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Mizuki Ohno

Publications and source records attributed to Mizuki Ohno.

10 recordsLinked to original sources

Quantum Hall effect in vacancy-engineered $\beta$-Ag$_2$Te

Accessing surface quantum transport in topological insulators is hampered by residual bulk conduction arising from lattice defects. Here, we demonstrate a novel synthesis pathway for realizing high mobility $\beta$-Ag$_2$Te thin films where surface transport is dominant. An \textit{in-situ} vacancy engineering step as part of the molecular beam epitaxy growth process acts to modify the stoichiometry and suppress donor-type defects, enabling continuous tuning of the sheet carrier density over more than an order of magnitude through the charge-neutrality point without an external gate electrode. In the lower-carrier-density films, a fully developed $\nu=1$ quantum Hall state is observed, and Landau-level energies extracted across samples collapse onto the $E_N=v_\mathrm{F}\sqrt{2e\hbar NB}$ relation, providing evidence for the massless Dirac dispersion of the top and bottom surface states. These results establish stoichiometry-driven vacancy engineering as a versatile lithography- and gate-free approach to accessing quantum Hall transport in epitaxial topological-insulator thin films.

cond-mat.mes-hall

Pair-Breaking and Dimensionality in Spin-Orbit Coupled Superconductors

The response of ultra-thin superconducting materials under parallel magnetic fields is often leveraged to obtain insight into the nature of the condensate, including features attributable to unconventional forms of pairing. Despite there being multiple competing mechanisms responsible for suppressing superconductivity, it is common for these analyses to overlook certain depairing channels. Here we report an analysis of thickness dependent superconductivity in thin films of \ce{LaBi2} using the multi-mechanism Kharitonov-Feigel'man framework . By resolving field-enhanced superconductivity in the thin-limit, we obtain an estimate the role of spin exchange scattering, in addition to paramagnetic and orbital effects. Our analyses offer insight into how fundamental quantities such as the critical temperature as well as Pauli limit are defined, recasting the landscape for how scattering times in two-dimensional superconductors can be interpreted.

cond-mat.supr-con

Anisotropic multiband magnetotransport in LaAg$_2$Ge$_2$ thin films

ThCr$_2$Si$_2$-type intermetallics are layered conductors in which crystallographic anisotropy and multiband electronic states often give rise to characteristic magnetotransport phenomena. Here, we report the molecular-beam epitaxy growth of LaAg$_2$Ge$_2$ thin films on MgO(001) and their magnetotransport properties. The Hall effect and magnetoresistance are captured by an effective two-carrier description with a high-mobility electron band, yielding a positive magnetoresistance of 22.5% at 9 T. Angle-dependent magnetoresistance exhibits a dominant twofold anisotropy and additional reproducible dip/peak features at characteristic tilt angles that are nearly independent of field and temperature. These results extend our understanding of the anisotropic electronic transport in thin-film germanides within the ThCr$_2$Si$_2$ family.

cond-mat.mtrl-sci

Relativistic Effects in LaBi$_2$ Thin Films

Chemical substitution in crystalline quantum materials is a powerful way to explore the consequences of strong spin-orbit coupling on their structural and electronic properties. In this work, we present an investigation of thin films of the La$\textit{Pn}_2$ ($\textit{Pn}$~=~Sb, Bi) class of layered square-net intermetallics. We report the growth of LaBi$_2$ with a pristine layer-by-layer growth mode, classifying it as a good metal displaying superconductivity at $\sim$0.55~K. Compared to LaSb$_2$, we attribute the enhanced metallic behavior and improved growth dynamics of LaBi$_2$ to significant relativistic corrections to its electronic band structure and the resulting impact on both surface energy and intrinsic phonon scattering.

cond-mat.mtrl-sci

Stacking-Selective Epitaxy of Rare-Earth Diantimonides

Deterministic control of the layering configuration of two-dimensional quantum materials plays a central role in studying their emergent electronic properties. Here we demonstrate in-situ control over competing stacking configurations in thin film crystals of the rare-earth diantimonides by synthesizing in proximity to competing structural orders. A crossover between the epitaxially stabilized monoclinic structure and the orthorhombic structure commonly observed in bulk crystals is navigated through three axes; the relative cation/anion ratio, growth temperature, and choice of lanthanide ion, culminating with a comparative magnetotransport study of single-yet-distinct phase CeSb2 films. These results set the stage for an expanded search for hidden stacking configurations in layered compounds which have evaded detection.

