arXiv subjects

Oliver Benson

Publications and source records attributed to Oliver Benson.

At least 19 recordsLinked to original sources

arXiv2026

Engineering Nanodiamonds for Quantum Sensing: Material Constraints at the Nanoscale

Optically addressable solid-state spin defects have emerged as powerful multimodal quantum sensors, with nitrogen-vacancy (NV) centers in bulk diamond providing benchmark quantum control and sensitivity under ambient conditions. Embedding such defects in nanodiamonds (NDs) extends these capabilities to mobile probes capable of accessing complex biological and nanoscale environments. Reduced dimensions, however, introduce constraints beyond volumetric spin impurities, notably enhanced lattice strain and surface-induced noise sources, which shorten NV spin relaxation times (T1 and T2) and destabilize the NV charge state, as well as resulting in pronounced particle-to-particle variability in NDs typically produced by top-down approaches. These effects complicate both sensing performance and the quantitative interpretation of multimodal signals in realistic environments. This article provides a structured perspective on the physical mechanisms by which material properties constrain NV behavior in NDs, together with mitigation strategies that shape the robust use of these mobile quantum sensors for biosensing and nanoscale science.

quant-ph↗

arXiv2026

Optimal stellar rank approximation of squeezed cat states with photon catalysis

Non-Gaussian quantum states and operations constitute essential resources for achieving quantum computational advantage and enabling quantum error correction in bosonic platforms. However, their generation in optical settings remains a challenging experimental task, often relying on probabilistic heralded protocols. Here, we present an in-depth analysis of the suitability of photon catalysis between low number Fock states and squeezed states for the generation of squeezed coherent state superpositions. We employ the stellar rank formalism to characterize the non-Gaussian complexity of input resources (including both states and measurements) and the generated states. This enables a systematic comparison of the fidelity between the catalyzed output and the target states to the maximum fidelity achievable by any protocol with the same non-Gaussian input resources. In this sense, we identify instances where the catalysis protocols considered here are provably optimal. We identify parameter regimes in which high-fidelity approximations of the target states can be achieved with minimal resources. Furthermore, we benchmark the performance of photon catalysis against Gaussian boson sampling-inspired protocols in terms of success probability and state quality, highlighting the advantages of deterministic Fock state sources. We also investigate the generation of related non-Gaussian resources including squeezed Fock states, relevant for quantum error correction. To account for experimental imperfections, we model losses across all optical modes using a Hilbert space truncation approach in the Fock basis and analyze the robustness of the generated states under realistic conditions. Our results quantify the trade-offs between non-Gaussian resource complexity, achievable fidelity, and losses in photon catalysis protocols, providing practical guidelines for near-term photonic implementations.

quant-ph↗

arXiv2025

The QTF-Backbone: Proposal for a Nationwide Optical Fibre Backbone in Germany for Quantum Technology and Time and Frequency Metrology

The recent breakthroughs in the distribution of quantum information and high-precision time and frequency (T&F) signals over long-haul optical fibre networks have transformative potential for physically secure communications, resilience of timing infrastructure (such as that supporting Global Navigation Satellite Systems (GNSS)) and fundamental physics. To date, these capabilities remain confined to isolated testbeds, with quantum and T&F signals accessible, for example in Germany, to only a few institutions. In this white paper we propose the QTF Backbone: a dedicated national fibre-optic infrastructure in Germany for the networked distribution of Quantum and T&F signals using dark fibres and specialised hardware. The QTF Backbone is planned as a four-phase deployment over ten years to ensure scalable, sustainable access for research institutions and industry. The concept builds on successful demonstrations of time and frequency distribution at high Technology Readiness Levels (TRLs) across Europe, including PTB-MPQ links in Germany, REFIMEVE in France, and the Italian LIFT network. The QTF Backbone will enable transformative Research and Development (R&D), support a nationwide QTF ecosystem, and ensure the transition from innovation to deployment. As a national and European hub, it will position Germany and Europe at the forefront of quantum networking, as well as T&F transfer.

physics.ins-det↗

arXiv2025

Light Storage in Light Cages: A Scalable Platform for Multiplexed Quantum Memories

Quantum memories are essential for photonic quantum technologies, enabling long-distance quantum communication and serving as delay units in quantum computing. Hot atomic vapors using electromagnetically induced transparency provide a simple platform with second-long photon storage capabilities. Light-guiding structures enhance performance, but current hollow-core fiber waveguides face significant limitations in filling time, physical size, fabrication versatility, and large-scale integration potential. In this work, we demonstrate the storage of attenuated coherent light pulses in a cesium (Cs) quantum memory based on a 3D-nanoprinted hollow-core waveguide, known as a light cage (LC), with several hundred nanoseconds of storage times. Leveraging the versatile fabrication process, we successfully integrated multiple LC memories onto a single chip within a Cs vapor cell, achieving consistent performance across all devices. We conducted a detailed investigation into storage efficiency, analyzing memory lifetime and bandwidth. These results represent a significant advancement toward spatially multiplexed quantum memories and have the potential to elevate memory integration to unprecedented levels. We anticipate applications in parallel single-photon synchronization for quantum repeater nodes and photonic quantum computing platforms.

