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P. C. E. Stamp

Publications and source records attributed to P. C. E. Stamp.

At least 37 records · Page 2Linked to original sources

Sharp transition for single polarons in the one-dimensional Su-Schrieffer-Heeger model

We study a single polaron in the Su-Schrieffer-Heeger (SSH) model using four different techniques (three numerical and one analytical). Polarons show a smooth crossover from weak to strong coupling, as a function of the electron-phonon coupling strength $λ$, in all models where this coupling depends only on phonon momentum $q$. In the SSH model the coupling also depends on the electron momentum $k$; we find it has a sharp transition, at a critical coupling strength $λ_c$, between states with zero and nonzero momentum of the ground state. All other properties of the polaron are also singular at $λ= λ_c$, except the average number of phonons in the polaronic cloud. This result is representative of all polarons with coupling depending on $k$ and $q$, and will have important experimental consequences (eg., in ARPES and conductivity experiments).

cond-mat.str-el↗

Tunneling and inversion symmetry in single-molecule magnets: the case of the Mn12 wheel molecule

We present a detailed study of the influence of various interactions on the spin quantum tunneling in a Mn12 wheel molecule. The effects of single-ion and exchange (spin-orbit) anisotropy are first considered, followed by an analysis of the roles played by secondary influences, e.g. disorder, dipolar and hyperfine fields, and magnetoacoustic interactions. Special attention is paid to the role of the antisymmetric Dzyaloshinski-Moriya (DM) interaction. This is done within the framework of a 12-spin microscopic model, and also using simplified dimer and tetramer approximations in which the electronic spins are grouped in 2 or 4 blocks, respectively. If the molecule is inversion symmetric, the DM interaction between the dimer halves must be zero. In an inversion symmetric tetramer, two independent DM vectors are allowed, but no new tunneling transitions are generated by the DM interaction. Experiments on the Mn12 wheel can only be explained if the molecular inversion symmetry is broken, and we explore this in detail using both models, focussing on the asymmetric disposition and rounding of Berry phase minima associated with quantum interference between states of opposite parity. A remarkable behavior exists for the `Berry phase zeroes' as a function of the directions of the internal DM vectors and the external transverse field. A rather drastic breaking of the molecular inversion-symmetry is required to explain the experiments; in the tetramer model this requires a reorientation of the DM vectors on one half of the molecule by nearly 180 degrees. This cannot be attributed to sample disorder. These results are of general interest for the quantum dynamics of tunneling spins, and lead to some interesting experimental predictions.

cond-mat.mtrl-sci↗

Pure Phase Decoherence in a Ring Geometry

We study the dynamics of pure phase decoherence for a particle hopping around an N-site ring, coupled both to a spin bath and to an Aharonov-Bohm flux which threads the ring. Analytic results are found for the dynamics of the influence functional and of the reduced density matrix of the particle, both for initial single wave-packet states, and for states split initially into 2 separate wave-packets moving at different velocities. We also give results for the dynamics of the current as a function of time.

quant-ph↗

Correlated random fields in dielectric and spin glasses

Both orientational glasses and dipolar glasses possess an intrinsic random field, coming from the volume difference between impurity and host ions. We show this suppresses the glass transition, causing instead a crossover to the low $T$ phase. Moreover the random field is correlated with the inter-impurity interactions, and has a broad distribution. This leads to a peculiar variant of the Imry-Ma mechanism, with 'domains' of impurities oriented by a few frozen pairs. These domains are small: predictions of domain size are given for specific systems, and their possible experimental verification is outlined. In magnetic glasses in zero field the glass transition survives, because the random fields are disallowed by time-reversal symmetry; applying a magnetic field then generates random fields, and suppresses the spin glass transition.

cond-mat.dis-nn↗

Manifestation of Spin Selection Rules on the Quantum Tunneling of Magnetization in a Single Molecule Magnet

We present low temperature magnetometry measurements on a new Mn3 single-molecule magnet (SMM) in which the quantum tunneling of magnetization (QTM) displays clear evidence for quantum mechanical selection rules. A QTM resonance appearing only at elevated temperatures demonstrates tunneling between excited states with spin projections differing by a multiple of three: this is dictated by the C3 symmetry of the molecule, which forbids pure tunneling from the lowest metastable state. Resonances forbidden by the molecular symmetry are explained by correctly orienting the Jahn-Teller axes of the individual manganese ions, and by including transverse dipolar fields. These factors are likely to be important for QTM in all SMMs.

