arXiv subjects

Milorad V. Milošević

Publications and source records attributed to Milorad V. Milošević.

At least 37 records · Page 2Linked to original sources

arXiv2025

Beyond the orbitally-resolved magnetic exchange in CrI$_{3}$ and NiI$_{2}$

The pertinent need for microscopic understanding of magnetic exchange motivated us to go beyond the existing theories and develop a systematic method to quantify all possible mechanisms that contribute to magnetic exchange for an arbitrary pair of atoms in a given material. We apply it to the archetypal 2D magnetic monolayers CrI3 and NiI2, to reveal the previously underrated dx2-y2,dx2-y2 contribution as either the leading or the second largest contribution to the total magnetic exchange. We proceed to explore the microscopic mechanisms behind all the non-zero orbital contributions in both CrI3 and NiI2, and generalize the findings to other magnetic monolayers dominated by d8 and d3 electronic configurations of the magnetic atoms.

cond-mat.mtrl-sci↗

arXiv2024

Towards Advanced Chiral Sensors: Enhanced Helicity-Dependent Photocurrent in Ultrathin Topological Insulator Films

Chirality, a fundamental property of asymmetric structures, plays a crucial role in pharmaceutical, biological and chemical systems, offering a powerful tool for screening organic compounds. While the conventional optical chirality detectors are often bulky and involuted, the topological insulators (TIs) offer a promising platform for developing compact yet sensitive devices - owing to their inherent chirality. However, the complex interplay of photoresponses in TIs can limit the ultimate accuracy of chirality detection. Therefore, we here analyze the underlying mechanisms governing the photoresponses in TIs and reveal strategies to enhance the helicity-dependent photocurrent (HDPC). By attentively analyzing the symmetries and behavior of competing photoresponses, we show that it is possible to effectively eliminate unwanted contributions and isolate the HDPC. Moreover, we reveal that HDPC is strongly amplified in ultrathin TI films, and can be further enhanced by optimizing the illumination parameters, sensor strain and/or back gating. Our findings thereby provide a roadmap for design and optimization of miniaturized, high-performance TI chirality detectors, with potential to revolutionize chiral analysis in biomedical and material sciences.

cond-mat.mes-hall↗

arXiv2024

Strain-tunable magnetic and magnonic states in Ni-dihalide monolayers

Monolayer NiI$_2$ garners large research interest due to its multiferroic behavior stemming from the interplay between its non-collinear magnetic order and the spin-orbit coupling. This prompts an investigation into the stability of the magnetic order in NiI$_2$ and similar materials under external stimuli. In this work, we report the effect of biaxial and uniaxial strain on the magnetic ground state, the critical temperature, and the magnonic properties of the NiX$_2$ (X = I, Br, Cl) monolayers. For all three materials, we reveal intricate strain-dependent phase diagrams, including ferromagnetic, helimagnetic, and skyrmionic phases. Moreover, we discuss the necessity of considering the biquadratic exchange interaction in the latter analysis. We reveal that the biquadratic exchange significantly alters both the magnetic ground state and the critical temperature of the magnetic order, and we demonstrate that its importance becomes even more explicit when monolayer Ni-dihalides are strained. Finally, we calculate the magnonic dispersion for the predicted magnetic states, showing that the skyrmionic phase functions as a magnonic crystal, and demonstrate the presence of strain-tunable soft magnon modes at finite wavevectors in the helimagnetic phase.

cond-mat.mes-hall↗

arXiv2024

Enhanced superconductivity of hydrogenated $β_{12}$ borophene

Borophene stands out among elemental two-dimensional materials due to its extraordinary physical properties, including structural polymorphism, strong anisotropy, metallicity, and the potential for phonon-mediated superconductivity. However, confirming superconductivity in borophene experimentally has been evasive to date, mainly due to the detrimental effects of metallic substrates and its susceptibility to oxidation. In this study, we present an \textit{ab initio} analysis of superconductivity in the experimentally synthesized hydrogenated $β_{12}$ borophene, which has been proven to be less prone to oxidation. Our findings demonstrate that hydrogenation significantly enhances both the stability and superconducting properties of $β_{12}$ borophene. Furthermore, we reveal that tensile strain and hole doping, achievable through various experimental methods, significantly enhance the critical temperature, reaching up to 29 K. These findings not only promote further fundamental research on superconducting borophene and its heterostructures, but also position hydrogenated borophene as a versatile platform for low-dimensional superconducting electronics.

cond-mat.supr-con↗

arXiv2024

First-principles exploration of superconductivity in intercalated bilayer borophene phases

