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O. Wieland

Publications and source records attributed to O. Wieland.

At least 19 recordsLinked to original sources

First Extraction of the Matter Radius of $^{132}$Sn via Proton Elastic Scattering at 200 MeV/Nucleon

The angular distribution of the differential cross sections for proton elastic scattering from $^{132}$Sn at 196-210 MeV/nucleon was successfully measured over a momentum transfer range of 0.80 to 2.1 fm$^{-1}$. Using a relativistic impulse approximation, the root-mean-square matter radius of $^{132}$Sn was extracted to be $4.758^{+0.023}_{-0.024}$ fm, which was compared with the state-of-the-art ab initio calculations. Combined with the charge radius measured at ISOLDE, there are no theoretical calculations consistent with both matter and charge radii within the experimental errors.

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Statistical properties and photon strength functions of the ${}^{112,114}$Sn isotopes below the neutron separation threshold

Here, we report on the measurements of the $γ$-ray strength functions and nuclear level densities of ${}^{112,114}$Sn performed for the first time at the 9~MV Tandem accelerator facilities at IFIN-HH using the Oslo method. We extract thermodynamic properties and gross and fine properties of the pygmy dipole resonance for systematic comparison in the chain of Sn isotopes. The results are compared with microscopic models implemented in the TALYS reaction code and the fully microscopic quasiparticle-phonon model for the underlying nuclear structure of the dipole strength in ${}^{112,114}$Sn. The quasiparticle-phonon model results show the importance of complex configurations to the low-energy dipole response in the pygmy dipole resonance energy region. The experimental data are further included in the cross-section and reaction rate calculations for the $(\mathrm{n},γ)$ reaction of the $p$-process nuclei ${}^{112,114}$Sn showing a significant increase in reaction rates at high temperatures compared to existing nuclear databases.

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PANDORA project: photo-nuclear reactions below $A=60$

Photo-nuclear reactions of light nuclei below a mass of $A=60$ are studied experimentally and theoretically by the PANDORA (Photo-Absorption of Nuclei and Decay Observation for Reactions in Astrophysics) project. Two experimental methods, virtual-photon excitation by proton scattering and real-photo absorption by a high-brilliance gamma-ray beam produced by laser Compton scattering, will be applied to measure the photo-absorption cross sections and the decay branching ratio of each decay channel as a function of the photon energy. Several nuclear models, e.g. anti-symmetrized molecular dynamics, mean-field type models, a large-scale shell model, and ab initio models, will be employed to predict the photo-nuclear reactions. The uncertainty in the model predictions will be evaluated from the discrepancies between the model predictions and the experimental data. The data and the predictions will be implemented in a general reaction calculation code TALYS . The results will be applied to the simulation of the photo-disintegration process of ultra-high-energy cosmic rays in inter-galactic propagation.

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Model-independent determination of the dipole response of $^{66}$Zn using quasi-monoenergetic and linearly-polarized photon beams

[Background] Photon strength functions are an important ingredient in calculations relevant for the nucleosynthesis of heavy elements. The relation to the photoabsorption cross section allows to experimentally constrain photon strength functions by investigating the photo-response of atomic nuclei. [Purpose] We determine the photoresponse of $^{66}$Zn in the energy region of 5.6 MeV to 9.9 MeV and analyze the contribution of the "elastic" decay channel back to the ground state. In addition, for the elastic channel electric and magnetic dipole transitions were separated. [Methods] Nuclear resonance fluorescence experiments were performed using a linearly-polarized quasi-monoenergetic photon beam at the High Intensity $γ$-ray Source. Photon beam energies from 5.6 to 9.9 MeV with an energy spread of about 3% were selected in steps of 200-300 keV. Two High Purity Germanium detectors were used for the subsequent $γ$-ray spectroscopy. [Results] Full photoabsorption cross sections are extracted from the data making use of the monoenergetic character of the photon beam. For the ground-state decay channel, the average contribution of electric and magnetic dipole strengths is disentangled. The average branching ratio back to the ground state is determined as well. [Conclusions] The new results indicate lower cross sections when compared to the values extracted from a former experiment using bremsstrahlung on $^{66}$Zn. In the latter, the average branching ratio to the ground state is estimated from statistical-model calculations in order to analyze the data. Corresponding estimates from statistical-model calculations underestimate this branching ratio compared to the values extracted from the present analysis, which would partly explain the high cross sections determined from the bremsstrahlung data.

