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Minjae Kim

Publications and source records attributed to Minjae Kim.

At least 73 records · Page 4Linked to original sources

Strain tunable electronic ground states in two-dimensional iridate thin films

Quantum phases of matter such as superconducting, ferromagnetic and Wigner crystal states are often driven by the two-dimensionality (2D) of correlated systems. Meanwhile, spin-orbit coupling (SOC) is a fundamental element leading to nontrivial topology which gives rise to quantum phenomena such as the large anomalous Hall effect and nontrivial superconductivity. However, the search for controllable platforms with both 2D and SOC has been relatively overlooked so far. Here, we control and study the electronic ground states of iridate ultrathin films having both 2D and SOC by angle-resolved photoemission spectroscopy (ARPES) and dynamical mean field theory (DMFT) calculations. The metallicity of SrIrO$_3$ ultrathin films is controlled down to a monolayer by dimensional and strain manipulation. Our results suggest that the iridate ultrathin films can be a controllable 2D SOC platform exhibiting a variety of phenomena for future functional devices.

cond-mat.str-el↗

The JWST Early Release Science Program for Direct Observations of Exoplanetary Systems V: Do Self-Consistent Atmospheric Models Represent JWST Spectra? A Showcase With VHS 1256 b

The unprecedented medium-resolution (R~1500-3500) near- and mid-infrared (1-18um) spectrum provided by JWST for the young (140+/-20Myr) low-mass (12-20MJup) L-T transition (L7) companion VHS1256b gives access to a catalogue of molecular absorptions. In this study, we present a comprehensive analysis of this dataset utilizing a forward modelling approach, applying our Bayesian framework, ForMoSA. We explore five distinct atmospheric models to assess their performance in estimating key atmospheric parameters: Teff, log(g), [M/H], C/O, gamma, fsed, and R. Our findings reveal that each parameter's estimate is significantly influenced by factors such as the wavelength range considered and the model chosen for the fit. This is attributed to systematic errors in the models and their challenges in accurately replicating the complex atmospheric structure of VHS1256b, notably the complexity of its clouds and dust distribution. To propagate the impact of these systematic uncertainties on our atmospheric property estimates, we introduce innovative fitting methodologies based on independent fits performed on different spectral windows. We finally derived a Teff consistent with the spectral type of the target, considering its young age, which is confirmed by our estimate of log(g). Despite the exceptional data quality, attaining robust estimates for chemical abundances [M/H] and C/O, often employed as indicators of formation history, remains challenging. Nevertheless, the pioneering case of JWST's data for VHS1256b has paved the way for future acquisitions of substellar spectra that will be systematically analyzed to directly compare the properties of these objects and correct the systematics in the models.

astro-ph.EP↗

Impact of discontinuous grain size distributions on the spectral energy distribution of debris disks

The collisional evolution of debris disks is expected to result in a characteristic wavy pattern of the grain size distributions, i.e., an under/overabundance of particles of specific sizes. This perturbed grain size distribution potentially leaves characteristic patterns in the spectral energy distribution (SED) of the disk system. We aim to quantify and understand the specific influence of discontinuous particle size distributions on the appearance of debris disks. For this purpose, we consider dust emission models based on two different grain size distributions, i.e., once with a single and once with a broken power law. We compare the spectral index $α$ ($F_ν\,\propto ν^{\rm{\,α}}$) in the case of a continuous grain size distribution with that of a discontinuous grain size distribution. We perform this comparison for central stars with different spectral types and two different disk structures (e.g., slim and broad debris dust rings). Within the considered parameter space, we find a characteristic difference between the spectral slopes of the SED in the different scenarios. More specifically, the overabundance of small grains leads to a steeper slope in the far-infrared/submillimeter regime, while the spectral index in the mm regime is hardly affected. On the other hand, the underabundance of medium-sized grains results in a slight steepening of the far-infrared slope of SED, while its primary effect is on the mm slope of SED, causing it to become shallower. We also find that the impact of an overabundance of small dust particles is more pronounced than that of an underabundance of medium-sized dust particles. Furthermore, we find that the difference between the spectral indices for the two different grain size distributions is largest for debris disks around brighter central stars and broader disks.

astro-ph.EP↗

Optical detection of bond-dependent and frustrated spin in the two-dimensional cobalt-based honeycomb antiferromagnet Cu3Co2SbO6

