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P. G. Pagliuso

Publications and source records attributed to P. G. Pagliuso.

At least 91 records · Page 5Linked to original sources

Two Superconducting Phases in CeRh_1-xIr_xIn_5

Pressure studies of CeRh_1-xIr_xIn_5 indicate two superconducting phases as a function of x, one with T_c >= 2 K for x < 0.9 and the other with T_c < 1.2 K for x > 0.9. The higher T_c phase, phase-1, emerges in proximity to an antiferromagnetic quantum-critical point; whereas, Cooper pairing in the lower T_c phase-2 is inferred to arise from fluctuations of a yet to be found magnetic state. The T-x-P phase diagram of CeRh_1-xIr_xIn_5, though qualitatively similar, is distinctly different from that of CeCu_2(Si_1-xGe_x)_2.

cond-mat.str-el↗

Non-Fermi Liquid behavior in CeIrIn$_5$ near a metamagnetic transition

We present specific heat and resistivity study of CeIrIn5 in magnetic fields up to 17 T and temperature down to 50 mK. Both quantities were measured with the magnetic field parallel to the c-axis (H || [001]) and within the a-b plane (H \perp [001]). Non-Fermi-liquid (NFL) behavior develops above 12 T for H || [001]. The Fermi liquid state is much more robust for H \perp [001] and is suppressed only moderately at the highest applied field. Based on the observed trends and the proximity to a metamagnetic phase transition, which exists at fields above 25 T for H || [001], we suggest that the observed NFL behavior in CeIrIn5 is a consequence of a metamagnetic quantum critical point.

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Crystalline Electric Field Effects in CeMIn5: Superconductivity and the Influence of Kondo Spin Fluctuations

We have measured the crystalline electric field (CEF) excitations of the CeMIn5 (M = Co, Rh, Ir) series of heavy fermion superconductors by means of inelastic neutron scattering. Fits to a CEF model reproduce the inelastic neutron scattering spectra and the high temperature magnetic susceptibility. The CEF parameters, energy level splittings, and wavefunctions are tabulated for each member of the CeMIn5 series and compared to each other as well as to the results of previous measurements. Our results indicate that the CEF level splitting in all three materials is similar, and can be thought of as being derived from the cubic parent compound CeIn3 in which an excited state quartet at ~12 meV is split into two doublets by the lower symmetry of the tetragonal environment of the CeMIn5 materials. In each case, the CEF excitations are observed as broad lines in the inelastic neutron scattering spectrum. We attribute this broadening to Kondo hybridization of the localized f moments with the conduction electrons. The evolution of the superconducting transition temperatures in the different members of CeMIn5 can then be understood as a direct consequence of the strength of this hybridization. Due to the importance of Kondo spin fluctuations in these materials, we also present calculations within the non-crossing approximation (NCA) to the Anderson impurity model including the effect of CEF level splitting for the inelastic neutron scattering spectra and the magnetic susceptibility.

cond-mat.str-el↗

Anomalous f-electron Hall Effect in the Heavy-Fermion System CeTIn$_{5}$ (T = Co, Ir, or Rh)

The in-plane Hall coefficient $R_{H}(T)$ of CeRhIn$_{5}$, CeIrIn$_{5}$, and CeCoIn$_{5}$ and their respective non-magnetic lanthanum analogs are reported in fields to 90 kOe and at temperatures from 2 K to 325 K. $R_{H}(T)$ is negative, field-independent, and dominated by skew-scattering above $\sim$ 50 K in the Ce compounds. $R_{H}(H \to 0)$ becomes increasingly negative below 50 K and varies with temperature in a manner that is inconsistent with skew scattering. Field-dependent measurements show that the low-T anomaly is strongly suppressed when the applied field is increased to 90 kOe. Measurements on LaRhIn$_{5}$, LaIrIn$_{5}$, and LaCoIn$_{5}$ indicate that the same anomalous temperature dependence is present in the Hall coefficient of these non-magnetic analogs, albeit with a reduced amplitude and no field dependence. Hall angle ($θ_{H}$) measurements find that the ratio $ρ_{xx}/ρ_{xy}=\cot(θ_{H})$ varies as $T^{2}$ below 20 K for all three Ce-115 compounds. The Hall angle of the La-115 compounds follow this T-dependence as well. These data suggest that the electronic-structure contribution dominates the Hall effect in the 115 compounds, with $f$-electron and Kondo interactions acting to magnify the influence of the underlying complex band structure. This is in stark contrast to the situation in most $4f$ and $5f$ heavy-fermion compounds where the normal carrier contribution to the Hall effect provides only a small, T-independent background to $R_{H}.$

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Crystal Field Effects in CeIrIn5

