arXiv subjects

Nelson Darkwah Oppong

Publications and source records attributed to Nelson Darkwah Oppong.

15 recordsLinked to original sources

arXiv2026

Local polarization control of optical tweezer arrays

Optical tweezer arrays trapping ultracold atoms and molecules are a versatile quantum science platform with broad impact in quantum simulation, quantum computation, and quantum metrology. The polarization dependence of anisotropic vector and tensor light shifts offers a degree of freedom for precise quantum state engineering of trapped particles. Similarly, state-selective operations depend on the polarization of the addressing light through the atom--light coupling strength. Yet, methods for controlling the polarization of individual tweezers or local addressing beams remain an experimental challenge. Here, we demonstrate independent, site-resolved linear polarization rotation across an optical tweezer array by exploiting the local birefringence tunability of a spatial light modulator. Applying this capability to an array of $^{88}\rm{Sr}$ atoms, we homogenize differential light shifts imparted by the 813-nm tweezers to the narrow ${^1{\rm S}_0}\leftrightarrow{^3{\rm P}_1}$ transition, enabling sideband cooling under a magic-angle condition. Furthermore, we show dynamic transport of trapped atoms across distinct polarization zones with high survival and preserved coherence. Finally, we characterize tweezer polarization noise and demonstrate closed-loop stabilization referenced to the atomic transition frequency, reaching mrad-level stability. Our work establishes a technique for manipulating polarization-sensitive atomic and molecular transitions in tweezer architectures, with immediate applications to optical tweezer clocks and multi-zone quantum processors.

physics.atom-ph↗

arXiv2025

Assembling a Bose-Hubbard superfluid from tweezer-controlled single atoms

Quantum simulation relies on the preparation and control of low-entropy many-body systems to reveal the behavior of classically intractable models. The development of new approaches for realizing such systems therefore represents a frontier in quantum science. Here we experimentally demonstrate a new protocol for generating ultracold, itinerant many-body states in a tunnel-coupled two-dimensional optical lattice. We do this by adiabatically connecting a near-ground-state-cooled array of up to 50 single strontium-86 atoms with a Bose-Hubbard superfluid. Through comparison with finite-temperature quantum-Monte-Carlo calculations, we estimate that the entropy per particle of the prepared many-body states is approximately $2 k_B$, and that the achieved temperatures are consistent with a significant superfluid fraction. This represents the first time that itinerant many-body systems have been prepared from rearranged atoms, opening the door to bottom-up assembly of a wide range of neutral-atom and molecular systems.

cond-mat.quant-gas↗

arXiv2025

Engineering the Kondo impurity problem with alkaline-earth atom arrays

We propose quantum simulation experiments of the Kondo impurity problem using cold alkaline-earth(-like) atoms (AEAs) in a combination of optical lattice and optical tweezer potentials. Within an ab initio model for atomic interactions in the optical potentials, we analyze hallmark signatures of the Kondo effect in a variety of observables accessible in cold-atom quantum simulators. We identify additional terms not part of the textbook Kondo problem, mostly ignored in previous works and giving rise to a direct competition between spin and charge correlations - strongly suppressing Kondo physics. We show that the Kondo effect can be restored by locally adjusting the chemical potential on the impurity site, and we identify realistic parameter regimes and preparation protocols suited to current experiments with AEA arrays. Our work paves the way for novel quantum simulations of the Kondo problem and offers new insights into Kondo physics in unconventional regimes.

cond-mat.quant-gas↗

arXiv2025

Autoionization-enhanced Rydberg dressing by fast contaminant removal

Rydberg dressing is a powerful tool for entanglement generation in long-lived atomic states. While already employed effectively in several demonstrations, a key challenge for this technique is the collective loss triggered by blackbody-radiation-driven transitions to contaminant Rydberg states of opposite parity. We demonstrate the rapid removal of such contaminants using autoionization (AI) transitions found in alkaline-earth-like atoms. The AI is shown to be compatible with coherent operation of an array of optical clock qubits. By incorporating AI pulses into a stroboscopic Rydberg dressing (SRD) sequence, we enhance lifetimes by an order of magnitude for system sizes of up to 144 atoms, while maintaining an order of magnitude larger duty cycle than previously achieved. To highlight the utility of our approach, we use the AI-enhanced SRD protocol to improve the degree of spin-squeezing achieved during early-time dressing dynamics. These results bring Rydberg dressing lifetimes closer to fundamental limits, opening the door to previously infeasible dressing proposals.

cond-mat.quant-gas↗

arXiv2024

Multi-qubit gates and Schrödinger cat states in an optical clock

Many-particle entanglement is a key resource for achieving the fundamental precision limits of a quantum sensor. Optical atomic clocks, the current state-of-the-art in frequency precision, are a rapidly emerging area of focus for entanglement-enhanced metrology. Augmenting tweezer-based clocks featuring microscopic control and detection with the high-fidelity entangling gates developed for atom-array information processing offers a promising route towards leveraging highly entangled quantum states for improved optical clocks. Here we develop and employ a family of multi-qubit Rydberg gates to generate Schrödinger cat states of the Greenberger-Horne-Zeilinger (GHZ) type with up to 9 optical clock qubits in a programmable atom array. In an atom-laser comparison at sufficiently short dark times, we demonstrate a fractional frequency instability below the standard quantum limit using GHZ states of up to 4 qubits. However, due to their reduced dynamic range, GHZ states of a single size fail to improve the achievable clock precision at the optimal dark time compared to unentangled atoms. Towards overcoming this hurdle, we simultaneously prepare a cascade of varying-size GHZ states to perform unambiguous phase estimation over an extended interval. These results demonstrate key building blocks for approaching Heisenberg-limited scaling of optical atomic clock precision.

