arXiv subjects

Michael G. Raymer

Publications and source records attributed to Michael G. Raymer.

At least 19 recordsLinked to original sources

arXiv2025

High-fidelity, quasi-deterministic entanglement generation using phase-matched spectral islands in a zero-added-loss multiplexing architecture

Spontaneous parametric down-converters (SPDCs) are the best available entanglement sources for distributing entanglement in a quantum internet. However, their intrinsically probabilistic nature, and their need to operate at low brightness to suppress multipair events, dictate that multiplexed SPDC arrays are required for high-rate distribution in that application. Early SPDC multiplexing proposals involved path switching, whose switching losses significantly degrade performance. The present paper proposes and analyzes a scheme for spectral multiplexing that provides entanglement-distribution rates well in excess of the state of the art. It builds on zero-added-loss multiplexing (ZALM)~[Phys. Rev. Appl. {\bf 19}, 054029 (2023)] for high-rate heralded entanglement generation, which does not require a switched array of SPDCs. Our ZALM's SPDCs rely on nonlinear crystals with $N_I$ phase-matched spectral islands, each generating two-mode squeezed-vacuum states. Also, our ZALM's multiplexing protocol uses both same-island and cross-island heralding, which allows the entanglement-delivery rate to approximately scale as $N_I^2$ in the realistic weak-squeezing regime. As a result, our scheme uses an order of magnitude fewer spectral channels than the original ZALM proposal, which may enable near-term implementations of satellite-to-ground or fiber-optic based ZALM architectures.

quant-ph↗

arXiv2025

Spectral compression of single-photon wave packets by sum-frequency conversion in slow-light waveguides

A slow-light scheme is proposed for simultaneous frequency conversion and spectral compression of a weak optical pulse, which may be in any quantum state including a single-photon state. Such a process plays crucial roles in a number of schemes for constructing quantum networks. Assuming that appropriate slow-light waveguides can be fabricated, theoretical modeling shows that a 3-ps pulse can be converted by sum-frequency generation into a pulse with duration in the ns regime with a corresponding spectral compression factor of the order of 1000 and a useful intrinsic efficiency up to 83%. Independent of the input pulse shape, the converted pulse will have a near-exponential rising shape, which is suitable for temporal-mode matching into an optical cavity.

quant-ph↗

arXiv2024

Entanglement source and quantum memory analysis for zero added-loss multiplexing

High-rate, high-fidelity entanglement distribution is essential to the creation of a quantum internet, but recent achievements in fiber and satellite-based entanglement distribution fall far short of what is needed. Chen et al. [Phys. Rev. Appl. 19, 054209 (2023)] proposed a means for dramatically increasing entanglement-distribution rates via zero added-loss multiplexing (ZALM). ZALM's quantum transmitter employs a pair of Sagnac-configured spontaneous parametric downconverters (SPDCs), channelization via dense wavelength-division multiplexing (DWDM) filtering, and partial Bell-state measurements (BSMs) to realize a heralded source of frequency-multiplexed polarization-entangled biphotons. Each biphoton is transmitted to Alice and Bob with a classical message identifying its frequency channel and the heralded entangled state. Their quantum receivers use DWDM filtering and mode conversion to interface their received biphotons to intra-cavity color-center quantum memories. This paper delves deeply into ZALM's SPDCs, partial-BSMs, and loading of Alice and Bob's quantum memories. It derives the density operators for the SPDC sources and the quantum memories, allowing heralding probability, heralding efficiency, and fidelity to be evaluated for both the polarization-entangled biphotons and the loaded quantum memories, thus enabling exploration of the parameter space for optimizing ZALM performance. Even without optimization analysis, the paper already demonstrates two critical features of the ZALM architecture: the necessity of achieving a near-separable channelized biphoton wave function to ensure the biphoton sent to Alice and Bob is of high purity; and the premium placed on Alice and Bob's temporal-mode converters' enabling narrowband push-pull memory loading to ensure the arriving biphoton's state is faithfully transferred to the intra-cavity color centers.

quant-ph↗

arXiv2024

The Duan-Kimble cavity-atom quantum memory loading scheme revisited

We reexamine the well-known Duan-Kimble entanglement scheme, wherein the state of a single-photon qubit is entangled with a quantum memory consisting of a single-atom qubit in a strongly coupled optical cavity, providing the capability to load the photon's state into the memory. We correct a common error appearing in some subsequent papers regarding the validity of the single-photon reflectivity function that characterizes the essential phase shift at the heart of the protocol. Using the validated analytical solution, we introduce an improved scheme-the push-pull configuration-where the photon and cavity are tuned at the midpoint between atomic resonances and show that it can outperform the original on-off configuration in which the photon and cavity are tuned exactly to one of the atomic resonances. The performance metric used is the final memory-state fidelity versus the heralding probability, which determines the memory loading rate. The results should play a role in optimizing future quantum repeater schemes based on the Duan-Kimble protocol.

