arXiv subjects

N. Millard-Pinard

Publications and source records attributed to N. Millard-Pinard.

5 recordsLinked to original sources

arXiv2026

Studies of $\rm ^{144,148}Sm+\alpha$ potential for the $p$-process nucleosynthesis

Nucleosynthesis reaction networks leading to $p$-nuclei involve a combination of different types of photodisintegration and capture reactions, as well as $\beta^+$ decays or electron captures. Photodisintegration reactions involving $\alpha$ particles present a particular interest as they serve as branching points of the reaction networks. The cross sections of these reactions depend crucially on the $\alpha$-nucleus interaction. The $\alpha$ optical model potential (AOMP) is determined mostly by means of experimental differential elastic scattering distributions. Several previous studies have focused on the case of $\rm ^{144}Sm$, an intriguing $p$-nucleus that is semi-magic with 82 neutrons. This work presents new experimental data on $\alpha$ elastic and inelastic scattering on $\rm ^{148}Sm$, its closest stable isotope. Isotopic effects on the description of the AOMP are studied, as well as their consequences on the prediction of $\alpha$-induced reaction cross sections at astrophysical energies. It is shown that the isotopic ratio for $(\alpha,\gamma)$ cross sections can be multiplied up to a factor of two when these effects are included.

nucl-ex↗

arXiv2024

Bayesian uncertainty quantification on nuclear level density data and their impact on $(p,γ)$ reactions of astrophysical interest

The $p$ process nucleosynthesis is responsible for the synthesis of 35 neutron-deficient nuclei from $^{35}$Se to $^{196}$Hg. An important input that can affect the modeling of this process is the nuclear level density at the relevant excitation energies of the nuclei involved in the reaction network. The OSLO method has been extensively used for the measurement of level densities in excitation energies of several MeV. In this work, Bayesian optimization has been used in order to estimate the 95% high density intervals for the parameters of two level density models optimized on the OSLO data. These uncertainties are then propagated on the cross sections of $(p,γ)$ reactions leading to the compound nuclei $^{105,106}$Pd and $^{105,106}$Cd inside the astrophysically relevant energy range. Imposing constraints in this region of the isotopic chart is important for network calculations involving the nearby $p$ nuclei $^{102}$Pd and $^{106}$Cd. We discuss the reduction of the range of cross sections due to the uncertainties arising from the level density data compared to the range of the six default level density models available in TALYS and we highlight the need for level density data inside the astrophysically relevant energy ranges.

nucl-th↗

arXiv2005

Role of proton irradiation and relative air humidity on iron corrosion

This paper presents a study of the effects of proton irradiation on iron corrosion. Since it is known that in humid atmospheres, iron corrosion is enhanced by the double influence of air and humidity, we studied the iron corrosion under irradiation with a 45% relative humidity. Three proton beam intensities (5, 10 and 20 nA) were used. To characterise the corrosion layer, we used ion beam methods (Rutherford Backscattering Spectrometry (RBS), Elastic Recoil Detection Analysis (ERDA)) and X-ray Diffraction (XRD) analysis. The corrosion kinetics are plotted for each proton flux. A diffusion model of the oxidant species is proposed, taking into account the fact that the flux through the surface is dependent on the kinetic factor K. This model provides evidence for the dependence of the diffusion coefficient, D, and the kinetic factor, K, on the proton beam intensity. Comparison of the values for D with the diffusion coefficients for thermal oxygen diffusion in iron at 300 K suggests an enhancement due to irradiation of 6 orders of magnitude.

physics.chem-ph↗

arXiv2005

Use ion beam techniques to study the coupling between air and its relative humidity on iron corrosion under irradiation

In this paper, the role of air humidity on the iron corrosion under irradiation is studied in the context of geological disposal of nuclear wastes. The irradiation experiments are performed at room temperature using a 3 MeV extracted proton beam with a 10 nA intensity. Different atmospheres are studied: Humid air with a relative humidity (RH) fixed at 45 %, dry air and a $^{15}N\_2$ atmosphere (45% RH). The hydrogen and oxygen distribution profiles at the iron surface in contact with atmosphere are measured by using respectively ERDA (Elastic Recoil Detection Analysis) and RBS (Rutherford Backscattering Spectrometry) analysis. From these experiments it is clearly demonstrated that the coupling of O$\_2$+H$\_2$O enhances iron oxidation whereas for iron hydrogenation, humidity is sufficient whatever the atmosphere. An interpretation is given, which is based on the reaction mechanisms and the species formed by air ionisation.

physics.chem-ph↗

arXiv2005

Origin of the hydrogen involved in iron corrosion under irradiation

In the perspective of long term geological storage, high level nuclear wastes will be overpacked in low carbon steel containers. In that context, we have studied the influence of oxygen dissolved in water on iron corrosion. Therefore, leaching experiments were performed in desaerated D$\_2$O and in aerated H$\_2$O and a kinetic study of iron corrosion under proton irradiation was lead in aqueous media with two different dissolved oxygen concentrations. The leaching experiments underline the major role of dissolved oxygen in oxydoreduction reactions which take place as far as iron is in contact with water. But the kinetic study of iron corrosion under irradiation put in evidence the balance between the oxydoreduction reactions and the corrosion rate induced by radicals species generated by water radiolysis. In addition, to check if, in the atomic % concentration range, hydrogen diffuse from the air/Fe interface through the foil an irradiation experiment was performed in argon. It proved that no hydrogen permeation occurs at a concentration level of the atomic percent.

physics.chem-ph↗