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Mengkun Liu

Publications and source records attributed to Mengkun Liu.

At least 19 recordsLinked to original sources

Scalable, Simple, and Versatile Encapsulation of 2D Materials and Devices

Air-sensitive 2D materials present a fundamental challenge for device integration. Encapsulation is often required to preserve intrinsic properties, yet conventional protection strategies often fail for thicker layers and complicate fabrication. Here, we demonstrate that electron-beam (e-beam) evaporated aluminum oxide ($\mathrm{AlO}_x$) serves as both an effective encapsulation layer and a platform for direct device fabrication. Unlike transfer-based approaches, this scalable method is compatible with thicker flakes and full device or wafer coverage. It requires no stacking procedures and enables contacts without post-encapsulation etching. Using rare-earth tritellurides ($\mathrm{RTe}_3$, R = La, Er), semimetallic $\mathrm{WTe}_2$, and superconducting $\mathrm{FeTe}_x\mathrm{Se}_{1-x}$, we show that $\mathrm{AlO}_x$ suppresses oxidation and preserves intrinsic optical and electronic properties. We establish substrate-dependent optimization of encapsulation across a range of flake thicknesses, demonstrate that ultrathin $\mathrm{AlO}_x$ preserves $\mathrm{WTe}_2$'s plasmonic response and maintains superconducting performance in $\mathrm{FeTe}_x\mathrm{Se}_{1-x}$. Thus we overcome the longstanding tradeoff between encapsulation and straightforward device fabrication in fragile quantum materials.

cond-mat.mes-hall

Quantum Light Nano-Imaging

Entanglement and quantum correlations are central to the physics of quantum materials, yet they have remained notoriously difficult to access experimentally. Accessing these phenomena in solids requires quantum optical probes that operate at the native length and time scales of material excitations, below the diffraction limit of light. Developing the requisite tools has previously been infeasible due to the weak intensities of state-of-the-art quantum light sources and the inefficiency of light coupling in near-field light-matter interactions. In this work, we address these challenges and report the development of a quantum light scattering-type scanning near-field optical microscope (q-SNOM) that enables quantum-optical studies of solid-state systems with nanoscale spatial resolution. As a first demonstration, we visualize the self-interference of single hybrid light-matter polaritons in the prototypical van der Waals semiconductor MoS2. We also introduce a polaritonic time-of-flight metrology that exploits the temporal correlations among entangled photons to observe the quasiparticle propagation dynamics at femtosecond time scales. This work establishes a new experimental paradigm for exploring quantum effects in materials at the nanoscale.

cond-mat.mes-hall

Magnetic-field-tunable cyclotron hyperbolic polaritons

Hyperbolic polaritons are conventionally associated with structural anisotropy or phononic Reststrahlen bands. Here, we predict a new class of hyperbolic polaritons arising from magnetic-field-induced cyclotron motion of charge carriers. When a perpendicular magnetic field is applied to high-mobility semimetals, the cyclotron response drives the in-plane dielectric function from metallic- to insulating-like below the cyclotron resonance frequency, while the out-of-plane response remains metallic. This anisotropy creates a hyperbolic dielectric environment that supports field-tunable hyperbolic polaritons. We develop a comprehensive theoretical framework incorporating coupling to other collective excitations and show that these modes can be directly visualized in real space via terahertz near-field nanoscopy. Our work identifies cyclotron motion as a new route to hyperbolic polaritons and establishes a versatile platform for magnetically programmable nanophotonics.

cond-mat.mes-hall

Quantum cascade laser roadmap

Quantum cascade lasers (QCLs) are unipolar semiconductor lasers first demonstrated in 1994. Since then, they have played a central role in advancing mid-infrared and terahertz photonics, becoming among the most reliable light sources in these regions of the electromagnetic spectrum. Their importance is further reinforced by their ability to generate self-starting optical frequency combs, whose investigation is motivated both by fundamental physics and by a wide range of applications, including molecular spectroscopy and free-space optical communications. This Roadmap provides a unified overview of current advances and emerging directions in QCL research. The chapters are organized into three main sections: device design and technology; frequency combs and pulse formation; and applications of QCLs. Each chapter reviews the relevant background, summarizes the current state of the art, and identifies key challenges and future directions within its specific research area.

