arXiv subjects

Michael Huth

Publications and source records attributed to Michael Huth.

At least 37 records · Page 2Linked to original sources

arXiv2017

Focused electron beam induced deposition meets materials science

Focused electron beam induced deposition (FEBID) is a direct-write method for the fabrication of nanostructures whose lateral resolution rivals that of advanced electron lithography but is in addition capable of creating complex three-dimensional nano-architectures. Over the last decade several new developments in FEBID and focused electron beam induced processing (FEBIP) have led to a growing number of scientific contributions in solid state physics and materials science based on FEBID-specific materials and particular shapes and arrangements of the employed nanostructures. In this review an attempt is made to give a broad overview of these developments and the resulting contributions in various research fields encompassing mesoscopic physics with nanostructured metals at low temperatures, direct-write of superconductors and nano-granular alloys or intermetallic compounds and their applications, the contributions of FEBID to the field of metamaterials, and the application of FEBID structures for sensing of force or strain, dielectric changes or magnetic stray fields. The very recent development of FEBID towards simulation-assisted growth of complex three-dimensional nano-architectures is also covered. In the review particular emphasis is laid on conceptual clarity in the description of the different developments, which is reflected in the mostly schematic nature of the presented figures, as well as in the recurring final sub-sections for each of the main topics discussing the respective "challenges and perspectives".

cond-mat.mes-hall↗

arXiv2017

Direct-write of free-form 3D nanostructures with controlled magnetic frustration

Building nanotechnological analogues of naturally occurring magnetic structures has proven to be a powerful approach to studying topics like geometry-induced magnetic frustration and to provide model systems for statistical physics. Moreover, it practically allows to engineer novel physical properties by realizing artificial lattice geometries that are not accessible via natural crystallization or chemical synthesis. This has been accomplished with great success in the field of two-dimensional artificial spin ice systems with important branches reaching into the field of magnetic logic devices. Although first proposals have been made to advance into three dimensions (3D), established nanofabrication pathways based on electron beam lithography have not been adapted to obtain free-form 3D nanostructures. Here we demonstrate the direct-write fabrication of freestanding ferromagnetic 3D nano-architectures with full control over the degree of magnetic frustration. By employing micro-Hall sensing, we have determined the magnetic stray field generated by our free-form structures in an externally applied magnetic field and we have performed micromagnetic and macro-spin simulations to deduce the spatial magnetization profiles in the structures and analyze their switching behavior. Furthermore we show that the magnetic 3D elements can be combined with other 3D elements of different chemical composition and intrinsic material properties.

cond-mat.mes-hall↗

arXiv2017

Pinning effects on flux flow instability in epitaxial Nb thin films

The flux flow properties of epitaxial niobium films with different pinning strengths are investigated by dc electrical resistance measurements and mapped to results derived within the framework of a theoretical model. Investigated are the cases of weak random pinning in as-grown films, strong random pinning in Ga ion-irradiated films, and strong periodic pinning induced by a nanogroove array milled by focused ion beam. The generic feature of the current-voltage curves of the films consists in instability jumps to the normal state at some instability current density $j^\ast$ as the vortex lattice reaches its critical velocity $v^\ast$. While $v^\ast(B)$ monotonically decreases for as-grown films, the irradiated films exhibit a non-monotonic dependence $v^\ast(B)$ attaining a maximum in the low-field range. In the case of nanopatterned films, this broad maximum is accompanied by a much sharper maximum in both, $v^\ast(B)$ and $j^\ast(B)$, which we attribute to the commensurability effect when the spacing between the vortex rows coincides with the location of the grooves. We argue that the observed behavior of $v^\ast(B)$ can be explained by the pinning effect on the vortex flow instability and support our claims by fitting the experimental data to theoretical expressions derived within a model accounting for the field dependence of the depinning current density.