In this work, we study crystalline electric field effects in the heavy fermion superconductor CeIrIn5. We observe two regions of broad magnetic response in the inelastic neutron scattering spectra at 10 K. The first corresponds to the transition between the gamma7 groundstate doublet and the first excited state doublet at 4 meV interwoven with a broad quasielastic contribution. The second region corresponds to the transition between the ground state and the second excited state doublet at 28 meV. The large Lorentzian half-widths of the peaks (~10 meV) calls into question calculations for the specific heat and magnetic susceptibility that assume sharp crystal field levels. Consequently, we have calculated the inelastic neutron scattering spectra and magnetic susceptibility using the Anderson impurity model within the non-crossing approximation (NCA) including the effects of crystal field level splitting.

cond-mat.str-el↗

Anisotropy of Thermal Conductivity and Possible Signature of the Fulde-Ferrell-Larkin-Ovchinnikov state in CeCoIn_5

We have measured the thermal conductivity of the heavy-fermion superconductor CeCoIn_5 in the vicinity of the upper critical field, with the magnetic field perpendicular to the c axis. Thermal conductivity displays a discontinuous jump at the superconducting phase boundary below critical temperature T_0 ~ 1 K, indicating a change from a second to first order transition and confirming the recent results of specific heat measurements on CeCoIn_5. In addition, the thermal conductivity data as a function of field display a kink at a field H_k below the superconducting critical field, which closely coincides with the recently discovered anomaly in specific heat, tentatively identified with the appearance of the spatially inhomogeneous Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconducting state. Our results indicate that the thermal conductivity is enhanced within the FFLO state, and call for further theoretical investigations of the order parameter's real space structure (and, in particular, the structure of vortices) and of the thermal transport within the inhomogeneous FFLO state.

cond-mat.str-el↗

Heat capacity studies of Ce and Rh site substitution in the heavy fermion antiferromagnet CeRhIn_5;: Short-range magnetic interactions and non-Fermi-liquid behavior

In heavy fermion materials superconductivity tends to appear when long range magnetic order is suppressed by chemical doping or applying pressure. Here we report heat capacity measurements on diluted alloyes of the heavy fermion superconductor CeRhIn_5;. Heat capacity measurements have been performed on CeRh_{1-y}Ir_{y}In_5; (y <= 0.10) and Ce_{1-x}La_{x}Rh_{1-y}Ir_{y}In_5; (x <= 0.50) in applied fields up to 90 kOe to study the affect of doping and magnetic field on the magnetic ground state. The magnetic phase diagram of CeRh_{0.9}Ir_{0.1}In_5; is consistent with the magnetic structure of CeRhIn_5; being unchanged by Ir doping. Doping of Ir in small concentrations is shown to slightly increase the antiferromagnetic transition temperature T_{N} (T_{N}=3.8 K in the undoped sample). La doping which causes disorder on the Ce sublattice is shown to lower T_{N} with no long range order observed above 0.34 K for Ce_{0.50}La_{0.50}RhIn_5;. Measurements on Ce_{0.50}La_{0.50}RhIn_5; show a coexistence of short range magnetic order and non-Fermi-liquid behavior. This dual nature of the Ce 4f-electrons is very similar to the observed results on CeRhIn_5; when long range magnetic order is suppressed at high pressure.

cond-mat.str-el↗

Magnetic structure of CeRhIn_5 as a function of pressure and temperature

We report magnetic neutron-diffraction and electrical resistivity studies on single crystals of the heavy-fermion antiferromagnet CeRhIn$_{5}$ at pressures up to 2.3 GPa. These experiments show that the staggered moment of Ce and the incommensurate magnetic structure change weakly with applied pressure up to 1.63 GPa, where resistivity, specific heat and NQR measurements confirm the presence of bulk superconductivity. This work places new constraints on an interpretation of the relationship between antiferromagnetism and unconventional superconductivity in CeRhIn$_{5}$.

cond-mat.str-el↗

Fulde-Ferrell-Larkin-Ovchinnikov Superconducting State in CeCoIn5

We report specific heat measurements of the heavy fermion superconductor CeCoIn5 in the vicinity of the superconducting critical field H_{c2}, with magnetic field in the [110], [100], and [001] directions, and at temperatures down to 50 mK. The superconducting phase transition changes from second to first order for field above 10 T for H || [110] and H || [100]. In the same range of magnetic field we observe a second specific heat anomaly within the superconducting state. We interpret this anomaly as a signature of a Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) inhomogeneous superconducting state. We obtain similar results for H || [001], with FFLO state occupying a smaller part of the phase diagram.

cond-mat.str-el↗

Avoided Antiferromagnetic Order and Quantum Critical Point in CeCoIn$_5$

We measured specific heat and resistivity of heavy fermion CeCoIn5 between the superconducting critical field $H_{c2} = 5 T$ and 9 T, with field in the [001] direction, and at temperatures down to 50mK. At 5T the data show Non Fermi Liquid behavior down to the lowest temperatures. At field above 8T the data exhibit crossover from the Fermi liquid to a Non Fermi Liquid behavior. We analyzed the scaling properties of the specific heat, and compared both resistivity and the specific heat with the predictions of a spin-fluctuation theory. Our analysis leads us to suggest that the NFL behavior is due to incipient antiferromagnetism (AF) in CeCoIn5, with the quantum critical point in the vicinity of the $H_{c2}$. Below $H_{c2}$ the AF phase which competes with the paramagnetic ground state is superseded by the superconducting transition.

