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Nishchhal Verma

Publications and source records attributed to Nishchhal Verma.

At least 19 recordsLinked to original sources

Cell Natural Orbitals in Interacting Topological Bands

Topological bands exhibit obstruction to exponentially localized and symmetric Wannier functions, challenging the standard paradigm of representing projected interactions in terms of local orbitals with finite range. To faithfully capture the form factors and quantum geometry of topological bands we introduce a singular-value decomposition of the band-projected density form factors, enabling a geometry-based truncation scheme of the Hilbert space, exposing an intrinsic hierarchy on band-projected interactions that is determined by the underlying wavefunctions. This decomposition is most naturally described in terms of Cell Natural Orbitals (CNOs), as the eigenstates of the unit-cell reduced one-particle density matrix, whose occupation provide a measure of the minimal orbital complexity required to faithfully represent the band wavefunctions overlaps. The CNO decomposition identifies systematically the minimal number of local orbitals needed to reproduce short-ranged interactions while resolving the hierarchy of interaction strengths across CNO channels. Applied to magic-angle twisted bilayer graphene in the chiral limit, we find that the dominant CNO is centered at the AA site, resembling the $f$-fermion of the heavy-fermion model. The subdominant CNO channels carry progressively weaker interaction matrix elements, allowing them to be treated at the static mean-field level, while the dominant channel requires a dynamical self-energy. The formalism illustrates how variations of charge density within the unit cell generate momentum dependence in the CNO envelope function and, consequently, dispersion in the single-particle spectral function. More broadly, our results establish CNOs as a geometry-informed bridge between band topology and real-space correlations, providing a systematic framework for analyzing interactions and emergent phases in quantum materials.

cond-mat.str-el

Cell Natural Orbitals in Quantum Materials

Understanding correlated quantum matter starts with an accurate model of the single-particle states that interact at low energies: their dispersion, band geometry, orbital content and charge density. In many cases, notably the topological bands of moire materials, it is not straightforward to find a real-space description with a few local orbitals that accomplishes this task. Here we provide a systematic way to identify the local degrees of freedom that best capture the band geometry and charge density of any chosen set of bands. We use the unit-cell one-particle reduced density matrix (UC-1pRDM), obtained by restricting the projector onto the target bands to a single unit cell. Its eigenstates, which we call cell natural orbitals (CNOs), form a local, symmetric basis uniquely determined by the Bloch wavefunctions and the choice of real-space partition. Their eigenvalues measure the occupation of each CNO in the target bands, quantifying entanglement across unit-cell boundaries and the importance of multi-orbital character. A set of CNOs that maximizes total spectral weight and reproduces the target band symmetries provides optimal trial states for Wannierization. We exemplify this by constructing a lattice model for twisted bilayer WSe$_2$ that tracks the orbital content across twist angles.

cond-mat.mtrl-sci

Long and short time linear response of metals: a geometric approach

The time-dependent quantum geometric tensor, which captures dipole fluctuations of bound electrons, is essential for understanding the electronic properties of insulators, superconductors, and flat bands. It is often considered subleading for low-energy descriptions of metals that are dominated by intra-band processes. Here, we revisit this perspective and highlight scenarios where the quantum geometry of the wavefunctions close to the Fermi surface plays a significant role. We compute the time-dependent quantum geometric tensor for metals, explain its divergence, and contrast it against singular geometric tensors of Dirac and Weyl semi-metals. We identify the ratio of Drude to total spectral weight, $D/\mathcal{S}_1$, as a lattice-scale probe of bound versus itinerant charge, and quantify it in the kagome metal, where the two van Hove fillings respond differently despite identical Fermi surfaces.

cond-mat.str-el

Plasmon dynamics in graphene

Plasmon are collective oscillations of mobile electrons with dynamics controlled by their charge stiffness("Drude weight"). Using terahertz spacetime metrology, we probe Plasmon dynamics of mono- and bi-layer graphene. In both systems, the experimentally measured Drude weight systematically exceeds the prediction based on non-interacting electronic system. The relative enhancement increases as the carrier density decreases. We attribute the observed deviation to the interplay of interactions and wave function structure of the Dirac fermions in multi-layer graphene. Our results establish that pseudospin structure of the single-particle electronic wave function can directly influence collective excitations, with implications that extend beyond graphene to a broad class of quantum materials.

