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N. Fukuda

Publications and source records attributed to N. Fukuda.

At least 19 recordsLinked to original sources

Femtoscopy Measurement with S$\pi$RIT TPC in Radioactive BeamHeavy-ion Collisions

Femtoscopy is a powerful tool for exploring the dynamic emitting structure in heavy-ion collisions, while radioactive beam heavy-ion collisions enable the investigation of nuclear matter under extreme isospin conditions. Here, we successfully perform femtoscopy measurements using the S$\pi$RIT Time Projection Chamber (TPC). A dedicated correction scheme for track merging and splitting is proposed, which is well applicable to rectangular TPCs housed inside dipole magnets and effectively improves the reconstructed correlation functions at small relative momenta. Focusing on the proton-proton (p-p) correlation function in the 270 MeV/u $^{132}\text{Sn}+^{124}\text{Sn}$ system, we successfully apply the track merging and splitting correction; additionally, the TPC angular acceptance exhibits a negligible impact on the correlation function. A systematic uncertainty quantification framework is established. The experimental results of the p-p correlation function confirm the feasibility of the S$\pi$RIT TPC for femtoscopy measurements and provide technical support for high-precision femtoscopy studies using rectangular TPCs in radioactive beam heavy-ion collisions.

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Large amplification of the isospin-dependence of proton emitting source size in radioactive heavy-ion collisions: a signal of n-p correlation

We report proton-proton correlation function measurements in central $^{132}$Sn+$^{124}$Sn and $^{108}$Sn+$^{112}$Sn collisions at 270 MeV/nucleon. The proton emitting source sizes are extracted for the systems by using femtoscopic imaging technique. The fast dynamic core radius for the neutron-rich system is found to be $2.22 \pm 0.13\ \text{(stat.)} \pm 0.07\ \text{(syst.)}$ fm, which is approximately 24\% larger than that for the neutron-deficient system, $1.74 \pm 0.08\ \text{(stat.)} \pm 0.05\ \text{(syst.)}$ fm. This difference is an order of magnitude larger than the $\sim$3\% difference in the ground-state charge radii of the projectile nuclei. Transport model simulations based on mean-field dynamics cannot reproduce this amplification. The observation reveals a beyond-mean-field mechanism associated to short-range neutron-proton correlations, which dynamically enhance the proton emitting source in the neutron-rich environment. Our results demonstrate that heavy-ion collisions induced by radioactive beam, combined with femtoscopic precision, provide a new hadronic probe of short-range correlation, and that careful treatment of the beyond-mean-field interactions are required in modeling such processes.

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The dipole strength distribution of $^8$He and decay characteristics

The weak binding and spatially extended neutron densities characteristic of drip-line nuclei give rise to a distinctive low-energy dipole response. The drip-line nucleus $^8$He is the most neutron-rich bound nucleus with a mass-to-charge ratio of $A/Z=4$. We measure the dipole response of $^8$He, including for the first time the four-neutron decay channel. A total dipole strength of $\sum B(E1)(E^*<15$~MeV$)=0.95(16)~e^2$fm$^2$ and a dipole polarizability of $\alpha_D = 0.61(1)$~fm$^3$ are extracted from the differential Coulomb-excitation cross section and compared to state-of-the-art theoretical calculations employing coupled cluster and three-body approaches. We find that the dipole continuum is dominated, even at high excitation energies well above the $4n$ decay threshold, by two-neutron emission, pointing to a $^6$He$+2n$ structure of the excited dipole mode. No indication was found for a $4n$ final-state correlation, while pronounced $nn$ and $^6$He-$n$ final-state correlations are apparent.

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Single-particle strength toward N = 32: Spectroscopy of 51 Ca via the 50 Ca(d, p) reaction

States in the neutron-rich isotope 51 Ca were populated via the 50 Ca(d, p) transfer reaction in inverse kinematics at a beam energy of about 14 AMeV. The experiment was performed using a decelerated radioactive 50 Ca beam from the OEDO facility and the TiNA2 silicon array in combination with the SHARAQ magnetic spectrometer at RIBF/RIKEN. The energies of excited states in 51 Ca were reconstructed via missing mass spectroscopy, and angular distributions of protons were measured to extract differential cross sections. From a comparison with adiabatic distorted wave approximation (ADWA) calculations, spectroscopic factors were deduced for several states, including the ground state and excited states up to 4.2 MeV. These results are compared with shell-model calculations, as well as ab initio valence-space in-medium similarity renormalization group (VS-IMSRG) predictions. The data support the assignment of the 1/2- and 5/2- single-particle states and provide evidence for a candidate 9/2+ state with a structure consistent with neutron excitation into the 0g9/2 orbital. These findings contribute new constraints on the single-particle structure and shell evolution in neutron-rich calcium isotopes.

