arXiv subjects

P. K. Sreejith

Publications and source records attributed to P. K. Sreejith.

3 recordsLinked to original sources

arXiv2024

Evidence of 3$d$-4$f$ antiferromagnetic coupling in strain-tuned PrCo$_{0.5}$Ni$_{0.5}$O$_{3-δ}$ epitaxial films

The strong exchange interaction between 3$d$-4$f$ magnetic sublattice in rare-earth perovskites introduces a variety of complex magnetic states hosting fascinating electronic ground states with exotic properties. Especially when it comes to rare-earth nickelate and cobaltite perovskites, tuning their rich magnetic phase diagram and spin-state transitions make them potential candidates for spintronic applications. Here, we report the observation of antiferromagnetic coupling between Pr 4$f$ and Ni/Co 3$d$ magnetic sublattices and its tunability with strain in PrCo$_{0.5}$Ni$_{0.5}$O$_{3-δ}$ (PCNO) thin films. SQUID magnetization measurements reveal ferromagnetic (FM) ordering around 25 K, followed by a spin glass transition at low temperatures subject to spin reorientation. Competing magnetic interactions arise owing to the 3$d$-4$f$ antiferromagnetic (AFM) coupling between Pr and Co/Ni sublattice as revealed by the X-ray absorption spectroscopy (XAS) and X-ray magnetic circular dichroism (XMCD) at the Pr $M_{4,5}$ and Co/Ni $L_{2,3}$ absorption edges. Strain dependence on these AFM coupling reveals an increase (decrease) in the AFM exchange interaction for tensile (compressive) strained films, leading to a net decrease (increase) in the magnetization of PCNO films at low temperatures. The relative increase in low-temperature negative magnetoresistance for compressively strained films also reflects the enhanced ferromagnetic ordering in the system. The angle-dependent magnetoresistance measurements reveal a two-fold anisotropic magnetoresistance (AMR) in tensile strained PCNO films. In contrast, temperature-dependent switching of AMR accompanied by a two- to four-fold symmetry crossover is observed for LaAlO$_3$-grown compressive strained films.

cond-mat.mtrl-sci↗

arXiv2023

Spin re-orientation induced anisotropic magnetoresistance switching in LaCo$_{0.5}$Ni$_{0.5}$O$_{3-δ}$ thin films

Realization of novel functionalities by tuning magnetic interactions in rare earth perovskite oxide thin films opens up exciting technological prospects. Strain-induced tuning of magnetic interactions in rare earth cobaltates and nickelates is of central importance due to their versatility in electronic transport properties. Here we reported the spin re-orientation induced switching of anisotropic magnetoresistance (AMR) and its tunability with strain in epitaxial LaCo$_{0.5}$Ni$_{0.5}$O$_{3-δ}$ thin films across the ferromagnetic transition. Moreover, with strain tuning, we could observe a two-fold to four-fold symmetry crossover in AMR across the magnetic transition temperature. The magnetization measurements revealed an onset of ferromagnetic transition around 50 K, and a further reduction in temperature showed a subtle change in the magnetization dynamics, which reduced the ferromagnetic long-range ordering and introduced glassiness in the system. X-ray absorption and X-ray magnetic circular dichroism spectroscopy measurements over Co and Ni L edges revealed the Co spin state transition below the magnetic transition temperature leading to the AMR switching and also the presence of Ni$^{2+}$ and Co$^{4+}$ ions evidencing the charge transfer from Ni to Co ions. Our work demonstrated the tunability of magnetic interactions mediated electronic transport in cobaltate-nickelate thin films, which is relevant in understanding Ni-Co interactions in oxides for their technological applications such as in AMR sensors.

cond-mat.mtrl-sci↗

arXiv2021

Response of the low pressure hot-filament discharge plasma to a positively biased auxiliary disk electrode

In steady-state, the plasma loss rate to the chamber wall is balanced by the ionization rate in the hot-filament discharges. This balance in the loss rate and ionization rate maintains the quasi--neutrality of the bulk plasma. In this report, we have studied the properties of bulk plasma in the presence of an auxiliary (additional) biased metal disk, which is working as a sink, in low-pressure helium plasma. A single Langmuir probe and emissive probe are used to characterize the plasma for various biases (positive and negative) to the metal disk, which was placed along the discharge axis inside the plasma. It is observed that only a positively biased disk increases the plasma potential, electron temperature, and plasma density. Moreover, the plasma parameters remain unaltered when the disk is negatively biased. The observed results for two different-sized positively metal disks are compared with an available theoretical model and found an opposite behavior of plasma density variation with the disk bias voltages at given discharge condition. The role of the primary energetic electron population in determining the plasma parameters is discussed. These experimental results are qualitatively explained on the basis of electrostatic confinement arising due to the loss of electrons to a biased metal disk electrode.

physics.plasm-ph↗