arXiv subjects

Milorad V. Milošević

Publications and source records attributed to Milorad V. Milošević.

At least 19 recordsLinked to original sources

arXiv2026

Optical activation of nonlinear Hall effect in topological insulators with warped Fermi surface

Topological insulators (TIs) with hexagonally warped Fermi surface are natural platforms for the nonlinear Hall effect, as warping breaks inversion symmetry while preserving time-reversal symmetry (TRS). Here we show that this inversion breaking alone is insufficient: although warping generates a strongly anisotropic Berry curvature, the preserved threefold rotational symmetry forces the equilibrium Berry curvature dipole (BCD) to vanish identically. We demonstrate that linearly polarized light removes this symmetry obstruction: in the off-resonant Floquet regime, it lowers the rotational symmetry while preserving TRS, thereby generating a finite BCD whose magnitude, orientation, and sign are continuously tunable by the light intensity and polarization. For realistic Bi$_2$Te$_3$ parameters, we show that the induced BCD reaches $\sim$0.03~nm, yielding microampere-scale nonlinear Hall currents under experimentally accessible conditions. Our results therefore establish Floquet symmetry engineering as a route to activating the symmetry-forbidden nonlinear transport on TI surfaces without breaking the TRS.

cond-mat.mes-hall↗

arXiv2026

Real-space Floquet topology written by the orbital angular momentum of light

Floquet engineering usually treats light as a uniform control field that changes the topology of an entire driven material. Here we show that structured light carrying orbital angular momentum (OAM) enables a different regime, in which topology is written directly in real space. For ultrathin topological insulator films, circularly polarized Laguerre--Gaussian beams generate a radial Floquet mass whose sign changes define a topological annulus bounded by two concentric chiral ring modes. The transition is helicity selective: below a thickness-dependent critical frequency, left-circularly polarized light drives mass inversion, whereas right-circularly polarized light increases the gap and leaves the film trivial. Independently, the OAM quantum number shifts and reshapes the annulus without changing the frequency, intensity, or helicity. In the decoupled-surfaces limit, the same mechanism produces a purely Floquet-induced topological mass and a vortex-core zero mode. These results identify photon OAM as a control parameter for nonequilibrium topology and provide a route to programmable topological landscapes in quantum materials.

cond-mat.mes-hall↗

arXiv2026

Imaging superconducting weak spots through vortex-assisted THz near-field photovoltage

Nanoscale inhomogeneities are a defining feature of many superconducting materials, yet their local electromagnetic response has remained difficult to access experimentally. This is because their relevant energy scale lies in the terahertz range, where wavelengths -- on the order of hundreds of microns -- are too large to spatially resolve nanoscopic variations. Here, we demonstrate the first application of THz near-field photovoltage nanoscopy in a superconductor, achieving 300 nm spatial resolution at 2.52 THz. Scanning a current-biased NbN strip, we reveal photovoltage peaks within the bulk associated with nanoscopic defects of reduced superfluid density. The observed photovoltage follows the evolution of the vortex-dissipative state and is attributed to enhanced vortex-antivortex pair nucleation at defect sites. Together, these results open a direct route to probing how material inhomogeneities influence light-matter interactions in superconductors, with implications for superconducting devices and strongly inhomogeneous systems such as high-Tc and moiré materials.

cond-mat.supr-con↗

arXiv2026

Bandwidth-Limited Critical Currents in Electrically Tunable Moiré Bands

Moiré superlattices host narrow minibands whose bandwidth governs correlated and topological phases. Here, we demonstrate that the bandwidth also sets the critical current for the onset of out-of-equilibrium transport. In bilayer graphene aligned to hexagonal boron nitride, we explore the high-current transport regime as we continuously flatten the valence miniband using an out-of-plane displacement field. We observe a significant reduction in the critical current, which is captured by a minimal analytical model and corresponds to the calculated narrowing of the miniband. Moreover, by comparing distinct moiré platforms, we show that the scaling between critical current and bandwidth is a universal feature of graphene superlattices. Our results reveal a direct link between miniband dispersion and high-current transport, and establish this regime as a fast and accessible electrical probe of bandwidth evolution.

