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Olena Gomonay

Publications and source records attributed to Olena Gomonay.

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Spin Hall magnetoresistance in antiferromagnetic insulators

Antiferromagnetic materials promise improved performance for spintronic applications, as they are robust against external magnetic field perturbations and allow for faster magnetization dynamics compared to ferromagnets. The direct observation of the antiferromagnetic state, however, is challenging due to the absence of a macroscopic magnetization. Here, we show that the spin Hall magnetoresistance (SMR) is a versatile tool to probe the antiferromagnetic spin structure via simple electrical transport experiments by investigating the easy-plane antiferromagnetic insulators $α$-Fe2O3 (hematite) and NiO in bilayer heterostructures with a Pt heavy metal top electrode. While rotating an external magnetic field in three orthogonal planes, we record the longitudinal and the transverse resistivities of Pt and observe characteristic resistivity modulations consistent with the SMR effect. We analyze both their amplitude and phase and compare the data to the results from a prototypical collinear ferrimagnetic Y3Fe5O12/Pt bilayer. The observed magnetic field dependence is explained in a comprehensive model, based on two magnetic sublattices and taking into account magnetic field-induced modifications of the domain structure. Our results show that the SMR allows us to understand the spin configuration and to investigate magnetoelastic effects in antiferromagnetic multi-domain materials. Furthermore, in $α$-Fe2O3/Pt bilayers, we find an unexpectedly large SMR amplitude of $2.5 \times 10^{-3}$, twice as high as for prototype Y3Fe5O12/Pt bilayers, making the system particularly interesting for room-temperature antiferromagnetic spintronic applications.

cond-mat.mtrl-sci↗

Theory of Current-Induced Angular Momentum Transfer Dynamics in Spin-Orbit Coupled Systems

Motivated by the importance of understanding competing mechanisms to current-induced spin-orbit torque in complex magnets, we develop a unified theory of current-induced spin-orbital coupled dynamics. The theory describes angular momentum transfer between different degrees of freedom in solids, e.g., the electron orbital and spin, the crystal lattice, and the magnetic order parameter. Based on the continuity equations for the spin and orbital angular momenta, we derive equations of motion that relate spin and orbital current fluxes and torques describing the transfer of angular momentum between different degrees of freedom. We then propose a classification scheme for the mechanisms of the current-induced torque in magnetic bilayers. Based on our first-principles implementation, we apply our formalism to two different magnetic bilayers, Fe/W(110) and Ni/W(110), which are chosen such that the orbital and spin Hall effects in W have opposite sign and the resulting spin- and orbital-mediated torques can compete with each other. We find that while the spin torque arising from the spin Hall effect of W is the dominant mechanism of the current-induced torque in Fe/W(110), the dominant mechanism in Ni/W(110) is the orbital torque originating in the orbital Hall effect of W. It leads to negative and positive effective spin Hall angles, respectively, which can be directly identified in experiments. This clearly demonstrates that our formalism is ideal for studying the angular momentum transfer dynamics in spin-orbit coupled systems as it goes beyond the "spin current picture" by naturally incorporating the spin and orbital degrees of freedom on an equal footing. Our calculations reveal that, in addition to the spin and orbital torque, other contributions such as the interfacial torque and self-induced anomalous torque within the ferromagnet are not negligible in both material systems.

cond-mat.mes-hall↗

Topological-chiral magnetic interactions driven by emergent orbital magnetism

Two hundred years ago, André-Marie Ampère discovered that electric loops in which currents of electrons are generated by a penetrating magnetic field can interact with each other. Here we show that Ampère's observation can be transferred to the quantum realm of interactions between triangular plaquettes of spins on a lattice, where the electrical currents at the atomic scale are associated with a peculiar type of the orbital motion of electrons in response to the non-coplanarity of neighbouring spins playing the role of a magnetic field. The resulting topological orbital moment underlies the relation of the orbital dynamics with the topology of the spin structure. We demonstrate that the interactions of the topological orbital moments with each other and with the spins of the underlying lattice give rise to a new class of magnetic interactions $-$ topological chiral interactions $-$ which can dominate over the celebrated Dzyaloshinskii-Moriya interaction, thus opening a path for the realization of new classes of chiral magnetic materials with three-dimensional magnetization textures such as magnetic hopfions.

