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N. Fukuda

Publications and source records attributed to N. Fukuda.

At least 37 records · Page 2Linked to original sources

First application of mass measurement with the Rare-RI Ring reveals the solar r-process abundance trend at A=122 and A=123

The Rare-RI Ring (R3) is a recently commissioned cyclotron-like storage ring mass spectrometer dedicated to mass measurements of exotic nuclei far from stability at Radioactive Isotope Beam Factory (RIBF) in RIKEN. The first application of mass measurement using the R3 mass spectrometer at RIBF is reported. Rare isotopes produced at RIBF, $^{127}$Sn, $^{126}$In, $^{125}$Cd, $^{124}$Ag, $^{123}$Pd, were injected in R3. Masses of $^{126}$In, $^{125}$Cd, and $^{123}$Pd were measured whereby the mass uncertainty of $^{123}$Pd was improved. This is the first reported measurement with a new storage ring mass spectrometery technique realized at a heavy-ion cyclotron and employing individual injection of the pre-identified rare nuclei. The latter is essential for the future mass measurements of the rarest isotopes produced at RIBF. The impact of the new $^{123}$Pd result on the solar $r$-process abundances in a neutron star merger event is investigated by performing reaction network calculations of 20 trajectories with varying electron fraction $Y_e$. It is found that the neutron capture cross section on $^{123}$Pd increases by a factor of 2.2 and $β$-delayed neutron emission probability, $P_\mathrm{1n}$, of $^{123}$Rh increases by 14\%. The neutron capture cross section on $^{122}$Pd decreases by a factor of 2.6 leading to pileup of material at $A=122$, thus reproducing the trend of the solar $r$-process abundances. The trend of the two-neutron separation energies (S$_\mathrm{2n}$) was investigated for the Pd isotopic chain. The new mass measurement with improved uncertainty excludes large changes of the S$_\mathrm{2n}$ value at $N=77$. Such large increase of the S$_\mathrm{2n}$ values before $N=82$ was proposed as an alternative to the quenching of the $N=82$ shell gap to reproduce $r$-process abundances in the mass region of $A=112-124$.

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Beta decay of the very neutron-deficient $^{60}$Ge and $^{62}$Ge nuclei

We report here the results of a study of the $β$ decay of the proton-rich Ge isotopes, $^{60}$Ge and $^{62}$Ge, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of $^{62}$Ge (73.5(1) ms), $^{60}$Ge (25.0(3) ms) and its daughter nucleus, $^{60}$Ga (69.4(2) ms). We measured individual $β$-delayed proton and $γ$ emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total $β$-delayed proton-emission branching ratio of 67(3)% has been obtained for $^{60}$Ge. New information has been obtained on the energy levels populated in $^{60}$Ga and on the 1/2$^-$ excited state in the $βp$ daughter $^{59}$Zn. We extracted a ground state to ground state feeding of 85.3(3)% for the decay of $^{62}$Ge. Eight new $γ$ lines have been added to the de-excitation of levels populated in the $^{62}$Ga daughter.

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Charge-changing cross sections for $^{42\textrm{--}51}$Ca and effect of charged-particle evaporation induced by neutron removal reaction

Charge-changing cross sections $σ_\mathrm{CC}$ for $^{42\textrm{--}51}$Ca on a carbon target at around 280~MeV/nucleon have been measured. The measured $σ_\mathrm{CC}$ values differ significantly from the previously developed calculations based on the Glauber model. However, through introduction of the charged-particle evaporation effect induced by the neutron-removal reaction in addition to the Glauber-model calculation, experimental $σ_\mathrm{CC}$ values on $^{12}$C at around 300~MeV/nucleon for nuclides from C to Fe isotopes are all reproduced with approximately 1\% accuracy. This proposed model systematically reproduces $σ_\mathrm{CC}$ data without phenomenological corrections, and can also explain experimental $σ_\mathrm{CC}$ values obtained in other energy regions.

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Probing the Symmetry Energy with the Spectral Pion Ratio

Many neutron star (NS) properties, such as the proton fraction within a NS, reflect the symmetry energy contributions to the Equation of State that dominate when neutron and proton densities differ strongly. To constrain these contributions at supra-saturation densities, we measure the spectra of charged pions produced by colliding rare isotope tin (Sn) beams with isotopically enriched Sn targets. Using ratios of the charged pion spectra measured at high transverse momenta, we deduce the slope of the symmetry energy to be $42 < L < 117$ MeV. This value is slightly lower but consistent with the $L$ values deduced from a recent measurement of the neutron skin thickness of $^{208}$Pb.