quant-ph↗

arXiv2025

Approaching Unity Photon Collection from NV Centers via Ultra-Precise Positioning of Nanodiamonds in Hybrid Nanoantennas

Efficient readout of nitrogen-vacancy (NV) centers in diamond is crucial for various quantum information technologies. However, achieving high-fidelity, single-shot readout at room temperature remains challenging due to limited photon collection efficiency (CE) and background noise. In this work, we enhance the readout efficiency of NV centers by integrating them into hybrid metal-dielectric bullseye nanoantennas using ultra-precise deterministic positioning. This approach enables highly directional emission while minimizing optical losses, resulting in a measured CE of 82\% into a numerical aperture (NA) as low as 0.5, and approaching unity for NA$>$0.8. This marks a substantial improvement over previous realizations using nanodiamonds, highlighting the advantage of combining hybrid nanoantennas with precise positioning. Our results mark a substantial advancement towards efficient single-shot readout of NV centers by significantly improving readout fidelity and efficiency in a simple on-chip configuration.

physics.optics↗

arXiv2025

Low-Noise Cascaded Frequency Conversion of $637.2$ nm Light to the Telecommunication C-Band in a Single-Waveguide Device

Interconnected quantum devices are the building blocks of quantum networks, where state transduction plays a central role. The frequency conversion of photons into the telecommunication C-band is decisive in taking advantage of current low-loss transmission lines. Here, we report the difference frequency conversion of $637.2$ nm fluorescent light from a cluster of NV centers in diamond to tunable wavelengths between $1559.6$ nm and $1565.2$ nm. In order to avoid detrimental noise from spontaneous emissions, we use a two-step conversion device based on a single-pumped periodic poled lithium niobate waveguide. We observed a total external (internal) conversion efficiency of $3.0\pm0.1$ ($20.5\pm0.8$) $\%$ with a noise rate of $2.4\pm0.8$ ($16\pm5$) cps/GHz.

quant-ph↗

arXiv2021

Time-frequency Quantum Key Distribution over a Free-Space Optical Link

We present an implementation of the time-frequency (TF) quantum key distribution (QKD) protocol realized mainly with standard telecommunication components at 1550 nm. TF-QKD is implemented with modulations in time and frequency, namely pulse position modulation (PPM) and frequency shift keying (FSK). The time-frequency uncertainty relation ensures the security of the protocol. We further demonstrate free-space optical QKD transmission over a 388-m distance. Since the QKD setup is single-mode fiber (SMF) -based, precise coupling in and out of the SMFs is crucial. Thus, we implemented an optical tracking system. The QKD signal is wavelength-multiplexed with a strong beacon for optical tracking. Strong spectral filtering is necessary to separate beacon and QKD signal. Together with spatial filtering caused by the SMF most background light is filtered, enabling daylight QKD transmission.

quant-ph↗

arXiv2021

Ground State Microwave-Stimulated Raman Transitions and Adiabatic Spin Transfer in the $^{15}$Nitrogen-Vacancy Center

Microwave pulse sequences are the basis of coherent manipulation of the electronic spin ground state in nitrogen-vacancy (NV) centers. In this work we demonstrate stimulated Raman transitions (SRT) and stimulated Raman adiabatic passage (STIRAP), two ways to drive the dipole-forbidden transition between two spin sublevels in the electronic triplet ground state of the NV center. This is achieved by a multitone Raman microwave pulse which simultaneously drives two detuned transitions via a virtual level for SRT or via two adiabatic and partially overlapping resonant microwave pulses for STIRAP. We lay the theoretical framework of SRT and STIRAP dynamics and verify experimentally the theoretical predictions of population inversion by observing the dipole-forbidden transition in the ground state of a single NV center. A comparison of the two schemes showed a better robustness and success of the spin swap for STIRAP as compared to SRT.

quant-ph↗

arXiv2020

Direct observation of the particle exchange phase of photons

Quantum theory stipulates that if two particles are identical in all physical aspects, the allowed states of the system are either symmetric or antisymmetric with respect to permutations of the particle labels. Experimentally, the symmetry of the states can be inferred indirectly from the fact that neglecting the correct exchange symmetry in the theoretical analysis leads to dramatic discrepancies with the observations. The only way to directly unveil the symmetry of the states for, say, two identical particles is through the interference of the original state and the physically permuted one, and measure the phase associated with the permutation process, the so-called particle exchange phase. Following this idea, we have measured the exchange phase of indistinguishable photons, providing direct evidence of the bosonic character of photons.