cond-mat.mes-hall↗

Mechanism of Néel order switching in antiferromagnetic thin films revealed by magnetotransport and direct imaging

We probe the current-induced magnetic switching of insulating antiferromagnet/heavy metals systems, by electrical spin Hall magnetoresistance measurements and direct imaging, identifying a reversal occurring by domain wall (DW) motion. We observe switching of more than one third of the antiferromagnetic domains by the application of current pulses. Our data reveal two different magnetic switching mechanisms leading together to an efficient switching, namely the spin-current induced effective magnetic anisotropy variation and the action of the spin torque on the DWs.

cond-mat.mtrl-sci↗

Spin eigen-excitations of an antiferromagnetic skyrmion

We theoretically predict and classify the localized modes of a skyrmion in a collinear uniaxial antiferromagnet and discuss how they can be excited. As a central result, we find two branches of skyrmion eigenmodes with distinct physical properties characterized by being low or high energy excitations. The frequency dependence of the low-energy modes scales as $R_0^{-2}$ for skyrmions with large radius $R_0$. Furthermore, we predict localized high-energy eigenmodes, which have no direct ferromagnetic counterpart. Except for the breathing mode, we find that all localized antiferromagnet skyrmion modes, both in the low and high-energy branch, are doubly degenerated in the absence of a magnetic field and split otherwise. We explain our numerical results for the low-energy modes within a string model representing the skyrmion boundary.

cond-mat.str-el↗

Dynamics of noncollinear antiferromagnetic textures driven by spin current injection

We present a theoretical formalism to address the dynamics of textured, noncolliear antiferromagnets subject to spin current injection. We derive sine-Gordon type equations of motion for the antiferromagnets, which are applicable to technologically important antiferromagnets such as Mn3Ir and Mn3Sn, and enables an analytical approach to domain wall dynamics in those materials. We obtain the expression for domain wall velocity, which is estimated to reach around 1 km/s in Mn3Ir by exploiting spin Hall effect with electric current density around 10^11A/m^2.

cond-mat.mes-hall↗

Anisotropies and magnetic phase transitions in insulating antiferromagnets determined by a Spin-Hall magnetoresistance probe

We demonstrate that we can determine the antiferromagnetic anisotropies and the bulk Dzyaloshinskii-Moriya fields of the insulating iron oxide hematite, α-Fe2O3, using a surface sensitive spin-Hall magnetoresistance (SMR) technique. We develop an analytical model that in combination with SMR measurements, allow for the identification of the material parameters of this prototypical antiferromagnet over a wide range of temperatures and magnetic field values. Using devices with different orientations, we demonstrate that the SMR response strongly depends on the direction of the charge current with respect to the magneto-crystalline anisotropies axis. We show that we can extract the anisotropies over a wide temperature range including across the Morin phase transition. We observe that the electrical response is dominated by the orientation of the antiferromagnetic Néel order parameter, rather than by the emergent weak magnetic moment. Our results highlight that the surface sensitivity of the SMR allows accessing the magnetic anisotropies of antiferromagnetic crystals and in particular thin films where other methods to determine anisotropies such as bulk-sensitive magnetic susceptibility measurements do not provide sufficient sensitivity.

cond-mat.mes-hall↗

Spin transfer torques and spin-dependent transport in a metallic F/AF/N tunneling junction

We study spin-dependent electron transport through a ferromagnetic-antiferromagnetic-normal metal tunneling junction subject to a voltage or temperature bias, in the absence of spin-orbit coupling. We derive microscopic formulas for various types of spin torque acting on the antiferromagnet as well as for charge and spin currents flowing through the junction. The obtained results are applicable in the limit of slow magnetization dynamics. We identify a parameter regime in which an unconventional damping-like torque can become comparable in magnitude to the equivalent of the conventional Slonczewski's torque generalized to antiferromagnets. Moreover, we show that the antiferromagnetic sublattice structure opens up a channel of electron transport which does not have a ferromagnetic analogue and that this mechanism leads to a pronounced field-like torque. Both charge conductance and spin current transmission through the junction depend on the relative orientation of the ferromagnetic and the antiferromagnetic vectors (order parameters). The obtained formulas for charge and spin currents allow us to identify the microscopic mechanisms responsible for this angular dependence and to assess the efficiency of an antiferromagnetic metal acting as a spin current polarizer.

