arXiv subjects

P. Senellart

Publications and source records attributed to P. Senellart.

At least 19 recordsLinked to original sources

arXiv2026

Dynamical decoupling of a quantum dot spin in a micropillar cavity for spin-multiphoton entanglement

Graph states of mutually entangled photons are key resources for quantum computation and communication and can be generated by leveraging the entanglement between a single resident spin and emitted photons from a charged semiconductor quantum dot (QD). This approach is intrinsically limited by the decoherence of the spin. We study how to mitigate this decoherence with dynamical decoupling of an electron spin in the weak transverse magnetic field regime using spin echo and Carr-Purcell-Meiboom-Gill (CPMG) techniques. Application of these techniques allows us to extend the coherence time of a spin by more than two orders of magnitude, extracting a $T_2^{CPMG}$ of $298\pm53$ ns. We further demonstrate that this technique is compatible with the generation of a spin-photon-photon entangled state at a high rate enabled by a micropillar cavity, with a 20% improvement in simulated state fidelity when using dynamical decoupling. These results pave the way for generating larger and more complex entangled states with QDs.

quant-ph↗

arXiv2026

Accessing which-path information in the absorption and emission of light by a quantum dot in a Ramsey sequence

We quantify which-path information in the absorption and emission of light by a quantum dot along a Ramsey-like sequence. The quantum dot is excited by two successive classical $\pi/2$-pulses with tunable relative phase, yielding the spontaneous release of coherent superpositions of zero- and one-photon Fock states into two successive time bins. Along the sequence, the first time bin extracts information on the quantum dot energy state, behaving as a which-path detector for the Ramsey interferometer. The which-path information increases over time, and is accessed through the reduction of contrast of the Ramsey fringes. After the second pulse, the information still present in the first time bin controls the emission of coherent light into the second time bin, which is measurable through the reduction of the contrast of self-homodyne interference fringes in a Mach-Zehnder interferometer. Both measurements are in remarkable agreement with theoretical predictions. Our results quantitatively illustrate how which-path information and more generally quantum correlations impact light-matter energy exchanges in the quantum realm.

quant-ph↗

arXiv2025

The impact of hole $g$-factor anisotropy on spin-photon entanglement generation with InGaAs quantum dots

Self-assembled InGaAs/GaAs quantum dots (QDs) are of particular importance for the deterministic generation of spin-photon entanglement. One promising scheme relies on the Larmor precession of a spin in a transverse magnetic field, which is governed by the in-plane $g$-factors of the electron and valence band heavy-hole. We probe the origin of heavy-hole $g$-factor anisotropy with respect to the in-plane magnetic field direction and uncover how it impacts the entanglement generated between the spin and the photon polarization. First, using polarization-resolved photoluminescence measurements on a single QD, we determine that the impact of valence-band mixing dominates over effects due to a confinement-renormalized cubic Luttinger $q$ parameter. From this, we construct a comprehensive hole $g$-tensor model. We then use this model to simulate the concurrence and fidelity of spin-photon entanglement generation with anisotropic hole $g$-factors, which can be tuned via magnetic field angle and excitation polarization. The results demonstrate that post-growth control of the hole $g$-factor can be used to improve spin-photon cluster state generation.

cond-mat.mes-hall↗

arXiv2024

Deterministic and reconfigurable graph state generation with a single solid-state quantum emitter

Measurement-based quantum computing offers a promising route towards scalable, universal photonic quantum computation. This approach relies on the deterministic and efficient generation of photonic graph states in which many photons are mutually entangled with various topologies. Recently, deterministic sources of graph states have been demonstrated with quantum emitters in both the optical and microwave domains. In this work, we demonstrate deterministic and reconfigurable graph state generation with optical solid-state integrated quantum emitters. Specifically, we use a single semiconductor quantum dot in a cavity to generate caterpillar graph states, the most general type of graph state that can be produced with a single emitter. By using fast detuned optical pulses, we achieve full control over the spin state, enabling us to vary the entanglement topology at will. We perform quantum state tomography of two successive photons, measuring Bell state fidelities up to 0.80$\pm$0.04 and concurrences up to 0.69$\pm$0.09, while maintaining high photon indistinguishability. This simple optical scheme, compatible with commercially available quantum dot-based single photon sources, brings us a step closer to fault-tolerant quantum computing with spins and photons.

