arXiv subjects

Md. Shafayat Hossain

Publications and source records attributed to Md. Shafayat Hossain.

At least 19 recordsLinked to original sources

arXiv2026

Phonon Signatures of Near-Room-Temperature Phase Transition in Quasi-One-Dimensional Bi4I4 Topological van der Waals Material

The quasi-one-dimensional material Bi4I4 hosts two crystallographically similar polymorphs that realize distinct topological insulating phases separated by a first-order structural transition near room temperature. This transition occurs without a change in space group, arising instead from a subtle rearrangement of chain stacking registry. Polarization-resolved Raman spectroscopy directly resolves this structural-topological phase transition through abrupt, hysteretic modifications of the phonon spectrum. Angle-dependent measurements establish the symmetry of the dominant Raman-active modes and require a complex Raman tensor formalism to account for absorption-induced phase effects. Across the transition, selected phonon modes exhibit discontinuous, reversible shifts in frequency, linewidth, and relative intensity despite the absence of a space-group change. Density functional theory calculations reproduce the direction of the observed phonon renormalizations and confirm their sensitivity to stacking-dependent force constants. These results demonstrate that polarization-resolved Raman spectroscopy can detect subtle stacking-driven structural rearrangements that underlie topological band character, even when global crystallographic symmetry remains unchanged. The obtained results provide valuable insights into the interplay among lattice dynamics, structural distortions, and topological properties in this class of low-dimensional materials, with strong potential for unique functionalities.

cond-mat.mtrl-sci↗

arXiv2024

Tunable Topological Phase Transitions in a Piezoelectric Janus Monolayer

Quantum Spin Hall (QSH) insulators represent a quintessential example of a topological phase of matter, characterized by a conducting edge mode within a bulk energy gap. The pursuit of a tunable QSH state stands as a pivotal objective in the development of QSH-based topological devices. In this study, we employ first-principles calculations to identify three strain-tunable QSH insulators based on monolayer MAlGaTe4 (where M represents Mg, Ca, or Sr). These monolayers exhibit dynamic stability, with no imaginary modes detected in their phonon dispersion. Additionally, they possess piezoelectric properties, rendering them amenable to strain-induced tuning. While MgAlGaTe4 is a normal insulator under zero strain, it transitions into the QSH phase when subjected to external strain. Conversely, CaAlGaTe4 and SrAlGaTe4 already exhibit the QSH phase at zero strain. Intriguingly, upon the application of biaxial strain, these two compounds undergo phase transitions, encompassing metallic (M), normal/trivial insulator (NI), and topological insulator (TI) phases, thereby illustrating their strain-tunable electronic and topological properties. (Ca, Sr)AlGaTe4, in particular, undergo M-TI/TI-M transitions under applied strain, while MgAlGaTe4 additionally experiences an M-NI/NI-M transition, signifying it as a material featuring a metal-insulator transition (MIT). Remarkably, the observation of metal-trivial insulator-topological insulator transitions in MgAlGaTe4 introduces it as a unique material platform in which both MIT and topological phase transitions can be controlled through the same physical parameter. Our study thus introduces a novel material platform distinguished by highly strain-tunable electronic and topological properties, offering promising prospects for the development of next-generation, low-power topological devices.

cond-mat.mtrl-sci↗

arXiv2023

Valley-tunable, even-denominator fractional quantum Hall state in the lowest Landau level of an anisotropic system

Fractional quantum Hall states (FQHSs) at even-denominator Landau level filling factors ($ν$) are of prime interest as they are predicted to host exotic, topological states of matter. We report here the observation of a FQHS at $ν=1/2$ in a two-dimensional electron system of exceptionally high quality, confined to a wide AlAs quantum well, where the electrons can occupy multiple conduction-band valleys with an anisotropic effective mass. The anisotropy and multi-valley degree of freedom offer an unprecedented tunability of the $ν=1/2$ FQHS as we can control both the valley occupancy via the application of in-plane strain, and the ratio between the strengths of the short- and long-range Coulomb interaction by tilting the sample in the magnetic field to change the electron charge distribution. Thanks to this tunability, we observe phase transitions from a compressible Fermi liquid to an incompressible FQHS and then to an insulating phase as a function of tilt angle. We find that this evolution and the energy gap of the $ν=1/2$ FQHS depend strongly on valley occupancy.

cond-mat.mes-hall↗

arXiv2022

Imaging real-space flat band localization in kagome magnet FeSn

Kagome lattices host flat bands due to their frustrated lattice geometry, which leads to destructive quantum interference of electron wave functions. Here, we report imaging of the kagome flat band localization in real-space using scanning tunneling microscopy. We identify both the Fe3Sn kagome lattice layer and the Sn2 honeycomb layer with atomic resolution in kagome antiferromagnet FeSn. On the Fe3Sn lattice, at the flat band energy determined by the angle resolved photoemission spectroscopy, tunneling spectroscopy detects an unusual state localized uniquely at the Fe kagome lattice network. We further show that the vectorial in-plane magnetic field manipulates the spatial anisotropy of the localization state within each kagome unit cell. Our results are consistent with the real-space flat band localization in the magnetic kagome lattice. We further discuss the magnetic tuning of flat band localization under the spin-orbit coupled magnetic kagome lattice model.