quant-ph↗

arXiv2024

Limitations in Fluorescence-Detected Entangled Two-Photon-Absorption Experiments: Exploring the Low- to High-Gain Squeezing Regimes

We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by using time-frequency-entangled photon pairs, and we found that in the low-flux regime, where such enhancement is theoretically predicted in-principle, the two-photon fluorescence signal is below detection threshold using current state-of-the-art methods. The results are important in the context of efforts to enable quantum-enhanced molecular spectroscopy and imaging at ultra-low optical flux. Using an optical parametric down-conversion photon-pair source that can be varied from the low-gain spontaneous regime to the high-gain squeezing regime, we observed two-photon-induced fluorescence in the high-gain regime but in the low-gain regime any fluorescence was below detection threshold. We supplemented the molecular fluorescence experiments with a study of nonlinear-optical sum-frequency generation, for which we are able to observe the low-to-high-gain crossover, thereby verifying our theoretical models and experimental techniques. The observed rates (or lack thereof) in both experiments are consistent with theoretical predictions and with our previous experiments, and indicate that time-frequency photon entanglement does not provide a practical means to enhance in-solution molecular two-photon fluorescence spectroscopy or imaging with current techniques.

quant-ph↗

arXiv2023

Classical Model for Broadband Squeezed Vacuum Driving Two-Photon Absorption or Sum Frequency Generation

We address theoretically the question of classical stochastic fields mimicking quantum states of light in the context of nonlinear spectroscopy and nonlinear optics, in particular two-photon absorption (TPA) and sum-frequency generation (SFG) driven by weak or bright broadband squeezed vacuum with time-frequency entanglement between photons. Upon using a well-defined but ad hoc subtraction of vacuum-energy terms (renormalization), we find that the classical stochastic model yields exactly the same predictions as the full quantum-field theory for all of the phenomena considered here, in both the low-gain and high-gain regimes of squeezed vacuum. Such predictions include the linear-flux scaling of TPA and SFG rates at low incident photon flux, as well as the dependence of TPA and SHG rates on the relative linewidths of the squeezed light and the ground-to-final-state transition in the material system, and the spectrum of SFG generated by bright squeezed vacuum.

quant-ph↗

arXiv2023

States, Modes, Fields, and Photons in Quantum Optics

The quantum nature of light enables potentially revolutionary communication technologies. Key to advancing this area of research is a clear understanding of the concepts of states, modes, fields, and photons. The concept of field modes carries over from classical optics, while the concept of state has to be considered carefully when treating light quantum mechanically. The term 'photon' is an overloaded identifier in the sense that it is often used to refer to either a quantum particle or the state of a field. This overloading, often used without placing in context, has the potential to obfuscate the physical processes that describe the reality we measure. We review the uses and relationships between these concepts using modern quantum optics theory, including the concept of a photon wave function, the modern history of which was moved forward in a groundbreaking paper in this journal by Iwo Bia{\l}ynicki-Birula, to whom this article is dedicated.

quant-ph↗

arXiv2022

Interferometric imaging using shared quantum entanglement

Quantum entanglement-based imaging promises significantly increased resolution by extending the spatial separation of optical collection apertures used in very-long-baseline interferometry for astronomy and geodesy. We report a table-top entanglement-based interferometric imaging technique that utilizes two entangled field modes serving as a phase reference between two apertures. The spatial distribution of a simulated thermal light source is determined by interfering light collected at each aperture with one of the entangled fields and performing joint measurements. This experiment demonstrates the ability of entanglement to implement interferometric imaging.

quant-ph↗

arXiv2022

Theory of Two-Photon Absorption with Broadband Squeezed Vacuum

We present an analytical quantum theoretic model for non-resonant molecular two-photon absorption (TPA) of broadband, spectrally multi-mode squeezed vacuum, including low-gain (isolated entangled photon pairs or EPP) and high-gain (bright squeezed vacuum or BSV) regimes. The results are relevant to the potential use of entangled-light TPA as a spectroscopic and imaging method. We treat the scenario that the exciting light is spatially single-mode and is non-resonant with all intermediate molecular states. In the case of high gain, we find that in the case that the linewidth of the final molecular state is much narrower than the bandwidth of the exciting light, bright squeezed vacuum is found to be equally (but no more) effective in driving TPA as is a quasi-monochromatic coherent-state (classical) pulse of the same temporal shape, duration and mean photon number. Therefore, in this case the sought-for advantage of observing TPA at extremely low optical flux is not provided by broadband bright squeezed vacuum. In the opposite case that the final-state linewidth is much broader than the bandwidth of the BSV exciting light, we show that the TPA rate is proportional to the second-order intensity autocorrelation function at zero time delay g^(2)(0), as expected. We derive and evaluate formulas describing the transition between these two limiting cases, that is, including the regime where the molecular linewidth and optical bandwidth are comparable, as is often the case in experimental studies. We also show that for g^(2)(0) to reach the idealized form g^(2)(0) = 3 + 1/n, with n being the mean number of photons per temporal mode, it is required to compensate the dispersion inherent in the nonlinear-optical crystal used to generate the BSV.