quant-ph↗

arXiv2024

A deterministic and efficient source of frequency-polarization hyper-encoded photonic qubits

The frequency or color of photons is an attractive degree of freedom to encode and distribute the quantum information over long distances. However, the generation of frequency-encoded photonic qubits has so far relied on probabilistic non-linear single-photon sources and inefficient gates. Here, we demonstrate the deterministic generation of photonic qubits hyper-encoded in frequency and polarization based on a semiconductor quantum dot in a cavity. We exploit the double dipole structure of a neutral exciton and demonstrate the generation of any quantum superposition in amplitude and phase, controlled by the polarization of the pump laser pulse. The source generates frequency-polarization single-photon qubits at a rate of 4 MHz corresponding to a generation probability at the first lens of 28 $\pm$ 2%, with a photon number purity > 98%. The photons show an indistinguishability > 91% for each dipole and 88% for a balanced quantum superposition of both. The density matrix of the hyper-encoded photonic state is measured by time-resolved polarization tomography, evidencing a fidelity to the target state of 94 $\pm$ 8% and concurrence of 77 $\pm$ 2%, here limited by frequency overlap in our device. Our approach brings the advantages of quantum dot sources to the field of quantum information processing based on frequency encoding.

quant-ph↗

arXiv2024

Quantum interferences and gates with emitter-based coherent photon sources

Quantum emitters such as quantum dots, defects in diamond or in silicon have emerged as efficient single photon sources that are progressively exploited in quantum technologies. In 2019, it was shown that the emitted single photon states often include coherence with the vacuum component. Here we investigate how such photon-number coherence alters quantum interference experiments that are routinely implemented both for characterising or exploiting the generated photons. We show that it strongly modifies intensity correlation measurements in a Hong-Ou-Mandel experiment and leads to errors in indistinguishability estimations. It also results in additional entanglement when performing partial measurements. We illustrate the impact on quantum protocols by evidencing modifications in heralding efficiency and fidelity of two-qubit gates.

quant-ph↗

arXiv2022

High-rate entanglement between a semiconductor spin and indistinguishable photons

Photonic graph states, quantum light states where multiple photons are mutually entangled, are key resources for optical quantum technologies. They are notably at the core of error-corrected measurement-based optical quantum computing and all-optical quantum networks. In the discrete variable framework, these applications require high efficiency generation of cluster-states whose nodes are indistinguishable photons. Such photonic cluster states can be generated with heralded single photon sources and probabilistic quantum gates, yet with challenging efficiency and scalability. Spin-photon entanglement has been proposed to deterministically generate linear cluster states. First demonstrations have been obtained with semiconductor spins achieving high photon indistinguishablity, and most recently with atomic systems at high collection efficiency and record length. Here we report on the efficient generation of three partite cluster states made of one semiconductor spin and two indistinguishable photons. We harness a semiconductor quantum dot inserted in an optical cavity for efficient photon collection and electrically controlled for high indistinguishability. We demonstrate two and three particle entanglement with fidelities of 80 % and 63 % respectively, with photon indistinguishability of 88%. The spin-photon and spin-photon-photon entanglement rates exceed by three and two orders of magnitude respectively the previous state of the art. Our system and experimental scheme, a monolithic solid-state device controlled with a resource efficient simple experimental configuration, are very promising for future scalable applications.

quant-ph↗

arXiv2022

Probing the dynamics and coherence of a semiconductor hole spin via acoustic phonon-assisted excitation

Spins in semiconductor quantum dots are promising local quantum memories to generate polarization-encoded photonic cluster states, as proposed in the pioneering Rudolph-Lindner scheme [1]. However, harnessing the polarization degree of freedom of the optical transitions is hindered by resonant excitation schemes that are widely used to obtain high photon indistinguishability. Here we show that acoustic phonon-assisted excitation, a scheme that preserves high indistinguishability, also allows to fully exploit the polarization selective optical transitions to initialise and measure single spin states. We access the coherence of hole spin systems in a low transverse magnetic field and directly monitor the spin Larmor precession both during the radiative emission process of an excited state or in the quantum dot ground state. We report a spin state detection fidelity of $94.7 \pm 0.2 \%$ granted by the optical selection rules and a $20\pm5$~ns hole spin coherence time, demonstrating the potential of this scheme and system to generate linear cluster states with a dozen of photons

cond-mat.mes-hall↗

arXiv2022

Photon-number entanglement generated by sequential excitation of a two-level atom

