arXiv subjects

Olivier J. F. Martin

Publications and source records attributed to Olivier J. F. Martin.

At least 37 records · Page 2Linked to original sources

arXiv2022

Multipolar expansions for scattering and optical force calculations beyond the long wavelength approximation

We review three different approaches for the calculation of electromagnetic multipoles, namely the Cartesian primitive multipoles, the Cartesian irreducible multipoles and the spherical multipoles. We identify the latter as the best suited to describe the scattering of electromagnetic radiation, as exemplified for an amorphous silicon sphere. These multipoles are then used to calculate the optical force acting on semiconductor, dielectric or metallic particles in a wide wavelength range, from the dipolar down to the Mie regimes.

physics.optics↗

arXiv2022

Probing surfactant bilayer interactions by tracking optically trapped single nanoparticles

Single-particle tracking and optical tweezers are powerful techniques for studying diverse processes at the microscopic scale. The stochastic behavior of a microscopically observable particle contains information about its interaction with surrounding molecules, and an optical tweezer can further facilitate this observation with its ability to constrain the particle to an area of interest. Although these techniques found their initial applications in biology, they can also shed new light on colloid and interface phenomena by unveiling nanoscale morphologies and molecular-level interactions in real time, which have been obscured in traditional ensemble analysis. Here we demonstrate the application of single-particle tracking and optical tweezers for studying molecular interactions at solid-liquid interfaces. Specifically, we investigate the behavior of surfactants at the water-glass interface by tracing their interactions with gold nanoparticles that are optically trapped on these molecules. We discover the underlying mechanisms governing the particle motion, which can be explained by hydrophobic interactions, disruptions, and rearrangements among surfactant monomers at the interfaces. Such interpretations are further supported by statistical analysis of an individual trajectory and comparison to theoretical predictions. Our findings provide new insights into the surfactant dynamics in this specific system but also illustrate the promise of single-particle tracking and optical manipulation in studying nanoscale physics and chemistry of surfaces and interfaces.

cond-mat.soft↗

arXiv2022

Crossing of the branch cut: the topological origin of a universal 2π-phase retardation in non-Hermitian metasurfaces

Full wavefront control by photonic components requires that the spatial phase modulation on an incoming optical beam ranges from 0 to 2π. Because of their radiative coupling to the environment, all optical components are intrinsically non-Hermitian systems, often described by reflection and transmission matrices with complex eigenfrequencies. Here, we show that Parity-Time symmetry breaking -- either explicit or spontaneous -- moves the position of Zero singularities of the reflection or transmission matrices from the real axis to the upper part of the complex frequency plane. A universal 0 to 2π-phase gradient of an output channel as a function of the real frequency excitation is thus realized whenever the discontinuity branch bridging a Zero and a Pole, i.e a pair of singularities, is crossing the real axis. This basic understanding is applied to engineer electromagnetic fields at interfaces, including, but not limited to, metasurfaces. Non-Hermitian topological features associated with exceptional degeneracies or branch cut crossing are shown to play a surprisingly pivotal role in the design of resonant photonic systems.

physics.optics↗

arXiv2021

Multipolar Modeling of Spatially Dispersive Metasurfaces

There is today a growing need to accurately model the angular scattering response of metasurfaces for optical analog processing applications. However, the current metasurface modeling techniques are not well suited for such a task since they are limited to small angular spectrum transformations, as shall be demonstrated. The goal of this work is to overcome this limitation by improving the modeling accuracy of these techniques and, specifically, to provide a better description of the angular response of metasurfaces. This is achieved by extending the current methods, which are restricted to dipolar responses and weak spatially dispersive effects, so as to include quadrupolar responses and higher-order spatially dispersive components. The accuracy of the newly derived multipolar model is demonstrated by predicting the angular scattering of a dielectric metasurface. This results in a modeling accuracy that is at least two times better than the standard dipolar model.

physics.optics↗

arXiv2021

Extension of Lorentz Reciprocity and Poynting Theorems for Spatially Dispersive Media with Quadrupolar Responses

We provide a self-consistent extension of the Lorentz reciprocity theorem and the Poynting theorem for media possessing electric and magnetic dipolar and quadrupolar responses related to electric and magnetic fields and field gradients. Using these two theorems, we respectively deduce the conditions of reciprocity and gainlessness and losslessness that apply to the various tensors mediating the interactions of these multipole moments and the associated fields and field gradients. We expect that these conditions will play an essential role in developing advanced metamaterial modeling techniques that include quadrupolar and spatially dispersive responses.

physics.optics↗

arXiv2021

Second harmonic generation from Chalcogenide metasurfaces via mode coupling engineering