cond-mat.mes-hall↗

arXiv2026

Fluctuation-enhanced electron-phonon coupling in FeSe

The interactions among lattice, charge, and spin degrees of freedom fundamentally shape material properties. In FeSe, symmetry-breaking perturbations serve as highly sensitive probes of these couplings. Previous work has shown that defects and isoelectronic substitution can substantially alter these interactions, giving rise to additional phonon modes. In this study, uniaxial strain is employed as a tunable symmetry-breaking control parameter to probe the intrinsic lattice response in the absence of disorder. The temperature evolution of phonon excitations was examined with fine temperature resolution in the vicinity of the nemato-structural transition temperature $T_s$, under strain applied along the $\langle 110 \rangle$ and $\langle 100 \rangle$ crystallographic directions. A subtle asymmetry of the $A_{1g}^{ph}$ mode appears in the unstrained crystal within a narrow temperature window around $T_s$, originating from the emergence of an additional mode in the fully symmetric channel. With applied strain, this feature becomes more distinctly resolved. The anomaly is attributed to modifications of the coupling between lattice and electronic degrees of freedom driven by the ordering fluctuations right above the nematic transition. These fluctuations enhance susceptibility for phonon-electron-phonon coupling in the vicinity of the X and R points of the Brillouin zone and promote two-phonon scattering close to the $A_{1g}^{ph}$ mode. The presence of this two-phonon scattering depends on both the strength and the direction of the applied strain, indicating a high sensitivity of FeSe to local symmetry breaking.

cond-mat.supr-con↗

arXiv2025

Benchmarking First-Principles Approaches for Extracting Magnetic Exchange Interactions

Magnetic exchange interactions govern the macroscopic magnetic behavior of solids and underpin both fundamental spin phenomena and emerging technologies. The accurate and efficient determination of these interactions is therefore critical for predictive modeling of magnetic materials. Here we present a systematic first-principles comparison of three widely used approaches-the Least-Squares Total Energy (LSTE), the Four-State Total Energy (FSTE), and the Green's function-based Liechtenstein \textit{et al.} (LKAG) methods-applied to thirteen antiferromagnetic compounds. We introduce an framework for identifying the minimal supercells required for an accurate exchange parameter extraction in the FSTE method, significantly reducing computational cost while preserving precision. Our results show that LSTE and FSTE yield nearly identical exchange parameters, whereas the LKAG method reproduces the dominant exchange interactions but exhibits quantitative deviations. A detailed analysis of computational efficiency versus accuracy reveals that the LSTE scheme offers the most favorable balance, establishing a general, reproducible, and scalable workflow for Heisenberg mapping, while the FSTE approach remains the most straightforward for extracting specific exchange interactions.

cond-mat.mtrl-sci↗

arXiv2025

Berezinskii-Kosterlitz-Thouless transition with enhanced phase stiffness in $d$-wave strongly coupled two-dimensional superconductors

We reveal the key role of the $d$-wave symmetry of the superconducting gap in strongly coupled two-dimensional superconductors in determining the properties of the Berezinskii-Kosterlitz-Thouless (BKT) transition, associated with a sizable enhancement of the phase stiffness compared to nodeless-gap superconductors. The enhanced stiffness originates from extended regions of vanishing gap around the nodal lines of the Brillouin zone (BZ). Our study, based on mean-field and BKT theory, presents a comparative analysis of $s$-wave and $d$-wave scenarios, highlighting the features of the latter that boost the stiffness and the BKT transition temperature (T$_{BKT}$). The comparison focuses on two quantities: the mean-field critical temperature and the maximum superconducting gap related to the pairing strengths. We present a phase diagram showing the scaling of T$_{BKT}$ with respect to the mean-field critical temperature across the BCS-BEC crossover and the evolution of the pseudogap. We also present a zero-temperature phase-stiffness intensity map over the Brillouin zone, displaying a two-component structure consisting of low- and high-stiffness regions whose extent depends on microscopic parameters. These results identify the nodal gap structure of strongly coupled two-dimensional superconductors as a key mechanism enabling enhanced stiffness and elevated T$_{BKT}$ compared to their $s$-wave counterparts.

cond-mat.supr-con↗

arXiv2025

Quantum Coherence in Superconducting Vortex States

Abrikosov vortices, where the superconducting gap is completely suppressed in the core, are dissipative, semi-classical entities that impact applications from high-current-density wires to superconducting quantum devices. In contrast, we present evidence that vortices trapped in granular superconducting films can behave as two-level systems, exhibiting microsecond-range quantum coherence and energy relaxation times that reach fractions of a millisecond. These findings support recent theoretical modeling of superconductors with granularity on the scale of the coherence length as tunnel junction networks, resulting in gapped vortices. Using the tools of circuit quantum electrodynamics, we perform coherent manipulation and quantum non-demolition readout of vortex states in granular aluminum microwave resonators, heralding new directions for quantum information processing, materials characterization, and sensing.

quant-ph↗

arXiv2025

Linearly polarized light enables chiral edge transport in quasi-2D Dirac materials