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Symmetry energy investigation with pion production from Sn+Sn systems

In the past two decades, pions created in the high density regions of heavy ion collisions have been predicted to be sensitive at high densities to the symmetry energy term in the nuclear equation of state, a property that is key to our understanding of neutron stars. In a new experiment designed to study the symmetry energy, the multiplicities of negatively and positively charged pions have been measured with high accuracy for central $^{132}$Sn+$^{124}$Sn, $^{112}$Sn+$^{124}$Sn, and $^{108}$Sn+$^{112}$Sn collisions at $E/A=270~\mathrm{MeV}$ with the S$π$RIT Time Projection Chamber. While the uncertainties of individual pion multiplicities are measured to 4\%, those of the charged pion multiplicity ratios are measured to 2\%. We compare these data to predictions from seven major transport models. The calculations reproduce qualitatively the dependence of the multiplicities and their ratios on the total neutron to proton number in the colliding systems. However, the predictions of the transport models from different codes differ too much to allow extraction of reliable constraints on the symmetry energy from the data. This finding may explain previous contradictory conclusions on symmetry energy constraints obtained from pion data in Au+Au system. These new results call for better understanding of the differences among transport codes, and new observables that are more sensitive to the density dependence of the symmetry energy.

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A two-neutron halo is unveiled in $^{29}$F

We report the measurement of reaction cross sections ($σ_R^{\rm ex}$) of $^{27,29}$F with a carbon target at RIKEN. The unexpectedly large $σ_R^{\rm ex}$ and derived matter radius identify $^{29}$F as the heaviest two-neutron Borromean halo to date. The halo is attributed to neutrons occupying the $2p_{3/2}$ orbital, thereby vanishing the shell closure associated with the neutron number $N = 20$. The results are explained by state-of-the-art shell model calculations. Coupled-cluster computations based on effective field theories of the strong nuclear force describe the matter radius of $^{27}$F but are challenged for $^{29}$F.

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$β$-Decay Half-Lives of 55 Neutron-Rich Isotopes beyond the N=82 Shell Gap

The $β$-decay half-lives of 55 neutron-rich nuclei $^{134-139}$Sn, $^{134-142}$Sb, $^{137-144}$Te, $^{140-146}$I, $^{142-148}$Xe, $^{145-151}$Cs, $^{148-153}$Ba, $^{151-155}$La were measured at the Radioactive Isotope Beam Factory (RIBF) employing the projectile fission fragments of $^{238}$U. The nuclear level structure, which relates to deformation, has a large effect on the half-lives. The impact of newly-measured half-lives on modeling the astrophysical origin of the heavy elements is studied in the context of $r$ process nucleosynthesis. For a wide variety of astrophysical conditions, including those in which fission recycling occurs, the half-lives have an important local impact on the second ($A$ $\approx$ 130) peak.

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Swelling of doubly magic $^{48}$Ca core in Ca isotopes beyond $N=28$

Interaction cross sections for $^{42\textrm{-}51}$Ca on a carbon target at 280 MeV/nucleon have been measured for the first time. The neutron number dependence of derived root-mean-square matter radii shows a significant increase beyond the neutron magic number $N=28$. Furthermore, this enhancement of matter radii is much larger than that of the previously measured charge radii, indicating a novel growth in neutron skin thickness. A simple examination based on the Fermi-type distribution, and the Mean-Field calculations point out that this anomalous enhancement of the nuclear size beyond $N=28$ results from an enlargement of the core by a sudden increase in the surface diffuseness of the neutron density distribution, which implies the swelling of the bare $^{48}$Ca core in Ca isotopes beyond $N=28$.

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Study of multi-neutron systems with SAMURAI spectrometer

The tetraneutron has been drawing the attention of the nuclear physics community for decades, but a firm conclusion on its existence and properties is still far from being reached despite many experimental and theoretical efforts. New measurements have recently been performed at RIBF with the SAMURAI spectrometer by applying complementary reaction probes, which will help to pin down the properties of this four-neutron system.

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Interplay between nuclear shell evolution and shape deformation revealed by magnetic moment of 75Cu

Exotic nuclei are characterized by a number of neutrons (or protons) in excess relative to stable nuclei. Their shell structure, which represents single-particle motion in a nucleus, may vary due to nuclear force and excess neutrons, in a phenomenon called shell evolution. This effect could be counterbalanced by collective modes causing deformations of the nuclear surface. Here, we study the interplay between shell evolution and shape deformation by focusing on the magnetic moment of an isomeric state of the neutron-rich nucleus 75Cu. We measure the magnetic moment using highly spin-controlled rare-isotope beams and achieving large spin alignment via a two-step reaction scheme that incorporates an angular-momentum-selecting nucleon removal. By combining our experiments with numerical simulations of many-fermion correlations, we find that the low-lying states in 75Cu are, to a large extent, of single-particle nature on top of a correlated 74Ni core. We elucidate the crucial role of shell evolution even in the presence of the collective mode, and within the same framework, we consider whether and how the double magicity of the 78Ni nucleus is restored, which is also of keen interest from the perspective of nucleosynthesis in explosive stellar processes.