physics.optics

Plasmon dynamics in graphene

Plasmon are collective oscillations of mobile electrons with dynamics controlled by their charge stiffness("Drude weight"). Using terahertz spacetime metrology, we probe Plasmon dynamics of mono- and bi-layer graphene. In both systems, the experimentally measured Drude weight systematically exceeds the prediction based on non-interacting electronic system. The relative enhancement increases as the carrier density decreases. We attribute the observed deviation to the interplay of interactions and wave function structure of the Dirac fermions in multi-layer graphene. Our results establish that pseudospin structure of the single-particle electronic wave function can directly influence collective excitations, with implications that extend beyond graphene to a broad class of quantum materials.

cond-mat.mes-hall

Lessons from $\alpha$-RuCl3 for pursuing quantum spin liquid physics in atomically thin materials

Quantum spin liquids can arise from Kitaev magnetic interactions, and exhibit fractionalized excitations with the potential for a topological form of quantum computation. This review surveys recent experimental and theoretical progress on the pursuit of phenomena related to Kitaev magnetism in layered and exfoliatable materials, which offer numerous opportunities to apply powerful techniques from the field of atomically thin materials. We primarily focus on the antiferromagnetic Mott insulator $\alpha$-RuCl3, which exhibits Kitaev couplings and is readily exfoliated to single- or few-layer sheets, and thus serves as a test bed for developing probes of Kitaev phenomena in atomically thin materials and devices. We introduce the Kitaev model and how it is realized in $\alpha$-RuCl3 and other material candidates; and cover $\alpha$-RuCl3 synthesis and fabrication into van der Waals heterostructure devices. A key discovery is a work-function-mediated charge transfer that heavily dopes both the $\alpha$-RuCl3 and proximate materials, and can enhance Kitaev interactions by up to 50%. We further discuss a wide range of recent results in electronic transport and optical and tunneling spectroscopies of $\alpha$-RuCl3 devices. The experimental techniques and theoretical insights developed for $\alpha$-RuCl3 establish a framework for discovering and engineering superior two-dimensional Kitaev materials that may ultimately realize elusive quantum spin liquid phases.

cond-mat.str-el

Polaritonic Quantum Matter

Polaritons are quantum mechanical superpositions of photon states with elementary excitations in molecules and solids. The light-matter admixture causes a characteristic frequency-momentum dispersion shared by all polaritons irrespective of the microscopic nature of material excitations that could entail charge, spin, lattice or orbital effects. Polaritons retain the strong nonlinearities of their matter component and simultaneously inherit ray-like propagation of light. Polaritons prompt new properties, enable new opportunities for spectroscopy/imaging, empower quantum simulations and give rise to new forms of synthetic quantum matter. Here, we review the emergent effects rooted in polaritonic quasiparticles in a wide variety of their physical implementations. We present a broad portfolio of the physical platforms and phenomena of what we term polaritonic quantum matter. We discuss the unifying aspects of polaritons across different platforms and physical implementations and focus on recent developments in: polaritonic imaging, cavity electrodynamics and cavity materials engineering, topology and nonlinearities, as well as quantum polaritonics.

cond-mat.mtrl-sci

Bolometric Superconducting Optical Nanoscopy (BOSON)

Superconducting transition-edge sensors are renowned for their extraordinary photon sensitivity and energy resolution, finding applications spanning quantum information, astronomy, and nanophotonics. Here, we report the development of BOlometric Superconducting Optical Nanoscopy (BOSON), a novel platform that integrates bolometric detection at the superconducting transition edges with near-field optical techniques. BOSON enables the mapping of photoinduced changes in superconductivity with unprecedented spatial resolution and photon sensitivity. By incorporating BOSON with low-dimensional materials, we achieved polariton imaging at nanowatt excitation levels--at least four orders of magnitude lower than the power typically required in prior near-field nanoscopy experiments. Our findings highlight the potential for BOSON to advance scanning probe based optical platforms to enable the detection of photons, polaritons, and Cooper pair dynamics at the nanoscale. This paves the way for quantum sensing applications using single-polariton detection and can offer deeper insights into quasiparticle dynamics.