cond-mat.str-el↗

arXiv2022

Fractional quantum Hall valley ferromagnetism in the extreme quantum limit

Electrons' multiple quantum degrees of freedom can lead to rich physics, including a competition between various exotic ground states, as well as novel applications such as spintronics and valleytronics. Here we report magneto-transport experiments demonstrating how the valley degree of freedom impacts the fractional quantum states (FQHSs), and the related magnetic-flux-electron composite fermions (CFs), at very high magnetic fields in the extreme quantum limit when only the lowest Landau level is occupied. Unlike in other multivalley two-dimensional electron systems such as Si or monolayer graphene and transition-metal dichalcogenides, in our AlAs sample we can continuously tune the valley polarization via the application of in-situ strain. We find that the FQHSs remain exceptionally strong even as they make valley polarization transitions, revealing a surprisingly robust ferromagnetism of the FQHSs and the underlying CFs. Our observation implies that the CFs are strongly interacting in our system. We are also able to obtain a phase diagram for the FQHS and CF valley polarization in the extreme quantum limit as we monitor transitions of the FHQSs with different valley polarizations.

cond-mat.mes-hall↗

arXiv2022

Discovery of charge order and corresponding edge state in kagome magnet FeGe

Kagome materials often host exotic quantum phases, including spin liquids, Chern gap, charge order, and superconductivity. Existing scanning microscopy studies of the kagome charge order have been limited to non-kagome surface layers. Here we tunnel into the kagome lattice of FeGe to uncover features of the charge order. Our spectroscopic imaging identifes a 2x2 charge order in the magnetic kagome lattice, resembling that discovered in kagome superconductors. Spin-mapping across steps of unit-cell-height demonstrates that this charge order emerges from spin-polarized electrons with an antiferromagnetic stacking order. We further uncover the correlation between antiferromagnetism and charge order anisotropy, highlighting the unusual magnetic coupling of the charge order. Finally, we detect a pronounced edge state within the charge order energy gap, which is robust against the irregular shape of the kagome lattice edges. We discuss our results with the theoretically considered topological features of the kagome charge order including orbital magnetism and bulk-boundary correspondence.

cond-mat.str-el↗

arXiv2022

Magnetization-direction-tunable kagome Weyl line

Kagome magnets provide a fascinating platform for a plethora of topological quantum phenomena. Here, utilizing angle-resolved photoemission spectroscopy, we demonstrate Weyl lines with strong out-of-plane dispersion in an A-A stacked kagome magnet TbxGd1-xMn6Sn6. On the Gd rich side, the Weyl line remains nearly spin-orbit-gapless due to a remarkable cooperative interplay between Kane-Mele spin-orbit-coupling, low site symmetry and in-plane magnetic order. Under Tb substitution, the kagome Weyl line gaps due to a magnetic reorientation to out-of-plane order. Our results illustrate the magnetic moment direction as an efficient tuning knob for realizing distinct three-dimensional topological phases.

cond-mat.str-el↗

arXiv2022

Visualizing the out-of-plane electronic dispersions in an intercalated transition metal dichalcogenide

Layered transition metal dichalcogenides have rich phase diagram and they feature two dimensionality on numerous physical properties. Co1/3NbS2 is one of the newest members of this family where Co atoms are intercalated into the Van der Waals gaps between NbS2 layers. We study the three-dimensional electronic band structure of Co1/3NbS2 using both surface and bulk sensitive angle-resolved photoemission spectroscopy. We show that the electronic bands do not fit into the rigid-band-shift picture after the Co intercalation. Instead, Co1/3NbS2 displays a different orbital character near the Fermi level compared to the pristine NbS2 compound and has a clear band dispersion in kz direction despite its layered structure. Our photoemission study demonstrates the out-of-plane electronic correlations introduced by the Co intercalation, thus offering a new perspective on this compound. Finally, we propose how Fermi level tuning could lead to exotic phases such as spin density wave instability.

cond-mat.mtrl-sci↗

arXiv2020

Competition between fractional quantum Hall liquid and Wigner solid at small fillings: Role of layer thickness and Landau level mixing