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First observation of 20B and 21B

The most neutron-rich boron isotopes 20B and 21B have been observed for the first time following proton removal from 22N and 22C at energies around 230 MeV/nucleon. Both nuclei were found to exist as resonances which were detected through their decay into 19B and one or two neutrons. Two-proton removal from 22N populated a prominent resonance-like structure in 20B at around 2.5 MeV above the one-neutron decay threshold, which is interpreted as arising from the closely spaced 1-,2- ground-state doublet predicted by the shell model. In the case of proton removal from 22C, the 19B plus one- and two-neutron channels were consistent with the population of a resonance in 21B 2.47+-0.19 MeV above the two-neutron decay threshold, which is found to exhibit direct two-neutron decay. The ground-state mass excesses determined for 20,21B are found to be in agreement with mass surface extrapolations derived within the latest atomic-mass evaluations.

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How different is the core of $^{25}$F from $^{24}$O$_{g.s.}$?

The neutron-shell structure of $^{25}$F was studied using quasi-free (p,2p) knockout reaction at 270A MeV in inverse kinematics. The sum of spectroscopic factors of $π$0d$_{5/2}$ orbital is found to be $1.0 \pm 0.3$. However, the spectroscopic factor for the ground-state to ground-state transition ($^{25}$F, $^{24}$O$_{g.s.}$) is only $0.36\pm 0.13$, and $^{24}$O excited states are produced from the 0d$_{5/2}$ proton knockout. The result shows that the $^{24}$O core of $^{25}$F nucleus significantly differs from a free $^{24}$O nucleus, and the core consists of 35% $^{24}$O$_{g.s}$. and 65% excited $^{24}$O.

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Commissioning of the BRIKEN detector for the measurement of very exotic beta-delayed neutron emitters

A new detection system has been installed at the RIKEN Nishina Center (Japan) to investigate decay properties of very neutron-rich nuclei. The setup consists of three main parts: a moderated neutron counter, a detection system sensitive to the implantation and decay of radioactive ions, and gamma-ray detectors. We describe here the setup, the commissioning experiment and some selected results demonstrating its performance for the measurement of half-lives and beta-delayed neutron emission probabilities. The methodology followed in the analysis of the data is described in detail. Particular emphasis is placed on the correction of the accidental neutron background.

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Spectroscopy of pionic atoms in $\mathbf{{}^{122}{\textbf Sn}({\textit d},{}^3{\textbf He})}$ reaction and angular dependence of the formation cross sections

We observed the atomic $1s$ and $2p$ states of $π^-$ bound to ${}^{121}{\rm Sn}$ nuclei as distinct peak structures in the missing mass spectra of the ${}^{122}{\rm Sn}(d,{}^3{\rm He})$ nuclear reaction. A very intense deuteron beam and a spectrometer with a large angular acceptance let us achieve potential of discovery, which includes capability of determining the angle-dependent cross sections with high statistics. The $2p$ state in a Sn nucleus was observed for the first time. The binding energies and widths of the pionic states are determined and found to be consistent with previous experimental results of other Sn isotopes. The spectrum is measured at finite reaction angles for the first time. The formation cross sections at the reaction angles between 0 and $2^\circ$ are determined. The observed reaction-angle dependence of each state is reproduced by theoretical calculations. However, the quantitative comparison with our high-precision data reveals a significant discrepancy between the measured and calculated formation cross sections of the pionic $1s$ state.