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Direct observation of three-neutron emission from $^7$He$^*$ and the search for the trineutron

Three-neutron emission from $^7$He has been directly measured for the first time, following neutron knockout from a $^8$He beam at 156 MeV/nucleon. A resonance-like structure at $2.08(4)$ MeV above the $^4$He+$3n$ threshold [$E_x=2.68(4)$ MeV] with a width of $3.9(2)$ MeV was observed and deduced to arise predominately from the predicted $J^{\pi}=3/2^{-}_2$ level. The three-neutron invariant-mass spectrum was reconstructed and found to peak at around 1 MeV and could, through complete simulations incorporating neutron-neutron correlations, be very well described by the sequential decay of $^7$He$^*$ via the $2_1^+$ excited state of $^6$He. No evidence was found for any significant three-neutron correlations beyond those expected from well-established two-body interactions, including a trineutron resonance.

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High-Precision Mass Measurements of Proton-Rich Rh, Pd, Cd isotopes in the vicinity of 100Sn and Impact on X-Ray Burst and Supernova Nucleosynthesis

Using the ZeroDegree multi-reflection time-of-flight mass spectrograph of the CRISMASS project at RIKEN Radioactive Isotope Beam Factory, we performed high-precision mass measurements of proton-rich nuclei near the doubly magic nucleus 100Sn, achieving uncertainties on the order of 10 keV. The masses of 91Rh, 92Pd, and 96Cd were determined for the first time with high precision, and the accuracy of several additional masses was substantially improved. Incorporating the new data into X-ray burst simulations significantly reduces the abundance uncertainties in the $A$ = 90-100 region, shifting the reaction flow toward $A$ = 90 production and suppressing the synthesis of heavier nuclei. Further investigation of the $\nu p$-process indicates that 99Rh plays a significant role in the reaction flow within the mass region studied. These high-precision mass measurements refine the mass surface near 100Sn and provide critical constraints on models of proton-rich nucleosynthesis.

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The beta decay of Tz=-2 64Se and its descendants: the T=2 isobaric multiplet

In this paper we present our results on the decay of 64Se. It is the heaviest Tz=-2 nucleus that both beta decays and has a stable mirror partner Tz=+2, thus allowing comparison with charge exchange reaction studies. The beta decays of 64Se and its descendants were studied at the RIKEN Nishina Center (Tokyo, Japan) following their production in the fragmentation of 78Kr on a beryllium target. Beta-delayed gamma-ray and particle radiation was identified for each of the nuclei in the decay chain allowing us to obtain decay schemes for 64Se, 64As, and 63Ge. Thus new excited states could be found for the descendant nuclei, including the interesting case of the N=Z nucleus 64Ge. Furthermore we observed for the first time the beta-delayed proton emission of 64Se and 64As. Based on these results we obtained proton branching ratios of 48.0(9)% in 64Se decay and 4.4(1)% in 64As decay. We obtained a half-life value of 22.5(6) ms for 64Se decay and half-lives slightly more precise than those in the literature for each nucleus involved in the decay chain. Using our results on the excited levels of 64As and the mass excess in the literature for 63Ge we obtained -39588(50) keV for the mass excess of 64As. Then based on the IMME we obtained the mass excess of -27429(88) keV for 64Se by extrapolation. The mirror process of 64Se beta decay, the charge exchange reaction 64Zn(3He,t)64Ga, has already been measured allowing us to study the mirror symmetry through the comparison of the weak force (beta decay) and strong force (charge exchange reaction). An interpretation of the decay schemes based on the idea of the Anti Analogue State is proposed.