quant-ph↗

arXiv2021

Building a Quantum Engineering Undergraduate Program

The rapidly growing quantum information science and engineering (QISE) industry will require both quantum-aware and quantum-proficient engineers at the bachelor's level. We provide a roadmap for building a quantum engineering education program to satisfy this need. For quantum-aware engineers, we describe how to design a first quantum engineering course accessible to all STEM students. For the education and training of quantum-proficient engineers, we detail both a quantum engineering minor accessible to all STEM majors, and a quantum track directly integrated into individual engineering majors. We propose that such programs typically require only three or four newly developed courses that complement existing engineering and science classes available on most larger campuses. We describe a conceptual quantum information science course for implementation at any post-secondary institution, including community colleges and military schools. QISE presents extraordinary opportunities to work towards rectifying issues of inclusivity and equity that continue to be pervasive within engineering. We present a plan to do so and describe how quantum engineering education presents an excellent set of education research opportunities. Finally, we outline a hands-on training plan on quantum hardware, a key component of any quantum engineering program, with a variety of technologies including optics, atoms and ions, cryogenic and solid-state technologies, nanofabrication, and control and readout electronics. Our recommendations provide a flexible framework that can be tailored for academic institutions ranging from teaching and undergraduate-focused two- and four-year colleges to research-intensive universities.

physics.ed-ph↗

arXiv2021

Quantifying the enhancement of two-photon absorption due to spectral-temporal entanglement

When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency correlations. We present a quantum-theoretic derivation of entangled TPA (ETPA) and calculate an upper bound on the amount of quantum enhancement that is possible in such systems. The derived bounds indicate that in order to observe ETPA the experiments would need to operate at a combination of significantly higher rates of EPP illumination, molecular concentrations, and conventional TPA cross sections than are achieved in typical experiments.

quant-ph↗

arXiv2021

Entangled Two-Photon Absorption by Atoms and Molecules: A Quantum Optics Tutorial

Two-photon absorption (TPA) and other nonlinear interactions of molecules with time-frequency-entangled photon pairs (EPP) has been predicted to display a variety of fascinating effects. Therefore, their potential use in practical quantum-enhanced molecular spectroscopy requires close examination. This paper presents in tutorial style a detailed theoretical study of one- and two-photon absorption by molecules, focusing on how to treat the quantum nature of light. We review some basic quantum optics theory, then we review the density-matrix (Liouville) derivation of molecular optical response, emphasizing how to incorporate quantum states of light into the treatment. For illustration we treat in detail the TPA of photon pairs created by spontaneous parametric down conversion, with an emphasis on how quantum light TPA differs from that with classical light. In particular, we treat the question of how much enhancement of the TPA rate can be achieved using entangled states. The paper includes review of known theoretical methods and results, as well as some extensions, especially the comparison of TPA processes that occur via far-off-resonant intermediate states only and those that involve off-resonant intermediate state by virtue of dephasing processes. A brief discussion of the main challenges facing experimental studies of entangled TPA is also given.

quant-ph↗

arXiv2020

Experimental feasibility of molecular two-photon absorption with isolated time-frequency-entangled photon pairs

Entangled photon pairs have been promised to deliver a substantial quantum advantage for two-photon absorption spectroscopy. However, recent work has challenged the previously reported magnitude of quantum enhancement in two-photon absorption. Here, we present an experimental comparison of sum-frequency generation and molecular absorption, each driven by isolated photon pairs. We establish an upper bound on the enhancement for entangled-two-photon absorption in Rhodamine-6G, which lies well below previously reported values.

quant-ph↗

arXiv2020

Two-photon absorption of time-frequency-entangled photon pairs by molecules: the roles of photon-number correlations and spectral correlations

While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in practical quantum-enhanced molecular spectroscopy requires close examination. This paper presents a detailed theoretical study of quantum-enhanced TPA by both photon-number correlations and spectral correlations, including an account of the deleterious effects of dispersion. While such correlations in EPP created by spontaneous parametric down conversion can increase the TPA rate significantly in the regime of extremely low optical flux, we find that for typical molecules in solution this regime corresponds to such low TPA event rates as to be unobservable in practice. Our results support the usefulness of EPP spectroscopy in atomic or other narrow-linewidth systems, while questioning the efficacy of such approaches for broadband systems including molecules in solution.

quant-ph↗

arXiv2020

Time-frequency optical filtering: efficiency vs. temporal-mode discrimination in incoherent and coherent implementations

