arXiv subjects

Michael G. Raymer

Publications and source records attributed to Michael G. Raymer.

28 records · Page 2Linked to original sources

arXiv2019

Temporal Modes in Quantum Optics: Then and Now

We review the concepts of temporal modes (TMs) in quantum optics, highlighting Roy Glauber's crucial and historic contributions to their development, and their growing importance in quantum information science. TMs are orthogonal sets of wave packets that can be used to represent a multimode light field. They are temporal counterparts to transverse spatial modes of light and play analogous roles - decomposing multimode light into the most natural basis for isolating statistically independent degrees of freedom. We discuss how TMs were developed to describe compactly various processes: superfluorescence, stimulated Raman scattering, spontaneous parametric down conversion, and spontaneous four-wave mixing. TMs can be manipulated, converted, demultiplexed, and detected using nonlinear optical processes such as three-wave mixing and quantum optical memories. As such, they play an increasingly important role in constructing quantum information networks.

quant-ph↗

arXiv2019

Phase-Modulated Interferometry, Spectroscopy, and Refractometry using Entangled Photon Pairs

The authors demonstrate a form of two-photon-counting interferometry by measuring the coincidence counts between single-photon-counting detectors at an output port of a Mach-Zehnder Interferometer (MZI) following injection of broad-band time-frequency-entangled photon pairs (EPP) generated from collinear spontaneous parametric down conversion into a single input port. Spectroscopy and refractometry are performed on a sample inserted in one internal path of the MZI by scanning the other path in length, which acquires phase and amplitude information about the samples linear response. Phase modulation and lock-in detection are introduced to increase detection signal-to-noise ratio and implement a down-sampling technique for scanning the interferometer delay, which reduces the sampling requirements needed to reproduce fully the temporal interference pattern. The phase-modulation technique also allows the contributions of various quantum-state pathways leading to the final detection outcomes to be extracted individually. Feynman diagrams frequently used in the context of molecular spectroscopy are used to describe the interferences resulting from the coherence properties of time-frequency EPPs passing through the MZI. These results are an important step toward implementation of a proposed method for molecular spectroscopy, i.e. quantum-light-enhanced two-dimensional spectroscopy.

quant-ph↗

arXiv2018

Temperature-dependent conformations of exciton-coupled Cy3 dimers in double-stranded DNA

Understanding the properties of electronically interacting molecular chromophores, which involve internally coupled electronic-vibrational motions, is important to the spectroscopy of many biologically relevant systems. Here we apply linear absorption, circular dichroism (CD), and two-dimensional fluorescence spectroscopy (2DFS) to study the polarized collective excitations of excitonically coupled cyanine dimers (Cy3)2 that are rigidly positioned within the opposing sugar-phosphate backbones of the double-stranded region of a double-stranded (ss) - single-stranded (ss) DNA fork construct. We show that the exciton-coupling strength of the (Cy3)2-DNA construct can be systematically varied with temperature below the ds - ss DNA denaturation transition. We interpret spectroscopic measurements in terms of the Holstein vibronic dimer model, from which we obtain information about the local conformation of the (Cy3)2 dimer, as well as the degree of static disorder experienced by the Cy3 monomer and the (Cy3)2 dimer probe locally within their respective DNA duplex environments. The properties of the (Cy3)2-DNA construct we determine suggest that it may be employed as a useful model system to test fundamental concepts of protein-DNA interactions, and the role of electronic-vibrational coherence in electronic energy migration within exciton-coupled bio-molecular arrays.

physics.chem-ph↗

arXiv2017

Temporal-mode-selective optical Ramsey interferometry via cascaded frequency conversion

Temporal modes (TM) are a new basis for storage and retrieval of quantum information in states of light. The full TM manipulation toolkit requires a practical quantum pulse gate (QPG), which is a device that unitarily maps any given TM component of the optical input field onto a different, easily separable subspace or degree of freedom. An ideal QPG must "separate" the selected TM component with unit efficiency, whilst avoiding crosstalk from orthogonal TMs. All attempts at implementing QPGs in pulsed-pump traveling-wave systems have been unable to satisfy both conditions simultaneously. This is due to a known selectivity limit in processes that rely on spatio-temporally local, nonlinear interactions between pulsed modes traveling at independent group velocities. This limit is a consequence of time ordering in the quantum dynamical evolution, which is predicted to be overcome by coherently cascading multiple stages of low-efficiency, but highly TM-discriminatory QPGs. Multi-stage interferometric quantum frequency conversion in nonlinear waveguides was first proposed for precisely this purpose. TM-nonselective cascaded frequency conversion, also called optical Ramsey interferometry, has recently been demonstrated with continuous-wave (CW) fields. Here, we present the first experimental demonstration of TM-selective optical Ramsey interferometry and show a significant enhancement in TM selectivity over single-stage schemes.

quant-ph↗

arXiv2017

Photonic temporal-mode multiplexing by quantum frequency conversion in a dichroic-finesse cavity