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Decay study of the most neutron-deficient Zn isotopes with the Warsaw Optical TPC detector

Results of decay studies of nuclei in the vicinity of 54Zn, which is the most neutron-deficient isotope of zinc and undergoes ground-state two-proton radioactivity (2p), are presented. The measurements were performed with a gaseous time projection chamber with optical readout which allowed us to record tracks of protons emitted in the decays. A new method of data analysis was used to reconstruct energies and emission angles of low-energy protons that were stopped within the active volume of the chamber. Half-lives and branching ratios for \b{eta}-delayed proton emission channels were determined for 56Zn, 55Zn, and 55Cu. The \b{eta}-delayed emission of two protons for 55Zn was observed for the first time. Five events of 2p radioactivity of 54Zn were detected and reconstructed. The distribution of the opening angle between momenta of the two protons is consistent with the findings published in [Ascher et al. PRL 107, 102502 (2011)]. The combination of all results suggests a flat angular distribution, in contrast to the one measured for 45Fe.

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Modeling of Light Production in Inorganic Scintillators

In recent experiments, inorganic scintillators have been used to study the decays of exotic nuclei, providing an alternative to silicon detectors and enabling measurements that were previously impossible. However, proper use of these materials requires us to understand and quantify the scintillation process. In this work, we propose a framework based on that of Birks [Proc. Phys. Soc. A 64, 874] and Meyer and Murray [Phys. Rev. 128, 98] to model the light output of inorganic scintillators in response to beams of energetic heavy ions over a broad range of energies. Our model suggests that, for sufficiently heavy ions at high energies, the majority of the light output is associated with the creation of delta electrons, which are induced by the passage of the beam through the material. These delta electrons dramatically impact the response of detection systems when subject to ions with velocities typical of beams in modern fragmentation facilities. We test the accuracy of our model with data from Lutetium Yttrium Orthosilicate (LYSO:Ce), a common inorganic scintillator. We compare calculated light production and quenching factors with experimental data for heavy ions of varying mass and energy as well as make a quantitative estimate of the effects of delta rays on overall light output. The model presented herein will serve as a basic framework for further studies of scintillator response to heavy ions. Our results are crucial in planning future experiments where relativistic exotic nuclei are interacting with scintillator detectors.

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Precision mass measurements around ${}^{84}$Mo rule out ZrNb cycle formation in the rapid proton-capture process at type I X-ray bursts

The rapid proton-capture ($rp$-) process is one of the primary, explosive thermonuclear burning processes that drive type I X-ray bursts. A possible termination of the $rp$-process at around ${}^{84}$Mo was previously suggested by the formation of a ZrNb cycle. We report here precision mass measurements at around ${}^{84}$Mo, which have concluded the possibility of the cycle. The experiment was conducted using the multi-reflection time-of-flight spectrograph at RIKEN RI Beam Factory, and the masses of ${}^{79}$Y, ${}^{83}$Nb, ${}^{84}$Mo, ${}^{88}$Ru, and an isomer in ${}^{78}$Y were measured. For ${}^{84}$Mo, and ${}^{88}$Ru, and the isomeric state of ${}^{78}$Y, their masses are experimentally determined for the first time with uncertainties of $\delta m \approx 20~{\rm keV/c^2}$. The mass precision of ${}^{79}$Y and ${}^{83}$Nb is improved to $13~{\rm keV/c^2}$ and $9.6~{\rm keV/c^2}$, respectively. The new $\alpha$-separation energy of ${}^{84}$Mo, 1.434(83) MeV, unambiguously rules out the possibility of forming the ZrNb cycle. The X-ray burst simulation with the new masses shows that our measurements effectively remove the large final abundance uncertainties in the $A=80-90$ mass region. The new mass values improve the prediction power for the composition of the nuclear ashes in X-ray bursts.

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Impact of newly measured $\beta$\nobreakdash-delayed neutron emitters around \myisoSimp{78}{Ni} on light element nucleosynthesis in the neutrino-wind following a neutron star merger

Neutron emission probabilities and half-lives of 37 beta-delayed neutron emitters from 75Ni to 92Br were measured at the RIKEN Nishina Center in Japan, including 11 one-neutron and 13 two-neutron emission probabilities and 6 half-lives measured for the first time, which supersede theoretical estimates. These nuclei lie in the path of the weak r-process occurring in neutrino-driven winds from the accretion disk formed after the merger of two neutron stars, synthesizing elements in the A~80 abundance peak. The presence of such elements dominates the accompanying kilonova emission over the first few days and has been identified in the AT2017gfo event, associated with the gravitational wave detection GW170817. Abundance calculations based on over 17000 simulated trajectories describing the evolution of matter properties in the merger outflows show that the new data lead to an increase of 50-70 percent in the abundance of Y, Zr, Nb, and Mo. This enhancement is large compared to the scatter of relative abundances observed in old very metal-poor stars and is therefore significant in the comparison with other possible astrophysical processes contributing to light-element production. These results underline the importance of including experimental decay data for very neutron-rich beta-delayed neutron emitters into r-process models.