Two-dimensional honeycomb antiferromagnet becomes an important class of materials as it can provide a route to Kitaev quantum spin liquid, characterized by massive quantum entanglement and fractional excitations. The signatures of its proximity to Kitaev quantum spin liquid in the honeycomb antiferromagnet includes anisotropic bond-dependent magnetic responses and persistent fluctuation by frustration in paramagnetic regime. Here, we propose Cu3Co2SbO6 heterostructures as an intriguing honeycomb antiferromagnet for quantum spin liquid, wherein bond-dependent and frustrated spins interact with optical excitons. This system exhibits antiferromagnetism at 16 K with different spin-flip magnetic fields between a bond-parallel and bond-perpendicular directions, aligning more closely with the generalized Heisenberg-Kitaev than the XXZ model. Optical spectroscopy reveals a strong excitonic transition coupled to the antiferromagnetism, enabling optical detection of its spin states. Particularly, such spin-exciton coupling presents anisotropic responses between bond-parallel and bond-perpendicular magnetic field as well as a finite spin-spin correlation function around 40 K, higher than twice its Néel temperature. The characteristic temperature that remains barely changed even under strong magnetic fields highlights the robustness of the spin-fluctuation region. Our results demonstrate Cu3Co2SbO6 as a unique candidate for the quantum spin liquid phase, where the spin Hamiltonian and quasiparticle excitations can be probed and potentially controlled by light.

cond-mat.str-el↗

Implementation Of MNIST Dataset Learning Using Analog Circuit

There have been many attempts to implement neural networks in the analog circuit. Most of them had a lot of input terms, and most studies implemented neural networks in the analog circuit through a circuit simulation program called Spice to avoid the need to design chips at a high cost and implement circuits directly to input them. In this study, we will implement neural networks using a capacitor and diode and use microcontrollers (Arduino Mega 2560 R3 boards) to drive real-world models and analyze the results.

cs.ET↗

Chiral magnetism and ordering of oxygen vacancies in SrTiO$_{2.5}$

Oxygen vacancies in the perovskite insulator SrTiO$_3$ free electrons that couple with other physical degrees of freedom such as lattice, orbital, and spin. This leads to the emergence of exotic quantum states such as superconductivity and unusual ferromagnetism. We perform density-functional theory and dynamical mean-field theory calculations and demonstrate that the orientation and ordering of the TiO$_5$ pentahedra plays a crucial role. Specifically, for vacancy-rich SrTiO$_{3-δ}$ ($δ\sim$0.5), we find a chiral ordering of the TiO$_5$ pentahedra in a sixfold superlattice. This chiral structure is accompanied by a chiral magnetic state with a net moment in the (111) direction at room temperature, which can explain several experimental observations.

cond-mat.str-el↗

Orbital Selective Mott Transition Effects and Non-Trivial Topology of Iron Chalcogenide

The iron-based superconductor FeSe$_{1-x}$Te$_{x}$ (FST) has recently gained significant attention as a host of two distinct physical phenomena: ($i$) Majorana zero modes which can serve as potential topologically protected qubits, and ($ii$) a realization of the orbital selective Mott transition (OSMT). In this Letter, we connect these two phenomena and provide new insights into the interplay between strong electronic correlations and non-trivial topology in FST. Using linearized quasiparticle self-consistent GW plus dynamical mean-field theory, we show that the topologically protected Dirac surface state has substantial Fe($d_{xy}$) character. The proximity to the OSMT plays a dual role, it facilitates the appearance of the topological surface state by bringing the Dirac cone close to the chemical potential, but destroys the Z$_{2}$ topological superconductivity when the system is too close to the orbital selective Mott phase (OSMP). We derive a reduced effective Hamiltonian that describes the topological band. Its parameters capture all the chemical trends found in the first principles calculation. Our findings provide a framework for further study of the interplay between strong electronic correlations and non-trivial topology in other iron-based superconductors.

cond-mat.str-el↗

Intersite Coulomb Interactions in Charge Ordered Systems

Using {\it ab initio} approaches for extended Hubbard interactions coupled to phonons, we reveal that the intersite Coulomb interaction plays important roles in determining various distinctive phases of the paradigmatic charge ordered materials of Ba$_{1-x}$K$_x A$O$_3$ ($A=$ Bi and Sb). We demonstrated that all their salient doping dependent experiment features such as breathing instabilities, anomalous phonon dispersions, and transition between charge-density wave and superconducting states can be accounted very well if self-consistently obtained nearest neighbor Hubbard interaction are included, thus establishing a minimal criterion for reliable descriptions of spontaneous charge orders in solids.

