arXiv subjects

Oliver G. Schmidt

Publications and source records attributed to Oliver G. Schmidt.

At least 37 records · Page 2Linked to original sources

arXiv2019

Real-time optoacoustic tracking of single moving micro-objects in deep tissue-mimicking phantoms

Medical imaging plays an important role in diagnosis and treatment of multiple diseases. It is a field under continuous development which seeks for improved sensitivity and spatiotemporal resolution to allow the dynamic monitoring of diverse biological processes that occur at the micro- and nanoscale. Emerging technologies for targeted diagnosis and therapy such as nanotherapeutics, micro-implants, catheters and small medical tools also need to be precisely located and monitored while performing their function inside the human body. In this work, we show for the first time the real-time tracking of moving single micro-objects below centimeter thick tissue-mimicking phantoms, using multispectral optoacoustic tomography (MSOT). This technique combines the advantages of ultrasound imaging regarding depth and resolution with the molecular specificity of optical methods, thereby facilitating the discrimination between the spectral signatures of the micro-objects from those of intrinsic tissue molecules. The resulting MSOT signal is further improved in terms of contrast and specificity by coating the micro-objects surface with gold nanorods, possessing a unique absorption spectrum, which will allow their discrimination from surrounding biological tissues when translated to in vivo settings.

physics.med-ph↗

arXiv2019

Slow and fast light behavior of single photons from a quantum dot interacting with the excited state hyperfine structure of the Cesium D1-line

Hybrid interfaces between distinct quantum systems play a major role in the implementation of quantum networks. Quantum states have to be stored in memories to synchronize the photon arrival times for entanglement swapping by projective measurements in quantum repeaters or for entanglement purification. Here, we analyze the distortion of a single photon wave packet propagating through a dispersive and absorptive medium with high spectral resolution. Single photons are generated from a single In(Ga)As quantum dot with its excitonic transition precisely set relative to the Cesium D1 transition. The delay of spectral components of the single photon wave packet with almost Fourier-limited width is investigated in detail with a 200 MHz narrow-band monolithic Fabry-Pérot resonator. Reflecting the excited state hyperfine structure of Cesium, "slow light" and "fast light" behavior is observed. As a step towards room-temperature alkali vapor memories, quantum dot photons are delayed for 5 ns by strong dispersion between the two 1.17 GHz hyperfine-split excited state transitions. Based on optical pumping on the hyperfine-split ground states, we propose a simple, all-optically controllable delay for synchronization of heralded narrow-band photons in a quantum network.

quant-ph↗

arXiv2019

Entanglement Swapping with Semiconductor-generated Photons

Transferring entangled states between photon pairs is essential for quantum communication technologies. Semiconductor quantum dots are the most promising candidate for generating polarization-entangled photons deterministically. Recent improvements in photonic quality and brightness now make them suited for complex quantum optical purposes in practical devices. Here we demonstrate for the first time swapping of entangled states between two pairs of photons emitted by a single quantum dot. A joint Bell measurement heralds the successful generation of the Bell state $Ψ^+$ with a fidelity of up to $0.81 \pm 0.04$. The state's nonlocal nature is confirmed by violating the CHSH-Bell inequality. Our photon source is compatible with atom-based quantum memories, enabling implementation of hybrid quantum repeaters. This experiment thus is a major step forward for semiconductor based quantum communication technologies.

quant-ph↗

arXiv2018

Uniaxial stress flips the natural quantization axis of a quantum dot for integrated quantum photonics

The optical selection rules in epitaxial quantum dots are strongly influenced by the orientation of their natural quantization axis, which is usually parallel to the growth direction. This configuration is well suited for vertically emitting devices, but not for planar photonic circuits because of the poorly controlled orientation of the transition dipoles in the growth plane. Here we show that the quantization axis of gallium arsenide dots can be flipped into the growth plane via moderate in plane uniaxial stress. By using piezoelectric strain actuators featuring strain-amplification we study the evolution of the selection rules and excitonic fine-structure in a regime, in which quantum confinement can be regarded as a perturbation compared to strain in determining the symmetry properties of the system. The experimental and computational results suggest that uniaxial stress, may be the right tool to obtain quantum light sources with ideally oriented transition dipoles and enhanced oscillator strengths for integrated quantum photonics.

