arXiv subjects

Milena Grifoni

Publications and source records attributed to Milena Grifoni.

At least 55 records · Page 3Linked to original sources

arXiv2012

Spin channel Keldysh field theory for weakly interacting quantum dots

We develop a low-energy nonequilibrium field theory for weakly interacting quantum dots. The theory is based on the Keldysh field integral in the spin channel of the quantum dot described by the single impurity Anderson Hamiltonian. The effective Keldysh action is a functional of the Hubbard-Stratonovich magnetization field decoupling the quantum dot spin channel. We expand this action up to the second order with respect to the magnetization field, which allows to describe nonequilibrium interacting quantum dots at low temperatures and weak electron-electron interactions,up to the contacts-dot coupling energy. Besides its simplicity, an additional advantage of the theory is that it correctly describes the unitary limit giving the correct result for the conductance maximum. Thus our theory establishes an alternative simple method relevant for investigation of weakly interacting nonequilibrium nanodevices.

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arXiv2012

Performance analysis of an interacting quantum dot thermoelectric system

We analyze the nanocaloritronic performance of an interacting quantum dot that is subject to an applied bias and an applied temperature gradient. It is now well known that, in the absence of phonon contribution, a weakly coupled non-interacting quantum dot can operate at thermoelectric efficiencies approaching the Carnot limit. However, it has also been recently pointed out that such peak efficiencies can only be achieved when operated in the reversible limit, with a vanishing current and hence a vanishing power output. In this paper, we point out three fundamental results affecting the thermoelectric performance due to the inclusion of Coulomb interactions: a) The reversible operating point carries zero efficiency, b) operation at finite power output is possible even at peak efficiencies approaching the Carnot value, and c) the evaluated trends of the the maximum efficiency deviate considerably from the conventional {\it{figure of merit}} $zT$ based result. Finally, we also analyze our system for thermoelectric operation at maximum power output.

cond-mat.mes-hall↗

arXiv2012

Spectrum and Franck-Condon factors of interacting suspended single-wall carbon nanotubes

A low energy theory of suspended carbon nanotube quantum dots in weak tunnelling coupling with metallic leads is presented. The focus is put on the dependence of the spectrum and the Franck-Condon factors on the geometry of the junction including several vibronic modes. The relative size and the relative position of the dot and its associated vibrons strongly influence the electromechanical properties of the system. A detailed analysis of the complete parameters space reveals different regimes: in the short vibron regime the tunnelling of an electron into the nanotube generates a plasmon-vibron excitation while in the long vibron regime polaron excitations dominate the scenario. The small, position dependent Franck-Condon couplings of the small vibron regime convert into uniform, large couplings in the long vibron regime. Selection rules for the excitations of the different plasmon-vibron modes via electronic tunnelling events are also derived.

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arXiv2012

Kondo effect in interacting nanoscopic systems: Keldysh field integral theory

Kondo physics in nonequilibrium interacting nanoscale devices is an attractive fundamental many-particle phenomenon with a rich potential for applications. Due to enormous complexity its clear and flexible theory is still highly desirable. We develop a physically transparent analytical theory capable to correctly describe the Kondo effect in strongly interacting systems at temperatures close to and above the Kondo temperature. We derive a nonequilibrium Keldysh field theory valid for a system with any finite electron-electron interaction which is much stronger than the coupling of the system to contacts. Finite electron-electron interactions are treated involving as many slave-boson degrees of freedom as one needs for a concrete many-body system. In a small vicinity of the zero slave-bosonic field configuration weak slave-bosonic oscillations, induced by the dot-contacts tunneling, are described by an effective Keldysh action quadratic in the slave-bosonic fields. For clarity the theory is presented for the single impurity Anderson model but the construction of the Keldysh field integral is universal and applicable to systems with more complex many-body spectra.

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arXiv2011

Dynamical symmetry breaking in vibration-assisted transport through nanostructures

A theoretical model of a single molecule coupled to many vibronic modes is presented. At low energies, transport is dominated by electron-vibron processes where transfer of an electron through the dot is accompanied by the excitation/emission of quanta (vibrons). Because the frequency of the $n$th mode is taken as an $n$th multiple of the frequency of the fundamental mode, several energetically degenerate or quasi-degenerate vibronic configurations can contribute to transport. We investigate the consequences of strong electron-vibron coupling in a fully \emph{symmetric} set-up. Several striking features are predicted. In particular, a gate-asymmetry and pronounced negative differential conductance features are observed. We attribute these features to the presence of slow channels originating from the interplay of Franck-Condon suppression of transport channels and spin/orbital degeneracies.

cond-mat.mes-hall↗

arXiv2011

Slave-boson Keldysh field theory for the Kondo effect in quantum dots

We present a {\it nonequilibrium nonperturbative} field theory for the Kondo effect in strongly interacting quantum dots at finite temperatures. Unifying the slave-boson representation with the Keldysh field integral an effective Keldysh action is derived and explored in the vicinity of the zero slave-bosonic field configuration. The theory properly reflects the essential features of the Kondo physics and at the same time significantly simplifies a field-theoretic treatment of the phenomenon, avoiding complicated saddle point analysis or 1/N expansions, used so far. Importantly, our theory admits a {\it closed analytical} solution which explains the mechanism of the Kondo effect in terms of an interplay between the real and imaginary parts of the slave-bosonic self-energy. It thus provides a convenient nonperturbative building block, playing the role of a "free propagator", for more advanced theories. We finally demonstrate that already this simplest possible field theory is able to correctly reproduce experimental data on the Kondo peak observed in the differential conductance, correctly predicts the Kondo temperature and, within its applicability range, has the same universal temperature dependence of the conductance as the one obtained in numerical renormalization group calculations.