Entanglement and spontaneous emission are fundamental quantum phenomena that drive many applications of quantum physics. During the spontaneous emission of light from an excited two-level atom, the atom briefly becomes entangled with the photonic field. Here, we show that this natural process can be used to produce photon-number entangled states of light distributed in time. By exciting a quantum dot -- an artificial two-level atom -- with two sequential $π$ pulses, we generate a photon-number Bell state. We characterise this state using time-resolved intensity and phase correlation measurements. Furthermore, we theoretically show that applying longer sequences of pulses to a two-level atom can produce a series of multi-temporal mode entangled states with properties intrinsically related to the Fibonacci sequence. Our results on photon-number entanglement can be further exploited to generate new states of quantum light with applications in quantum technologies.

quant-ph↗

arXiv2022

Experimental analysis of energy transfers between a quantum emitter and light fields

Energy transfer between quantum systems can either be achieved through an effective unitary interaction or through the generation of entanglement. This observation defines two types of energy exchange: unitary and correlation energy. Here we propose and implement experimental protocols to access these energy transfers in interactions between a quantum emitter and light fields. Upon spontaneous emission, we measure the unitary energy transfer from the emitter to the optical field and show that it never exceeds half of the total energy and is reduced when introducing decoherence. We then study the interference of the emitted field and a laser field at a beam splitter and show that the energy transfers quantitatively depend on the quantum purity of the emitted field.

quant-ph↗

arXiv2021

Three-dimensional electrical control of the excitonic fine structure for a quantum dot in a cavity

The excitonic fine structure plays a key role for the quantum light generated by semiconductor quantum dots, both for entangled photon pairs and single photons. Controlling the excitonic fine structure has been demonstrated using electric, magnetic, or strain fields, but not for quantum dots in optical cavities, a key requirement to obtain high source efficiency and near-unity photon indistinguishability. Here, we demonstrate the control of the fine structure splitting for quantum dots embedded in micropillar cavities. We propose a scheme based on remote electrical contacts connected to the pillar cavity through narrow ridges. Numerical simulations show that such a geometry allows for a three-dimensional control of the electrical field. We experimentally demonstrate tuning and reproducible canceling of the fine structure, a crucial step for the reproducibility of quantum light source technology.

quant-ph↗

arXiv2021

Bright Polarized Single-Photon Source Based on a Linear Dipole

Semiconductor quantum dots in cavities are promising single-photon sources. Here, we present a path to deterministic operation, by harnessing the intrinsic linear dipole in a neutral quantum dot via phonon-assisted excitation. This enables emission of fully polarized single photons, with a measured degree of linear polarization up to 0.994 $\pm$ 0.007, and high population inversion -- 85\% as high as resonant excitation. We demonstrate a single-photon source with a polarized first lens brightness of 0.50 $\pm $ 0.01, a single-photon purity of 0.954 $\pm$ 0.001 and single-photon indistinguishability of 0.909 $\pm$ 0.004.

quant-ph↗

arXiv2020

Fiber-based angular filtering for high-resolution Brillouin spectroscopy in the 20-300 GHz frequency range

Brillouin spectroscopy emerges as a promising non-invasive tool for nanoscale imaging and sensing. One-dimensional semiconductor superlattice structures are eminently used for selectively enhancing the generation or detection of phonons at few GHz. While commercially available Brillouin spectrometers provide high-resolution spectra, they consist of complex experimental techniques and are not suitable for semiconductor cavities operating at a wide range of optical wavelengths. We develop a pragmatic experimental approach for conventional Brillouin spectroscopy integrating a widely tunable excitation-source. Our setup combines a fibered-based angular filtering and a spectral filtering based on a single etalon and a double grating spectrometer. This configuration allows probing confined acoustic phonon modes in the 20-300 GHz frequency range with excellent laser rejection and high spectral resolution. Remarkably, our scheme based on the excitation and collection of the enhanced Brillouin scattering signals through the optical cavity, allows for better angular filtering for low phonon frequency. It can be implemented for the study of cavity optomechanics and stimulated Brillouin scattering over broadband optical and acoustic frequency ranges.

physics.optics↗

arXiv2020

Fiber-integrated microcavities for efficient generation of coherent acoustic phonons