quant-ph↗

arXiv2018

Topological phase transition in a stretchable photonic crystal

We design a setup to realize tunable topological phases in elastic photonic crystals. Using the Su-Schrieffer-Heeger (SSH) model as a canonical example, we show how a system can be continuously tuned across its topological phase transition by stretching. We examine the setup both analytically and numerically, showing how the phase transition point may be identified from the behavior of bulk modes. Our design principle is generic as it can be applied to a variety of systems, and enables multiple new theoretical predictions to be experimentally tested by continuously strain-tuning system properties, such as the shape of the bandstructure and the topological invariant. In addition, it allows for cost-effective device fabrication, since a wide range of parameter space can be accessed on a single photonic crystal chip.

cond-mat.mes-hall↗

arXiv2018

Tuning emission energy and fine structure splitting in quantum dots emitting in the telecom O-band

We report on optical investigations of MOVPE-grown InGaAs/GaAs quantum dots emitting at the telecom O-band that were integrated onto uniaxial piezoelectric actuators. This promising technique, which does not degrade the optical quality or performances of the quantum emitters, enables us to tune the quantum dot emission wavelengths and their fine-structure splitting. By spectrally analyzing the emitted light with respect to its polarization, we are able to demonstrate the cancelation of the fine structure splitting within the experimental resolution limit. This work represents an important step towards the high-yield generation of entangled photon pairs at telecommunication wavelength, together with the capability to precisely tune the emission to target wavelengths.

cond-mat.mes-hall↗

arXiv2018

Coupling a single solid state quantum emitter to an array of resonant plasmonic antennas

Plasmon resonant arrays or meta-surfaces shape both the incoming optical field and the local density of states for emission processes. They provide large regions of enhanced emission from emitters and greater design flexibility than single nanoantennas. This makes them of great interest for engineering optical absorption and emission. Here we study the coupling of a single quantum emitter, a self-assembled semiconductor quantum dot, to a plasmonic meta-surface. We investigate the influence of the spectral properties of the nanoantennas and the position of the emitter in the unit cell of the structure. We observe a resonant enhancement due to emitter-array coupling in the far-field regime and find a clear difference from the interaction of an emitter with a single antenna.

physics.optics↗

arXiv2017

Frequency Feedback for Two-Photon Interference from Separate Quantum Dots

We employ active feedback to stabilize the frequency of single photons emitted by two separate quantum dots to an atomic standard. The transmission of a single, rubidium-based Faraday filter serves as the error signal for frequency stabilization to less than 1.5% of the emission linewidth. Long-term stability is demonstrated by Hong-Ou-Mandel interference between photons from the two quantum dots. The observed visibility of $V_{\mathrm{lock}}=(41 \pm 5)$% is limited only by internal dephasing of the dots. Our approach facilitates quantum networks with indistinguishable photons from distributed emitters.

quant-ph↗

arXiv2017

Multiharmonic frequency-chirped transducers for surface-acoustic-wave optomechanics

Wide passband interdigital transducers are employed to establish a stable phase-lock between a train of laser pulses emitted by a mode-locked laser and a surface acoustic wave generated electrically by the transducer. The transducer design is based on a multi-harmonic split-finger architecture for the excitation of a fundamental surface acoustic wave and a discrete number of its overtones. Simply by introducing a variation of the transducer's periodicity $p$, a frequency chirp is added. This combination results in wide frequency bands for each harmonic. The transducer's conversion efficiency from the electrical to the acoustic domain was characterized optomechanically using single quantum dots acting as nanoscale pressure sensors. The ability to generate surface acoustic waves over a wide band of frequencies enables advanced acousto-optic spectroscopy using mode-locked lasers with fixed repetition rate. Stable phase-locking between the electrically generated acoustic wave and the train of laser pulses was confirmed by performing stroboscopic spectroscopy on a single quantum dot at a frequency of 320 MHz. Finally, the dynamic spectral modulation of the quantum dot was directly monitored in the time domain combining stable phase-locked optical excitation and time-correlated single photon counting. The demonstrated scheme will be particularly useful for the experimental implementation of surface acoustic wave-driven quantum gates of optically addressable qubits or collective quantum states or for multi-component Fourier synthesis of tailored nanomechanical waveforms.

physics.app-ph↗

arXiv2017

On-demand semiconductor source of 780 nm single photons with controlled temporal wave packets

We report on a fast, bandwidth-tunable single-photon source based on an epitaxial GaAs quantum dot. Exploiting spontaneous spin-flip Raman transitions, single photons at $780\,$nm are generated on-demand with tailored temporal profiles of durations exceeding the intrinsic quantum dot lifetime by up to three orders of magnitude. Second-order correlation measurements show a low multi-photon emission probability ($g^{2}(0)\sim\,0.10-0.15$) at a generation rate up to $10\,$MHz. We observe Raman photons with linewidths as low as $200\,$MHz, narrow compared to the $1.1\,$GHz linewidth measured in resonance fluorescence. The generation of such narrow-band single photons with controlled temporal shapes at the rubidium wavelength is a crucial step towards the development of an optimized hybrid semiconductor-atom interface.