We explore the emergence of phonon-mediated superconductivity in bilayer borophenes by controlled intercalation with elements from the groups of alkali, alkaline-earth, and transition metals, using systematic first-principles and Eliashberg calculations. We show that the superconducting properties are primarily governed by the interplay between the out-of-plane ($p_{z}$) boron states and the partially occupied in-plane ($s+p_{x,y}$) bonding states at the Fermi level. Our Eliashberg calculations indicate that intercalation with alkaline-earth elements leads to the highest superconducting critical temperatures ($T_{c}$). Specifically, Be in $δ_{4}$, Mg in $χ_{3}$, and Ca in the kagome bilayer borophene demonstrate superior performance with $T_{c}$ reaching up to 58~K. Our study therefore reveals that intercalated bilayer borophene phases are not only more resilient to chemical deterioration, but also harbor enhanced $T_{c}$ values compared to their monolayer counterparts, underscoring their substantial potential for the development of boron-based two-dimensional superconductors.

cond-mat.supr-con↗

arXiv2024

High-$T_c$ Berezinskii-Kosterlitz-Thouless transition in 2D superconducting systems with coupled deep and quasi-flat electronic bands with van Hove singularities

In the pursuit of higher critical temperature of superconductivity, quasi-flat electronic bands and van Hove singularities in two dimensions (2D) have emerged as a potential approach to enhance Cooper pairing on the basis of mean-field expectations. However, these special electronic features suppress the superfluid stiffness and, hence, the Berezinskii-Kosterlitz-Thouless (BKT) transition in 2D superconducting systems, leading to the emergence of a significant pseudogap regime due to superconducting fluctuations. In the strong-coupling regime, one finds that superfluid stiffness is inversely proportional to the superconducting gap, which is the predominant factor contributing to the strong suppression of superfluid stiffness. Here we reveal that the aforementioned limitation is avoided in a 2D superconducting electronic system with a quasi-flat electronic band with a strong pairing strength coupled to a deep band with weak electronic pairing strength. Owing to the multiband effects, we demonstrate a screening-like mechanism that circumvents the suppression of the superfluid stiffness. We report the optimal conditions for achieving a large enhancement of the BKT transition temperature and a substantial shrinking of the pseudogap regime by tuning the intraband couplings and the pair-exchange coupling between the two band-condensates.

cond-mat.supr-con↗

arXiv2024

Realization of a Two-Dimensional Lieb Lattice in a Metal-Inorganic Framework with Flat Bands and Topological Edge States

Flat bands and Dirac cones in materials are at the source of the exotic electronic and topological properties. The Lieb lattice is expected to host these electronic structures, arising from quantum destructive interference. Nevertheless, the experimental realization of a two-dimensional Lieb lattice remained challenging to date due to its intrinsic structural instability. After computationally designing a Platinum-Phosphorus (Pt-P) Lieb lattice, we have successfully overcome its structural instability and synthesized it on a gold substrate via molecular beam epitaxy. Low-temperature scanning tunneling microscopy and spectroscopy verified the Lieb lattice's morphology and electronic flat bands. Furthermore, topological Dirac edge states stemming from pronounced spin-orbit coupling induced by heavy Pt atoms have been predicted. These findings convincingly open perspectives for creating metal-inorganic framework-based atomic lattices, offering prospects for strongly correlated phases interplayed with topology.

physics.app-ph↗

arXiv2024

Unconventional superconducting diode effects via antisymmetry and antisymmetry breaking

Symmetry-breaking plays a pivotal role in unlocking intriguing properties and functionalities in material systems. For example, the breaking of spatial and temporal symmetries leads to a fascinating phenomenon of superconducting diode effect. However, generating and precisely controlling the superconducting diode effect poses significant challenges. Here, we take a novel route with deliberate manipulation of magnetic charge potentials to realize unconventional superconducting flux-quantum diode effects. We achieve this through suitably tailored nanoengineered arrays of nanobar magnets on top of a superconducting thin film. We demonstrate the vital roles of inversion antisymmetry and its breaking in evoking unconventional superconducting effects-a magnetically symmetric diode effect and an odd-parity magnetotransport effect. These effects are non-volatilely controllable through in-situ magnetization switching of the nanobar magnets. Our findings promote the use of antisymmetry (breaking) for initiating unconventional superconducting properties, paving the way for exciting prospects and innovative functionalities in superconducting electronics.