quant-ph↗

arXiv2020

Vacuum-Induced Saturation in Plasmonic Nanoparticles

Vacuum fluctuations are a fundamental feature of quantized fields. It is usually assumed that observations connected to vacuum fluctuations require a system well isolated from other influences. In this work, we demonstrate that effects of the quantum vacuum can already occur in simple colloidal nano-assemblies prepared by wet chemistry. We claim that the electromagnetic field fluctuations at the zero-point level saturate the absorption of dye molecules self-assembled at the surface of plasmonic nano-resonators. For this effect to occur, reaching the strong coupling regime between the plasmons and excitons is not required. This intriguing effect of vacuum-induced saturation (VISA) is discussed within a simple quantum optics picture and demonstrated by comparing the optical spectra of hybrid gold-core dye-shell nanorods to electromagnetic simulations.

physics.optics↗

arXiv2020

General and complete description of temporal photon correlations in cavity-enhanced spontaneous parametric down-conversion

Heralded single photon sources are the most commonly used sources for optical quantum technology applications. There is strong demand for accurate prediction of their spectral features and temporal correlations with ever increasing precision. This is particularly important in connection with the intrinsically stochastic photon-pair generation process in heralded sources. Here we present a complete theoretical description of the temporal correlation of a signal-idler, signal-signal and signal-signal-idler coincidences of photons generated by continuous wave pumped cavity-enhanced spontaneous parametric down-conversion. The theory excellently predicts the measurements, which has been experimentally confirmed in our setup utilizing single photon detectors with high temporal resolution. This enables us to resolve and analyze the multi-photon correlation functions in great detail.

quant-ph↗

arXiv2020

Real-time estimation of the optically detected magnetic resonance shift in diamond quantum thermometry

We investigate the real-time estimation protocols for the frequency shift of optically detected magnetic resonance (ODMR) of nitrogen-vacancy (NV) centers in nanodiamonds (NDs). Efficiently integrating multipoint ODMR measurements and ND particle tracking into fluorescence microscopy has recently demonstrated stable monitoring of the temperature inside living animals. We analyze the multipoint ODMR measurement techniques (3-, 4-, and 6-point methods) in detail and quantify the amount of measurement artifact owing to several systematic errors derived from instrumental errors of experimental hardware and ODMR spectral shape. We propose a practical approach to minimize the effect of these factors, which allows for measuring accurate temperatures of single NDs during dynamic thermal events. We also discuss integration of noise filters, data estimation protocols, and possible artifacts for further developments in real-time temperature estimation. The present study provides technical details of quantum diamond thermometry and discusses factors that may affect the temperature estimation in biological applications.

physics.app-ph↗

arXiv2020

A Hahn-Ramsey Scheme for Dynamical Decoupling and DC Magnetometry with Single Solid-State Qubits

Spin systems in solid state materials are promising qubit candidates for quantum information or quantum sensing. A major prerequisite here is the coherence of spin phase oscillations. In this work, we show a control sequence which, by applying RF pulses of variable detuning, allows to increase the spin phase oscillation visibility and to perform DC magnetometry as well. We experimentally demonstrate the scheme on single NV centers in diamond and analytically describe how the NV electron spin phase oscillations behave in the presence of classical noise models. We hereby introduce detuning as the enabling factor that modulates the filter function of the sequence, in order to achieve a visibility of the Ramsey fringes comparable to or longer than the Hahn-echo $T_2$ time and an improved sensitivity to DC magnetic fields in various experimental settings.

quant-ph↗

arXiv2020

An efficient, tunable, and robust source of narrow-band photon pairs at the $^{87}$Rb D1 line

We present an efficient and robust source of photons at the $^{87}$Rb D1-line (795 nm) with a narrow bandwidth of $δ=226(1)$ MHz. The source is based on non-degenerate, cavity-enhanced spontaneous parametric down-conversion in a monolithic optical parametric oscillator far below threshold. The setup allows for efficient coupling to single mode fibers. A heralding efficiency of $η_{\mathrm{heralded}}=45(5)$ % is achieved, and the uncorrected number of detected photon pairs is $3.8 \times 10^{3}/(\textrm{s mW})$. For pair generation rates up to $5\times 10^{5}/$s, the source emits heralded single photons with a normalized, heralded, second-order correlation function $g^{(2)}_{c}<0.01$. The source is intrinsically stable due to the monolithic configuration. Frequency drifts are on the order of $δ/20$ per hour without active feedback on the emission frequency. We achieved fine-tuning of the source frequency within a range of $ > 2$ GHz by applying mechanical strain.