What is the fate of the ground state of a two-dimensional electron system (2DES) at very low Landau level filling factors ($ν$) where interaction reigns supreme? An ordered array of electrons, the so-called Wigner crystal, has long been believed to be the answer. It was in fact the search for the elusive Wigner crystal that led to the discovery of an unexpected, incompressible liquid state, namely the fractional quantum Hall state at $ν=1/3$. Understanding the competition between the liquid and solid ground states has since remained an active field of fundamental research. Here we report experimental data for a new two-dimensional system where the electrons are confined to an AlAs quantum well. The exceptionally high quality of the samples and the large electron effective mass allow us to determine the liquid-solid phase diagram for the two-dimensional electrons in a large range of filling factors near $\simeq 1/3$ and $\simeq 1/5$. The data and their comparison with an available theoretical phase diagram reveal the crucial role of Landau level mixing and finite electron layer thickness in determining the prevailing ground states.

cond-mat.mes-hall↗

arXiv2020

Bloch Ferromagnetism of Composite Fermions

In 1929 Felix Bloch suggested that the paramagnetic Fermi sea of electrons should make a spontaneous transition to a fully-magnetized state at very low densities, because the exchange energy gained by aligning the spins exceeds the enhancement in the kinetic energy. We report here the observation of an abrupt, interaction-driven transition to full magnetization, highly reminiscent of Bloch ferromagnetism that has eluded experiments for the last ninety years. Our platform is the exotic two-dimensional Fermi sea of composite fermions at half-filling of the lowest Landau level. Via quantitative measurements of the Fermi wavevector, which provides a direct measure of the spin polarization, we observe a sudden transition from a partially-spin-polarized to a fully-spin-polarized ground state as we lower the composite fermions' density. Our detailed theoretical calculations provide a semi-quantitative account of this phenomenon.

cond-mat.str-el↗

arXiv2019

Geometric Resonance of Four-Flux Composite Fermions

Two-dimensional interacting electrons exposed to strong perpendicular magnetic fields generate emergent, exotic quasiparticles phenomenologically distinct from electrons. Specifically, electrons bind with an even number of flux quanta, and transform into composite fermions (CFs). Besides providing an intuitive explanation for the fractional quantum Hall states, CFs also possess Fermi-liquid-like properties, including a well-defined Fermi sea, at and near even-denominator Landau level filling factors such as $ν=1/2$ or $1/4$. Here, we directly probe the Fermi sea of the rarely studied four-flux CFs near $ν=1/4$ via geometric resonance experiments. The data reveal some unique characteristics. Unlike in the case of two-flux CFs, the magnetic field positions of the geometric resonance resistance minima for $ν<1/4$ and $ν>1/4$ are symmetric with respect to the position of $ν=1/4$. However, when an in-plane magnetic field is applied, the minima positions become asymmetric, implying a mysterious asymmetry in the CF Fermi sea anisotropy for $ν<1/4$ and $ν>1/4$. This asymmetry, which is in stark contrast to the two-flux CFs, suggests that the four-flux CFs on the two sides of $ν=1/4$ have very different effective masses, possibly because of the proximity of the Wigner crystal formation at small $ν$.

cond-mat.str-el↗

arXiv2018

Unconventional anisotropic even-denominator fractional quantum Hall state in a system with mass anisotropy

The fractional quantum Hall state (FQHS) observed at a half-filled Landau level in an interacting two-dimensional electron system (2DES) is among the most exotic states of matter as its quasiparticles are expected to be Majoranas with non-Abelian statistics. We demonstrate here the unexpected presence of such a state in a novel 2DES with a strong band-mass anisotropy. The FQHS we observe has unusual characteristics. While its Hall resistance is well-quantized at low temperatures, it exhibits highly-anisotropic in-plane transport resembling compressible stripe/nematic charge-density-wave phases. More striking, the anisotropy sets in suddenly below a critical temperature, suggesting a finite-temperature phase transition. Our observations highlight how anisotropy modifies the many-body phases of a 2DES, and should further fuel the discussion surrounding the enigmatic even-denominator FQHS.

cond-mat.mes-hall↗

arXiv2018

Anomalous coupling between magnetic and nematic orders in quantum Hall systems

The interplay between different orders is of fundamental importance in physics. The spontaneous, symmetry-breaking charge order, responsible for the stripe or the nematic phase, has been of great interest in many contexts where strong correlations are present, such as high-temperature superconductivity and quantum Hall effect. In this article we show the unexpected result that in an interacting two-dimensional electron system, the robustness of the nematic phase, which represents an order in the charge degree of freedom, not only depends on the orbital index of the topmost, half-filled Landau level, but it is also strongly correlated with the magnetic order of the system. Intriguingly, when the system is fully magnetized, the nematic phase is particularly robust and persists to much higher temperatures compared to the nematic phases observed previously in quantum Hall systems. Our results give fundamental new insight into the role of magnetization in stabilizing the nematic phase, while also providing a new knob with which it can be effectively tuned.