cond-mat.str-el↗

Flybys in debris disk systems with Gaia eDR3

We aim to observationally and statistically constrain the influence of flybys in the formation and evolution of debris disks. We compiled a sample of 254 debris disks with ages between 2 Myr and 8 Gyr that are either part of an association or isolated, drawing the binary and planetary companions of the systems mainly from the literature. Using the Gaia eDR3 astrometric data and radial velocities of our sample, as well as all the sources in a specific region of the sky, we reconstructed the relative linear motions in the last 5 Myr and made predictions for the next 2 Myr. Relating the Hill radius of each debris disk system and the closest distances reached by the two sources, we defined the flyby events in terms of position and time. We find that in the period between the last 5 Myrs and the next 2 Myrs, 90% of the analyzed systems have experienced at least a close flyby, while 7% of them have experienced flybys at distances greater than 0.5R Hill. In particular, 75% of them have experienced at least one past close encounter and 36% multiple past close encounters. From the sub-sample of resolved debris disk (41 out of 94), 80% of the analyzed systems experience at least an encounter within 0.8 pc. From the subsample of 10 debris disks with planets, half of these systems do show misalignments between disk and planet, stirring, or asymmetries. Systems with a misalignment between the planetary orbit and the disk do indeed experience at least one flyby event. In particular, when the planet orbits have a difference with the disk inclination higher than about 20 degree, as in the case of HD 38529, we find that multiple close encounters have taken place in the last 5 Myr, as theoretically predicted. The high incidence of encounters, particularly close encounters, experienced by the systems in the last 5 Myr suggests the fundamental impact of flybys on the evolution of debris disks.

astro-ph.EP↗

Honeycomb oxide heterostructure: a new platform for Kitaev quantum spin liquid

Kitaev quantum spin liquid, massively quantum entangled states, is so scarce in nature that searching for new candidate systems remains a great challenge. Honeycomb heterostructure could be a promising route to realize and utilize such an exotic quantum phase by providing additional controllability of Hamiltonian and device compatibility, respectively. Here, we provide epitaxial honeycomb oxide thin film Na3Co2SbO6, a candidate of Kitaev quantum spin liquid proposed recently. We found a spin glass and antiferromagnetic ground states depending on Na stoichiometry, signifying not only the importance of Na vacancy control but also strong frustration in Na3Co2SbO6. Despite its classical ground state, the field-dependent magnetic susceptibility shows remarkable scaling collapse with a single critical exponent, which can be interpreted as evidence of quantum criticality. Its electronic ground state and derived spin Hamiltonian from spectroscopies are consistent with the predicted Kitaev model. Our work provides a unique route to the realization and utilization of Kitaev quantum spin liquid.

cond-mat.str-el↗

Metal to Mott Insulator Transition in Two-dimensional 1T-TaSe$_2$

When electron-electron interaction dominates over other electronic energy scales, exotic, collective phenomena often emerge out of seemingly ordinary matter. The strongly correlated phenomena, such as quantum spin liquid and unconventional superconductivity, represent a major research frontier and a constant source of inspiration. Central to strongly correlated physics is the concept of Mott insulator, from which various other correlated phases derive. The advent of two-dimensional (2D) materials brings unprecedented opportunities to the study of strongly correlated physics in the 2D limit. In particular, the enhanced correlation and extreme tunability of 2D materials enables exploring strongly correlated systems across uncharted parameter space. Here, we discover an intriguing metal to Mott insulator transition in 1T-TaSe$_2$ as the material is thinned down to atomic thicknesses. Specifically, we discover, for the first time, that the bulk metallicity of 1T-TaSe$_2$ arises from a band crossing Fermi level. Reducing the dimensionality effectively quenches the kinetic energy of the initially itinerant electrons and drives the material into a Mott insulating state. The dimensionality-driven Metal to Mott insulator transition resolves the long-standing dichotomy between metallic bulk and insulating surface of 1T-TaSe$_2$. Our results additionally establish 1T-TaSe$_2$ as an ideal variable system for exploring various strongly correlated phenomena.

cond-mat.str-el↗

Style-Guided Inference of Transformer for High-resolution Image Synthesis

Transformer is eminently suitable for auto-regressive image synthesis which predicts discrete value from the past values recursively to make up full image. Especially, combined with vector quantised latent representation, the state-of-the-art auto-regressive transformer displays realistic high-resolution images. However, sampling the latent code from discrete probability distribution makes the output unpredictable. Therefore, it requires to generate lots of diverse samples to acquire desired outputs. To alleviate the process of generating lots of samples repetitively, in this article, we propose to take a desired output, a style image, as an additional condition without re-training the transformer. To this end, our method transfers the style to a probability constraint to re-balance the prior, thereby specifying the target distribution instead of the original prior. Thus, generated samples from the re-balanced prior have similar styles to reference style. In practice, we can choose either an image or a category of images as an additional condition. In our qualitative assessment, we show that styles of majority of outputs are similar to the input style.

cs.CV↗

Tunable electronic and magnetic phases in layered ruthenates: SrRuO3-SrTiO3 heterostructure upon strain