quant-ph

Photocurrent Nanoscopy of Quantum Hall Bulk

Understanding nanoscale electronic and thermal transport of two-dimensional (2D) electron systems in the quantum Hall regime, particularly in the bulk insulating state, poses considerable challenges. One of the primary difficulties arises from the presence of chiral edge channels, whose transport behavior obscures the investigation of the insulating bulk. Using near-field (NF) optical and photocurrent (PC) nanoscopy, we probe real-space variations of the optical and thermal dynamics of graphene in the quantum Hall regime without relying on complex sample or electrode geometries. Near the charge neutrality point (CNP), we detect strong optical and photothermal signals from resonant inter-Landau level (LL) magnetoexciton excitations between the 0th and +-1st LLs, which gradually weaken with increasing doping due to Pauli blocking. Interestingly, at higher doping levels and full integer LL fillings, photothermal signals reappear across the entire sample over a ~10-micrometer scale, indicating unexpectedly long cooling lengths and nonlocal photothermal heating through the insulating bulk. This observation suggests thermal conductivity persists for the localized states even as electronic transport is suppressed - a clear violation of the Wiedemann-Franz (WF) law. Our experiments provide novel insights into nanoscale thermal and electronic transport in incompressible 2D gases, highlighting the roles of magnetoexcitons and chiral edge states in the thermo-optoelectric dynamics of Dirac quantum Hall state.

cond-mat.mes-hall

Terahertz-induced tunnel ionization drives coherent Raman-active phonon in Bismuth

Driving coherent lattice motion with THz pulses has emerged as a novel pathway for achieving dynamic stabilization of exotic phases that are inaccessible in equilibrium quantum materials. In this work, we present a previously unexplored mechanism for THz excitation of Raman-active phonons. We show that intense THz pulses centered at 1 THz can excite the Raman-active $A_{1g}$ phonon mode at 2.9 THz in a bismuth film. We rule out the possibilities of the phonon being excited through conventional anharmonic coupling to other modes or via a THz sum frequency process. Instead, we demonstrate that the THz-driven tunnel ionization provides a plausible means of creating a displacive driving force to initiate the phonon oscillations. Our work highlights a new mechanism for exciting coherent phonons, offering potential for dynamic control over the electronic and structural properties of semimetals and narrow-band semiconductors on ultrafast timescales.

cond-mat.mes-hall

Electronic structure, magnetic and transport properties of antiferromagnetic Weyl semimetal GdAlSi

We report the topological electronic structure, magnetic, and magnetotransport properties of a noncentrosymmetric compound GdAlSi. Magnetic susceptibility shows an antiferromagnetic transition at $T_\mathrm{N}$ = 32 K. In-plane isothermal magnetization exhibits an unusual hysteresis behavior at higher magnetic field, rather than near zero field. Moreover, the hysteresis behavior is asymmetric under positive and negative magnetic fields. First-principles calculations were performed on various magnetic configurations, revealing that the antiferromagnetic state is the ground state, and the spiral antiferromagnetic state is a close competing state. The calculations also reveal that GdAlSi hosts multiple Weyl points near the Fermi energy. The band structure measured by angle-resolved photoemission spectroscopy (ARPES) shows relatively good agreement with the theory, with the possibility of Weyl nodes slightly above the Fermi energy. Within the magnetic ordered state, we observe an exceptionally large anomalous Hall conductivity (AHC) of ~ 1310 $\Omega^{-1}$cm$^{-1}$ at 2 K. Interestingly, the anomalous Hall effect persists up to room temperature with a significant value of AHC (~ 155 $\Omega^{-1}$cm$^{-1}$). Our analysis indicates that the large AHC originates from the Berry curvature associated with the multiple pairs of Weyl points near Fermi energy.

cond-mat.str-el

Nano-Imaging of Landau-Phonon Polaritons in Dirac Heterostructures

Polaritons are light-matter quasiparticles that govern the optical response of quantum materials and enable their nanophotonic applications. We have studied a new type of polaritons arising in magnetized graphene encapsulated in hexagonal boron nitride (hBN). These polaritons stem from hybridization of Dirac magnetoexciton modes of graphene with waveguide phonon modes of hBN crystals. We refer to these quasiparticles as the Landau-phonon polaritons (LPPs). Using infrared magneto nanoscopy, we imaged LPPs and controlled their real-space propagation by varying the magnetic field. These LLPs have large in-plane momenta and are not bound by the conventional optical selection rules, granting us access to the "forbidden" inter-Landau level transitions (ILTs). We observed avoided crossings in the LPP dispersion - a hallmark of the strong coupling regime - occurring when the magnetoexciton and hBN phonon frequencies matched. Our LPP-based nanoscopy also enabled us to resolve two fundamental many-body effects: the graphene Fermi velocity renormalization and ILT-dependent magnetoexciton binding energies. These results indicate that magnetic-field-tuned Dirac heterostructures are promising platforms for precise nanoscale control and sensing of light-matter interaction.

physics.optics

Electronic interactions in Dirac fluids visualized by nano-terahertz spacetime interference of electron-photon quasiparticles