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of nonlinear effects due to their high intrinsic nonlinearities. Here, we demonstrate, experimentally and theoretically, that significant second harmonic generation can be obtained within amorphous chalcogenide based metasurfaces by relying on the coupling between lattice and particle resonances. We further show that the high quality factor resonance at the origin of the second harmonic generation can be tuned over a wide wavelength range using a simple and versatile fabrication approach. The measured second harmonic intensity is orders of magnitude higher than that from a deposited chalcogenide film, and more than three orders of magnitude higher than conventional plasmonic and Silicon-based structures. Fabricated via a simple and scalable technique, these all-dielectric architectures are ideal candidates for the design of flat non-linear optical components on flexible substrates.

physics.optics↗

arXiv2021

Multipolar scattering analysis of hybrid metal-dielectric nanostructures

We perform a systematic study showing the evolution of the multipoles along with the spectra for a hybrid metal-dielectric nanoantenna, a Si cylinder and an Ag disk stacked one on top of another, as its dimensions are varied one by one. We broaden our analysis to demonstrate the "magnetic light" at energies above 1 eV by varying the height of the Ag on the Si cylinder and below 1 eV by introducing insulating spacing between them. We also explore the appearance of the anapole state along with some exceptionally narrow spectral features by varying the radius of the Ag disk.

cond-mat.mes-hall↗

arXiv2020

Fundamental Properties and Classification of Polarization Converting Bianisotropic Metasurfaces

We provide a detailed discussion on the electromagnetic modeling and classification of polarization converting bianisotropic metasurfaces. To do so, we first present a general approach to compute the scattering response of such metasurfaces, which relies on a generalized sheet transition conditions based susceptibility model. Then, we review how the fundamental properties of reciprocity, energy conservation, rotation invariance and matching may be expressed in terms of metasurface susceptibilities and scattering parameters, and show how these properties may affect and limit the polarization effects of metasurfaces. Finally, we connect together the metasurface susceptibility model to the structural symmetries of scattering particles and their associated polarization effects. This work thus provides a detailed understanding of the polarization conversion properties of metasurfaces and may prove to be of particular interest for their practical implementation.

physics.optics↗

arXiv2020

Successive Training of a Generative Adversarial Network for the Design of an Optical Cloak

We present an optimization algorithm based on a deep convolution generative adversarial network (DCGAN) to design a 2-Dimensional optical cloak. The optical cloak consists in a shell of uniform and isotropical dielectric material, and the cloaking is achieved via the geometry of the shell. We use a feedback loop from the solutions of the DCGAN to successively retrain it and improve its ability to predict and find optimal geometries.

eess.IV↗

arXiv2020

Multipolar Origin of the Unexpected Transverse Force Resulting from Two-Wave Interference

We propose a theoretical study on the electromagnetic forces resulting from the superposition of a TE and TM plane waves interacting with a sphere. Specifically, we first show that, under such an illumination condition, the sphere is subjected to a force transverse to the propagation direction of the waves. We then analyze the physical origin of this counter-intuitive behavior using a multipolar decomposition of the electromagnetic modes involved in that scattering process. This analysis reveals that interference effects, due to the two-wave illumination, lead to a Kerker-like asymmetric scattering behavior resulting in this peculiar transverse force.

physics.optics↗

arXiv2018

Influence of Reciprocity, Symmetry and Normal Polarizations on the Angular Scattering Properties of Bianisotropic Metasurfaces

This paper aims at studying the angular scattering properties of bianisotropic metasurfaces and at clarifying the different roles played by tangential and normal polarization densities. Different types of metasurfaces are considered for this study and are classified according to their symmetrical/asymmetrical and reciprocal/nonreciprocal angular scattering behavior. Finally, the paper presents the relationships between the symmetrical angular scattering properties of reciprocal metasurfaces and the structural symmetries of their scattering particles. This may prove to be practically useful for the implementation of metasurfaces with complex angular scattering characteristics.

physics.optics↗

arXiv2018

Less is more - enhancement of second-harmonic generation from metasurfaces by reduced nanoparticle density

We investigate optical second-harmonic generation (SHG) from metasurfaces where noncentrosymmetric V-shaped gold nanoparticles are ordered into regular array configurations. In contrast to expectations, a substantial enhancement of the SHG signal is observed when the number density of the particles in the array is reduced. More specifically, by halving the number density, we obtain over five-fold enhancement in SHG intensity. This striking result is attributed to favorable interparticle interactions mediated by the lattice, where surface-lattice resonances lead to spectral narrowing of the plasmon resonances. Importantly, however, the results cannot be explained by the improved quality of the plasmon resonance alone. Instead, the lattice interactions also lead to further enhancement of the local fields at the particles. The experimental observations agree very well with results obtained from numerical simulations including lattice interactions.