cond-mat.supr-con↗

arXiv2023

Probing confined vortices with a superconducting nanobridge

We realize a superconducting nanodevice in which vortex traps in the form of an aluminum square are integrated with a Dayem nanobridge. We perform field-cooling of the traps arriving to different vortex configurations, dependent on the applied magnetic field, to demonstrate that the switching current of the bridge is highly sensitive to the presence and location of vortices in the trap. Our measurements exhibit unprecedented precision and ability to detect the first and successive vortex entries into all fabricated traps, from few hundred nm to 2 $μ$m in size. The experimental results are corroborated by Ginzburg-Landau simulations, which reveal the subtle yet crucial changes in the density of the superconducting condensate in the vicinity of the bridge with every additional vortex entry and relocation inside the trap. An ease of integration and simplicity make our design a convenient platform for studying dynamics of vortices in strongly confining geometries, involving a promise to manipulate vortex states electronically with simultaneous in situ control and monitoring.

cond-mat.supr-con↗

arXiv2023

Flattening conduction and valence bands for interlayer excitons in a moiré MoS$_2$/WSe$_2$ heterobilayer

We explore the flatness of conduction and valence bands of interlayer excitons in MoS$_2$/WSe$_2$ van der Waals heterobilayers, tuned by interlayer twist angle, pressure, and external electric field. We employ an efficient continuum model where the moiré pattern from lattice mismatch and/or twisting is represented by an equivalent mesoscopic periodic potential. We demonstrate that the mismatch moiré potential is too weak to produce significant flattening. Moreover, we draw attention to the fact that the quasi-particle effective masses around the $Γ$-point and the band flattening are \textit{reduced} with twisting. As an alternative approach, we show (i) that reducing the interlayer distance by uniform vertical pressure can significantly increase the effective mass of the moiré hole, and (ii) that the moiré depth and its band flattening effects are strongly enhanced by accessible electric gating fields perpendicular to the heterobilayer, with resulting electron and hole effective masses increased by more than an order of magnitude leading to record-flat bands. These findings impose boundaries on the commonly generalized benefits of moiré twistronics, while also revealing alternate feasible routes to achieve truly flat electron and hole bands to carry us to strongly correlated excitonic phenomena on demand.

cond-mat.mes-hall↗

arXiv2023

Strong gate-tunability of flat bands in bilayer graphene due to moiré encapsulation between hBN monolayers

When using hexagonal boron-nitride (hBN) as a substrate for graphene, the resulting moiré pattern creates secondary Dirac points. By encapsulating a multilayer graphene within aligned hBN sheets the controlled moiré stacking may offer even richer benefits. Using advanced tight-binding simulations on atomistically-relaxed heterostructures, here we show that the gap at the secondary Dirac point can be opened in selected moiré-stacking configurations, and is independent of any additional vertical gating of the heterostructure. On the other hand, gating can broadly tune the gap at the principal Dirac point, and may thereby strongly compress the first moiré mini-band in width against the moiré-induced gap at the secondary Dirac point. We reveal that in hBN-encapsulated bilayer graphene this novel mechanism can lead to isolated bands flatter than 10~meV under moderate gating, hence presenting a convenient pathway towards electronically-controlled strongly-correlated states on demand.

cond-mat.mes-hall↗

arXiv2023

Towards Magnonic Logic and Neuromorphic Computing: Controlling Spin-Waves by Spin-Polarized Current

Spin-waves (magnons) are among the prime candidates for building fast yet energy-efficient platforms for information transport and computing. We here demonstrate theoretically and in state-of-the-art micromagnetic simulation the effects that strategically-injected spin-polarized current can have on controlling magnonic transport. We reveal analytically that the Zhang-Li spin-transfer-torque induced by applied current is analogous to the Dzyaloshinskii-Moriya interaction for scattering the magnons in the linear regime, to then provide a generalized Snell's law that describes the spin-wave propagation across regions with different current densities. We validate the latter in numerical simulations of realistic systems, and exemplify how these findings may help advance the design of spin-wave logic and neuromorphic computing devices.

cond-mat.mtrl-sci↗

arXiv2022

Vortical versus skyrmionic states in the topological phase of a twisted bilayer with $d$-wave superconducting pairing

It was recently shown that a chiral topological phase emerges from the coupling of two twisted monolayers of superconducting Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ for certain twist angles. In this work, we reveal the behavior of such twisted superconducting bilayers with $d_{x^2-y^2}$ pairing symmetry in presence of applied magnetic field. Specifically, we show that the emergent vortex matter can serve as smoking gun for detection of topological superconductivity in such bilayers. Moreover, we report two distinct skyrmionic states that characterize the chiral topological phase, and provide full account of their experimental signatures and their evolution with the twist angle.