cond-mat.mes-hall

Observing unconventional superconductivity via kinetic inductance in Weyl semimetal MoTe$_2$

Identifying the pairing symmetry of unconventional superconductors plays an essential role in the ongoing quest to understand correlated electronic matter. A long-standing approach is to study the temperature dependence of the London penetration depth $\lambda$ for evidence of nodal points where the superconducting gap vanishes. However, experimental reports can be ambiguous due to the requisite low-temperature resolution, and the similarity in signatures of nodal quasiparticles and impurity states. Here we study the pairing symmetry of Weyl semimetal $T_d$-MoTe$_2$, where previous measurements of $\lambda$ have yielded conflicting results. We utilize a novel technique based on a microwave resontor to measure the kinetic inductance of MoTe$_2$, which is directly related to $\lambda$. The high precision of this technique allows us to observe power-law temperature dependence of $\lambda$, and to measure the anomalous nonlinear Meissner effect -- the current dependence of $\lambda$ arising from nodal quasiparticles. Together, these measurements provide smoking gun signatures of nodal superconductivity.

cond-mat.supr-con

Cyclic structure of Landau levels in transition metal dichalcogenide semiconductors

Transition metal dichalcogenides (TMDs) exhibit unconventional Landau level (LL) spectra that cannot be fully captured by an effective mass approximation or a minimal two-band Dirac model. Namely, TMDs show an anomalous, upward-sloping zeroth LL in the valence band and an asymmetric orbital magnetization between electron and hole bands. In this paper, we employ a continuum three-band model to derive analytic constraints on the LL spectrum of the $K$ and $K'$ valleys at weak magnetic fields. This model highlights the cyclic structure of the LL spectrum inherited from $C_3$ symmetry, providing both analytical tractability and an accurate description of the band geometry in the low energy approximation of the valleys. We compare our results against numerical calculations using the three-band tight-binding model of Ref.[1] and a distorted kagome lattice model. We find that the Landau levels of the $K$ and $K'$ valleys show a cyclic structure which explains their anomalous slope and magnetization asymmetry. This asymmetry can be traced to the topological obstruction of TMD semiconductors. We further analyze the impact of disorder, finding that the zeroth LL exhibits partial robustness against certain off-diagonal perturbations, in contrast to the exact index-theorem protection of massive Dirac particles. Our results establish a direct link between orbital structure, band topology, and magnetic response in TMDs.

cond-mat.mtrl-sci

Mapping the moir\'e potential in multi-layer rhombohedral graphene

Rhombohedral graphene (rG) aligned with hexagonal boron nitride (hBN) has been shown to host flat bands that stabilize various strongly correlated quantum phases, including Mott insulators, integer, and fractional quantum anomalous Hall phases. In this work, we use scanning tunneling microscopy/spectroscopy (STM/STS) to visualize the dispersion of flat bands with doping and applied displacement fields in a hBN-aligned rhombohedral trilayer graphene (rtG)/hBN moir\'e superlattice. In addition to the intrinsic flat bands of rtG induced by the displacement field, we observe low-energy features originating from moir\'e potential-induced band folding. Real-space variations of the spectroscopic features allow us to quantify the spatial structure of the moir\'e potential at the rtG/hBN interface. Importantly, we find that accurately capturing the moir\'e site-dependent spectra requires incorporating a moir\'e potential acting on the top graphene layer with a sign opposite to that of the bottom layer into the continuum model. Our results thus provide key experimental and theoretical insights into understanding the role of the moire superlattice in rG/hBN heterostructures.