quant-ph↗

arXiv2023

State-dependent potentials for the $^1\text{S}_{0}$ and $^3\text{P}_{0}$ clock states of neutral ytterbium atoms

We present measurements of three distinctive state-(in)dependent wavelengths for the $^1\text{S}_{0}-^3\text{P}_{0}$ clock transition in $^{174}\text{Yb}$ atoms. Specifically, we determine two magic wavelengths at $652.281(21)\,$THz and $542.50205(19)\,$THz, where the differential light shift on the $^1\text{S}_{0}-^3\text{P}_{0}$ clock transition vanishes, and one tune-out wavelength at $541.8325(5)\,$THz, where the polarizability of the $^1\text{S}_{0}$ ground state exhibits a zero crossing. The two new magic wavelengths are identified by spectroscopically interrogating cold $^{174}\text{Yb}$ atoms on the clock transition in a one-dimensional optical lattice. The ground-state tune-out wavelength is determined via a parametric heating scheme. With a simple empirical model, we then extrapolate the ground and excited state polarizability over a broad range of wavelengths in the visible spectrum.

physics.atom-ph↗

arXiv2023

Realizing spin squeezing with Rydberg interactions in a programmable optical clock

Neutral-atom arrays trapped in optical potentials are a powerful platform for studying quantum physics, combining precise single-particle control and detection with a range of tunable entangling interactions. For example, these capabilities have been leveraged for state-of-the-art frequency metrology as well as microscopic studies of entangled many-particle states. In this work, we combine these applications to realize spin squeezing - a widely studied operation for producing metrologically useful entanglement - in an optical atomic clock based on a programmable array of interacting optical qubits. In this first demonstration of Rydberg-mediated squeezing with a neutral-atom optical clock, we generate states that have almost 4 dB of metrological gain. Additionally, we perform a synchronous frequency comparison between independent squeezed states and observe a fractional frequency stability of $1.087(1)\times 10^{-15}$ at one-second averaging time, which is 1.94(1) dB below the standard quantum limit, and reaches a fractional precision at the $10^{-17}$ level during a half-hour measurement. We further leverage the programmable control afforded by optical tweezer arrays to apply local phase shifts in order to explore spin squeezing in measurements that operate beyond the relative coherence time with the optical local oscillator. The realization of this spin-squeezing protocol in a programmable atom-array clock opens the door to a wide range of quantum-information inspired techniques for optimal phase estimation and Heisenberg-limited optical atomic clocks.

quant-ph↗

arXiv2023

Equation of State and Thermometry of the 2D SU($N$) Fermi-Hubbard Model

We characterize the equation of state (EoS) of the SU($N>2$) Fermi-Hubbard Model (FHM) in a two-dimensional single-layer square optical lattice. We probe the density and the site occupation probabilities as functions of interaction strength and temperature for $N = 3, 4$ and 6. Our measurements are used as a benchmark for state-of-the-art numerical methods including determinantal quantum Monte Carlo (DQMC) and numerical linked cluster expansion (NLCE). By probing the density fluctuations, we compare temperatures determined in a model-independent way by fitting measurements to numerically calculated EoS results, making this a particularly interesting new step in the exploration and characterization of the SU($N$) FHM.

cond-mat.quant-gas↗

arXiv2023

$Ab\,initio$ derivation of lattice gauge theory dynamics for cold gases in optical lattices

We introduce a method for quantum simulation of U$(1)$ lattice gauge theories coupled to matter, utilizing alkaline-earth(-like) atoms in state-dependent optical lattices. The proposal enables the study of both gauge and fermionic-matter fields without integrating out one of them in one and two dimensions. We focus on a realistic and robust implementation that utilizes the long-lived metastable clock state available in alkaline-earth(-like) atomic species. Starting from an $ab\,initio$ modelling of the experimental setting, we systematically carry out a derivation of the target U$(1)$ gauge theory. This approach allows us to identify and address conceptual and practical challenges for the implementation of lattice gauge theories that - while pivotal for a successful implementation - have never been rigorously addressed in the literature: those include the specific engineering of lattice potentials to achieve the desired structure of Wannier functions, and the subtleties involved in realizing the proper separation of energy scales to enable gauge-invariant dynamics. We discuss realistic experiments that can be carried out within such a platform using the fermionic isotope $^{173}$Yb, addressing via simulations all key sources of imperfections, and provide concrete parameter estimates for relevant energy scales in both one- and two-dimensional settings.