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Coulomb and nuclear excitations of $^{70}$Zn and $^{68}$Ni at intermediate energy

The reduced transition probabilities $B(E2; 0^+_{g.s.}\rightarrow2_1^+,2^+_2)$ in $^{70}$Zn and the full $B(E2; 0^+_{g.s.}\rightarrow2^+)$ strength up to S$_n$=7.79 MeV in $^{68}$Ni have been determined at the LISE/GANIL facility using the Coulomb-excitation technique at intermediate beam energy on a $^{208}$Pb target. The $γ$ rays emitted in-flight were detected with an array of 46 BaF$_2$ crystals. The angles of the deflected nuclei were determined in order to disentangle and extract the Coulomb and nuclear contributions to the excitation of the 2$^+$ states. The measured $B(E2; 0^+_{g.s.}\rightarrow2_1^+)$ of 1432(124) e$^2$fm$^4$ for $^{70}$Zn falls in the lower part of the published values which clustered either around 1600 or above 2000 e$^2$fm$^4$, while the $B(E2; 0^+_{g.s.}\rightarrow2^+_2)$ of 53(7) e$^2$fm$^4$ agrees very well with the two published values. The relatively low $B(E2; 0^+_{g.s.}\rightarrow2_1^+)$ of 301(38) e$^2$fm$^4$ for $^{68}$Ni agrees with previous studies and confirms a local magicity at $Z=28, N=40$. Combining the results of the low-energy spectra of $^{68}$Ni and $^{70}$Zn and their shell-model interpretations, it is interesting to notice that four different shapes (spherical, oblate, prolate and triaxial) are present. Finally, a summed $E2$ strength of only about 150 e$^2$fm$^4$ has been found experimentally at high excitation energy, likely due to proton excitations across the $Z=28$ gap. The experimental distribution of this high-energy $E2$ excitation agrees with SM calculations, but its strength is about two times weaker.

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Complete set of bound negative-parity states in the neutron-rich 18N nucleus

High-resolution gamma-ray spectroscopy of 18N is performed with the Advanced GAmma Tracking Array AGATA, following deep-inelastic processes induced by an 18O beam on a 181Ta target. Six states are newly identified, which together with the three known excitations exhaust all negative-parity excited states expected in 18N below the neutron threshold. Spin and parities are proposed for all located states on the basis of decay branchings and comparison with large-scale shell-model calculations performed in the p-sd space, with the YSOX interaction. Of particular interest is the location of the 0^-_1 and 1^-_2 excitations, which provide strong constrains for cross-shell p-sd matrix elements based on realistic interactions, and help to simultaneously reproduce the ground and first-excited states in 16N and 18N, for the first time. Understanding the 18N structure may also have significant impact on neutron-capture cross-section calculations in r-process modeling including light neutron-rich nuclei.

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Accessing tens-to-hundreds femtoseconds nuclear state lifetimes with low-energy binary heavy-ion reactions

A novel Monte Carlo technique has been developed to determine lifetimes of excited states in the tens-to-hundreds femtoseconds range. The method is applied to low-energy heavy-ion binary reactions populating nuclei with complex velocity distributions. Its relevance is demonstrated in connection with the $^{18}$O(7.0 MeV/u) + $^{181}$Ta experiment, performed at GANIL with the AGATA+VAMOS+PARIS setup, to study neutron-rich O, C, N, ... nuclei. Excited states in $^{17}$O and $^{19}$O, with known lifetimes, are used to validate the method over the $\sim$20-400 fs lifetime-sensitivity range. Emphasis is given to the unprecedented position resolution provided by $γ$-tracking arrays, which turns out to be essential for reaching the required accuracy in Doppler-shift correction, at the basis of the detailed analysis of $γ$-ray lineshape and resulting state lifetime determination. The technique is anticipated to be an important tool for lifetime investigations in exotic neutron-rich nuclei, produced with intense ISOL-type beams.