cond-mat.mes-hall

Quantum Geometry and the Hidden Scales in Materials

Electronic properties of quantum materials solids are often well understood via the low energy dispersion of Bloch bands, motivating single band approximations in many metals and semiconductors. However, a closer look reveals length and time scales introduced by quantum dipole fluctuations due to interband mixing, which are reflected in the momentum space textures of the electronic wavefunctions. This structure is usually referred to as quantum geometry. These new scales not only qualitatively modify the linear and nonlinear responses of a material but can also have a vital role in determining the many-body ground state at low temperatures. In this Perspective, we explore how quantum geometry impacts properties of materials and outline recent experimental advances that have begun to explore quantum geometric effects in various condensed matter platforms. We discuss the separation of scales that can allow us to estimate the significance of quantum geometry in various response functions.

cond-mat.mtrl-sci

Local basis for interacting topological bands

The discovery of correlated states in moire materials has challenged the established methods of projecting interactions into a local Wannier basis due to topological obstructions that manifest in extended interactions. This difficulty can sometimes be evaded by decomposing the band into a basis of extended itinerant states and a lattice of local states, using the heavy fermion prescription. We revisit this framework by systematically identifying the dominant interaction channels guided by the eigenvalues of the projected density operator. This approach can be applied both to tight-binding and continuum models, allowing us to identify a hierarchy in interaction scales that can be universally used to reduce the Hilbert space dimension and determine an appropriate local basis for modeling electronic correlations in interacting topological materials.

cond-mat.str-el

Obstructed Cooper pairs in flat band systems -- weakly-coherent superfluids and exact spin liquids

Superconductivity in a partially filled flat band presents a vexing conceptual hurdle because the absence of a Fermi surface precludes a weak-coupling regime where one can extend insights from the Bardeen-Cooper-Schrieffer picture of a Fermi surface instability. We approach the strongly correlated problem of flat band superconductivity from the strong coupling limit of local attractive interactions on line-graph lattices, whose non-interacting bandstructures host exactly flat bands due to frustrated hopping. In this limit, the pair kinetic energy which sets the superfluid stiffness is expected to scale inversely with the pair binding interaction. Here we demonstrate a striking counterexample. We show that when doped charges propagate on the line-graph of a lattice with strong pairing interaction and broken time-reversal symmetry, they bind into obstructed Cooper pairs whose motion is frustrated by destructive interference. As a result, the leading-order pair kinetic energy vanishes identically in the strong-coupling expansion, producing a flat bosonic band of compact localised pair states, zero superfluid stiffness at leading order, and an extensively degenerate many-body ground state manifold. At quarter filling, the frustrated pair dynamics maps onto a quantum dimer model which has a $d$-wave resonating-valence-bond ground state when time-reversal is broken. The pairing Hamiltonian in this limit thus has a topologically ordered spin liquid ground state which becomes exact at the analytically solvable Rokhsar-Kivelson point with long-range entanglement and deconfined holon excitations. Interestingly, we find exact compact localised eigenstates and extensive degeneracies in the many-body eigenstates of this emergent dimer model. Our results establish a disorder-free mechanism for interaction-driven localisation, in which strong pairing collapses the kinetic energy of Cooper pairs.

cond-mat.supr-con

Measuring kinetic inductance and superfluid stiffness of two-dimensional superconductors using high-quality transmission-line resonators

The discovery of van der Waals superconductors in recent years has generated a lot of excitement for their potentially novel pairing mechanisms. However, their typical atomic-scale thickness and micrometer-scale lateral dimensions impose severe challenges to investigations of pairing symmetry by conventional methods. In this report we demonstrate a new technique that employs high-quality-factor superconducting resonators to measure the kinetic inductance -- up to a part per million -- and loss of a van der Waals superconductor. We analyze the equivalent circuit model to extract the kinetic inductance, superfluid stiffness, penetration depth, and ratio of imaginary and real parts of the complex conductivity. We validate the technique by measuring aluminum and finding excellent agreement in both the zero-temperature superconducting gap as well as the complex conductivity data when compared with BCS theory. We then demonstrate the utility of the technique by measuring the kinetic inductance of multi-layered niobium diselenide and discuss the limits to the accuracy of our technique when the transition temperature of the sample, NbSe$_2$ at 7.06 K, approaches our Nb probe resonator at 8.59 K. Our method will be useful for practitioners in the growing fields of superconducting physics, materials science, and quantum sensing, as a means of characterizing superconducting circuit components and studying pairing mechanisms of the novel superconducting states which arise in layered 2D materials and heterostructures.