Ultraclean graphene at charge neutrality hosts a quantum critical Dirac fluid of interacting electrons and holes. Interactions profoundly affect the charge dynamics of graphene, which is encoded in the properties of its electron-photon collective modes: surface plasmon polaritons (SPPs). Here we show that polaritonic interference patterns are particularly well suited to unveil the interactions in Dirac fluids by tracking polaritonic interference in time at temporal scales commensurate with the electronic scattering. Spacetime SPP interference patterns recorded in tera-hertz (THz) frequency range provided unobstructed readouts of the group velocity and lifetime of polariton that can be directly mapped onto the electronic spectral weight and the relaxation rate. Our data uncovered prominent departures of the electron dynamics from the predictions of the conventional Fermi-liquid theory. The deviations are particularly strong when the densities of electrons and holes are approximately equal. The proposed spacetime imaging methodology can be broadly applied to probe the electrodynamics of quantum materials.

cond-mat.str-el

Harnessing excitons at the nanoscale -- photoelectrical platform for quantitative sensing and imaging

Excitons -- quasiparticles formed by the binding of an electron and a hole through electrostatic attraction -- hold promise in the fields of quantum light confinement and optoelectronic sensing. Atomically thin transition metal dichalcogenides (TMDs) provide a versatile platform for hosting and manipulating excitons, given their robust Coulomb interactions and exceptional sensitivity to dielectric environments. In this study, we introduce a cryogenic scanning probe photoelectrical sensing platform, termed exciton-resonant microwave impedance microscopy (ER-MIM). ER-MIM enables ultra-sensitive probing of exciton polarons and their Rydberg states at the nanoscale. Utilizing this technique, we explore the interplay between excitons and material properties, including carrier density, in-plane electric field, and dielectric screening. Furthermore, we employ deep learning for automated data analysis and quantitative extraction of electrical information, unveiling the potential of exciton-assisted nano-electrometry. Our findings establish an invaluable sensing platform and readout mechanism, advancing our understanding of exciton excitations and their applications in the quantum realm.

cond-mat.mes-hall

Visualizing moiré ferroelectricity via plasmons and nano-photocurrent in graphene/twisted-WSe2 structures

Ferroelectricity, a spontaneous and reversible electric polarization, is found in certain classes of van der Waals (vdW) material heterostructures. The discovery of ferroelectricity in twisted vdW layers provides new opportunities to engineer spatially dependent electric and optical properties associated with the configuration of moiré superlattice domains and the network of domain walls. Here, we employ near-field infrared nano-imaging and nano-photocurrent measurements to study ferroelectricity in minimally twisted WSe2. The ferroelectric domains are visualized through the imaging of the plasmonic response in a graphene monolayer adjacent to the moiré WSe2 bilayers. Specifically, we find that the ferroelectric polarization in moiré domains is imprinted on the plasmonic response of the graphene. Complementary nano-photocurrent measurements demonstrate that the optoelectronic properties of graphene are also modulated by the proximal ferroelectric domains. Our approach represents an alternative strategy for studying moiré ferroelectricity at native length scales and opens promising prospects for (opto)electronic devices.

cond-mat.mes-hall

Machine Learning for Optical Scanning Probe Nanoscopy

The ability to perform nanometer-scale optical imaging and spectroscopy is key to deciphering the low-energy effects in quantum materials, as well as vibrational fingerprints in planetary and extraterrestrial particles, catalytic substances, and aqueous biological samples. The scattering-type scanning near-field optical microscopy (s-SNOM) technique has recently spread to many research fields and enabled notable discoveries. In this brief perspective, we show that the s-SNOM, together with scanning probe research in general, can benefit in many ways from artificial intelligence (AI) and machine learning (ML) algorithms. We show that, with the help of AI- and ML-enhanced data acquisition and analysis, scanning probe optical nanoscopy is poised to become more efficient, accurate, and intelligent.

physics.optics

Deep-Learning-Aided Extraction of Optical Constants in Scanning Near-Field Optical Microscopy

Scanning near-field optical microscopy is one of the most effective techniques for spectroscopy of nanoscale systems. However, inferring optical constants from the measured near-field signal can be challenging because of a complicated and highly nonlinear interaction between the scanned probe and the sample. Conventional fitting methods applied to this problem often suffer from the lack of convergence or require human intervention. Here we develop an alternative approach where the optical parameter extraction is automated by a deep learning network. Compared to its traditional counterparts, our method demonstrates superior accuracy, stability against noise, and computational speed when applied to simulated near-field spectra.

physics.optics