cond-mat.mes-hall↗

Spin colossal magnetoresistance in an antiferromagnetic insulator

Colossal magnetoresistance (CMR) refers to a large change in electrical conductivity induced by a magnetic field in the vicinity of a metal-insulator transition and has inspired extensive studies for decades\cite{Ramirez1997, Tokura2006}. Here we demonstrate an analogous spin effect near the Néel temperature $T_{\rm{N}}$=296 K of the antiferromagnetic insulator \CrO. Using a yttrium iron garnet \YIG/\CrO/Pt trilayer, we injected a spin current from the YIG into the \CrO layer, and collected via the inverse spin Hall effect the signal transmitted in the heavy metal Pt. We observed a change by two orders of magnitude in the transmitted spin current within 14 K of the Néel temperature. This transition between spin conducting and nonconducting states could be also modulated by a magnetic field in isothermal conditions. This effect, that we term spin colossal magnetoresistance (SCMR), has the potential to simplify the design of fundamental spintronics components, for instance enabling the realization of spin current switches or spin-current based memories.

cond-mat.mtrl-sci↗

Spin caloric effects in antiferromagnets assisted by an external spin current

Searching for novel spin caloric effects in antiferromagnets we study the properties of thermally activated magnons in the presence of an external spin current and temperature gradient. We predict the spin Peltier effect -- generation of a heat flux by spin accumulation -- in an antiferromagnetic insulator with cubic or uniaxial magnetic symmetry. This effect is related with spin-current induced splitting of the relaxation times of the magnons with opposite spin direction. We show that the Peltier effect can trigger antiferromagnetic domain wall motion with a force whose value grows with the temperature of a sample. At a temperature, larger than the energy of the low-frequency magnons, this force is much larger than the force caused by direct spin transfer between the spin current and the domain wall. We also demonstrate that the external spin current can induce the magnon spin Seebeck effect. The corresponding Seebeck coefficient is controlled by the current density. These spin-current assisted caloric effects open new ways for the manipulation of the magnetic states in antiferromagnets.

cond-mat.mes-hall↗

Roles of chiral renormalization on magnetization dynamics in chiral magnets

In metallic ferromagnets, the interaction between local magnetic moments and conduction electrons renormalizes parameters of the Landau-Lifshitz-Gilbert equation such as the gyromagnetic ratio and the Gilbert damping, and makes them dependent on the magnetic configurations. Although the effects of the renormalization for nonchiral ferromagnets are usually minor and hardly detectable, we show that the renormalization does play a crucial role for chiral magnets. Here the renormalization is chiral and as such we predict experimentally identifiable effects on the phenomenology of magnetization dynamics. In particular, our theory for the self-consistent magnetization dynamics of chiral magnets allows for a concise interpretation of domain wall creep motion. We also argue that the conventional creep theory of the domain wall motion, which assumes Markovian dynamics, needs critical reexamination since the gyromagnetic ratio makes the motion non-Markovian. The non-Markovian nature of the domain wall dynamics is experimentally checkable by the chirality of the renormalization.

cond-mat.mes-hall↗

Spin Hall magnetoresistance in antiferromagnet/heavy-metal heterostructures

We investigate the spin Hall magnetoresistance in thin film bilayer heterostructures of the heavy metal Pt and the antiferromagnetic insulator NiO. While rotating an external magnetic field in the easy plane of NiO, we record the longitudinal and the transverse resistivity of the Pt layer and observe an amplitude modulation consistent with the spin Hall magnetoresistance. In comparison to Pt on collinear ferrimagnets, the modulation is phase shifted by 90° and its amplitude strongly increases with the magnitude of the magnetic field. We explain the observed magnetic field-dependence of the spin Hall magnetoresistance in a comprehensive model taking into account magnetic field induced modifications of the domain structure in antiferromagnets. With this generic model we are further able to estimate the strength of the magnetoelastic coupling in antiferromagnets. Our detailed study shows that the spin Hall magnetoresistance is a versatile tool to investigate the magnetic spin structure as well as magnetoelastic effects, even in antiferromagnetic multidomain materials.