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Isospin breaking in the $^{71}$Kr and $^{71}$Br mirror system

Isospin symmetry is a fundamental concept in nuclear physics. Even though isospin symmetry is partially broken, it holds approximately for most nuclear systems, which makes exceptions very interesting from the nuclear structure perspective. In this framework, it is expected that the spins and parities of the ground states of mirror nuclei should be the same, in particular for the simplest systems where a proton is exchanged with a neutron or vice versa. In this work, we present evidence that this assumption is broken in the mirror pair $^{71}$Br and $^{71}$Kr system. Our conclusions are based on a high-statistics $\beta$ decay study of $^{71}$Kr and on state-of-the-art shell model calculations. In our work, we also found evidence of a new state in $^{70}$Se, populated in the $\beta$-delayed proton emission process which can be interpreted as the long sought coexisting 0$^+$ state.

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First Exploration of Monopole-Driven Shell Evolution above the N = 126 shell closure: new Millisecond Isomers in 213Tl and 215Tl

Isomer spectroscopy of heavy neutron-rich nuclei beyond the N=126 closed shell has been performed for the first time at the Radioactive Isotope Beam Factory of the RIKEN Nishina Center. New millisecond isomers have been identified at low excitation energies, 985.3(19) keV in 213Tl and 874(5) keV in 215Tl. The measured half-lives of 1.34(5) ms in 213Tl and 3.0(3) ms in 215Tl suggest spins and parities 11/2- with the single proton-hole configuration h11/2 as leading component. They are populated via E1 transitions by the decay of higher-lying isomeric states with proposed spin and parity 17/2+, interpreted as arising from a single s1/2 proton hole coupled to the 8+ seniority isomer in the (A+1)Pb cores. The lowering of the 11/2- states is ascribed to an increase of the h11/2 proton effective single-particle energy as the second g9/2 orbital is filled by neutrons, owing to a significant reduction of the proton-neutron monopole interaction between the h11/2 and g9/2 orbitals. The new ms-isomers provide the first experimental observation of shell evolution in the almost unexplored N>126 nuclear region below doubly-magic 208Pb.

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Constraining nucleon effective masses with flow and stopping observables from the S$\pi$RIT experiment

Properties of the nuclear equation of state (EoS) can be probed by measuring the dynamical properties of nucleus-nucleus collisions. In this study, we present the directed flow ($v_1$), elliptic flow ($v_2$) and stopping (VarXZ) measured in fixed target Sn + Sn collisions at 270 AMeV with the S$\pi$RIT Time Projection Chamber. We perform Bayesian analyses in which EoS parameters are varied simultaneously within the Improved Quantum Molecular Dynamics-Skyrme (ImQMD-Sky) transport code to obtain a multivariate correlated constraint. The varied parameters include symmetry energy, $S_0$, and slope of the symmetry energy, $L$, at saturation density, isoscalar effective mass, $m_{s}^*/m_{N}$, isovector effective mass, $m_{v}^{*}/m_{N}$ and the in-medium cross-section enhancement factor $\eta$. We find that the flow and VarXZ observables are sensitive to the splitting of proton and neutron effective masses and the in-medium cross-section. Comparisons of ImQMD-Sky predictions to the S$\pi$RIT data suggest a narrow range of preferred values for $m_{s}^*/m_{N}$, $m_{v}^{*}/m_{N}$ and $\eta$.

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Silicon tracker array for RIB experiments at SAMURAI

This work describes a silicon tracker system developed for experiments with proton-rich radioactive ion beams at the SAMURAI superconducting spectrometer of RIBF at RIKEN. The system is designed for accurate angular reconstruction and atomic number identification of relativistic heavy ions and protons which are simultaneously produced in reactions motivated by studies of proton capture reactions of interest for nuclear astrophysics. The technical characteristics of the tracking array are described in detail as are its performance in two pilot experiments. The physics justification for such a system is also presented.