Layered ruthenates are a unique class of systems which manifests a variety of electronic and magnetic features emerged from competing energy scales. At the heart of such features lies the multi-orbital physics, especially, the orbital-selective behavior. Here, we propose that the SrRuO3-SrTiO3 heterostructure is a highly tunable platform to obtain the various emergent properties. Employing the density functional theory plus dynamical mean-field theory, we thoroughly investigate the orbital-dependent physics of the system and identify the competing magnetic fluctuations. We show that the epitaxial strain drives the system towards multi-orbital or orbital selective Mott phases from the Hund metal regime. At the same time, the two different types of static magnetism are stabilized, ferromagnetism and checkerboard antiferromagnetism, from the competition with the spin-density wave instability.

cond-mat.str-el↗

Competing spin-fluctuations in Sr$_2$RuO$_4$ and their tuning through epitaxial strain

In this study, we report the magnetic energy landscape of Sr2RuO4 employing the generalized Bloch approach within density functional theory. We identify the two dominant magnetic instabilities, ferromagnetic and spin-density-wave, together with other predominant instabilities. We show that epitaxial strain can change the overall magnetic tendency of the system, and tune the relative weight of the various magnetic instabilities in the system. Especially, the balance between spin-density wave and ferromagnetic instabilities can be controlled by the strain, and, eventually can lead to the new magnetic phases as well as superconducting phases with possibly altered pairing channels. Our findings are compared with previous theoretical models and experimental reports for the various magnetic features of the system and offer a first-principles explanation to them.

cond-mat.str-el↗

Growth of delafossite CuAlO2 single crystals in a reactive crucible

Delafossite oxide CuAlO2 has engaged great attention as a promising p-type conducting oxide. In this work, high-quality CuAlO2 single crystals with a size of several millimeters (mm) are successfully achieved with a reactive crucible melting method. The crystals are characterized by X-ray diffraction, scanning electron microscopy with energy-dispersive spectroscopy, transport measurement, and magnetic susceptibility measurement. The grown single crystals are free of contamination from a copper oxide flux. This work provides a new approach to growing high-quality delafossite oxide CuAlO2 with a few mm size.

cond-mat.mtrl-sci↗

StyLandGAN: A StyleGAN based Landscape Image Synthesis using Depth-map

Despite recent success in conditional image synthesis, prevalent input conditions such as semantics and edges are not clear enough to express `Linear (Ridges)' and `Planar (Scale)' representations. To address this problem, we propose a novel framework StyLandGAN, which synthesizes desired landscape images using a depth map which has higher expressive power. Our StyleLandGAN is extended from the unconditional generation model to accept input conditions. We also propose a '2-phase inference' pipeline which generates diverse depth maps and shifts local parts so that it can easily reflect user's intend. As a comparison, we modified the existing semantic image synthesis models to accept a depth map as well. Experimental results show that our method is superior to existing methods in quality, diversity, and depth-accuracy.

cs.CV↗

Social norms in indirect reciprocity with ternary reputations

Indirect reciprocity is a key mechanism that promotes cooperation in social dilemmas by means of reputation. Although it has been a common practice to represent reputations by binary values, either `good' or `bad', such a dichotomy is a crude approximation considering the complexity of reality. In this work, we studied norms with three different reputations, i.e., `good', `neutral', and `bad'. Through massive supercomputing for handling more than thirty billion possibilities, we fully identified which norms achieve cooperation and possess evolutionary stability against behavioural mutants. By systematically categorizing all these norms according to their behaviours, we found similarities and dissimilarities to their binary-reputation counterpart, the leading eight. We obtained four rules that should be satisfied by the successful norms, and the behaviour of the leading eight can be understood as a special case of these rules. A couple of norms that show counter-intuitive behaviours are also presented. We believe the findings are also useful for designing successful norms with more general reputation systems.

q-bio.PE↗

Observation of spin-dependent dual ferromagnetism in perovskite ruthenates

We performed in-situ angle-resolved photoemission spectroscopy (ARPES) and spin-resolved ARPES (SARPES) experiments to investigate the relationship between electronic band structures and ferromagnetism in SrRuO$_3$ (SRO) thin films. Our high-quality ARPES and SARPES results show clear spin-lifted band structures. The spin polarization is strongly dependent on momentum around the Fermi level, whereas it becomes less dependent at high-binding energies. This experimental observation matches our dynamical mean-field theory (DMFT) results very well. As temperature increases from low to the Curie temperature, spin-splitting gap decreases and band dispersions become incoherent. Based on the ARPES study and theoretical calculation results, we found that SRO possesses spin-dependent electron correlations in which majority and minority spins are localized and itinerant, respectively. Our finding explains how ferromagnetism and electronic structure are connected, which has been under debate for decades in SRO.

cond-mat.str-el↗