cond-mat.mes-hall↗

arXiv2018

Realization of a Valley Superlattice

In a number of widely-studied materials, such as Si, AlAs, Bi, graphene, MoS2, and many transition metal dichalcogenide monolayers, electrons acquire an additional, spin-like degree of freedom at the degenerate conduction band minima, also known as "valleys". External symmetry breaking fields such as mechanical strain, or electric or magnetic fields, can tune the valley-polarization of these materials making them suitable candidates for "valleytronics". Here we study a quantum well of AlAs, where the two-dimensional electrons reside in two energetically degenerate valleys. By fabricating a strain-inducing grating on the sample surface, we engineer a spatial modulation of the electron population in different valleys, i.e., a "valley superlattice" in the quantum well plane. Our results establish a novel manipulation technique of the valley degree of freedom, paving the way to realizing a valley-selective layered structure in multi-valley materials, with potential application in valleytronics.

cond-mat.mes-hall↗

arXiv2018

Direct observation of composite fermions and their fully spin-polarized Fermi sea near $ν=5/2$

The enigmatic even-denominator fractional quantum Hall state at Landau level filling factor $ν=5/2$ is arguably the most promising candidate for harboring Majorana quasi-particles with non-Abelian statistics and thus of potential use for topological quantum computing. The theoretical description of the $ν=5/2$ state is generally believed to involve a topological p-wave pairing of fully spin-polarized composite fermions through their condensation into a non-Abelian Moore-Read Pfaffian state. There is, however, no direct and conclusive experimental evidence for the existence of composite fermions near $ν=5/2$ or for an underlying fully spin-polarized Fermi sea. Here, we report the observation of composite fermions very near $ν=5/2$ through geometric resonance measurements, and find that the measured Fermi wavevector provides direct demonstration of a Fermi sea with full spin polarization. This lends crucial credence to the model of $5/2$ fractional quantum Hall effect as a topological p-wave paired state of composite fermions.

cond-mat.mes-hall↗

arXiv2017

Observation of fractional quantum Hall effect in an InAs quantum well

The two-dimensional electron system in an InAs quantum well has emerged as a prime candidate for hosting exotic quasi-particles with non-Abelian statistics such as Majorana fermions and parafermions. To attain its full promise, however, the electron system has to be clean enough to exhibit electron-electron interaction phenomena. Here we report the observation of fractional quantum Hall effect in a very low disorder InAs quantum well with a well-width of 24 nm, containing a two-dimensional electron system with a density $n=7.8 \times 10^{11}$ cm$^{-2}$ and low-temperature mobility $1.8 \times 10^6$ cm$^2$/Vs. At a temperature of $\simeq35$ mK and $B\simeq24$ T, we observe a deep minimum in the longitudinal resistance, accompanied by a nearly quantized Hall plateau at Landau level filling factor $ν=4/3$.

physics.app-ph↗

arXiv2017

Search for Composite Fermions at Filling Factor 5/2: Role of Landau Level and Subband Index

The pairing of composite fermions (CFs), electron-flux quasi-particles, is commonly proposed to explain the even-denominator fractional quantum Hall state observed at $ν=5/2$ in the first excited ($N=1$) Landau level (LL) of a two-dimensional electron system (2DES). While well-established to exist in the lowest ($N=0$) LL, much is unknown about CFs in the $N=1$ LL. Here we carry out geometric resonance measurements to detect CFs at $ν=5/2$ by subjecting the 2DES to a one-dimensional density modulation. Our data, taken at a temperature of 0.3 K, reveal no geometric resonances for CFs in the $N=1$ LL. In stark contrast, we observe clear signatures of such resonances when $ν=5/2$ is placed in the $N=0$ LL of the anti-symmetric subband by varying the 2DES width. This finding implies that the CFs' mean-free-path is significantly smaller in the $N=1$ LL compared to the $N=0$ LL. Our additional data as a function of in-plane magnetic field highlight the role of subband index and establish that CFs at $ν=5/2$ in the $N=0$ LL are more anisotropic in the symmetric subband than in the anti-symmetric subband.

cond-mat.mes-hall↗

arXiv2016

Reorientation of the stripe Phase of 2D Electrons by a Minute Density Modulation

Interacting two-dimensional electrons confined in a GaAs quantum well exhibit isotropic transport when the Fermi level resides in the first excited ($N=1$) Landau level. Adding an in-plane magnetic field ($B_{||}$) typically leads to an anisotropic, stripe-like (nematic) phase of electrons with the stripes oriented perpendicular to the $B_{||}$ direction. Our experimental data reveal how a periodic density modulation, induced by a surface strain grating from strips of negative electron-beam resist, competes against the $B_{||}$-induced orientational order of the stripe phase. Even a minute ($<0.25\%$) density modulation is sufficient to reorient the stripes along the direction of the surface grating.

cond-mat.mes-hall↗