cond-mat.mes-hall↗

dHvA Oscillations in High-Tc Compounds

Recent de Haas-van Alphen (dHvA) experiments on high-Tc compounds have been interpreted using Lifshitz-Kosevich (LK) theory, which ignores many-body effects. However in quasi-2d systems, interactions plus Landau level quantization give strong singularities in the self-energy $Σ$ and the thermodynamic potential $Ω$. These are rapidly suppressed as one increases the c-axis tunneling amplitude $t_\perp$ and/or impurity scattering. We show that 2d-3d crossover and interaction effects should show up in these experiments, and that they can lead to strong deviations from LK behaviour. Moreover, dHvA experiments in quasi-2d systems should clearly distinguish between Fermi liquid and non-Fermi liquid states, for sufficiently weak impurity scattering.

cond-mat.str-el↗

What are the interactions in quantum glasses?

The form of the low-temperature interactions between defects in neutral glasses is reconsidered. We analyse the case where the defects can be modelled either as simple 2-level tunneling systems, or tunneling rotational impurities. The coupling to strain fields is determined up to 2nd order in the displacement field. It is shown that the linear coupling generates not only the usual $1/r^3$ Ising-like interaction between the rotational tunneling defect modes, which cause them to freeze around a temperature $T_G$, but also a random field term. At lower temperatures the inversion symmetric tunneling modes are still active - however the coupling of these to the frozen rotational modes, now via the 2nd-order coupling to phonons, generates another random field term acting on the inversion symmetric modes (as well as shorter-range $1/r^5$ interactions between them). Detailed expressions for all these couplings are given.

cond-mat.dis-nn↗

The low-$T$ phase diagram of ${\rm LiHo_xY_{1-x}F_4}$

The ${\rm LiHo_xY_{1-x}F_4}$ compound is widely considered to be the archetypal dipolar Quantum Ising system, with longitudinal dipolar interactions $V_{ij}^{zz}$ between ${\rm Ho}$ spins $\{i,j \}$ competing with transverse field-induced tunneling, to give a T=0 quantum phase transition. By varying the ${\rm Ho}$ concentration x, the typical strength $V_0$ of $V_{ij}^{zz}$ can be varied over many orders of magnitude; and so can the transverse field $H_{\perp}$. A new effective Hamiltonian is derived, starting from the electronuclear degrees of freedom, and valid at low and intermediate temperatures. For any such dipolar Quantum Ising system, the hyperfine interaction will dominate the physics at low temperatures, even if its strength $A_0 < V_0$: one must therefore go beyond an electronic transverse field Quantum Ising model. We derive the full phase diagram of this system, including all nuclear levels, as a function of transverse field $H_{\perp}$, temperature $T$, and dipole concentration x. For ${\rm LiHo_xY_{1-x}F_4}$ we predict a re-entrant critical field as a function of x. We also predict the phase diagram for x$=0.045$, and the behavior of the system in magnetic resonance and $μ$SR experiments.

cond-mat.str-el↗

Topological multicritical point in the Toric Code and 3D gauge Higgs Models

We report a new type of multicritical point that arises from competition between the Higgs and confinement transitions in a Z_2 gauge system. The phase diagram of the 3d gauge Higgs model has been obtained by Monte-Carlo simulation on large (up to 60^3) lattices. We find the transition lines continue as 2nd-order until merging into a 1st-order line. These findings pose the question of an effective field theory for a multicritical point involving noncommuting order parameters. A similar phase diagram is predicted for the 2-dimensional quantum toric code model with two external fields, h_z and h_x; this problem can be mapped onto an anisotropic 3D gauge Higgs model.

cond-mat.stat-mech↗

Stability of Bose Einstein condensates of hot magnons in YIG

We investigate the stability of the recently discovered room temperature Bose-Einstein condensate (BEC) of magnons in Ytrrium Iron Garnet (YIG) films. We show that magnon-magnon interactions depend strongly on the external field orientation, and that the BEC in current experiments is actually metastable - it only survives because of finite size effects, and because the BEC density is very low. On the other hand a strong field applied perpendicular to the sample plane leads to a repulsive magnon-magnon interaction; we predict that a high-density magnon BEC can then be formed in this perpendicular field geometry.