cond-mat.supr-con

Quantum Metric in Step Response

Quantum geometry of Bloch wavefunctions has gained considerable interest with the discovery of moir\'e materials that exhibit bands flattened by quantum interference. The quantum metric, the symmetric part of the quantum geometric tensor, influences several observables, such as the dielectric constant, superfluid stiffness and optical spectral weight. However, a direct measurement of the metric itself has remained elusive so far. In linear response functions such as the conductivity, the matrix elements of the metric typically appear convoluted with energy prefactors, preventing finding an observable that is directly proportional to the total quantum metric. The only observable that may extract it is the integrated optical spectral weight weighted by the inverse frequency, a generalized sum rule known as the Souza-Wilkens-Martin (SWM) sum rule. However, the sum rule comes with experimental challenges, such as requiring a large spectrum of frequency resolution. In this work, we propose relaxation from constrained equilibrium as a method to directly measure the symmetric part of the time-dependent quantum geometric tensor (tQGT), which at $t=0$ is the quantum metric. Additionally, we comment on other geometric properties of insulators that are absent in the frequency expansions of conductivity in insulators but can, in principle, be revealed in step response.

cond-mat.mes-hall

Topologically protected flatness in chiral moir\'e heterostructures

The observation of delicate correlated phases in twisted heterostructures of graphene and transition metal dichalcogenides suggests that moir\'e flat bands are intrinsically resilient against certain types of disorder. Here, we investigate the robustness of moir\'e flat bands in the chiral limit of the Bistrizer-MacDonald model -- applicable to both platforms in certain limits -- and demonstrate drastic differences between the first magic angle and higher magic angles in response to chiral symmetric disorder that arise, for instance, from lattice relaxation. Using a hidden constant of motion, we decompose the non-abelian gauge field induced by interlayer tunnelings into two decoupled abelian ones, whose effective magnetic field splits into an anomalous contribution and a fluctuating part. The anomalous field maps the moir\'e flat bands onto a zeroth Dirac Landau level, whose flatness withstands any chiral symmetric perturbation due to a topological index theorem -- thereby underscoring a topological mechanism for band flatness. Only the first magic angle can fully harness this topological protection due to its weak fluctuating magnetic field. In higher magic angles, the amplitude of fluctuations largely exceeds the anomalous contribution, which we find results in an extremely large sensitivity to microscopic details. Through numerical simulations, we study various types of disorder and identify the processes that are enhanced or suppressed in the chiral limit. Interestingly, we find that the topological suppression of disorder broadening persists away from the chiral limit and is further accentuated by isolating a single sublattice polarized flat band in energy. Our analysis suggests the Berry curvature hotspot at the top of the $K$ and $K'$ valence band in the transition metal dichalcogenide monolayers is essential for the stability of its moir\'e flat bands and their correlated states.

cond-mat.mes-hall

Instantaneous response and quantum geometry of insulators

We present the time-dependent Quantum Geometric Tensor (tQGT) as a comprehensive tool for capturing the geometric character of insulators observable within linear response. We show that tQGT describes the zero-point motion of bound electrons and acts as a generating function for generalized sum rules of electronic conductivity. It therefore enables a systematic framework for computing the instantaneous response of insulators, including optical mass, orbital angular momentum, and dielectric constant. This construction guarantees a consistent approximation across these quantities upon restricting the number of occupied and unoccupied states in a low-energy description of an infinite quantum system. We outline how quantum geometry can be generated in periodic systems by lattice interference and examine spectral weight transfer from small frequencies to high frequencies by creating geometrically frustrated flat bands.