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Simultaneous investigation of the $\mathbf{T=1~ (J^π=0^+)}$ and $\mathbf{T=0 ~ (J^π=9^+)}$ $β$ decays in $^{70}$Br

The $β$ decay of the odd-odd nucleus $^{70}$Br has been investigated with the BigRIPS and EURICA setups at the Radioactive Ion Beam Factory (RIBF) of the RIKEN Nishina Center. The $T=0$ ($J^π=9^+$) and $T=1$ ($J^π=0^+$) isomers have both been produced in in-flight fragmentation of $^{78}$Kr with ratios of 41.6(8)\% and 58.4(8)\%, respectively. A half-life of $t_{1/2}=2157^{+53}_{-49}$ ms has been measured for the $J^π=9^+$ isomer from $γ$-ray time decay analysis. Based on this result, we provide a new value of the half-life for the $J^π=0^+$ ground state of $^{70}$Br, $t_{1/2}=78.42\pm0.51$ ms, which is slightly more precise, and in excellent agreement, with the best measurement reported hitherto in the literature. For this decay, we provide the first estimate of the total branching fraction decaying through the $2^+_1$ state in the daughter nucleus $^{70}$Se, $R(2^+_1)=1.3\pm1.1\%$. We also report four new low-intensity $γ$-ray transitions at 661, 1103, 1561, and 1749 keV following the $β$ decay of the $J^π=9^+$ isomer. Based on their coincidence relationships, we tentatively propose two new excited states at 3945 and 4752 keV in $^{70}$Se with most probable spins and parities of $J^π=(6^+)$ and $(8^+)$, respectively. The observed structure is interpreted with the help of shell-model calculations, which predict a complex interplay between oblate and prolate configurations at low excitation energies.

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Single-neutron knockout from $^{20}\textrm{C}$ and the structure of $^{19}\textrm{C}$

The low-lying unbound level structure of the halo nucleus $^{19}\textrm{C}$ has been investigated using single-neutron knockout from $^{20}\textrm{C}$ on a carbon target at 280 MeV/nucleon. The invariant mass spectrum, derived from the momenta of the forward going beam velocity $^{18}\textrm{C}$ fragment and neutrons, was found to be dominated by a very narrow near threshold ($E_\textrm{rel}$ = 0.036(1) MeV) peak. Two less strongly populated resonance-like features were also observed at $E_\textrm{rel}$ = 0.84(4) and 2.31(3) MeV, both of which exhibit characteristics consistent with neutron $p$-shell hole states. Comparisons of the energies, measured cross sections and parallel momentum distributions to the results of shell-model and eikonal reaction calculations lead to spin-parity assignments of $5/2^+_1$ and $1/2^-_1$ for the levels at $E_x$ = 0.62(9) and 2.89(10) MeV with $S_n$ = 0.58(9) MeV. Spectroscopic factors were also deduced and found to be in reasonable accord with shell-model calculations. The valence neutron configuration of the $^{20}\textrm{C}$ ground state is thus seen to include, in addition to the known $1s^2_{1/2}$ component, a significant $0d^2_{5/2}$ contribution. The level scheme of $^{19}\textrm{C}$, including significantly the $1/2^-_1$ cross-shell state, is well accounted for by the YSOX shell-model interaction developed from the monopole-based universal interaction.

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New neutron-deficient isotopes from $^{78}$Kr fragmentation

In an experiment with the BigRIPS separator at the RIKEN Nishina Center, the fragmentation of a $^{78}$Kr beam allowed the observation of new neutron-deficient isotopes at the proton drip-line. Clean identification spectra could be produced and $^{63}$Se, $^{67}$Kr, and $^{68}$Kr were identified for the first time. In addition, $^{59}$Ge was also observed. Three of these isotopes, $^{59}$Ge, $^{63}$Se, and $^{67}$Kr, are potential candidates for ground-state two-proton radioactivity. In addition, the isotopes $^{58}$Ge, $^{62}$Se, and $^{66}$Kr were also sought but without success. The present experiment also allowed the determination of production cross sections for some of the most exotic isotopes. These measurements confirm the trend already observed that the empirical parameterization of fragmentation cross sections, EPAX, significantly overestimates experimental cross sections in this mass region.

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Nuclear structure of 140Te with N = 88: Structural symmetry and asymmetry in Te isotopes with respect to the double-shell closure Z = 50 and N = 82

We study for the first time the internal structure of 140Te through the beta-delayed gamma-ray spectroscopy of 140Sb. The very neutron-rich 140Sb, Z = 51 and N = 89, ions were produced by the in-flight fission of 238U beam on a 9Be target at 345 MeV per nucleon at the Radioactive Ion Beam Factory, RIKEN. The half-life and spin-parity of 140Sb are reported as 124(30) ms and (4-), respectively. In addition to the excited states of 140Te produced by the beta-decay branch, the beta-delayed one-neutron and two-neutron emission branches were also established. By identifying the first 2+ and 4+ excited states of 140Te, we found that Te isotopes persist their vibrator character with E(4+)/E(2+) = 2. We discuss the distinctive features manifest in this region, such as valence neutron symmetry and asymmetry, revealed in pairs of isotopes with the same neutron holes and particles with respect to N = 82.

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