cond-mat.supr-con↗

arXiv2017

Optimizing Governed Blockchains for Financial Process Authentications

We propose the formal study of governed blockchains that are owned and controlled by organizations and that neither create cryptocurrencies nor provide any incentives to solvers of cryptographic puzzles. We view such approaches as frameworks in which system parts, such as the cryptographic puzzle, may be instantiated with different technology. Owners of such a blockchain procure puzzle solvers as resources they control, and use a mathematical model to compute optimal parameters for the cryptographic puzzle mechanism or other parts of the blockchain. We illustrate this approach with a use case in which blockchains record hashes of financial process transactions to increase their trustworthiness and that of their audits. For Proof of Work as cryptographic puzzle, we develop a detailed mathematical model to derive MINLP optimization problems for computing optimal Proof of Work configuration parameters that trade off potentially conflicting aspects such as availability, resiliency, security, and cost in this governed setting. We demonstrate the utility of such a mining calculus by solving some instances of this problem. This experimental validation is strengthened by statistical experiments that confirm the validity of random variables used in formulating our mathematical model. We hope that our work may facilitate the creation of domain-specific blockchains for a wide range of applications such as trustworthy information in Internet of Things systems and bespoke improvements of legacy financial services.

cs.CR↗

arXiv2017

Constrained Bayesian Networks: Theory, Optimization, and Applications

We develop the theory and practice of an approach to modelling and probabilistic inference in causal networks that is suitable when application-specific or analysis-specific constraints should inform such inference or when little or no data for the learning of causal network structure or probability values at nodes are available. Constrained Bayesian Networks generalize a Bayesian Network such that probabilities can be symbolic, arithmetic expressions and where the meaning of the network is constrained by finitely many formulas from the theory of the reals. A formal semantics for constrained Bayesian Networks over first-order logic of the reals is given, which enables non-linear and non-convex optimisation algorithms that rely on decision procedures for this logic, and supports the composition of several constrained Bayesian Networks. A non-trivial case study in arms control, where few or no data are available to assess the effectiveness of an arms inspection process, evaluates our approach. An open-access prototype implementation of these foundations and their algorithms uses the SMT solver Z3 as decision procedure, leverages an open-source package for Bayesian inference to symbolic computation, and is evaluated experimentally.

cs.AI↗

arXiv2017

Manyopt: An Extensible Tool for Mixed, Non-Linear Optimization Through SMT Solving

Optimization of Mixed-Integer Non-Linear Programming (MINLP) supports important decisions in applications such as Chemical Process Engineering. But current solvers have limited ability for deductive reasoning or the use of domain-specific theories, and the management of integrality constraints does not yet exploit automated reasoning tools such as SMT solvers. This seems to limit both scalability and reach of such tools in practice. We therefore present a tool, ManyOpt, for MINLP optimization that enables experimentation with reduction techniques which transform a MINLP problem to feasibility checking realized by an SMT solver. ManyOpt is similar to the SAT solver ManySAT in that it runs a specified number of such reduction techniques in parallel to get the strongest result on a given MINLP problem. The tool is implemented in layers, which we may see as features and where reduction techniques are feature vectors. Some of these features are inspired by known MINLP techniques whereas others are novel and specific to SMT. Our experimental results on standard benchmarks demonstrate the benefits of this approach. The tool supports a variety of SMT solvers and is easily extensible with new features, courtesy of its layered structure. For example, logical formulas for deductive reasoning are easily added to constrain further the optimization of a MINLP problem of interest.

cs.AI↗

arXiv2016

Partial Solvers for Parity Games: Effective Polynomial-Time Composition

Partial methods play an important role in formal methods and beyond. Recently such methods were developed for parity games, where polynomial-time partial solvers decide the winners of a subset of nodes. We investigate here how effective polynomial-time partial solvers can be by studying interactions of partial solvers based on generic composition patterns that preserve polynomial-time computability. We show that use of such composition patterns discovers new partial solvers - including those that merge node sets that have the same but unknown winner - by studying games that composed partial solvers can neither solve nor simplify. We experimentally validate that this data-driven approach to refinement leads to polynomial-time partial solvers that can solve all standard benchmarks of structured games. For one of these polynomial-time partial solvers not even a sole random game from a few billion random games of varying configuration was found that it won't solve completely.

cs.LO↗

arXiv2016

Evidence for eight node mixed-symmetry superconductivity in a correlated organic metal

