimming medium. By simultaneous visualisation of the chemical and hydrodynamic fields, supported quantitatively by an advection-diffusion model, we show that higher hydrodynamic modes become excitable with increasing viscosity, while the recurrent mode-switching is driven by the droplet's interaction with self-generated chemical gradients. We further demonstrate that this gradient interaction results in anomalous diffusive swimming akin to self-avoiding spatial exploration strategies observed in nature.

cond-mat.soft↗

arXiv2020

Spreading of viscoplastic droplets

The spreading under surface tension and gravity of a droplet of yield-stress fluid over a thin film of the same material is studied. The droplet converges to a final equilibrium shape once the driving stresses inside the droplet fall below the yield stress. Scaling laws are presented for the final radius and complemented with an asymptotic analysis for shallow droplets. Moreover, numerical simulations using the volume-of-fluid method and a regularized constitutive law, and experiments with an aqueous solution of Carbopol are presented.

physics.flu-dyn↗

arXiv2020

Stress-Induced Dinoflagellate Bioluminescence at the Single Cell Level

One of the characteristic features of many marine dinoflagellates is their bioluminescence, which lights up nighttime breaking waves or seawater sliced by a ship's prow. While the internal biochemistry of light production by these microorganisms is well established, the manner by which fluid shear or mechanical forces trigger bioluminescence is still poorly understood. We report controlled measurements of the relation between mechanical stress and light production at the single-cell level, using high-speed imaging of micropipette-held cells of the marine dinoflagellate $Pyrocystis~lunula$ subjected to localized fluid flows or direct indentation. We find a viscoelastic response in which light intensity depends on both the amplitude and rate of deformation, consistent with the action of stretch-activated ion channels. A phenomenological model captures the experimental observations.

cond-mat.soft↗

arXiv2019

Ripples in Thin Films

Capillary ripples on thin viscous films are important features of coating and lubrication flows. Here we present experiments based on Digital Holographic Microscopy, measuring the morphology of capillary ripples ahead of a viscous drop spreading on a prewetted surface with a nanoscale resolution. Our experiments reveal that upon increasing the spreading velocity, the amplitude of the ripples first increases and subsequently decreases. Above a critical spreading velocity, the ripples even disappear completely and this transition is accompanied by a divergence of the ripple wavelength. These observations are explained quantitatively using linear wave analysis, beyond the usual lubrication approximation, illustrating that new phenomena arise when the capillary number becomes order unity.

physics.flu-dyn↗