quant-ph↗

arXiv2017

Superconducting Micro- and Nanohelices

Superconducting micro- and nanohelices are proposed for the first time. A theoretical investigation of the superconducting state in the helical coils at the micro- and nanoscale is performed within the time-dependent Ginzburg-Landau approach. The pattern and number of vortices in a stationary distribution are determined by their confinement to the ultrathin helical spiral and can therefore be efficiently controlled by the helical stripe width and the helical pitch distance for both dense and sparse helices. Quasi-degeneracy of vortex patterns is manifested in the helical spiral when the number of vortices is incommensurable with the total number of half-turns. With increasing radius, superconducting helical spirals provide a physical realization of a transition from the vortex pattern peculiar to an open tube to that of a planar stripe.

cond-mat.supr-con↗

arXiv2017

Sperm-hybrid micromotor for drug delivery in the female reproductive tract

A sperm-driven micromotor is presented as cargo-delivery system for the treatment of gynecological cancers. This particular hybrid micromotor is appealing to treat diseases in the female reproductive tract, the physiological environment that sperm cells are naturally adapted to swim in. Here, the single sperm cell serves as an active drug carrier and as driving force, taking advantage of its swimming capability, while a laser-printed microstructure coated with a nanometric layer of iron is used to guide and release the sperm in the desired area by an external magnet and structurally imposed mechanical actuation, respectively. The printed tubular microstructure features four arms which release the drug-loaded sperm cell in situ when they bend upon pushing against a tumor spheroid, resulting in the drug delivery, which occurs when the sperm squeezes through the cancer cells and fuses with cell membrane. Sperms also offer higher drug encapsulation capability and carrying stability compared to other nano and microcarriers, minimizing toxic effects and unwanted drug accumulation. Moreover, sperms neither express pathogenic proteins nor proliferate to form undesirable colonies, unlike other cells or microorganisms do, making this bio-hybrid system a unique and biocompatible cargo delivery platform for various biomedical applications, especially in gynecological healthcare.

physics.med-ph↗

arXiv2016

A quantum plasmonic nanocircuit on a semiconductor platform

Quantum photonics holds great promise for future technologies such as secure communication, quantum computation, quantum simulation, and quantum metrology. An outstanding challenge for quantum photonics is to develop scalable miniature circuits that integrate single-photon sources, linear optical components, and detectors on a chip. Plasmonic nanocircuits will play essential roles in such developments. Plasmonic components feature ultracompact geometries and can be controlled more flexibly and more energy-efficiently compared to conventional dielectric components due to strong field confinement and enhancement. Moreover, plasmonic components are compatible with electronic circuits, thanks to their deep subwavelength sizes as well as their electrically conducting materials. However, for quantum plasmonic circuits, integration of stable, bright, and narrow-band single photon sources in the structure has so far not been reported. Here we present a quantum plasmonic nanocircuit driven by a self-assembled GaAs quantum dot. The quantum dot efficiently excites narrow-band single plasmons that are guided in a two-wire transmission line until they are converted into single photons by an optical antenna. Our work demonstrates the feasibility of fully on-chip plasmonic nanocircuits for quantum optical applications.

physics.optics↗

arXiv2016

Electrically-Pumped Wavelength-Tunable GaAs Quantum Dots Interfaced with Rubidium Atoms

We demonstrate the first wavelength-tunable electrically-pumped source of non-classical light that can emit photons with wavelength in resonance with the D2 transitions of 87Rb atoms. The device is fabricated by integrating a novel GaAs single-quantum-dot light-emitting-diode (LED) onto a piezoelectric actuator. By feeding the emitted photons into a 75-mm-long cell containing warm 87Rb atom vapor, we observe slow-light with a temporal delay of up to 3.4 ns. In view of the possibility of using 87Rb atomic vapors as quantum memories, this work makes an important step towards the realization of hybrid-quantum systems for future quantum networks.