We report a combined theoretical and experimental investigation of the superconducting state in the quasi-two-dimensional organic superconductor $κ$-(ET)$_2$Cu[N(CN)$_2$]Br. Applying spin-fluctuation theory to a low-energy material-specific Hamiltonian derived from ab initio density functional theory we calculate the quasiparticle density of states in the superconducting state. We find a distinct three-peak structure that results from a strongly anisotropic mixed-symmetry superconducting gap with eight nodes and twofold rotational symmetry. This theoretical prediction is supported by low-temperature scanning tunneling spectroscopy on in situ cleaved single crystals of $κ$-(ET)$_2$Cu[N(CN)$_2$]Br with the tunneling direction parallel to the layered structure.

cond-mat.supr-con↗

arXiv2016

Interplay of flux guiding and Hall effect in Nb films with nanogrooves

The interplay between vortex guiding and the Hall effect in superconducting Nb films with periodically arranged nanogrooves is studied via four-probe measurements in standard and Hall configurations and accompanying theoretical modeling. The nanogrooves are milled by focused ion beam and induce a symmetric pinning potential of the washboard type. The resistivity tensor of the films is determined in the limit of small current densities at temperatures close to the critical temperature for the fundamental matching configuration of the vortex lattice with respect to the pinning nanolandscape. The angle between the current direction with respect to the grooves is set at seven fixed values between $0^\circ$ and $90^\circ$. A sign change is observed in the temperature dependence of the Hall resistivity $ρ_\perp^-$ of as-grown films in a narrow temperature range near $T_c$. By contrast, for all nanopatterned films $ρ_\perp^-$ is nonzero in a broader temperature range below $T_c$, allowing us to discriminate between two contributions in $ρ_\perp^-$, namely one contribution originating from the guided vortex motion and the other one caused by the Hall anomaly just as in as-grown Nb films. All four measured resistivity components are successfully fitted to analytical expressions derived within the framework of a stochastic model of competing isotropic and anisotropic pinning. This provides evidence of the model validity for the description of the resistive response of superconductor thin films with washboard pinning nanolandscapes.

cond-mat.supr-con↗

arXiv2015

AC-driven microwave loss modulation in a fluxonic metamaterial

We introduce a fluxonic metamaterial on the basis of nanopatterned superconducting Nb microstrips and employ it for modulation and synthesis of quantized loss levels in the lower GHz range by a sine-wave quasistatic ac drive. The nanopatterns are uniaxial nanogrooves with identical and different slope steepness, which induce a pinning potential of the washboard type for Abrikosov vortices. For the fundamental matching field, when the location of vortex rows geometrically matches the nanogrooves, the following effects are observed: The forward transmission coefficient $S_{21}(f)$ of the microstrips can be controllably modulated within a range of about $3$\,dB by the ac current. For the sample with symmetric grooves, depending on the choice of the operation point in the current-voltage curve, the shape and the duty cycle of the output signal can be tuned. For the sample with asymmetric grooves, depending on the ac amplitude, a sine-to-triangular or a sine-to-rectangular pulse shape conversion is observed. The possibility of synthesizing quantized loss levels by a serial connection of the two samples with different nanopatterns is exemplified and can be used for the development of multilevel excess-loss-based fluxonic devices.

cond-mat.supr-con↗

arXiv2015

Mn$_3$O$_4$(001) film growth on Ag(001) - a systematic study using NEXAFS, STM, and LEED

The film growth of Mn$_3$O$_4$(001) films on Ag(001) up to film thicknesses of almost seven unit cells of Mn$_3$O$_4$ has been monitored using a complementary combination of near-edge X-ray absorption fine structure spectroscopy (NEXAFS), scanning tunneling microscopy (STM), and low-energy electron diffraction (LEED). The oxide films have been prepared by molecular beam epitaxy. Using NEXAFS, the identity of the Mn oxide has clearly been determined as Mn$_3$O$_4$. For the initial stages of growth, oxide islands with p(2$\times$1) and p(2$\times$2) structures are formed, which are embedded into the substrate. For Mn$_3$O$_4$ coverages up to 1.5 unit cells a p(2$\times$1) structure of the films is visible in STM and LEED. Further increase of the thickness leads to a phase transition of the oxide films resulting in an additional c(2$\times$2) structure with a 45$^\circ$ rotated atomic pattern. The emerging film structures are discussed on the basis of a sublayer model of the Mn$_3$O$_4$ spinel unit cell. While the polarity of the island edges determines the structure of initial islands, the surface energy of thicker layers is remarkably reduced by a film restructuring.