cond-mat.mes-hall

Geometric Stiffness in Interlayer Exciton Condensates

Recent experiments have confirmed the presence of interlayer excitons in the ground state of transition metal dichalcogenide (TMD) bilayers. The interlayer excitons are expected to show remarkable transport properties when they undergo Bose condensation. In this work, we demonstrate that quantum geometry of Bloch wavefunctions plays an important role in the phase stiffness of the Interlayer Exciton Condensate (IEC). Notably, we identify a geometric contribution that amplifies the stiffness, leading to the formation of a robust condensate with an increased BKT temperature. Our results have direct implications for the ongoing experimental efforts on interlayer excitons in materials that have non-trivial quantum geometry. We provide quantitative estimates for the geometric contribution in TMD bilayers through a realistic continuum model with gated Coulomb interaction, and find that the substantially increased stiffness allows for an IEC to be realized at amenable experimental conditions.

cond-mat.mes-hall

Unified Theory of the Anomalous and Topological Hall Effects with Phase Space Berry Curvatures

Hall experiments in chiral magnets are often analyzed as the sum of an anomalous Hall effect, dominated by momentum-space Berry curvature, and a topological Hall effect, arising from the real-space Berry curvature in the presence of skyrmions, in addition to the ordinary Hall resistivity. This raises the questions of how one can incorporate, on an equal footing, the effects of the anomalous velocity and the real space winding of the magnetization, and when such a decomposition of the resistivity is justified. We provide definitive answers to these questions by including the effects of all phase-space Berry curvatures in a semi-classical approach and by solving the Boltzmann equation in a weak spin-orbit coupling regime when the magnetization texture varies slowly on the scale of the mean free path. We show that the Hall resistivity is then just the sum of the anomalous and topological contributions, with negligible corrections from Berry curvature-independent and mixed curvature terms. We also use an exact Kubo formalism to numerically investigate the opposite limit of infinite mean path, and show that the results are similar to the semi-classical results.

cond-mat.mes-hall

Enhancing Perpendicular Magnetic Anisotropy in Garnet Ferrimagnet by Interfacing with Few-Layer WTe2

Engineering magnetic anisotropy in a ferro- or ferrimagnetic (FM) thin film is crucial in spintronic device. One way to modify the magnetic anisotropy is through the surface of the FM thin film. Here, we report the emergence of a perpendicular magnetic anisotropy (PMA) induced by interfacial interactions in a heterostructure comprised of a garnet ferrimagnet, Y3Fe5O12 (YIG), and the low-symmetry, high spin orbit coupling (SOC) transition metal dichalcogenide, WTe2. At the same time, we also observed an enhancement in Gilbert damping in the WTe2 covered YIG area. Both the magnitude of interface-induced PMA and the Gilbert damping enhancement have no observable WTe2 thickness dependence down to single quadruple-layer, indicating that the interfacial interaction plays a critical role. The ability of WTe2 to enhance the PMA in FM thin film, combined with its previously reported capability to generate out-of-plane damping like spin torque, makes it desirable for magnetic memory applications.

cond-mat.mtrl-sci

Optical Spectral Weight, Phase Stiffness and Tc Bounds for Trivial and Topological Flat Band Superconductors

We present exact results that give insight into how interactions lead to transport and superconductivity in a flat band where the electrons have no kinetic energy. We obtain bounds for the optical spectral weight for flat band superconductors, that lead to upper bounds for the superfluid stiffness and the 2D $T_c$. We focus on on-site attraction $|U|$ on the Lieb lattice with trivial flat bands and on the $π$-flux model with topological flat bands. For trivial flat bands, the low-energy optical spectral weight $\widetilde{D}_\text{low} \leq \widetilde{n} |U| Ω/2$ with $\widetilde{n} = \min\left(n,2-n\right)$, where $n$ is the flat band density and $Ω$ the Marzari-Vanderbilt spread of the Wannier functions (WFs). We also obtain a lower bound involving the quantum metric. For topological flat bands, with an obstruction to localized WFs respecting all symmetries, we again obtain an upper bound for $D_{\rm low}$ linear in $|U|$. We discuss the insights obtained from our bounds by comparing them with mean-field and quantum Monte-Carlo results.

cond-mat.supr-con