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Manifestation of the Berry phase in the atomic nucleus $^{213}$Pb

The neutron-rich $^{213}$Pb isotope was produced in the fragmentation of a primary 1 GeV $A$ $^{238}$U beam, separated in FRS in mass and atomic number, and then implanted for isomer decay $γ$-ray spectroscopy with the RISING setup at GSI. A newly observed isomer and its measured decay properties indicate that states in $^{213}$Pb are characterized by the seniority quantum number that counts the nucleons not in pairs coupled to angular momentum $J=0$. The conservation of seniority is a consequence of the Berry phase associated with particle-hole conjugation, which becomes gauge invariant and therefore observable in semi-magic nuclei where nucleons half-fill the valence shell. The $γ$-ray spectroscopic observables in $^{213}$Pb are thus found to be driven by two mechanisms, particle-hole conjugation and seniority conservation, which are intertwined through the Berry phase.

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Testing ab initio nuclear structure in neutron-rich nuclei: lifetime measurements of second 2+ states in 16C and 20O

To test the predictive power of ab initio nuclear structure theory, the lifetime of the second 2+ state in neutron-rich 20O, tau(2+_2 ) = 150(+80-30) fs, and an estimate for the lifetime of the second 2+ state in 16C have been obtained, for the first time. The results were achieved via a novel Monte Carlo technique that allowed us to measure nuclear state lifetimes in the tens-to-hundreds femtoseconds range, by analyzing the Doppler-shifted gamma-transition line shapes of products of low-energy transfer and deep-inelastic processes in the reaction 18O (7.0 MeV/u) + 181Ta. The requested sensitivity could only be reached owing to the excellent performances of the AGATA gamma-tracking array, coupled to the PARIS scintillator array and to the VAMOS++ magnetic spectrometer. The experimental lifetimes agree with predictions of ab initio calculations using two- and three-nucleon interactions, obtained with the valence-space in-medium similarity renormalization group for 20O, and with the no-core shell model for 16C. The present measurement shows the power of electromagnetic observables, determined with high-precision gamma spectroscopy, to assess the quality of first-principles nuclear structure calculations, complementing common benchmarks based on nuclear energies. The proposed experimental approach will be essential for short lifetimes measurements in unexplored regions of the nuclear chart, including r-process nuclei, when intense ISOL-type beams become available.

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Is Seniority a Partial Dynamic Symmetry in the First $νg_{9/2}$ Shell?

The low-lying structures of the midshell $νg_{9/2}$ Ni isotopes $^{72}$Ni and $^{74}$Ni have been investigated at the RIBF facility in RIKEN within the EURICA collaboration. Previously unobserved low-lying states were accessed for the first time following $β$ decay of the mother nuclei $^{72}$Co and $^{74}$Co. As a result, we provide a complete picture in terms of the seniority scheme up to the first $(8^+)$ levels for both nuclei. The experimental results are compared to shell-model calculations in order to define to what extent the seniority quantum number is preserved in the first neutron $g_{9/2}$ shell. We find that the disappearance of the seniority isomerism in the $(8^+_1)$ states can be explained by a lowering of the seniority-four $(6^+)$ levels as predicted years ago. For $^{74}$Ni, the internal de-excitation pattern of the newly observed $(6^+_2)$ state supports a restoration of the normal seniority ordering up to spin $J=4$. This property, unexplained by the shell-model calculations, is in agreement with a dominance of the single-particle spherical regime near $^{78}$Ni.