physics.atom-ph↗

arXiv2015

Dual cut-off dc-tunable microwave low-pass filter on superconducting Nb microstrips with asymmetric nanogrooves

We present a dual cut-off, dc-tunable low-pass microwave filter on a superconducting Nb microstrip with uniaxial asymmetric nanogrooves. The frequency response of the device was measured in the range $300$\,KHz to $14$\,GHz at different temperatures, magnetic fields, and dc current values. The microwave loss is most effectively reduced when the Abrikosov vortex lattice spatially matches the underlying washboard pinning landscape. The forward transmission coefficient $S_{21}(f)$ of the microstrip has a dc-tunable cut-off frequency $f_d$ which notably changes under dc bias reversal, due to the two different slope steepnesses of the pinning landscape. The device's operation principle relies upon a crossover from the weakly dissipative response of vortices at low frequencies when they are driven over the grooves, to the strongly dissipative response at high frequencies when the vortices are oscillating within one groove. The filter's cut-off frequency is the vortex depinning frequency tunable by the dc bias as it diminishes the pinning effect induced by the nanopattern. The reported results unveil an advanced microwave functionality of superconducting films with asymmetric (ratchet) pinning landscapes and are relevant for tuning the microwave loss in superconducting planar transmission lines.

cond-mat.supr-con↗

arXiv2015

$^4$He sample probe for combined microwave and dc transport measurements

Combined microwave and dc electrical transport measurements at low temperatures represent a valuable experimental method in many research areas. In particular, when samples are conventional superconductors, a typical experiment requires a combination of helium temperatures, a wide range of magnetic fields, and the utilization of coaxial lines along with the usual dc wiring. We report on the general design features and the microwave performance of a custom-made low-temperature sample probe, with a measurement bandwidth tested from dc to 20 GHz. Equipped with 6 coaxial cables, a heater, Hall and temperature sensors, the probe fits into a d32 mm shaft. We present our setup, analyze its microwave performance, and describe two representative experiments enabled by this system. The proposed setup will be essential for a systematic study of the dc and ac response of the vortex dynamics in nanopatterned superconductors subject to combined dc and microwave stimuli. Besides, it will be valuable for the investigation of a broad class of nonlinear stochastic systems where a combination of dc and high-frequency ac driving in a wide temperature range is necessary.

cond-mat.supr-con↗

arXiv2015

Post-growth purification of Co nanostructures prepared by focused electron beam induced deposition

In the majority of cases nanostructures prepared by focused electron beam induced deposition (FEBID) employing an organometallic precursor contain predominantly carbon-based ligand dissociation products. This is unfortunate with regard to using this high-resolution direct-write approach for the preparation of nanostructures for various fields, such as mesoscopic physics, micromagnetism, electronic correlations, spin-dependent transport and numerous applications. Here we present an in-situ cleaning approach to obtain pure Co-FEBID nanostructures. The purification procedure lies in the exposure of heated samples to a H$_2$ atmosphere in conjunction with the irradiation by low-energy electrons. The key finding is that the combination of annealing at $300^\circ$C, H$_2$ exposure and electron irradiation leads to compact, carbon- and oxygen free Co layers down to a thickness of about 20\,nm starting from as-deposited Co-FEBID structures. In addition to this, in temperature-dependent electrical resistance measurements on post-processed samples we find a typical metallic behavior. In low-temperature magneto-resistance and Hall effect measurements we observe ferromagnetic behavior.

cond-mat.mes-hall↗

arXiv2015

Tunable magnetism on the lateral mesoscale by post-processing of Co/Pt heterostructures

