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Nobuo Furukawa

Publications and source records attributed to Nobuo Furukawa.

At least 55 records · Page 3Linked to original sources

Non-Degenerate Ground State in the Antiferromagnetic Double-Exchange Model on a Triangular Lattice

In order to study effects of frustration in an itinerant electron system, we investigate ground states of the antiferromagnetic double-exchange model on a triangular lattice. In this model, pseudo-spins are coupled to electron transfer integrals in such a way that antiparallel configurations of pseudo-spins gain kinetic energies. Although the antiferromagnetic Ising model on a triangular lattice shows macroscopic dengenerate ground states, the present model shows that the degeneracy is lifted due to long-range natures of the double exchange interactions. Spin ordering at the ground state is also discussed.

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Frustration-induced Dodecamer Ordering in the Double-Exchange Spin Ice Model on the Kagomé Lattice

We investigate a detail of a dodecamer cluster ordering in a double-exchange spin ice model on a kagomé lattice. In frustrated systems, ordinary spin orderings are suppressed and macroscopic degeneracy remains down to low temperatures. In some frustrated systems, the degeneracy is lifted due to residual interactions and cluster orderings are stabilized. In the present model, the spin ice state is first formed at intermediate temperatures, and further entropies are released at lower temperatures as the dodecamer phase emerges. Since the spin symmetry is not broken in the dodecamer phase, there still exists macroscopic degeneracy. At further low temperatures, a possible spin ordering due to inter-dodecamer interactions is proposed. We discuss that such a multiple-site clustering larger than a bond-pair might be generic to frustrated systems where macroscopic degeneracy is lifted by residual interactions.

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Mechanism for lifting the degeneracy in the double-exchange spin ice model on a kagomé lattice: Dodecamer formation

We investigated the double-exchange spin ice model on a kagomé lattice by Monte Carlo simulation in order to study a mechanism for lifting the degeneracy in frustrated electron systems. We show specific heat and vector spin chirality data on a finite lattice. Specific heat has a double-peak structure: A broad peak and a sharp peak are at $k_{\rm B}T/t \sim 0.15$ and 0.015, respectively, where $t$ is the transfer integral of electrons. The broad peak corresponds to a crossover to the spin ice-like state, on the other hand, the sharp one a transition to a dodecagonal spin cluster (dodecamer) state. We discuss the interplay between the formation of the dodecamer state and the lifting of the macroscopic degeneracy.

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Colossal magnetoresistance and quenched disorder in manganese oxides

We give an overview on several recent topics of colossal magnetoresistive manganites in both experiments and theories, focusing on the effect of quenched disorder. The disorder is intrinsically involved since the compounds are solid solutions, and its importance has been pointed out in several experiments of transport and magnetic properties. Recent progress in the experimental control of the strength of disorder is also reviewed. Theoretically, the effect of the disorder has been explored within the framework of the double-exchange mechanism. Several efforts to understand the phase diagram and the electronic properties are reviewed. We also briefly discuss a recent topic on the effect of disorder on competing phases and the origin of colossal magnetoresistance.

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Entropy-Driven Reentrant Behavior in CMR Manganites

We discuss the origin of the reentrant behaviors of insulating states above the Curie temperature of the colossal magnetoresistance manganites. We consider a system where charge ordering and ferromagnetism compete with each other. In the presence of randomness which pins charge order fluctuations, entropy-driven reentrant behaviors will appear, which explains the typical temperature dependence of the resistivity for CMR manganites.

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An Origin of CMR: Competing Phases and Disorder-Induced Insulator-to-Metal Transition in Manganites

We theoretically explore the mechanism of the colossal magnetoresistance in manganese oxides by explicitly taking into account the phase competition between the double-exchange ferromagnetism and the charge-ordered insulator. We find that quenched disorder causes a drastic change of the multicritical phase diagram by destroying the charge-ordered state selectively. As a result, there appears a nontrivial phenomenon of the disorder-induced insulator-to-metal transition in the multicritical regime. On the contrary, the disorder induces a highly-insulating state above the transition temperature where charge-ordering fluctuations are much enhanced. The contrasting effects provide an understanding of the mechanism of the colossal magnetoresistance. The obtained scenario is discussed in comparison with other theoretical proposals such as the polaron theory, the Anderson localization, the multicritical-fluctuation scenario, and the percolation scenario.