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arXiv2011

Dynamical symmetry breaking in vibration-assisted transport through nanostructures

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arXiv2011

Inelastic cotunneling in quantum dots and molecules with weakly broken degeneracies

We calculate the nonlinear cotunneling conductance through interacting quantum dot systems in the deep Coulomb blockade regime using a rate equation approach based on the T-matrix formalism, which shows in the concerned regions very good agreement with a generalized master equation approach. Our focus is on inelastic cotunneling in systems with weakly broken degeneracies, such as complex quantum dots or molecules. We find for these systems a characteristic gate dependence of the non-equilibrium cotunneling conductance. While on one side of a Coulomb diamond the conductance decreases after the inelastic cotunneling threshold towards its saturation value, on the other side it increases monotonously even after the threshold. We show that this behavior originates from an asymmetric gate voltage dependence of the effective cotunneling amplitudes.

cond-mat.mes-hall↗

arXiv2011

Qubit-oscillator system under ultrastrong coupling and extreme driving

We introduce an approach to studying a driven qubit-oscillator system in the ultrastrong coupling regime, where the ratio $g/Ω$ between coupling strength and oscillator frequency approaches unity or goes beyond, and simultaneously for driving strengths much bigger than the qubit energy splitting (extreme driving). Both qubit-oscillator coupling and external driving lead to a dressing of the qubit tunneling matrix element of different nature: the former can be used to suppress selectively certain oscillator modes in the spectrum, while the latter can bring the qubit's dynamics to a standstill at short times (coherent destruction of tunneling) even in the case of ultrastrong coupling.

quant-ph↗

arXiv2011

Signatures of spin-orbit interaction in transport properties of finite carbon nanotubes in a parallel magnetic field

The transport properties of finite nanotubes placed in a magnetic field parallel to their axes are investigated. Upon including spin-orbit coupling and curvature effects, two main phenomena are analyzed which crucially depend on the tube's chirality: i) Finite carbon nanotubes in a parallel magnetic field may present a suppression of current due to the localization at the edges of otherwise conducting states. This phenomenon occurs due to the magnetic-field dependent open boundary conditions obeyed by the carbon nanotube's wave functions. The transport is fully suppressed above threshold values of the magnetic field which depend on the nanotube chirality, length and on the spin-orbit coupling. ii) Reversible spin polarized currents can be obtained upon tuning the magnetic field, exploiting the curvature-induced spin-orbit splitting.

cond-mat.mes-hall↗

arXiv2011

Magnetic field induced localization in carbon nanotubes

The electronic spectra of long carbon nanotubes (CNTs) can, to a very good approximation, be obtained using the dispersion relation of graphene with both angular and axial periodic boundary conditions. In short CNTs one must account for the presence of open ends, which may give rise to states localized at the edges. We show that when a magnetic field is applied parallel to the tube axis, it modifies both momentum quantization conditions, causing hitherto extended states to localize near the ends. This localization is gradual and initially the involved states are still conducting. Beyond a threshold value of the magnetic field, which depends on the nanotube chirality and length, the localization is complete and the transport is suppressed.

cond-mat.mes-hall↗

arXiv2010

Qubit-oscillator system: An analytical treatment of the ultra-strong coupling regime

We examine a two-level system coupled to a quantum oscillator, typically representing experiments in cavity and circuit quantum electrodynamics. We show how such a system can be treated analytically in the ultrastrong coupling limit, where the ratio $g/Ω$ between coupling strength and oscillator frequency approaches unity and goes beyond. In this regime the Jaynes-Cummings model is known to fail, because counter-rotating terms have to be taken into account. By using Van Vleck perturbation theory to higher orders in the qubit tunneling matrix element $Δ$ we are able to enlarge the regime of applicability of existing analytical treatments, including in particular also the finite bias case. We present a detailed discussion on the energy spectrum of the system and on the dynamics of the qubit for an oscillator at low temperature. We consider the coupling strength $g$ to all orders, and the validity of our approach is even enhanced in the ultrastrong coupling regime. Looking at the Fourier spectrum of the population difference, we find that many frequencies are contributing to the dynamics. They are gathered into groups whose spacing depends on the qubit-oscillator detuning. Furthermore, the dynamics is not governed anymore by a vacuum Rabi splitting which scales linearly with $g$, but by a non-trivial dressing of the tunneling matrix element, which can be used to suppress specific frequencies through a variation of the coupling.