Controlling magnetic properties on the nm-scale is essential for basic research in micro-magnetism and spin-dependent transport, as well as for various applications such as magnetic recording, imaging and sensing. This has been accomplished to a very high degree by means of layered heterostructures in the vertical dimension. Here we present a complementary approach that allows for a controlled tuning of the magnetic properties of Co/Pt heterostructures on the lateral mesoscale. By means of in-situ post-processing of Pt- and Co-based nano-stripes prepared by focused electron beam induced deposition (FEBID) we are able to locally tune their coercive field and remanent magnetization. Whereas single Co-FEBID nano-stripes show no hysteresis, we find hard-magnetic behavior for post-processed Co/Pt nano-stripes with coercive fields up to 850 Oe. We attribute the observed effects to the locally controlled formation of the CoPt L1$_{0}$ phase, whose presence has been revealed by transmission electron microscopy.

cond-mat.mes-hall↗

arXiv2015

Magnetization reversal assisted by half antivortex states in nanostructured circular cobalt disks

The half antivortex, a fundamental topological structure which determines magnetization reversal of submicron magnetic devices with domain walls, has been suggested also to play a crucial role in spin torque induced vortex core reversal in circular disks. Here we report on magnetization reversal in circular disks with nanoholes through consecutive metastable states with half antivortices. In-plane anisotropic magnetoresistance and broadband susceptibility measurements accompanied by micromagnetic simulations reveal that cobalt disks with two and three linearly arranged nanoholes directed at 45 and 135 degrees with respect to the external magnetic field show reproducible step-like changes in the anisotropic magnetoresistance and magnetic permeability due to transitions between different intermediate states mediated by vortices and half antivortices confined to the dot nanoholes and edges, respectively. Our findings are relevant for the development of multi-hole based spintronic and magnetic memory devices.

cond-mat.mes-hall↗

arXiv2014

Local density of states in the superconductor $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br

Low temperature scanning tunneling spectroscopy reveals the local density of states of the organic superconductor $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br, that was cut in-situ in ultra-high vacuum perpendicular to the superconducting BEDT-TTF layers. The spectra confirm that superconductivity is confined to the conducting BEDT-TTF layers, while the Cu[N(CN)$_2$]Br anion layers are insulating. The density of states comprises a twofold superconducting gap, which is attributed to the two separated bands crossing the Fermi surface.

cond-mat.str-el↗

arXiv2014

Comparing charge transfer tuning effects by chemical substitution and uniaxial pressure in the organic charge transfer complex tetramethoxypyrene-tetracyanoquinodimethane

In the search for novel organic charge transfer salts with variable charge transfer degree we study the effects of two modifications to the recently synthesized donor-acceptor Tetramethoxypyrene (TMP)-Tetracyanoquinodimethane (TCNQ). One is of chemical nature by substituting the acceptor TCNQ molecules by F4TCNQ molecules. The second consists in simulating the application of uniaxial pressure along the stacking axis of the system. In order to test the chemical substitution, we have grown single crystals of TMP-F4TCNQ and analyzed its electronic structure via electronic transport measurements, ab initio density functional theory (DFT) calculations and UV/VIS/IR absorption spectroscopy. This system shows an almost ideal geometrical overlap of nearly planar molecules alternately stacked (mixed stack) and this arrangement is echoed by a semiconductor-like transport behavior with an increased conductivity along the stacking direction. This is in contrast to TMP-TCNQ which shows a less pronounced anisotropy and a smaller conductivity response. Our bandstructure calculations confirm the one-dimensional behavior of TMP-F4TCNQ with pro- nounced dispersion only along the stacking axis. Infrared measurements illustrating the CN vibration frequency shift in F4TCNQ suggest however no improvement on the degree of charge transfer in TMP-F4TCNQ with respect to TMP-TCNQ. In both complexes about 0.1 is transferred from TMP to the acceptor. Concerning the pressure effect, our DFT calculations on designed TMP-TCNQ and TMP-F4TCNQ structures under different pressure conditions show that application of uniaxial pressure along the stacking axis of TMP-TCNQ may be the route to follow in order to obtain a much more pronounced charge transfer.

cond-mat.mtrl-sci↗