cond-mat.mes-hall↗

Part of a collection of reviews on antiferromagnetic spintronics. Antiferromagnetic dynamics, spin-texures, and nanostructures

Antiferromagnets as active elements of spintronics can be faster than their ferromagnetic counterparts and more robust to magnetic noise. Owing to the strongly exchange-coupled magnetic sublattice structure, antiferromagnetic order parameter dynamics are qualitatively different and thus capable of engendering novel device functionalities. In this review, we discuss antiferromagnetic textures -- nanoparticles, domain walls, and skyrmions, -- under the action of different spin torques. We contrast the antiferromagnetic and ferromagnetic dynamics, with a focus on the features that can be relevant for applications.

cond-mat.mes-hall↗

Cross effect of magnetic field and charge current on antiferromagnetic dynamics

We theoretically examine a cross effect of magnetic field and charge current on antiferromagnetic domain wall dynamics. Since antiferromagnetic materials are largely insensitive to external magnetic fields in general, charge current has been shown recently as an alternative and efficient way to manipulate antiferromagnets. We find a new role of the magnetic field in the antiferromagnetic dynamics that appears when it is combined with charge current, demonstrating a domain wall motion in the presence of both field and current. We show that a spatially-varying magnetic field can shift the current-driven domain-wall velocity, depending on the domain-wall structure and the direction of the field-gradient. Our result suggests a novel concept of field-control of current-driven antiferromagnetic dynamics.

cond-mat.mes-hall↗

Manipulating antiferromagnets with magnetic fields: ratchet motion of multiple domain walls induced by asymmetric field pulses

Future applications of antiferromagnets (AFs) in many spintronics devices rely on the precise manipulation of domain walls. The conventional approach using static magnetic fields is inefficient due to the low susceptibility of AFs. Recently proposed electrical manipulation with spin-orbit torques is restricted to metals with a specific crystal structure. Here we propose an alternative, broadly applicable approach: using asymmetric magnetic field pulses to induce controlled ratchet motion of AF domain walls. The efficiency of this approach is based on three peculiarities of AF dynamics. First, a time-dependent magnetic field couples with an AF order parameter stronger than a static magnetic field, which leads to higher mobility of the domain walls. Second, the rate of change of the magnetic field couples with the spatial variation of the AF order parameter inside the domain and this enables synchronous motion of multiple domain walls with the same structure. Third, tailored asymmetric field pulses in combination with static friction can prevent backward motion of domain walls and thus lead to the desired controlled ratchet effect. The proposed use of an external field, rather than internal spin-orbit torques, avoids any restrictions on size, conductivity, and crystal structure of the AF material. We believe that our approach paves a way for the development of new AF-based devices based on controlled motion of AF domain walls.

cond-mat.mtrl-sci↗

Phenomenology of current-induced skyrmion motion in antiferromagnets

We study current-driven skyrmion motion in uniaxial thin film antiferromagnets in the presence of the Dzyaloshinskii-Moriya interactions and in an external magnetic field. We phenomenologically include relaxation and current-induced torques due to both spin-orbit coupling and spatially inhomogeneous magnetic textures in the equation for the Néel vector of the antiferromagnet. Using the collective coordinate approach we apply the theory to a two-dimensional antiferromagnetic skyrmion and estimate the skyrmion velocity under an applied DC electric current.

cond-mat.mes-hall↗

Magnetostriction-induced anisotropy in the exchange biased bilayers

The exchange bias at ferromagnetic/antiferromagnetic interfaces strongly depends upon the state of antiferromagnetic (AF) layer which, due to strong magnetoelastic coupling, is sensitive to mechanical stresses. In the present paper we consider magnetoelastic effects that arise at FM/AF interface due to lattice misfit and magnetic ordering. We show how magnetostriction affects mutual orientation of AF and FM vectors and easy-axis direction in thin AF layer. The results obtained could be used for tailoring exchange biased systems.

cond-mat.mtrl-sci↗