Floquet engineering with high-frequency light offers dynamic control over topological phases in quantum materials. While in 3D Dirac systems circularly polarized light is known to induce topological phase transitions via gap opening, linearly polarized light (LPL) has generally been considered ineffective. Here we show that in quasi-2D Dirac materials the second-order momentum term arising from the intersurface coupling can induce a topological phase transition under LPL, leading to chiral edge channels. Considering an ultrathin Bi$_2$Se$_3$ film as a representative system, we show that this transition occurs at experimentally accessible light intensities. Our results thus promote quasi-2D materials as viable platforms for light-controlled topological phases, expanding the potential of Floquet topological engineering.

cond-mat.mes-hall↗

arXiv2025

Dissipationless transport by design in ultrathin magnetic topological insulator films

Magnetic topological insulators (MTIs) are among the prominent platforms for the next generation of high-speed and low-power spintronic devices. However, unlike their non-magnetic counterparts, where the surface spin-momentum locking prevents electrons from being scattered by non-magnetic impurities and results in a dissipationless electronic flow, magnetic impurities in MTIs cause dissipation by exerting magnetic torque on the electron spin. Decreasing this resistance is desired to reduce energy consumption and optimize performance of MTIs in envisaged applications. Here we reveal how electronic backscattering can be suppressed in a MTI thin film by external magnetic and/or electronic stimuli, to yield an entirely dissipationless spin-polarized charge transport. Our findings thus present an effective route to preserve spin coherence and enhance spin-current functionality in magnetic topological materials, suggesting design strategies for magneto-electronic and spintronic devices with strongly reduced energy consumption.

cond-mat.mes-hall↗

arXiv2025

Strain-tuned magnetoelectric properties of monolayer NiX$_2$ (X = I, Br): a first-principles analysis

Using \textit{ab initio} methodology, we reveal a strain-mediated approach to precisely tune the magnetoelectric coupling and spin-driven emergent polarization of NiX$_2$ (X = I, Br) monolayers. In the absence of strain, these systems spontaneously stabilize non-collinear spin states that break the inversion symmetry, inducing a ferroelectric polarization in the plane of the material. We show that biaxial and uniaxial strains broadly modulate the magnetoelectric response in these materials through two distinct mechanisms: (i) direct modification of the magnetoelectric tensor components, and (ii) tuning of the characteristic propagation vectors of a spin texture. This dual mechanism enables precise control over the magnitude of the spin-induced electric polarization of these materials. With respect to the achievable magnitude of the electric polarization, we demonstrate the critical role of third-nearest-neighbor spin-pair contributions, which can increase under strain to levels that compete with or even exceed the polarization driven by first-nearest-neighbor effects. These findings offer important insights into low-dimensional piezo-magnetoelectricity and expand the possibilities for designing multifunctional two-dimensional straintronic devices.

cond-mat.mtrl-sci↗

arXiv2025

mumax+: extensible GPU-accelerated micromagnetics and beyond

We present mumax+, an extensible GPU-accelerated micromagnetic simulator with a Python user interface, to address the challenges posed by current magnetism research into systems with complex magnetic ordering and interfaces. It is a general solver for the space- and time-dependent evolution of the magnetization and related vector quantities, using finite difference discretization. Here, we present its application and design and discuss features not available in \mumaxthree{}, such as the modeling of antiferromagnets with magnetoelastic coupling. As an illustration of its capabilities, we use \mumaxp{} to simulate state of the art magnetic systems. Specifically, we demonstrate the current induced domain wall motion in a polycrystalline antiferromagnet, we simulate the working principle of a strain-driven antiferromagnetic racetrack memory and we reproduce experimentally observed domain structures in a non-collinear antiferromagnet.

cond-mat.mes-hall↗

arXiv2025

Scalable High-Temperature Superconducting Diodes in Intrinsic Josephson Junctions

Superconducting diodes, characterized by nonreciprocal supercurrent transport, offer transformative opportunities for ultra-low-power circuits. However, achieving reliable operation at temperatures above liquid nitrogen remains a major challenge, limiting their practical applicability. Here, we present a scalable strategy for high-temperature superconducting diodes based on intrinsic Josephson junctions naturally present in a cuprate superconductor. We demonstrate that strong nonreciprocity arises not only from broken spatial and time-reversal symmetries, but also from enhanced anharmonicity in the current-phase relation, enabled by the atomically thin barrier of the intrinsic junction. The diode efficiency strongly depends on the number of stacked intrinsic junctions, with the highest efficiency occurring in single-junction devices. Notably, these high-temperature superconducting diodes are readily scalable to large arrays, marking a critical step toward practical implementation in energy-efficient computing architectures.

cond-mat.supr-con↗

arXiv2025

Single-photon detection enabled by negative differential conductivity in moiré superlattices