Time-frequency (TF) filtering of analog signals has played a crucial role in the development of radio-frequency communications, and is currently being recognized as an essential capability for communications, both classical and quantum, in the optical frequency domain. How best to design optical time-frequency (TF) filters to pass a targeted temporal mode (TM), and to reject background (noise) photons in the TF detection window? The solution for coherent TF filtering is known, the quantum pulse gate, whereas the conventional, more common method is implemented by a sequence of incoherent spectral filtering and temporal gating operations. To compare these two methods, we derive a general formalism for two-stage incoherent time frequency filtering, finding expressions for signal pulse transmission efficiency, and for the ability to discriminate TMs, which allows the blocking of unwanted background light. We derive the tradeoff between efficiency and TM discrimination ability, and find a remarkably concise relation between these two quantities and the time-bandwidth product of the combined filters. We apply the formalism to two examples, rectangular filters or Gaussian filters, both of which have known orthogonal-function decompositions. The formalism can be applied to any state of light occupying the input temporal mode, e.g., classical coherent-state signals or pulsed single photon states of light. We point out implications in classical and quantum optical communications. As an example, we study quantum key distribution, wherein strong rejection of background noise is necessary to maintain a high quality of entanglement, while high signal transmission is needed to ensure a useful key generation rate.

quant-ph↗

arXiv2020

Fluorescence-detected Fourier transform electronic spectroscopy by phase-tagged photon counting

Fluorescence-detected Fourier transform (FT) spectroscopy is a technique in which the relative paths of an optical interferometer are controlled to excite a material sample, and the ensuing fluorescence is detected as a function of the interferometer path delay and relative phase. A common approach to enhance the signal-to-noise ratio in these experiments is to apply a continuous phase sweep to the relative optical path, and to detect the resulting modulated fluorescence using a phase-sensitive lock-in amplifier. In many important situations, the fluorescence signal is too weak to be measured using a lock-in amplifier, so that photon counting techniques are preferred. Here we introduce an approach to low-signal fluorescence-detected FT spectroscopy, in which individual photon counts are assigned to a modulated interferometer phase ('phase-tagged photon counting,' or PTPC), and the resulting data are processed to construct optical spectra. We studied the fluorescence signals of a molecular sample excited resonantly by a pulsed coherent laser over a range of photon flux and visibility levels. We compare the performance of PTPC to standard lock-in detection methods and establish the range of signal parameters over which meaningful measurements can be carried out. We find that PTPC generally outperforms the lock-in detection method, with the dominant source of measurement uncertainty being associated with the statistics of the finite number of samples of the photon detection rate.

physics.optics↗

arXiv2019

Development of Quantum InterConnects for Next-Generation Information Technologies

Just as classical information technology rests on a foundation built of interconnected information-processing systems, quantum information technology (QIT) must do the same. A critical component of such systems is the interconnect, a device or process that allows transfer of information between disparate physical media, for example, semiconductor electronics, individual atoms, light pulses in optical fiber, or microwave fields. While interconnects have been well engineered for decades in the realm of classical information technology, quantum interconnects (QuICs) present special challenges, as they must allow the transfer of fragile quantum states between different physical parts or degrees of freedom of the system. The diversity of QIT platforms (superconducting, atomic, solid-state color center, optical, etc.) that will form a quantum internet poses additional challenges. As quantum systems scale to larger size, the quantum interconnect bottleneck is imminent, and is emerging as a grand challenge for QIT. For these reasons, it is the position of the community represented by participants of the NSF workshop on Quantum Interconnects that accelerating QuIC research is crucial for sustained development of a national quantum science and technology program. Given the diversity of QIT platforms, materials used, applications, and infrastructure required, a convergent research program including partnership between academia, industry and national laboratories is required. This document is a summary from a U.S. National Science Foundation supported workshop held on 31 October - 1 November 2019 in Alexandria, VA. Attendees were charged to identify the scientific and community needs, opportunities, and significant challenges for quantum interconnects over the next 2-5 years.

quant-ph↗

arXiv2019

Temporal Modes in Quantum Optics: Then and Now

We review the concepts of temporal modes (TMs) in quantum optics, highlighting Roy Glauber's crucial and historic contributions to their development, and their growing importance in quantum information science. TMs are orthogonal sets of wave packets that can be used to represent a multimode light field. They are temporal counterparts to transverse spatial modes of light and play analogous roles - decomposing multimode light into the most natural basis for isolating statistically independent degrees of freedom. We discuss how TMs were developed to describe compactly various processes: superfluorescence, stimulated Raman scattering, spontaneous parametric down conversion, and spontaneous four-wave mixing. TMs can be manipulated, converted, demultiplexed, and detected using nonlinear optical processes such as three-wave mixing and quantum optical memories. As such, they play an increasingly important role in constructing quantum information networks.

quant-ph↗