cond-mat.other↗

Decoherence in quantum walks and quantum computers

Decoherence is the major stumbling block in the realization of a large-scale quantum computer. Ingenious methods have been devised to overcome decoherence, but their success has been proven only for over-simplified models of system-environment interaction. Whether such methods will be reliable in the face of more realistic models is a fundamental open question. In this partly pedagogical article, we study two toy models of quantum information processing, using the language of \emph{quantum walks}. Decoherence is incorporated in 3 ways - by coupling to a noisy `projective measurement' system, and by coupling to oscillator and spin baths.

quant-ph↗

Quantum Walks, Quantum Gates and Quantum Computers

The physics of quantum walks on graphs is formulated in Hamiltonian language, both for simple quantum walks and for composite walks, where extra discrete degrees of freedom live at each node of the graph. It is shown how to map between quantum walk Hamiltonians and Hamiltonians for qubit systems and quantum circuits; this is done for both a single- and multi-excitation coding, and for more general mappings. Specific examples of spin chains, as well as static and dynamic systems of qubits, are mapped to quantum walks, and walks on hyperlattices and hypercubes are mapped to various gate systems. We also show how to map a quantum circuit performing the quantum Fourier transform, the key element of Shor's algorithm, to a quantum walk system doing the same. The results herein are an essential preliminary to a Hamiltonian formulation of quantum walks in which coupling to a dynamic quantum environment is included.

quant-ph↗

Pair-wise decoherence in coupled spin qubit networks

Experiments involving phase coherent dynamics of networks of spins, such as echo experiments, will only work if decoherence can be suppressed. We show here, by analyzing the particular example of a crystalline network of Fe8 molecules, that most decoherence typically comes from pairwise interactions (particularly dipolar interactions) between the spins, which cause `correlated errors'. However at very low T these are strongly suppressed. These results have important implications for the design of quantum information processing systems using electronic spins.

cond-mat.mes-hall↗

Quantum spin glass in anisotropic dipolar systems

The spin-glass phase in the $\LHx$ compound is considered. At zero transverse field this system is well described by the classical Ising model. At finite transverse field deviations from the transverse field quantum Ising model are significant, and one must take properly into account the hyperfine interactions, the off-diagonal terms in the dipolar interactions, and details of the full J=8 spin Hamiltonian to obtain the correct physical picture. In particular, the system is not a spin glass at finite transverse fields and does not show quantum criticality.

cond-mat.dis-nn↗

Significance of the Hyperfine Interactions in the Phase Diagram of ${\rm LiHo_xY_{1-x}F_4}$

We consider the quantum magnet $\rm LiHo_xY_{1-x}F_4$ at $x = 0.167$. Experimentally the spin glass to paramagnet transition in this system was studied as a function of the transverse magnetic field and temperature, showing peculiar features: for example (i) the spin glass order is destroyed much faster by thermal fluctuations than by the transverse field; and (ii) the cusp in the nonlinear susceptibility signaling the glass state {\it decreases} in size at lower temperature. Here we show that the hyperfine interactions of the Ho atom must dominate in this system, and that along with the transverse inter-Ho dipolar interactions they dictate the structure of the phase diagram. The experimental observations are shown to be natural consequences of this.

cond-mat.dis-nn↗

Critical Boundary Sine-Gordon Revisited

We revisit the exact solution of the two space-time dimensional quantum field theory of a free massless boson with a periodic boundary interaction and self-dual period. We analyze the model by using a mapping to free fermions with a boundary mass term originally suggested in ref.[22]. We find that the entire SL(2,C) family of boundary states of a single boson are boundary sine-Gordon states and we derive a simple explicit expression for the boundary state in fermion variables and as a function of sine-Gordon coupling constants. We use this expression to compute the partition function. We observe that the solution of the model has a strong-weak coupling generalization of T-duality. We then examine a class of recently discovered conformal boundary states for compact bosons with radii which are rational numbers times the self-dual radius. These have simple expression in fermion variables. We postulate sine-Gordon-like field theories with discrete gauge symmmetries for which they are the appropriate boundary states.

hep-th↗