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Decay Pattern of Pygmy States Observed in Neutron-Rich 26 Ne

Coulomb excitation of the exotic neutron-rich nucleus Ne26 on a Pb208 target was measured at 58 MeV/u in order to search for low-lying E1 strength above the neutron emission threshold. This radioactive beam experiment was carried out at the RIKEN Accelerator Research Facility. Using the invariant mass method in the Ne25+n channel, we observe a sizable amount of E1 strength between 6 and 10 MeV excitation energy. By performing a multipole decomposition of the differential cross section, a reduced dipole transition probability of B(E1)=0.49+-0.16e2fm2 is deduced, corresponding to 4.9+-1.6% of the Thomas-Reiche-Kuhn sum rule. For the first time, the decay pattern of low-lying strength in a neutron-rich nucleus is measured. The extracted decay pattern is not consistent with several mean-field theory descriptions of the pygmy states.

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Isoscaling in central Sn+Sn collisions at 270 MeV/u

Experimental information on fragment emissions is important in understanding the dynamics of nuclear collisions and in the development of transport model simulating heavy-ion collisions. The composition of complex fragments emitted in the heavy-ion collisions can be explained by statistical models, which assume that thermal equilibrium is achieved at collision energies below 100 MeV/u. Our new experimental data together with theoretical analyses for light particles from Sn+Sn collisions at 270 MeV/u, suggest that the hypothesis of thermal equilibrium breaks down for particles emitted with high transfer momentum. To inspect the system's properties in such limit, the scaling features of the yield ratios of particles from two systems, a neutron-rich system of ${}^{132}\mathrm{Sn}+{}^{124}\mathrm{Sn}$ and a nearly symmetric system of ${}^{108}\mathrm{Sn}+{}^{112}\mathrm{Sn}$, are examined in the framework of the statistical multifragmentation model and the antisymmetrized molecular dynamics model. The isoscaling from low energy particles agree with both models. However the observed breakdown of isoscaling for particles with high transverse momentum cannot be explained by the antisymmetrized molecular dynamics model.

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First application of mass measurement with the Rare-RI Ring reveals the solar r-process abundance trend at A=122 and A=123

The Rare-RI Ring (R3) is a recently commissioned cyclotron-like storage ring mass spectrometer dedicated to mass measurements of exotic nuclei far from stability at Radioactive Isotope Beam Factory (RIBF) in RIKEN. The first application of mass measurement using the R3 mass spectrometer at RIBF is reported. Rare isotopes produced at RIBF, $^{127}$Sn, $^{126}$In, $^{125}$Cd, $^{124}$Ag, $^{123}$Pd, were injected in R3. Masses of $^{126}$In, $^{125}$Cd, and $^{123}$Pd were measured whereby the mass uncertainty of $^{123}$Pd was improved. This is the first reported measurement with a new storage ring mass spectrometery technique realized at a heavy-ion cyclotron and employing individual injection of the pre-identified rare nuclei. The latter is essential for the future mass measurements of the rarest isotopes produced at RIBF. The impact of the new $^{123}$Pd result on the solar $r$-process abundances in a neutron star merger event is investigated by performing reaction network calculations of 20 trajectories with varying electron fraction $Y_e$. It is found that the neutron capture cross section on $^{123}$Pd increases by a factor of 2.2 and $β$-delayed neutron emission probability, $P_\mathrm{1n}$, of $^{123}$Rh increases by 14\%. The neutron capture cross section on $^{122}$Pd decreases by a factor of 2.6 leading to pileup of material at $A=122$, thus reproducing the trend of the solar $r$-process abundances. The trend of the two-neutron separation energies (S$_\mathrm{2n}$) was investigated for the Pd isotopic chain. The new mass measurement with improved uncertainty excludes large changes of the S$_\mathrm{2n}$ value at $N=77$. Such large increase of the S$_\mathrm{2n}$ values before $N=82$ was proposed as an alternative to the quenching of the $N=82$ shell gap to reproduce $r$-process abundances in the mass region of $A=112-124$.

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