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Spin Dodecamer Formation in the Double-Exchange Spin Ice Model

We investigated the double-exchange spin ice (DESI) model on a kagomé lattice by Monte Carlo simulation to study the effects of a geometrical frustration, and the mechanism that generates an ordered state in a metallic system. The DESI model on the kagomé lattice is a frustrated metallic system due to an effective ferromagnetic interaction between localized spins caused by the double-exchange (DE) mechanism and a uniaxial anisotropy for the localized spins. A dodecagonal spin cluster (named dodecamer), which consists of twelve localized spins, appears at low temperature when the number of particles per site $n \simeq 1/3 \sim 1/2$. Such a dodecamer order is driven by both the kinetic energy gain due to the DE mechanism and the geometrical frustration. We discuss that cluster orders, in general, may be a common feature in itinerant electron systems coupled with frustrated adiabatic fields.

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Order N Monte Carlo Algorithm for Fermion Systems Coupled with Fluctuating Adiabatical Fields

An improved algorithm is proposed for Monte Carlo methods to study fermion systems interacting with adiabatical fields. To obtain a weight for each Monte Carlo sample with a fixed configuration of adiabatical fields, a series expansion using Chebyshev polynomials is applied. By introducing truncations of matrix operations in a systematic and controlled way, it is shown that the cpu time is reduced from O(N^3) to O(N) where N is the system size. Benchmark results show that the implementation of the algorithm makes it possible to perform systematic investigations of critical phenomena using system-size scalings even for an electronic model in three dimensions, within a realistic cpu timescale.

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Competing Orders and Disorder-induced Insulator to Metal Transition in Manganites

Effects of disorder on the two competing phases, i.e., the ferromagnetic metal and the commensurate charge/lattice ordered insulator, are studied by Monte Carlo simulation. The disorder suppresses the charge/lattice ordering more strongly than the ferromagnetic order, driving the commensurate insulator to the ferromagnetic metal near the phase boundary in the pure case. Above the ferromagnetic transition temperature, on the contrary, the disorder makes the system more insulating, which might cause an enhanced colossal magnetoresistance as observed in the half-doped or Cr-substituted manganites. No indication of the percolation or the cluster formation is found, and there remain the charge/lattice fluctuations instead which are enhanced toward the transition temperature.

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Disorder Effect on Spin Excitation in Double Exchange Systems

Spin excitation spectrum is studied in the double exchange model in the presence of disorder. Spin wave approximation is applied in the lowest order of 1/S expansion. The disorder causes anomalies in the spin excitation spectrum such as broadening, branching, anticrossing with gap opening. The origin of the anomalies is the Friedel oscillation, in which the perfectly polarized electrons form the charge density wave to screen the disorder effect. Near the zone center $q = 0$, the linewidth has a $q$ linear component while the excitation energy scales to $q^2$, which indicates that the magnon excitation is incoherent. As $q$ increases, there appears a crossover from this incoherent behavior to the marginally coherent one in which both the linewidth and the excitation energy are proportional to $q^2$. The results are compared with experimental results in colossal magnetoresistance manganese oxides. Quantitative comparison of the linewidth suggests that spatially-correlated or mesoscopic-scale disorder is more relevant in real compounds than local or atomic-scale disorder. Comparison with other theoretical proposals is also discussed. Experimental tests are proposed for the relevance of disorder.

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Monte Carlo Study of Doping Change and Disorder Effect on Double Exchange Ferromagnetism

Phase diagram and critical properties are studied for three-dimensional double exchange model with and without quenched disorder. Employing the Monte Carlo method and the systematic analysis on the finite-size effect, we estimate the Curie temperature and the critical exponent as functions of the doping concentration and the strength of the random potential. The Curie temperature well scales to the kinetic energy of electrons in the ground state as expected for this kinetics-driven ferromagnetism. The universality class of this transition is described by the short-range Heisenberg fixed point. The results are compared with the experimental results in the colossal magnetoresistance manganites.