Detecting individual light quanta is essential for quantum information, space exploration, advanced machine vision, and fundamental science. Here, we introduce a novel single photon detection mechanism using highly photosensitive non-equilibrium electron phases in moiré materials. Using tunable bands in bilayer graphene/hexagonal-boron nitride superlattices, we engineer negative differential conductance and a sensitive bistable state capable of detecting single photons. Operating in this regime, we demonstrate single-photon counting at mid-infrared (11.3 microns) and visible wavelengths (675 nanometres) and temperatures up to 25 K. This detector offers new prospects for broadband, high-temperature quantum technologies with CMOS compatibility and seamless integration into photonic integrated circuits (PICs). Our analysis suggests the mechanism underlying our device operation originates from negative differential velocity, and represents an important milestone in the field of high-bias transport in two-dimensional moiré quantum materials.

cond-mat.mes-hall↗

arXiv2025

Real-space superconducting properties in the atomically-thin limit: Ab initio approach and its application to Josephson junctions

Real-space superconducting properties are increasingly important to characterize low-dimensional, layered, and nanostructured materials. Here, we present a method to extract the real-space superconducting order parameter from the superconducting gap spectrum obtained via anisotropic Migdal-Eliashberg calculations, using the Bloch wave functions of the Fermi states. We apply this approach to a selection of atomically thin material systems. Our analysis of gallenene, a monolayer of gallium atoms, shows that its planar and buckled phases exhibit distinct superconducting order parameter behaviors, shaped by their structural and electronic properties. Furthermore, we demonstrate that our real-space approach is exceptionally suited to identify and characterize Josephson junctions made from van der Waals materials. Our examination of a bilayer of NbSe$_2$ reveals that the van der Waals gap acts as an intrinsic weak link between the superconducting NbSe$_2$ layers. Therefore, a bilayer of NbSe$_2$ represents one of the thinnest and most tunable Josephson junction architectures, with potential applications in quantum devices. Our findings underscore the utility of transformation into real-space in understanding superconducting properties through ab initio calculations.

cond-mat.supr-con↗

arXiv2025

Planar Hall effect in ultrathin topological insulator films

The planar Hall effect (PHE), previously observed in Weyl and Dirac semimetals due to the chiral anomaly, emerges with a different origin in topological insulators (TIs), where in-plane magnetic fields induce resistivity anisotropy. In strictly two-dimensional TIs, PHE is generally suppressed due to the inability of the out-of-plane Berry curvature to couple to the in-plane band velocity of the charge carriers. Here, we demonstrate that in ultrathin TI films, a quasi-two-dimensional system, intersurface tunneling coupling with in-plane magnetization induces electronic anisotropy, enabling a finite PHE. In addition, we reveal that strong in-plane magnetization can stabilize the thickness-dependent quantum anomalous Hall effect, typically associated with out-of-plane magnetization. These insights advance the understanding of magnetic topological phases, paving the way for next-generation spintronic devices and magnetic sensing technologies.

cond-mat.mes-hall↗

arXiv2025

Machine-Learning Interatomic Potential for Twisted Hexagonal Boron Nitride: Accurate Structural Relaxation and Emergent Polarization

The emerging ferroelectric properties of two-dimensional (2D) heterostructures are at the forefront of science and prospective technology. In moiré bilayers, twisting or heterostructuring causes local atomic reconstruction, which even at picometer scale, can lead to pronounced ferroelectric polarization. Accurately determining this reconstruction utilizing ab initio methods is unfeasible for the relevant system sizes, but modern machine-learning interatomic potentials offer a viable solution. Here, we present the Gaussian Approximation Potential for twisted hexagonal boron nitride (hBN) layers validated against ab initio datasets. This approach enables the precise analysis of their structural properties, which is particularly relevant at small twist angles. We couple the structural information to a tight-binding model based on accurate interatomic positioning, and determine the twist-dependent polarization, yielding results that closely align with previous experimental findings - even at room temperature. This methodology enables further studies that are unattainable otherwise and is transferable to other 2D materials of interest.

cond-mat.mtrl-sci↗

arXiv2025

Light-induced dissipationless states in magnetic topological insulators with hexagonal warping

Magnetic impurities in topological insulators (TIs) induce backscattering via magnetic torque, unlike pristine TIs where spin-orbit locking promotes dissipationless surface states. Here we reveal that one can suppress that unwanted backscattering and dissipation in magnetic TIs using high-frequency linearly polarized light (LPL). By carefully considering the hexagonal warping of the Fermi surface of the TI, we demonstrate how the coupling between Dirac surface states and LPL can effectively reduce backscattering on magnetic dopants, enhance carrier mobility and suppress resistance, even entirely. These findings open up avenues for designing ultra low-power sensing and spintronic technology.

cond-mat.mes-hall↗