cond-mat.supr-con↗

arXiv2021

High-temperature multigap superconductivity in two-dimensional metal-borides

Using first-principles calculations in combination with the Eliashberg formalism, we systematically investigated phonon-mediated superconductivity in two-dimensional (2D) metal-boride crystals, consisting of a boron honeycomb network doped by diverse metal elements. Such 2D metal-boride compounds, named MBenes, are chemically exfoliable from single-crystalline layered ternary borides (MAB phases). First, we identified the MBene layers with potential for superconductivity via isotropic Eliashberg calculations, considering a wide range of metal elements, with focus on alkaline earth and transition metals. Subsequently, we performed a detailed analysis of the prominent superconducting MBenes by solving the anisotropic Eliashberg equations. The obtained high critical temperatures (up to 72 K), as well as the rich multigap superconducting behavior, recommend these crystals for further use in multifunctional 2D heterostructures and superconducting device applications.

cond-mat.supr-con↗

arXiv2021

Tailoring High-Frequency Magnonics in Monolayer Chromium Trihalides

Monolayer chromium trihalides, the archetypal two dimensional (2D) magnetic materials, are readily suggested as a promising platform for high frequency magnonics. Here we detail the spin wave properties of monolayer CrBr$_3$ and CrI$_3$, using spin dynamics simulations parametrized from the first principles. We reveal that spin wave dispersion can be tuned in a broad range of frequencies by strain, paving the way towards flexo magnonic applications. We further show that ever present halide vacancies in these monolayers host sufficiently strong Dzyaloshinskii Moriya interaction to scatter spin waves, which promotes design of spin-wave guides by defect engineering. Finally we discuss the spectra of spin-waves propagating across a moiré periodic modulation of magnetic parameters in a van der Waals heterobilayer, and show that the nanoscale moiré periodicities in such samples are ideal for realization of a magnonic crystal in the terahertz frequency range. Recalling the additional tunability of magnetic 2D materials by electronic gating, our results situate these systems among the front-runners for prospective high frequency magnonic applications.

physics.comp-ph↗

arXiv2021

Superconducting diode effect via conformal-mapped nanoholes

A superconducting diode is an electronic device that conducts supercurrent and exhibits zero resistance primarily for one direction of applied current. Such a dissipationless diode is a desirable unit for constructing electronic circuits with ultralow power consumption. However, realizing a superconducting diode is fundamentally and technologically challenging, as it usually requires a material structure without a centre of inversion, which is scarce among superconducting materials. Here, we demonstrate a superconducting diode achieved in a conventional superconducting film patterned with a conformal array of nanoscale holes, which breaks the spatial inversion symmetry. We showcase the superconducting diode effect through switchable and reversible rectification signals, which can be three orders of magnitude larger than that from a flux-quantum diode. The introduction of conformal potential landscapes for creating a superconducting diode is thereby proven as a convenient, tunable, yet vastly advantageous tool for superconducting electronics. This could be readily applicable to any superconducting materials, including cuprates and iron-based superconductors that have higher transition temperatures and are desirable in device applications.

cond-mat.supr-con↗

arXiv2020

2D ferromagnetism at finite temperatures under quantum scrutiny

Recent years have seen a tremendous rise of two-dimensional (2D) magnetic materials, several of which verified experimentally. However, most of the theoretical predictions to date rely on ab-initio methods, at zero temperature and fluctuations-free, while one certainly expects detrimental quantum fluctuations at finite temperatures. Here we present the solution of the quantum Heisenberg model for honeycomb/hexagonal lattices with anisotropic exchange interaction up to third nearest neighbors and in an applied field in arbitrary direction, that answers the question whether long-range magnetization can indeed survive in the ultrathin limit of materials, up to which temperature, and what the characteristic excitation (magnon) frequencies are, all essential to envisaged applications of magnetic 2D materials. We find that long-range magnetic order persists at finite temperature for materials with overall easy-axis anisotropy. We validate the calculations on the examples of monolayer CrI3, CrBr3 and MnSe2. Moreover, we provide an easy-to-use tool to calculate Curie temperatures of new 2D computational materials.

cond-mat.stat-mech↗

arXiv2020

Spin textures in chiral magnetic monolayers with suppressed nearest-neighbor exchange

High tunability of two dimensional magnetic materials (by strain, gating, heterostructuring or otherwise) provides unique conditions for studying versatile magnetic properties and controlling emergent magnetic phases. Expanding the scope of achievable magnetic phenomena in such materials is important for both fundamental and technological advances. Here we perform atomistic spin-dynamics simulations to explore the (chiral) magnetic phases of atomic monolayers in the limit of suppressed first-neighbors exchange interaction. We report the rich phase diagram of exotic magnetic configurations, obtained for both square and honeycomb lattice symmetries, comprising coexistence of ferromagnetic and antiferromagnetic spin-cycloids, as well as multiple types of magnetic skyrmions. We perform a minimum-energy path analysis for the skyrmion collapse to evaluate the stability of such topological objects, and reveal that magnetic monolayers could be good candidates to host the antiferromagnetic skyrmions that are experimentally evasive to date.

physics.comp-ph↗