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Randomness Effect on Multicritical Phenomena in Double-Exchange Systems

Double-exchange model interacting with adiabatic phonons is studied in the presence of randomness by using the Monte-Carlo method and the systematic size-scaling analysis. A bicritical behavior is found between the ferromagnetic metal and the charge-ordered insulator. We find the distinct response to the randomness between these two states, which agrees well with the experimental results in the colossal magnetoresistance manganites.

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Universality Class of Ferromagnetic Transition in Three-Dimensional Double-Exchange System - O(N) Monte Carlo Study -

Curie temperature and exponents are studied for the three-dimensional double-exchange model. Applying the O(N) Monte Carlo algorithm, we perform systematic finite-size scaling analyses on the data up to $20^3$ sites. The obtained values of the critical exponents are consistent with those of the Heisenberg universality class, and clearly distinct from the mean-field values.

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Spectral Function Analysis on Spin Dynamics in Double-Exchange Systems with Randomness

Spin excitation spectrum is studied in the double-exchange model with randomness. Applying the spin wave approximation and the spectral function analysis, we examine excitation energy and linewidth using analytical as well as numerical methods. For small wave number $q \sim 0$, the excitation energy is cosine-like and the linewidth shows a $q$-linear behavior. This indicates that the spin excitation becomes incoherent or localized near $q = 0$. Crossover takes place to marginally-coherent regime where both the excitation energy and the linewidth are proportional to $q^2$. The incoherence is due to local fluctuations of the kinetic energy of electrons. Comparison with experimental results in colossal magnetoresistance manganites suggests that spatially-correlated or mesoscopic-scale fluctuations are more important in real compounds than local or atomic-scale ones.

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Spin-wave Hamiltonian in double-exchange systems

A simple derivation of the effective spin-wave Hamiltonian for a double-exchange system with infinitely large Hund's-rule coupling is demonstrated. The formalism can be applied to models with arbitrary range of hopping as well as those with randomness. The result shows that, within the leading order of the 1/S expansion, one magnon excitation spectrum can be described by the Heisenberg model.

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Impurity Effect on Ferromagnetic Transition in Double-Exchange Systems

Effect of randomness in the double-exchange model is studied. Large fluctuations and spatial random distribution of impurities are taken into account in an essentially exact manner by using the Monte Carlo calculation. The randomness suppresses the ferromagnetism by reducing the coherence of itinerant electrons. The suppression is significant in the critical region where the fluctuations are dominant. Temperature dependences of the magnetization are estimated for finite-size clusters. A characteristic temperature for phase transition $T^{*}$ is estimated from the inflection point, which is expected to give a good approximation for the critical temperature in the thermodynamic limit. Our results suggest that the ferromagnetism becomes unstable more rapidly than predicted in the previous theoretical results by the coherent-potential approximation.

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Anomaly in Spin Excitation Spectrum of Double-Exchange Systems with Randomness

Spin excitation spectrum of the double-exchange model is studied in the presence of randomness. Spin wave approximation in the ground state shows that the randomness significantly modifies the spectrum from the cosine-like one in the pure system to that with anomalies such as broadening, anti-crossing and gap opening. The origin of anomalies is speculated to be modulation of effective ferromagnetic coupling by the Friedel oscillation. These anomalies qualitatively reproduce the spin excitation spectrum in colossal magnetoresistance manganites whose Curie temperatures are relatively low. Our results suggest that randomness control is an important notion to understand effects of the A-site substitution which has previously been understood as the bandwidth control.

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Critical Exponents for the Ferromagnetism in Colossal Magnetoresistance Manganites

Critical phenomena of ferromagnetic transition in colossal magnetoresistance manganites are theoretically studied. Concerning the critical exponents for this transition, there still remains controversy among experimental results. In order to clarify intrinsic physics of the manganites through a comparison with theoretical prediction, we investigate the critical phenomena of double-exchange models by using finite-size scaling analysis on unbiased numerical results. As a result, we show that the critical exponents of the ferromagnetic transition of the three-dimensional double-exchange model is consistent with those of the Heisenberg model, but are distinct from the mean-field one.

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