cond-mat.mes-hall↗

arXiv2016

Topology induced anomalous plasmon modes in metallic Mobius nanorings

We report on the investigation of plasmonic resonances in metallic Möbius nanorings. Half-integer numbers of resonant modes are observed due to the presence of an extra phase π provided by the topology of the Möbius nanostrip. Anomalous plasmon modes located at the non-orientable surface of the Möbius nanoring break the symmetry that exist in conventional ring cavities, thus enable far-field excitation and emission as bright modes. The far-field resonant wavelength as well as the feature of half-integer mode numbers is invariant to the change of charge distribution on the Möbius nanoring due to the nontrivial topology. Owing to the ultra-small mode volume induced by the remaining dark feature, an extremely high sensitivity as well as a remarkable figure of merit is obtained in sensing performance. The topological metallic nanostructure provides a novel platform for the investigation of localized surface plasmon modes exhibiting unique phenomena in plasmonic applications such as high sensitive detection and plasmonic nanolasers.

physics.optics↗

arXiv2016

Purely Antiferromagnetic Magnetoelectric Random Access Memory

Magnetic random access memory schemes employing magnetoelectric coupling to write binary information promise outstanding energy efficiency. We propose and demonstrate a purely antiferromagnetic magnetoelectric random access memory (AF-MERAM) that offers a remarkable 50 fold reduction of the writing threshold compared to ferromagnet-based counterparts, is robust against magnetic disturbances and exhibits no ferromagnetic hysteresis losses. Using the magnetoelectric antiferromagnet Cr2O3, we demonstrate reliable isothermal switching via gate voltage pulses and all-electric readout at room temperature. As no ferromagnetic component is present in the system, the writing magnetic field does not need to be pulsed for readout, allowing permanent magnets to be used. Based on our prototypes of these novel systems, we construct a comprehensive model of the magnetoelectric selection mechanism in thin films of magnetoelectric antiferromagnets. We identify that growth induced effects lead to emergent ferrimagnetism, which is detrimental to the robustness of the storage. After pinpointing lattice misfit as the likely origin, we provide routes to enhance or mitigate this emergent ferrimagnetism as desired. Beyond memory applications, the AF-MERAM concept introduces a general all-electric interface for antiferromagnets and should find wide applicability in purely antiferromagnetic spintronics devices.

cond-mat.mes-hall↗

arXiv2016

Solid-state ensemble of highly entangled photon sources at rubidium atomic transitions

Semiconductor InAs/GaAs quantum dots grown by the Stranski-Krastanov method are among the leading candidates for the deterministic generation of polarization entangled photon pairs. Despite remarkable progress in the last twenty years, many challenges still remain for this material, such as the extremely low yield (<1% quantum dots can emit entangled photons), the low degree of entanglement, and the large wavelength distribution. Here we show that, with an emerging family of GaAs/AlGaAs quantum dots grown by droplet etching and nanohole infilling, it is possible to obtain a large ensemble (close to 100%) of polarization-entangled photon emitters on a wafer without any post-growth tuning. Under pulsed resonant two-photon excitation, all measured quantum dots emit single pairs of entangled photons with ultra-high purity, high degree of entanglement (fidelity up to F=0.91, with a record high concurrence C=0.90), and ultra-narrow wavelength distribution at rubidium transitions. Therefore, a solid-state quantum repeater - among many other key enabling quantum photonic elements - can be practically implemented with this new material.

quant-ph↗

arXiv2016

Highly indistinguishable and strongly entangled photons from symmetric GaAs quantum dots

The development of scalable sources of non-classical light is fundamental to unlock the technological potential of quantum photonics\cite{Kimble:Nat2008}. Among the systems under investigation, semiconductor quantum dots are currently emerging as near-optimal sources of indistinguishable single photons. However, their performances as sources of entangled-photon pairs are in comparison still modest. Experiments on conventional Stranski-Krastanow InGaAs quantum dots have reported non-optimal levels of entanglement and indistinguishability of the emitted photons. For applications such as entanglement teleportation and quantum repeaters, both criteria have to be met simultaneously. In this work, we show that this is possible focusing on a system that has received limited attention so far: GaAs quantum dots grown via droplet etching. Using a two-photon resonant excitation scheme, we demonstrate that these quantum dots can emit triggered polarization-entangled photons with high purity (g^(2)(0)=0.002 +/-0.002), high indistinguishability (0.93 +/-0.07) and high entanglement fidelity (0.94 +/-0.01). Such unprecedented degree of entanglement, which in contrast to InGaAs can theoretically reach near-unity values, allows Bell's inequality (2.64 +/-0.01) to be violated without the aid of temporal or spectral filtering. Our results show that if quantum-dot entanglement resources are to be used for future quantum technologies, GaAs might be the system of choice.

quant-ph↗