cond-mat.mtrl-sci

Berry curvature derived negative magnetoconductivity observed in type-II magnetic Weyl semimetal films

Here we study nonmonotonic features which appear both in magnetoresistivity and anomalous Hall resistivity during the simple magnetization process, by systematically measuring type-II magnetic Weyl semimetal EuCd$_2$Sb$_2$ films over a wide carrier density range. We find that a positive magnetoresistivity hump can be explained as manifestation of a field-linear term in the generalized magnetoconductivity formula including the Berry curvature. As also confirmed by model calculation, the term can be negative and pronounced near the Weyl point energy in the case that the Weyl cones are heavily tilted. Our findings demonstrate extensive effects of the Berry curvature on various magnetotransport in magnetic Weyl semimetals beyond the anomalous Hall effect.

cond-mat.mtrl-sci

Intrinsic insulating transport characteristics in low-carrier density EuCd2As2 films

Searching for an ideal magnetic Weyl semimetal hosting only a single pair of Weyl points has been a focal point for systematic clarification of its unique magnetotransport derived from the interplay between topology and magnetization. Among the candidates, triangular-lattice antiferromagnet EuCd$_2$As$_2$ has been attracting special attention due to the prediction of the ideal Weyl semimetal phase in the ferromagnetic state, however, transport properties of low-carrier density samples have remained elusive. Here we report molecular beam epitaxy growth of EuCd$_2$As$_2$ films, achieving low-hole density in the range of $10^{15}$-$10^{16}$ cm$^{-3}$ at low temperature. Transport measurements of such low-carrier density films reveal an insulating behavior with an activation gap of about 200 meV, which persists even in the field-induced ferromagnetic state. Our work provides an important experimental clue that EuCd$_2$As$_2$ is intrinsically insulating, contrary to the previous prediction.

cond-mat.mtrl-sci

Maximizing intrinsic anomalous Hall effect by controlling the Fermi level in simple Weyl semimetal films

Large intrinsic anomalous Hall effect (AHE) originating in the Berry curvature has attracted growing attention for potential applications. Recently proposed magnetic Weyl semimetal EuCd$_2$Sb$_{\mathrm{2}}$ provides an excellent platform for controlling the intrinsic AHE because it only hosts a Weyl-points related band structure near the Fermi energy. Here we report the fabrication of EuCd$_2$Sb$_{\mathrm{2}}$ single-crystalline films and control of their anomalous Hall effect by film technique. As also analyzed by first-principles calculations of energy-dependent intrinsic anomalous Hall conductivity, the obtained anomalous Hall effect shows a sharp peak as a function of carrier density, demonstrating clear energy dependence of the intrinsic AHE.

cond-mat.str-el

Quantum transport observed in films of magnetic topological semimetal EuSb$_2$

We report fabrication of EuSb$_2$ single-crystalline films and investigation of their quantum transport. First-principles calculations demonstrate that EuSb$_2$ is a magnetic topological nodal-line semimetal protected by nonsymmorphic symmetry. Observed Shubnikov-de Haas oscillations with multiple frequency components exhibit small effective masses and two-dimensional field-angle dependence even in a 250 nm thick film, further suggesting possible contributions of surface states. This finding of the high-mobility magnetic topological semimetal will trigger further investigation of exotic quantum transport phenomena by controlling magnetic order in topological semimetal films.

cond-mat.mtrl-sci

Enhancement of spin-orbit coupling in Dirac semimetal Cd$_{3}$As$_{2}$ films by Sb-doping

We present a study on magnetotransport in films of the topological Dirac semimetal Cd$_{3}$As$_{2}$ doped with Sb grown by molecular beam epitaxy. In our weak antilocalization analysis, we find a significant enhancement of the spin-orbit scattering rate, indicating that Sb doping leads to a strong increase of the pristine band-inversion energy. We discuss possible origins of this large enhancement by comparing Sb-doped Cd$_{3}$As$_{2}$ with other compound semiconductors. Sb-doped Cd$_{3}$As$_{2}$ will be a suitable system for further investigations and functionalization of topological Dirac semimetals.

cond-mat.str-el