arXiv subjects

Oliver G. Schmidt

Publications and source records attributed to Oliver G. Schmidt.

At least 55 records · Page 3Linked to original sources

arXiv2016

Hybridization of photon-plasmon modes in metal-coated microtubular cavities

The coupling of resonant light and surface plasmons in metal layer coated optical microcavities results in the formation of hybrid photon-plasmon modes. Here, we comprehensively investigate the hybridization mechanism of photon-plasmon modes based on opto-plasmonic microtubular cavities. By changing the cavity structure and the metal layer thickness, weakly, moderately and strongly hybridized resonant modes are demonstrated depending on the photon-plasmon coupling strength. An effective potential approach is applied to illustrate the hybridization of photon-plasmon modes relying on the competition between light confinement by the cavity wall and the potential barrier introduced by the metal layer. Our work reveals the basic physical mechanisms for the generation of hybrid modes in metal-coated whispering-gallery-mode microcavities, and is of importance for the study of enhanced light-matter interactions and potential sensing applications.

physics.optics↗

arXiv2016

Electric-field-induced energy tuning of on-demand entangled-photon emission from self-assembled quantum dots

The scalability of quantum dot based non-classical light sources relies on the control over their dissimilar emission energies. Electric fields offer a promising route to tune the quantum dot emission energy through the quantum-confined Stark effect. However, electric fields have been mostly used for tuning the energy of single-photon emission from quantum dots, while electrical control over the energy of entangled-photon emission, which is crucial for building a solid-state quantum repeater using indistinguishable entangled photons, has not been realized yet. Here, we present a method to achieve electrical control over the energy of entangled-photon emission from quantum dots. The device consists of an electrically-tunable quantum diode integrated onto a piezoactuator. We find that, through application of a vertical electric field, the critical uniaxial stress used to eliminate the fine-structure-splitting of quantum dots can be linearly tuned. This allows realization of a triggered source of energy-tunable entangled-photon emission, an important step towards a solid-state quantum repeater application.

physics.optics↗

arXiv2016

Localized surface plasmons selectively coupled to resonant light in tubular microcavities

Vertical gold-nanogaps are created on microtubular cavities to explore the coupling between resonant light supported by the microcavities and surface plasmons localized at the nanogaps. Selective coupling of optical axial modes and localized surface plasmons critically depends on the exact location of the gold-nanogap on the microcavities which is conveniently achieved by rolling-up specially designed thin dielectric films into three dimensional microtube ring resonators. The coupling phenomenon is explained by a modified quasi-potential model based on perturbation theory. Our work reveals the coupling of surface plasmon resonances localized at the nanoscale to optical resonances confined in microtubular cavities at the microscale, implying a promising strategy for the investigation of light-matter interactions.

physics.optics↗

arXiv2016

An artificial Rb atom in a semiconductor with lifetime-limited linewidth

We report results important for the creation of a best-of-both-worlds quantum hybrid system consisting of a solid-state source of single photons and an atomic ensemble as quantum memory. We generate single photons from a GaAs quantum dot (QD) frequency-matched to the Rb D2-transitions and then use the Rb transitions to analyze spectrally the quantum dot photons. We demonstrate lifetime-limited QD linewidths (1.48 GHz) with both resonant and non-resonant excitation. The QD resonance fluorescence in the low power regime is dominated by Rayleigh scattering, a route to match quantum dot and Rb atom linewidths and to shape the temporal wave packet of the QD photons. Noise in the solid-state environment is relatively benign: there is a blinking of the resonance fluorescence at MHz rates but negligible upper state dephasing of the QD transition. We therefore establish a close-to-ideal solid-state source of single photons at a key wavelength for quantum technologies.