Coherent phonon generation by optical pump-probe experiments has enabled the study of acoustic properties at the nanoscale in planar heterostructures, plasmonic resonators, micropillars and nanowires. Focalizing both pump and probe on the same spot of the sample is a critical part of pump-probe experiments. This is particularly relevant in the case of small objects. The main practical challenges for the actual implementation of this technique are: stability of the spatio-temporal overlap, reproducibility of the focalization and optical mode matching conditions. In this work, we solve these three challenges for the case of planar and micropillar optophononic cavities. We integrate the studied samples to single mode fibers lifting the need for focusing optics to excite and detect coherent acoustic phonons. The resulting excellent reflectivity contrast of at least 66% achieved in our samples allows us to observe stable coherent phonon signals over at least a full day and signals at extremely low excitation powers of 1uW. The monolithic sample structure is transportable and could provide a means to perform reproducible plug-and-play experiments.

physics.optics↗

arXiv2020

Hong-Ou-Mandel Interference with Imperfect Single Photon Sources

Hong-Ou-Mandel interference is a cornerstone of optical quantum technologies. We explore both theoretically and experimentally how the nature of unwanted multi-photon components of single photon sources affect the interference visibility. We apply our approach to quantum dot single photon sources in order to access the mean wavepacket overlap of the single-photon component - an important metric to understand the limitations of current sources. We find that the impact of multi-photon events has thus far been underestimated, and that the effect of pure dephasing is even milder than previously expected.

quant-ph↗

arXiv2020

Deterministic assembly of a charged quantum dot-micropillar cavity device

Developing future quantum communication may rely on the ability to engineer cavity-mediated interactions between photons and solid-state artificial atoms, in a deterministic way. Here, we report a set of technological and experimental developments for the deterministic coupling between the optical mode of a micropillar cavity and a quantum dot trion transition. We first identify a charged transition through in-plane magnetic field spectroscopy, and then tune the optical cavity mode to its energy via in-situ lithography. In addition, we design an asymmetric tunneling barrier to allow the optical trapping of the charge, assisted by a quasi-resonant pumping scheme, in order to control its occupation probability. We evaluate the generation of a positively-charged quantum dot through second order auto-correlation measurements of its resonance fluorescence, and the quality of light-matter interaction for these spin-photon interfaces is assessed by measuring the performance of the device as a single-photon source.

quant-ph↗

arXiv2020

Sequential generation of linear cluster states from a single photon emitter

Light states composed of multiple entangled photons - such as cluster states - are essential for developing and scaling-up quantum computing networks. Photonic cluster states with discrete variables can be obtained from single-photon sources and entangling gates, but so far this has only been done with probabilistic sources constrained to intrinsically-low efficiencies, and an increasing hardware overhead. Here, we report the resource-efficient generation of polarization-encoded, individually-addressable, photons in linear cluster states occupying a single spatial mode. We employ a single entangling-gate in a fiber loop configuration to sequentially entangle an ever-growing stream of photons originating from the currently most efficient single-photon source technology - a semiconductor quantum dot. With this apparatus, we demonstrate the generation of linear cluster states up to four photons in a single-mode fiber. The reported architecture can be programmed to generate linear-cluster states of any number of photons with record scaling ratios, potentially enabling practical implementation of photonic quantum computing schemes.

quant-ph↗

arXiv2019

Interfacing scalable photonic platforms: solid-state based multi-photon interference in a reconfigurable glass chip

Scaling-up optical quantum technologies requires to combine highly efficient multi-photon sources and integrated waveguide components. Here, we interface these scalable platforms: a quantum dot based multi-photon source and a reconfigurable photonic chip on glass are combined to demonstrate high-rate three-photon interference. The temporal train of single-photons obtained from a quantum emitter is actively demultiplexed to generate a 3.8 kHz three-photon source, which is then sent to the input of a tuneable tritter circuit, demonstrating the on-chip quantum interference of three indistinguishable single-photons. Pseudo number-resolving photon detection characterising the output distribution shows that this first combination of scalable sources and reconfigurable photonic circuits compares favourably in performance with respect to previous implementations. A detailed loss-budget shows that merging solid-state based multi-photon sources and reconfigurable photonic chips could allow ten-photon experiments on chip at ${\sim}40$ Hz rate in a foreseeable future.

quant-ph↗