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Charged particle decay of hot and rotating $^{88}$Mo nuclei in fusion-evaporation reactions

A study of fusion-evaporation and (partly) fusion-fission channels for the $^{88}$Mo compound nucleus, produced at different excitation energies in the reaction $^{48}$Ti + $^{40}$Ca at 300, 450 and 600 MeV beam energies, is presented. Fusion-evaporation and fusion-fission cross sections have been extracted and compared with the existing systematics. Experimental data concerning light charged particles have been compared with the prediction of the statistical model in its implementation in the Gemini++ code, well suited even for high spin systems, in order to tune the main model parameters in a mass region not abundantly covered by exclusive experimental data. Multiplicities for light charged particles emitted in fusion evaporation events are also presented. Some discrepancies with respect to the prediction of the statistical model have been found for forward emitted $α$-particles; they may be due both to pre-equilibrium emission and to reaction channels (such as Deep Inelastic Collisions, QuasiFission/QuasiFusion) different from the compound nucleus formation.

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A new study of $^{25}$Mg($α$,n)$^{28}$Si angular distributions at $E_α$ = 3 - 5 MeV

The observation of $^{26}$Al gives us the proof of active nucleosynthesis in the Milky Way. However the identification of the main producers of $^{26}$Al is still a matter of debate. Many sites have been proposed, but our poor knowledge of the nuclear processes involved introduces high uncertainties. In particular, the limited accuracy on the $^{25}$Mg($α$,n)$^{28}$Si reaction cross section has been identified as the main source of nuclear uncertainty in the production of $^{26}$Al in C/Ne explosive burning in massive stars, which has been suggested to be the main source of $^{26}$Al in the Galaxy. We studied this reaction through neutron spectroscopy at the CN Van de Graaff accelerator of the Legnaro National Laboratories. Thanks to this technique we are able to discriminate the ($α$,n) events from possible contamination arising from parasitic reactions. In particular, we measured the neutron angular distributions at 5 different beam energies (between 3 and 5 MeV) in the \ang{17.5}-\ang{106} laboratory system angular range. The presented results disagree with the assumptions introduced in the analysis of a previous experiment.

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Pre-equilibrium α-particle emission as a probe to study α-clustering in nuclei

A theoretical approach was developed to describe secondary particle emission in heavy ion collisions, with special regards to pre-equilibrium α-particle production. Griffin's model of non-equilibrium processes is used to account for the first stage of the compound system formation, while a Monte Carlo statistical approach was used to describe the further decay from a hot source at thermal equilibrium. The probabilities of neutron, proton and α-particle emission have been evaluated for both the equilibrium and pre-equilibrium stages of the process. Fission and γ-ray emission competition were also considered after equilibration. Effects due the possible cluster structure of the projectile which has been excited during the collisions have been experimentally evidenced studying the double differential cross sections of p and α-particles emitted in the E=250MeV 16O +116Sn reaction. Calculations within the present model with different clusterization probabilities have been compared to the experimental data.

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Measurement of light charged particles in the decay channels of medium-mass excited compound nuclei

The 48Ti on 40Ca reactions have been studied at 300 and 600 MeV focusing on the fusion-evaporation (FE) and fusion-fission (FF) exit channels. Energy spectra and multiplicities of the emitted light charged particles have been compared to Monte Carlo simulations based on the statistical model. Indeed, in this mass region (A about 100) models predict that shape transitions can occur at high spin values and relatively scarce data exist in the literature about coincidence measurements between evaporation residues and light charged particles. Signals of shape transitions can be found in the variations of the lineshape of high energy gamma rays emitted from the de-excitation of GDR states gated on different region of angular momenta. For this purpose it is important to keep under control the FE and FF processes, to regulate the statistical model parameters and to control the onset of possible preequilibrium emissions from 300 to 600 MeV bombarding energy.