quant-ph↗

arXiv2016

Fourier synthesis of radio frequency nanomechanical pulses with different shapes

The concept of Fourier synthesis is heavily employed in both consumer electronic products and fundamental research. In the latter, pulse shaping is key to dynamically initialize, probe and manipulate the state of classical or quantum systems. In nuclear magnetic resonance, for instance, shaped pulses have a long-standing tradition and the underlying fundamental concepts have subsequently been successfully extended to optical frequencies and even to implement quantum gate operations. Transferring these paradigms to nanomechanical systems requires tailored nanomechanical waveforms. Here, we report on an additive Fourier synthesizer for nanomechanical waveforms based on monochromatic surface acoustic waves. As a proof of concept, we electrically synthesize four different elementary nanomechanical waveforms from a fundamental surface acoustic wave at $ f_1 \sim 150$ MHz using a superposition of up to three discrete harmonics $f_n$. We employ these shaped pulses to interact with an individual sensor quantum dot and detect their deliberately and temporally modulated strain component via the opto-mechanical quantum dot response. Importantly, and in contrast to the direct mechanical actuation by bulk piezoactuators, surface acoustic waves provide much higher frequencies (> 20 GHz) to resonantly drive mechanical motion. Thus, our technique uniquely allows coherent mechanical control of localized vibronic modes of optomechanical crystals, even in the quantum limit when cooled to the vibrational ground state.

cond-mat.mes-hall↗

arXiv2015

Energy-tunable entangled photon sources on a III-V/Silicon chip

Many of the envisioned quantum photonic technologies, e.g. a quantum repeater, rely on an energy- (wavelength-) tunable source of polarization entangled photon pairs. The energy tunability is a fundamental requirement to perform two-photon-interference between different sources and to swap the entanglement. Parametric-down-conversion and four-wave-mixing sources of entangled photons have shown energy tunability, however the probabilistic nature of the sources limits their applications in complex quantum protocols. Here we report a silicon-based hybrid photonic chip where energy-tunable polarization entangled photons are generated by deterministic and scalable III-V quantum light sources. This device is based on a micro-electromechanical system (MEMS) incorporating InAs/GaAs quantum dots (QDs) on a PMNPT-on-silicon substrate. The entangled photon emissions from single QDs can be tuned by more than 3000 times of the radiative linewidth without spoiling the entanglement. With a footprint of several hundred microns, our design facilitates the miniaturization and scalable integration of indistinguishable entangled photon sources on silicon. When interfaced with silicon-based quantum photonic circuits, this device will offer a vast range of exciting possibilities.

cond-mat.mes-hall↗

arXiv2015

Scalable Sources of Entangled Photons with Wavelength on Demand

The prospect of using the quantum nature of light for secure communication keeps spurring the search and investigation of suitable sources of entangled-photons. Semiconductor quantum dots are arguably the most attractive. They can generate indistinguishable entangled-photons deterministically, and are compatible with current photonic-integration technologies, a set of properties not shared by any other entanglement resource. However, as no two quantum dots are identical, they emit entangled-photons with random energies. This hinders their exploitation in communication protocols requiring entangled-states with well-defined energies. Here, we introduce scalable quantum-dot-based sources of polarization-entangled-photons whose energy can be controlled via dynamic strain-engineering without degrading the degree of entanglement of the source. As a test-bench, we interface quantum dots with clouds of atomic vapours, and we demonstrate slow-entangled-photons from a single quantum emitter. These results pave the way towards the implementation of hybrid quantum networks where entanglement is distributed among distant parties using scalable optoelectronic devices.

cond-mat.mes-hall↗

arXiv2015

Electron and nuclear spin properties of the nanohole-filled GaAs/AlGaAs quantum dots

GaAs/AlGaAs quantum dots grown by in-situ droplet etching and nanohole infilling offer a combination of strong charge confinement, optical efficiency, and spatial symmetry required for polarization entanglement and spin-photon interface. Here we study spin properties of such dots. We find nearly vanishing electron $g$-factor ($g_e<0.05$), providing a route for electrically driven spin control schemes. Optical manipulation of the nuclear spin environment is demonstrated with nuclear spin polarization up to $60\%$ achieved. NMR spectroscopy reveals the structure of two types of quantum dots and yields the small magnitude of residual strain $ε_b<0.02\%$ which nevertheless leads to long nuclear spin lifetimes exceeding 1000 s. The stability of the nuclear spin environment is advantageous for applications in quantum information processing.

cond-mat.mes-hall↗

arXiv2015

Nonlinear surface magneto-plasmonics in Kretschmann multilayers

The nonlinear magneto-plasmonics aims to utilize plasmonic excitations to control the mechanisms and taylor the efficiencies of the non-linear light frequency conversion at the nanoscale. We investigate the mechanisms of magnetic second harmonic generation in hybrid gold-cobalt-silver multilayer structures, which support propagating surface plasmon polaritons at both fundamental and second harmonic frequencies. Using magneto-optical spectroscopy in Kretschmann geometry, we show that the huge magneto-optical modulation of the second harmonic intensity is dominated by the excitation of surface plasmon polaritons at the second harmonic frequency, as shown by tuning the optical wavelength over the spectral region of strong plasmonic dispersion. Our proof-of-principle experiment highlights bright prospects of nonlinear magneto-plasmonics and contributes to the general understanding of the nonlinear optics of magnetic surfaces and interfaces.