Orthogonal temporal modes (TMs) form a field-orthogonal, continuous-variable degree of freedom that is in principle infinite dimensional, and create a promising resource for quantum information science and technology. The ideal quantum pulse gate (QPG) is a device that multiplexes and demultiplexes temporally orthogonal optical pulses that have the same carrier frequency, spatial mode, and polarization. The QPG is the chief enabling technology for usage of orthogonal temporal modes as a basis for high-dimensional quantum information storage and processing. The greatest hurdle for QPG implementation using nonlinear-optical, parametric processes with time-varying pump or control fields is the limitation on achievable temporal mode selectivity, defined as perfect TM discrimination combined with unity efficiency. We propose the use of pulsed nonlinear frequency conversion in an optical cavity having greatly different finesses for different frequencies to implement a nearly perfectly TM-selective QPG in a low-loss integrated-optics platform.

quant-ph↗

arXiv2017

Engineering temporal-mode-selective frequency conversion in off-the-shelf nonlinear optical waveguides: From theory to experiment

Quantum frequency conversion (QFC) in nonlinear optical media is a powerful tool for temporal-mode selective manipulation of light. Recent attempts at achieving high mode selectivities and/or fidelities have had to resort to multi-dimensional optimization schemes to determine the system's natural Schmidt modes. Certain combinations of relative-group velocities between the relevant frequency bands, medium length, and temporal pulse widths have been known to achieve good selectivities (exceeding 80%) for temporal modes that are nearly identical to pump pulse shapes, even for high conversion efficiencies. Working in this parameter regime using an off-the-shelf, second-harmonic generation, MgO:PPLN waveguide, and with pulses on the order of 500 fs at wavelengths around 800 nm, we verify experimentally that model-predicted Schmidt modes provide the high temporal-mode selectivity expected. This paves the way to the implementation of a proposed two-stage QFC scheme that is predicted to reach near-perfect (100%) selectivity.

physics.optics↗

arXiv2017

Observation of Interaction of Spin and Intrinsic Orbital Angular Momentum of Light

Interaction of spin and intrinsic orbital angular momentum of light is observed, as evidenced by length-dependent rotations of both spatial patterns and optical polarization in a cylindrically-symmetric isotropic optical fiber. Such rotations occur in straight few-mode fiber when superpositions of two modes with parallel and anti-parallel orientation of spin and intrinsic orbital angular momentum (IOAM=$2\hslash$) are excited, resulting from a degeneracy splitting of the propagation constants of the modes.

physics.optics↗

arXiv2014

Efficient sorting of quantum-optical wave packets by temporal-mode interferometry

Long-distance quantum communication relies on storing and retrieving photonic qubits in orthogonal field modes. The available degrees of freedom for photons are polarization, spatial-mode profile, and temporal/spectral profile. To date, methods exist for decomposing, manipulating, and analyzing photons into orthogonal polarization modes and spatial modes. Here we propose and theoretically verify the first highly efficient method to carry out analogous operations for temporally and spectrally overlapping, but field-orthogonal, temporal modes. The method relies on cascaded nonlinear-optical quantum frequency conversion.

quant-ph↗

arXiv2013

Temporal mode selectivity by frequency conversion in second-order nonlinear optical waveguides

We explore theoretically the feasibility of using frequency conversion by sum- or difference-frequency generation, enabled by three- wave-mixing, for selectively multiplexing orthogonal input waveforms that overlap in time and frequency. Such a process would enable a drop device for use in a transparent optical network using temporally orthogonal waveforms to encode different channels. We model the process using coupled-mode equations appropriate for wave mixing in a uniform second- order nonlinear optical medium pumped by a strong laser pulse. We find Green functions describing the process, and employ Schmidt (singular- value) decompositions thereof to quantify its viability in functioning as a coherent waveform discriminator. We define a selectivity figure of merit in terms of the Schmidt coefficients, and use it to compare and contrast various parameter regimes via extensive numerical computations. We identify the most favorable regime (at least in the case of no pump chirp) and derive the complete analytical solution for the same. We bound the maximum achievable selectivity in this parameter space. We show that including a frequency chirp in the pump does not improve selectivity in this optimal regime. We also find an operating regime in which high-efficiency frequency conversion without temporal-shape selectivity can be achieved while preserving the shapes of a wide class of input pulses. The results are applicable to both classical and quantum frequency conversion.

quant-ph↗

arXiv2006

Generation of Pure-State Single-Photon Wavepackets by Conditional Preparation Based on Spontaneous Parametric Downconversion

We study the conditional preparation of single photons based on parametric downconversion, where the detection of one photon from a given pair heralds the existence of a single photon in the conjugate mode. We derive conditions on the modal characteristics of the photon pairs, which ensure that the conditionally prepared single photons are quantum-mechanically pure. We propose specific experimental techniques that yield photon pairs ideally suited for single-photon conditional preparation.

quant-ph↗