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Characterization of Large Volume 3.5 x 8 inches LaBr3:Ce Detectors

The properties of large volume cylindrical 3.5 x 8 inches (89 mm x 203 mm) LaBr3:Ce scintillation detectors coupled to the Hamamatsu R10233-100SEL photo-multiplier tube were investigated. These crystals are among the largest ones ever produced and still need to be fully characterized to determine how these detectors can be utilized and in which applications. We tested the detectors using monochromatic gamma-ray sources and in-beam reactions producing gamma rays up to 22.6 MeV; we acquired PMT signal pulses and calculated detector energy resolution and response linearity as a function of gamma-ray energy. Two different voltage dividers were coupled to the Hamamatsu R10233-100SEL PMT: the Hamamatsu E1198-26, based on straightforward resistive network design, and the LABRVD, specifically designed for our large volume LaBr3:Ce scintillation detectors, which also includes active semiconductor devices. Because of the extremely high light yield of LaBr3:Ce crystals we observed that, depending on the choice of PMT, voltage divider and applied voltage, some significant deviation from the ideally proportional response of the detector and some pulse shape deformation appear. In addition, crystal non-homogeneities and PMT gain drifts affect the (measured) energy resolution especially in case of high-energy gamma rays. We also measured the time resolution of detectors with different sizes (from 1x1 inches up to 3.5x8 inches), correlating the results with both the intrinsic properties of PMTs and GEANT simulations of the scintillation light collection process. The detector absolute full energy efficiency was measured and simulated up to gamma-rays of 30 MeV

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Core-coupled states and split proton-neutron quasi-particle multiplets in 122-126Ag

Neutron-rich silver isotopes were populated in the fragmentation of a 136Xe beam and the relativistic fission of 238U. The fragments were mass analyzed with the GSI Fragment separator and subsequently implanted into a passive stopper. Isomeric transitions were detected by 105 HPGe detectors. Eight isomeric states were observed in 122-126Ag nuclei. The level schemes of 122,123,125Ag were revised and extended with isomeric transitions being observed for the first time. The excited states in the odd-mass silver isotopes are interpreted as core-coupled states. The isomeric states in the even-mass silver isotopes are discussed in the framework of the proton-neutron split multiplets. The results of shell-model calculations, performed for the most neutron-rich silver nuclei are compared to the experimental data.

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Response of AGATA Segmented HPGe Detectors to Gamma Rays up to 15.1 MeV

The response of AGATA segmented HPGe detectors to gamma rays in the energy range 2-15 MeV was measured. The 15.1 MeV gamma rays were produced using the reaction d(11B,ng)12C at Ebeam = 19.1 MeV, while gamma-rays between 2 to 9 MeV were produced using an Am-Be-Fe radioactive source. The energy resolution and linearity were studied and the energy-to-pulse-height conversion resulted to be linear within 0.05%. Experimental interaction multiplicity distributions are discussed and compared with the results of Geant4 simulations. It is shown that the application of gamma-ray tracking allows a suppression of background radiation following neutron capture by Ge nuclei. Finally the Doppler correction for the 15.1 MeV gamma line, performed using the position information extracted with Pulse-shape Analysis, is discussed.

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Neutron-skin thickness from the study of the anti-analog giant dipole resonance

The gamma-decay of the anti-analog of the giant dipole resonance (AGDR) has been measured to the isobaric analog state excited in the p(124Sn,n) reaction at a beam energy of 600 MeV/nucleon. The energy of the transition was also calculated with state-of-the-art self-consistent random-phase approximation (RPA) and turned out to be very sensitive to the neutron-skin thickness (\DeltaR_(pn)). By comparing the theoretical results with the measured one, the \DeltaR_(pn) value for 124Sn was deduced to be 0.175 \pm 0.048 fm, which agrees well with the previous results. The energy of the AGDR measured previously for ^(208)Pb was also used to determine the \DeltaR_(pn) for ^(208)Pb. In this way a very precise \DeltaR_(pn) = 0.181 \pm 0.031 neutron-skin thickness has been obtained for 208Pb. The present method offers new possibilities for measuring the neutron-skin thicknesses of very exotic isotopes.

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