physics.optics↗

arXiv2015

Vertical optical ring resonators fully integrated with nanophotonic waveguides on silicon-on-insulator substrates

We demonstrate full integration of vertical optical ring resonators with silicon nanophotonic waveguides on silicon-on-insulator substrates to accomplish a significant step towards 3D photonic integration. The on-chip integration is realized by rolling up 2D differentially strained TiO2 nanomembranes into 3D microtube cavities on a nanophotonic microchip. The integration configuration allows for out of plane optical coupling between the in-plane nanowaveguides and the vertical microtube cavities as a compact and mechanically stable optical unit, which could enable refined vertical light transfer in 3D stacks of multiple photonic layers. In this vertical transmission scheme, resonant filtering of optical signals at telecommunication wavelengths is demonstrated based on subwavelength thick walled microcavities. Moreover, an array of microtube cavities is prepared and each microtube cavity is integrated with multiple waveguides which opens up interesting perspectives towards parallel and multi-routing through a single cavity device as well as high-throughput optofluidic sensing schemes.

physics.optics↗

arXiv2015

Atomic Clouds as Spectrally-Selective and Tunable Delay Lines for Single Photons from Quantum Dots

We demonstrate a compact, spectrally-selective, and tunable delay line for single photons emitted by quantum dots. This is achieved by fine-tuning the wavelength of the optical transitions of such "artificial atoms" into a spectral window in which a cloud of natural atoms behaves as slow-light medium. By employing the ground-state fine-structure-split exciton confined in an InGaAs/GaAs quantum dot as a source of single photons at different frequencies and the hyperfine-structure-split $D_1$ transition of Cs-vapors as a tunable delay-medium, we achieve a differential delay of up 2.4 ns on a 7.5 cm long path for photons that are only 60 μeV (14.5 GHz) apart. To quantitatively explain the experimental data we develop a theoretical model that accounts for both the inhomogeneously broadening of the quantum-dot emission lines and the Doppler-broadening of the atomic lines. The concept we proposed here may be used to implement time-reordering operations aimed at erasing the "which-path" information that deteriorates entangled-photon emission from excitons with finite fine-structure-splitting.

cond-mat.mes-hall↗

arXiv2015

Strain-tunable entangled-light-emitting diodes with high yield and fast operation speed

Triggered sources of entangled photons play crucial roles in almost any existing protocol of quantum information science. The possibility to generate these non-classical states of light with high speed and using electrical pulses could revolutionize the field. Entangled-light-emitting-diodes (ELEDs) based on semiconductor quantum dots (QDs) are at present the only devices that can address this task 5. However, ELEDs are plagued by a source of randomness that hampers their practical exploitation in the foreseen applications: the very low probability (~10-2) of finding QDs with sufficiently small fine-structure-splitting for entangled-photon-generation. Here, we overcome this hurdle by introducing the first strain-tunable ELEDs (S-ELEDs) that exploit piezoelectric-induced strains to tune QDs for entangled-photon-generation. We demonstrate that up to 30% of the QDs in S-ELEDs emit polarization-entangled photon pairs with entanglement-fidelities as high as f+ = 0.83(5). Driven at the highest operation speed of 400 MHz ever reported so far, S-ELEDs emerge as unique devices for high-data rate entangled-photon applications.

quant-ph↗

arXiv2015

Pseudo-ballistic transport in 3D topological insulator quantum wires

Quantum conductance fluctuations are investigated in disordered 3D topological insulator quantum wires. Both experiments and theory reveal a new transport regime in a mesoscopic conductor, pseudo-ballistic transport, for which ballistic properties persist beyond the transport mean free path, characteristic of diffusive transport. It results in non-universal conductance fluctuations due to quasi-1D surface modes, as observed in long and narrow Bi$_2$Se$_3$ nanoribbons. Spin helical Dirac fermions in quantum wires retain pseudo-ballistic properties over an unusually broad energy range, due to strong quantum confinement and weak momentum scattering.