cond-mat.quant-gas↗

arXiv2022

Probing transport and slow relaxation in the mass-imbalanced Fermi-Hubbard model

Constraints in the dynamics of quantum many-body systems can dramatically alter transport properties and relaxation timescales even in the absence of static disorder. Here, we report on the observation of such constrained dynamics arising from the distinct mobility of two species in the one-dimensional mass-imbalanced Fermi-Hubbard model, realized with ultracold ytterbium atoms in a state-dependent optical lattice. By displacing the trap potential and monitoring the subsequent dynamical response of the system, we identify suppressed transport and slow relaxation with a strong dependence on the mass imbalance and interspecies interaction strength, consistent with eventual thermalization for long times. Our observations demonstrate the potential for quantum simulators to provide insights into unconventional relaxation dynamics arising from constraints.

cond-mat.quant-gas↗

arXiv2021

Quasiparticle lifetime of the repulsive Fermi polaron

We investigate the metastable repulsive branch of a mobile impurity coupled to a degenerate Fermi gas via short-range interactions. We show that the quasiparticle lifetime of this repulsive Fermi polaron can be experimentally probed by driving Rabi oscillations between weakly and strongly interacting impurity states. Using a time-dependent variational approach, we find that we can accurately model the impurity Rabi oscillations that were recently measured for repulsive Fermi polarons in both two and three dimensions. Crucially, our theoretical description does not include relaxation processes to the lower-lying attractive branch. Thus, the theory-experiment agreement demonstrates that the quasiparticle lifetime is determined by many-body dephasing within the upper repulsive branch rather than by the metastability of the upper branch itself. Our findings shed light on recent experimental observations of persistent repulsive correlations, and have important consequences for the nature and stability of the strongly repulsive Fermi gas.

cond-mat.quant-gas↗

arXiv2020

Orbital ordering of ultracold alkaline-earth atoms in optical lattices

We report on a dynamical mean-field theoretical analysis of emerging low-temperature phases in multicomponent gases of fermionic alkaline-earth(-like) atoms in state-dependent optical lattices. Using the example of $^{173}$Yb atoms, we show that a two-orbital mixture with two nuclear spin components is a promising candidate for studies of not only magnetic but also staggered orbital ordering peculiar to certain solid-state materials. We calculate and study the phase diagram of the full Hamiltonian with parameters similar to existing experiments and reveal an antiferroorbital phase. This long-range-ordered phase is inherently stable, and we analyze the change of local and global observables across the corresponding transition lines, paving the way for experimental observations. Furthermore, we suggest a realistic extension of the system to include and probe a Jahn-Teller source field playing one of the key roles in real crystals.

cond-mat.quant-gas↗

arXiv2020

Clock-line photoassociation of strongly bound dimers in a magic-wavelength lattice

We report on the direct optical production and spectroscopy of $^1\mathrm{S}_0\mbox{-}^3\mathrm{P}_0$ molecules with large binding energy using the clock transition of $^{171}\mathrm{Yb}$, and on the observation of the associated orbital Feshbach resonance near $1300\,\mathrm{G}$. We measure the magnetic field dependence of the closed-channel dimer and of the open-channel pair state energy via clock-line spectroscopy in a deep optical lattice. In addition, we show that the free-to-bound transition into the dimer can be made first-order insensitive to the trap depth by choice of the lattice wavelength. Finally, we determine the fundamental intra- and interorbital scattering lengths and probe the stability of the corresponding pair states, finding long lifetimes in both interorbital interaction channels. These results are promising both for molecular clocks and for the preparation of strongly-interacting multiorbital Fermi gases.

cond-mat.quant-gas↗

arXiv2019

Observation of coherent multiorbital polarons in a two-dimensional Fermi gas

We report on the experimental observation of multiorbital polarons in a two-dimensional Fermi gas of $^{173}\mathrm{Yb}$ atoms formed by mobile impurities in the metastable $^3\mathrm{P}_0$ orbital and a Fermi sea in the ground-state $^1\mathrm{S}_0$ orbital. We spectroscopically probe the energies of attractive and repulsive polarons close to an orbital Feshbach resonance and characterize their coherence by measuring the quasiparticle residue. For all probed interaction parameters, the repulsive polaron is a long-lived quasiparticle with a decay rate more than 2 orders of magnitude below its energy. We formulate a many-body theory, which accurately treats the interorbital interactions in two dimensions and agrees well with the experimental results. Our work paves the way for the investigation of many-body physics in multiorbital ultracold Fermi gases.

cond-mat.quant-gas↗

arXiv2018

Localized magnetic moments with tunable spin exchange in a gas of ultracold fermions

We report on the experimental realization of a state-dependent lattice for a two-orbital fermionic quantum gas with strong interorbital spin exchange. In our state-dependent lattice, the ground and metastable excited electronic states of $^{173}$Yb take the roles of itinerant and localized magnetic moments, respectively. Repulsive on-site interactions in conjunction with the tunnel mobility lead to spin exchange between mobile and localized particles, modeling the coupling term in the well-known Kondo Hamiltonian. In addition, we find that this exchange process can be tuned resonantly by varying the on-site confinement. We attribute this to a resonant coupling to center-of-mass excited bound states of one interorbital scattering channel.

cond-mat.quant-gas↗