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arXiv2010

Dynamics of a qubit coupled to a dissipative nonlinear quantum oscillator: an effective bath approach

We consider a qubit coupled to a nonlinear quantum oscillator, the latter coupled to an Ohmic bath, and investigate the qubit dynamics. This composed system can be mapped onto that of a qubit coupled to an effective bath. An approximate mapping procedure to determine the spectral density of the effective bath is given. Specifically, within a linear response approximation the effective spectral density is given by the knowledge of the linear susceptibility of the nonlinear quantum oscillator. To determine the actual form of the susceptibility, we consider its periodically driven counterpart, the problem of the quantum Duffing oscillator within linear response theory in the driving amplitude. Knowing the effective spectral density, the qubit dynamics is investigated. In particular, an analytic formula for the qubit's population difference is derived. Within the regime of validity of our theory, a very good agreement is found with predictions obtained from a Bloch-Redfield master equation approach applied to the composite qubit-nonlinear oscillator system.

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arXiv2010

Interference effects in the Coulomb blockade regime: current blocking and spin preparation in symmetric nanojunctions

We consider nanojunctions in the single-electron tunnelling regime which, due to a high degree of spatial symmetry, have a degenerate many body spectrum. As a consequence, interference phenomena which cause a current blocking can occur at specific values of the bias and gate voltage. We present here a general formalism to give necessary and sufficient conditions for interference blockade also in the presence of spin polarized leads. As an example we analyze a triple quantum dot single electron transistor (SET). For a set-up with parallel polarized leads, we show how to selectively prepare the system in each of the three states of an excited spin triplet without application of any external magnetic field.

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arXiv2010

Spin-dependent transport through interacting graphene armchair nanoribbons

We investigate spin effects in transport across fully interacting, finite size graphene armchair nanoribbons (ACNs) contacted to collinearly spin-polarized leads. In such systems, the presence of short ranged Coulomb interaction between bulk states and states localized at the ribbon ends leads to novel spin-dependent phenomena. Specifically, the total spin of the low energy many-body states is conserved during tunneling but that of the bulk and end states is not. As a consequence, in the single-electron regime, dominated by Coulomb blockade phenomena, we find pronounced negative differential conductance features for ACNs contacted to parallel polarized leads. These features are however absent for an anti-parallel contact configuration, which in turn leads within a certain gate and bias voltage region to a negative tunneling magneto-resistance. Moreover, we analyze the changes in the transport characteristics under the influence of an external magnetic field.

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arXiv2010

Exchange effects in spin polarized transport through carbon nanotube quantum dots

We investigate linear and nonlinear transport across single-walled carbon nanotube quantum dots weakly coupled to spin-polarized leads. We consider tubes of finite length and small diameter, where not only forward scattering contributions of the Coulomb potential, but also short-ranged processes play an important role. In particular, they induce exchange effects leading for electron fillings 4n+2 either to a non-degenerate groundstate of spin S=0 or to a triplet groundstate. In the linear regime we present analytical results for the conductance - for both the S=0 and the triplet groundstate - and demonstrate that an external magnetic field is crucial to reveal the spin nature of the groundstates. In the nonlinear regime we show stability diagrams that clearly distinguish between the different groundstates. We observe a negative differential conductance (NDC) effect in the S=0 groundstate for antiparallel lead magnetization. In presence of an external magnetic field spin blockade effects can be detected, again leading to NDC effects for both groundstates.

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arXiv2010

The dissipative quantum Duffing oscillator: a comparison of Floquet-based approaches

We study the dissipative quantum Duffing oscillator in the deep quantum regime with two different approaches: The first is based on the exact Floquet states of the linear oscillator and the nonlinearity is treated perturbatively. It well describes the nonlinear oscillator dynamics away from resonance. The second, in contrast, is applicable at and in the vicinity of a N-photon resonance and it exploits quasi-degenerate perturbation theory for the nonlinear oscillator in Floquet space. It is perturbative both in driving and nonlinearity. A combination of both approaches yields the possibility to cover the whole range of driving frequencies. As an example we discuss the dissipative dynamics of the Duffing oscillator near and at the one-photon resonance.

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arXiv2010

The dissipative two-level system under strong ac-driving: a combination of Floquet and Van Vleck perturbation theory

We study the dissipative dynamics of a two-level system (TLS) exposed to strong ac driving. By combing Floquet theory with Van Vleck perturbation theory in the TLS tunneling matrix element, we diagonalize the time-dependent Hamiltonian and provide corrections to the renormalized Rabi frequency of the TLS, which are valid for both a biased and unbiased TLS and go beyond the known high-frequency and rotating-wave results. In order to mimic environmental influences on the TLS, we couple the system weakly to a thermal bath and solve analytically the corresponding Floquet-Bloch-Redfield master equation. We give a closed expression for the relaxation and dephasing rates of the TLS and discuss their behavior under variation of the driving amplitude. Further, we examine the robustness of coherent destruction of tunneling (CDT) and driving-induced tunneling oscillations (DITO). We show that also for a moderate driving frequency an almost complete suppression of tunneling can be achieved for short times and demonstrate the sensitiveness of DITO to a change of the external parameters.

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