cond-mat.mes-hall↗

arXiv2014

Magnetochiral symmetry breaking in a Möbius ring

We show that the interaction of the magnetic subsystem of a curved magnet with the magnet curvature results in coupling of a topologically nontrivial magnetization pattern and topology of the object. The mechanism of this coupling is explored and illustrated by an example of ferromagnetic Möbius ring, where a topologically induced domain wall appears as a ground state in case of strong easy-normal anisotropy. For the Möbius geometry the curvilinear form of the exchange interaction produces an additional effective Dzyaloshinskii-like term which leads to the coupling of the magnetochirality of the domain wall and chirality of the Möbius ring. Two types of domain walls are found, transversal and longitudinal, which are oriented across and along the Möbius ring, respectively. In both cases the effect of magnetochirality symmetry breaking is established. The dependence of the ground state of the Möbius ring on its geometrical parameters and on the value of the easy-normal anisotropy is explored numerically.

cond-mat.mes-hall↗

arXiv2014

Experimental realization of coexisting states of rolled-up and wrinkled nanomembranes by strain and etching control

Self-positioned nanomembranes such as rolled-up tubes and wrinkled thin films have been potential systems for a variety of applications and basic studies on elastic properties of nanometer-thick systems. Although there is a clear driving force towards elastic energy 1 minimization in each system, the exploration of intermediate states where specific characteristics could be chosen by a slight modification of a processing parameter had not been experimentally realized. In this work, arrays of freestanding III-V nanomembranes (NM) supported on one edge and presenting a coexistence of these two main behaviors were obtained by design of strain conditions in the NMs and controlled selective etching of patterned substrates. As the etching process continues a mixture of wrinkled and rolled-up states is achieved. For very long etching times an onset of plastic cracks was observed in the points with localized stress. The well- defined morphological periodicity of the relaxed NMs was compared with finite element simulations of their elastic relaxation. The evolution of strain in the NMs with etching time was directly evaluated by X-ray diffraction, providing a comprehensive scenario of transitions among competing and coexisting strain states.

cond-mat.mes-hall↗

arXiv2014

Highly entangled photons from hybrid piezoelectric-semiconductor quantum dot devices

Entanglement resources are key ingredients of future quantum technologies. If they could be efficiently integrated into a semiconductor platform a new generation of devices could be envisioned, whose quantum-mechanical functionalities are controlled via the mature semiconductor technology. Epitaxial quantum dots (QDs) embedded in diodes would embody such ideal quantum devices, but QD structural asymmetries lower dramatically the degree of entanglement of the sources and hamper severely their real exploitation in the foreseen applications. In this work, we overcome this hurdle using strain-tunable optoelectronic devices, where any QD can be tuned for the emission of highly polarization-entangled photons. The electrically-controlled sources violate Bell inequalities without the need of spectral or temporal filtering and they feature the highest degree of entanglement ever reported for QDs, with concurrence as high as 0.75(2). These quantum-devices are at present the most promising candidates for the direct implementation of QD-based entanglement-resources in quantum information science and technology.

cond-mat.mes-hall↗

arXiv2013

Non-integer optical modes in a Möbius-ring resonator

In-plane polarized light experiences a non-trivial topological evolution as it propagates resonantly in a Möbius ring resonator. The resultant geometric phase varies continuously when changing the light ellipticity, which leads to constructive interference for a non-integer number of wavelengths, and therefore to the occurrence of an arbitrary fractional number of optical modes. The geometric phase in Möbius-ring resonators is topologically robust and implies excellent intrinsic fault-tolerance.

physics.optics↗

arXiv2012

Monolithic growth of ultra-thin Ge nanowires on Si(001)

Self-assembled Ge wires with a height of only 3 unit cells and a length of up to 2 micrometers were grown on Si(001) by means of a catalyst-free method based on molecular beam epitaxy. The wires grow horizontally along either the [100] or the [010] direction. On atomically flat surfaces, they exhibit a highly uniform, triangular cross section. A simple thermodynamic model accounts for the existence of a preferential base width for longitudinal expansion, in quantitative agreement with the experimental findings. Despite the absence of intentional doping, first transistor-type devices made from single wires show low-resistive electrical contacts and single hole transport at sub-Kelvin temperatures. In view of their exceptionally small and self-defined cross section, these Ge wires hold promise for the realization of hole systems with exotic properties and provide a new development route for silicon-based nanoelectronics.

cond-mat.mtrl-sci↗