physics.optics↗

arXiv2018

Surface-Wave Dispersion Retrieval Method and Synthesis Technique for Bianisotropic Metasurfaces

We propose a surface-wave dispersion retrieval method and synthesis technique that applies to bianisotropic metasurfaces that are embedded in symmetric or asymmetric environments. Specifically, we use general zero-thickness sheet transition conditions to relate the propagation constants of surface-wave modes to the bianisotropic susceptibility components of the metasurface, which can themselves be directly related to its scattering parameters. It is then possible to either obtain the metasurface dispersion diagram from its known susceptibilities or, alternatively, compute the susceptibilities required to achieve a desired surface-wave propagation. The validity of the method is demonstrated by comparing its results to those obtained with exact dispersion relations of well known structures such as the propagation of surface plasmons on thin metallic films. In particular, this work reveals that it is possible to achieve surface-wave propagation only on one side of the metasurface either by superposition of symmetric and asymmetric modes in the case of anisotropic metasurfaces or by completely forbidding the existence of the surface wave on one side of the structure using bianisotropic metasurfaces.

physics.optics↗

arXiv2018

Revealing a mode interplay that controls second harmonic radiation in gold nanoantennas

In this work, we investigate the generation of second harmonic light by gold nanorods and demonstrate that the collected nonlinear intensity depends upon a phase interplay between different modes available in the nanostructure. By recording the backward and forward emitted second harmonic signals from nanorods with various lengths, we find that the maximum nonlinear signal emitted in the forward and backward directions is not obtained for the same nanorod length. We confirm the experimental results with the help of full-wave computations done with a surface integral equation method. These observations are explained by the multipolar nature of the second harmonic emission, which emphasizes the role played by the relative phase between the second harmonic modes. Our findings are of a particular importance for the design of plasmonic nanostructures with controllable nonlinear emission and nonlinear plasmonic sensors as well as for the coherent control of harmonic generations in plasmonic nanostructures.

physics.optics↗

arXiv2018

Homogenization and Scattering Analysis of Second-Harmonic Generation in Nonlinear Metasurfaces

We propose an extensive discussion on the homogenization and scattering analysis of second-order nonlinear metasurfaces. Our developments are based on the generalized sheet transition conditions (GSTCs) which are used to model the electromagnetic responses of nonlinear metasurfaces. The GSTCs are solved both in the frequency domain, assuming an undepleted pump regime, and in the time-domain, assuming dispersionless material properties but a possible depleted pump regime. Based on these two modeling approaches, we derive the general second-harmonic reflectionless and transmissionless conditions as well as the conditions of asymmetric reflection and transmission. We also discuss and clarify the concept of nonreciprocal scattering pertaining to nonlinear metasurfaces.

physics.optics↗

arXiv2012

Coherent perfect absorption mediated anomalous reflection and refraction

We demonstrate bending of light on the same side of the normal in a free standing corrugated metal film under bi-directional illumination. Coherent perfect absorption (CPA) is exploited to suppress the specular zeroth order leading to effective back-bending of light into the `-1' order, while the `+1' order is resonant with the surface mode. The effect is shown to be phase sensitive yielding CPA and superscattering in the same geometry.

physics.optics↗

arXiv2011

Controllable coherent perfect absorption in a composite film

We exploit the versatility provided by metal--dielectric composites to demonstrate controllable coherent perfect absorption (CPA) in a slab of heterogeneous medium. The slab is illuminated by coherent light from both sides, at the same angle of incidence and the conditions required for CPA are investigated as a function of the different geometrical parameters. The simultaneous realization of CPA at two distinct frequencies is also shown. Finally, our calculations clearly elucidate the role of absorption as a necessary prerequisite for CPA.

physics.optics↗

arXiv2011

Ab initio theory of Fano resonances in plasmonic nanostructures and metamaterials

An ab initio theory for Fano resonances in plasmonic nanostructures and metamaterials is developed using Feshbach formalism. It reveals the role played by the electromagnetic modes and material losses in the system, and enables the engineering of Fano resonances in arbitrary geometries. A general formula for the asymmetric resonance in a non-conservative system is derived. The influence of the electromagnetic interactions on the resonance line shape is discussed and it is shown that intrinsic losses drive the resonance contrast, while its width is mostly determined by the coupling strength between the non-radiative mode and the continuum. The analytical model is in perfect agreement with numerical simulations.

cond-mat.mes-hall↗