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Magnetism and superconductivity in CeRh_{1-x}Ir_xIn_5 heavy fermion materials

We report on zero-field muon spin relaxation studies of cerium based heavy-fermion materials CeRh_{1-x}Ir_xIn_5. In the superconducting x=0.75 and 1 compositions muon spin relaxation functions were found to be temperature independent across T_c; no evidence for the presence of electronic magnetic moments was observed. The x=0.5 material is antiferromagnetic below T_N=3.75 K and superconducting below T_c=0.8 K. Muon spin realxation spectra show the gradual onset of damped coherent oscillations characteristic of magnetic order below T_N. At 1.65 K the total oscillating amplitude accounts for at least 85% of the sample volume. No change in muon precession frequency or amplitude is detected on cooling below T_c, indicating the microscopic coexistence of magnetism and superconductivity in this material.

cond-mat.supr-con↗

Magnetism and superconductivity in Ce_2RhIn_8

We report the discovery of pressure-induced superconductivity, with T_c=2 K, in the heavy-fermion antiferromagnet Ce_2RhIn_8, where superconductivity and magnetic order coexist over an extended pressure interval. A T-linear resistivity in the normal state, accessed by an applied magnetic field, does not appear to derive from the existence of a 2D quantum-critical spin-density wave.

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Low Frequency Spin Dynamics in the CeMIn_5 Materials

We measure the spin lattice relaxation of the In(1) nuclei in the CeMIn_5 materials, extract quantitative information about the low energy spin dynamics of the lattice of Ce moments in both CeRhIn_5 and CeCoIn_5, and identify a crossover in the normal state. Above a temperature T* the Ce lattice exhibits "Kondo gas" behavior characterized by local fluctuations of independently screened moments; below T* both systems exhibit a "Kondo liquid" regime in which interactions between the local moments contribute to the spin dynamics. Both the antiferromagnetic and superconducting ground states in these systems emerge from the "Kondo liquid" regime. Our analysis provides strong evidence for quantum criticality in CeCoIn_5.

cond-mat.str-el↗

Superconductivity and Quantum Criticality in CeCoIn_5

Electrical resistivity measurements on a single crystal of the heavy-fermion superconductor CeCoIn_5 at pressures to 4.2 GPa reveal a strong crossover in transport properties near P^* \approx 1.6 GPa, where T_c is a maximum. The temperature-pressure phase diagram constructed from these data provides a natural connection to cuprate physics, including the possible existence of a pseudogap.

cond-mat.str-el↗

Unconventional Metallic Magnetism in LaCrSb{3}

Neutron-diffraction measurements in LaCrSb{3} show a coexistence of ferromagnetic and antiferromagnetic sublattices below Tc=126 K, with ordered moments of 1.65(4) and 0.49(4) Bohr magnetons per formula unit, respectively (T=10 K), and a spin reorientation transition at ~95 K. No clear peak or step was observed in the specific heat at Tc. Coexisting localized and itinerant spins are suggested.

cond-mat↗

Magnetic structure of antiferromagnetic NdRhIn5

The magnetic structure of antiferromagnetic NdRhIn5 has been determined using neutron diffraction. It has a commensurate antiferromagnetic structure with a magnetic wave vector (1/2,0,1/2) below T_N = 11K. The staggered Nd moment at 1.6K is 2.6mu_B aligned along the c-axis. We find the magnetic structure to be closely related to that of its cubic parent compound NdIn3 below 4.6K. The enhanced T_N and the absence of additional transitions below T_N for NdRhIn5 are interpreted in terms of an improved matching of the crystalline-electric-field (CEF), magnetocrystalline, and exchange interaction anisotropies. In comparison, the role of these competing anisotropies on the magnetic properties of the structurally related compound CeRhIn5 is discussed.

cond-mat.str-el↗

Intersite coupling effects in a Kondo lattice

The La dilution of the Kondo lattice CeCoIn_5 is studied. The scaling laws found for the magnetic susceptibility and the specific heat reveal two well-separated energy scales, corresponding to the single impurity Kondo temperature T_K and an intersite spin-liquid temperature T^*. The Ce-dilute alloy has the expected Fermi liquid ground state, while the specific heat and resistivity in the dense Kondo regime exhibit non-Fermi-liquid behavior, which scales with T^*. These observations indicate that the screening of the magnetic moments in the lattice involves antiferromagnetic intersite correlations with a larger energy scale in comparison with the Kondo impurity case.

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