quant-ph↗

arXiv2020

Real-time nanodiamond thermometry probing in-vivo thermogenic responses

Real-time temperature monitoring inside living organisms provides a direct measure of their biological activities, such as homeostatic thermoregulation and energy metabolism. However, it is challenging to reduce the size of bio-compatible thermometers down to submicrometers despite their potential applications for the thermal imaging of subtissue structures with single-cell resolution. Light-emitting nanothermometers that remotely sense temperature via optical signals exhibit considerable potential in such \textit{in-vivo} high-spatial-resolution thermometry. Here, using quantum nanothermometers based on optically accessible electron spins in nanodiamonds (NDs), we demonstrate \textit{in-vivo} real-time temperature monitoring inside \textit{Caenorhabditis elegans} (\textit{C. elegans}) worms. We developed a thermometry system that can measure the temperatures of movable NDs inside live adult worms with a precision of $\pm 0.22^{\circ}{\rm C}$. Using this system, we determined the increase in temperature based on the thermogenic responses of the worms during the chemical stimuli of mitochondrial uncouplers. Our technique demonstrates sub-micrometer localization of real-time temperature information in living animals and direct identification of their pharmacological thermogenesis. The results obtained facilitate the development of a method to probe subcellular temperature variation inside living organisms and may allow for quantification of their biological activities based on their energy expenditures.

q-bio.QM↗

arXiv2019

Extending Quantum Links: Modules for Fiber- and Memory-Based Quantum Repeaters

We analyze elementary building blocks for quantum repeaters based on fiber channels and memory stations. Implementations are considered for three different physical platforms, for which suitable components are available: quantum dots, trapped atoms and ions, and color centers in diamond. We evaluate and compare the performances of basic quantum repeater links for these platforms both for present-day, state-of-the-art experimental parameters as well as for parameters that could in principle be reached in the future. The ultimate goal is to experimentally explore regimes at intermediate distances, up to a few 100 km, in which the repeater-assisted secret key transmission rates exceed the maximal rate achievable via direct transmission. We consider two different protocols, one of which is better adapted to the higher source clock rate and lower memory coherence time of the quantum dot platform, while the other circumvents the need of writing photonic quantum states into the memories in a heralded, non-destructive fashion. The elementary building blocks and protocols can be connected in a modular form to construct a quantum repeater system that is potentially scalable to large distances.

quant-ph↗

arXiv2019

On-Chip Integration of Single Solid-State Quantum Emitters with a SiO$_2$ Photonic Platform

One important building block for future integrated nanophotonic devices is the scalable on-chip interfacing of single photon emitters and quantum memories with single optical modes. Here we present the deterministic integration of a single solid-state qubit, the nitrogen-vacancy (NV) center, with a photonic platform consisting exclusively of SiO$_2$ grown thermally on a Si substrate. The platform stands out by its ultra-low fluorescence and the ability to produce various passive structures such as high-Q microresonators and mode-size converters. By numerical analysis an optimal structure for the efficient coupling of a dipole emitter to the guided mode could be determined. Experimentally, the integration of a preselected NV emitter was performed with an atomic force microscope and the on-chip excitation of the quantum emitter as well as the coupling of single photons to the guided mode of the integrated structure could be demonstrated. Our approach shows the potential of this platform as a robust nanoscale interface of on-chip photonic structures with solid-state qubits.

physics.optics↗

arXiv2019

Slow and fast light behavior of single photons from a quantum dot interacting with the excited state hyperfine structure of the Cesium D1-line

Hybrid interfaces between distinct quantum systems play a major role in the implementation of quantum networks. Quantum states have to be stored in memories to synchronize the photon arrival times for entanglement swapping by projective measurements in quantum repeaters or for entanglement purification. Here, we analyze the distortion of a single photon wave packet propagating through a dispersive and absorptive medium with high spectral resolution. Single photons are generated from a single In(Ga)As quantum dot with its excitonic transition precisely set relative to the Cesium D1 transition. The delay of spectral components of the single photon wave packet with almost Fourier-limited width is investigated in detail with a 200 MHz narrow-band monolithic Fabry-Pérot resonator. Reflecting the excited state hyperfine structure of Cesium, "slow light" and "fast light" behavior is observed. As a step towards room-temperature alkali vapor memories, quantum dot photons are delayed for 5 ns by strong dispersion between the two 1.17 GHz hyperfine-split excited state transitions. Based on optical pumping on the hyperfine-split ground states, we propose a simple, all-optically controllable delay for synchronization of heralded narrow-band photons in a quantum network.

quant-ph↗