arXiv subjects

P. Senellart

Publications and source records attributed to P. Senellart.

At least 37 records · Page 2Linked to original sources

arXiv2018

Brillouin Scattering in Hybrid Optophononic Bragg Micropillar Resonators at 300 GHz

We introduce a monolithic Brillouin generator based on a semiconductor micropillar cavity embedding a high frequency nanoacoustic resonator operating in the hundreds of GHz range. The concept of two nested resonators allows an independent design of the ultrahigh frequency Brillouin spectrum and of the optical device. We develop an optical free-space technique to characterize spontaneous Brillouin scattering in this monolithic device and propose a measurement protocol that maximizes the Brillouin generation efficiency in the presence of optically induced thermal effects. The compact and versatile Brillouin generator studied here could be readily integrated into fibered and on-chip architectures.

physics.optics↗

arXiv2018

Generation of non-classical light in a photon-number superposition

The ability to generate light in a pure quantum state is essential for advances in optical quantum technologies. However, obtaining quantum states with control in the photon-number has remained elusive. Optical light fields with zero and one photon can be produced by single atoms, but so far it has been limited to generating incoherent mixtures, or coherent superpositions with a very small one-photon term. Here, we report on the on-demand generation of quantum superpositions of zero, one, and even two photons, via pulsed coherent control of a single artificial atom. Driving the system up to full atomic inversion leads to the generation of quantum superpositions of vacuum and one photon, with their relative populations controlled by the driving laser intensity. A stronger driving of the system, with $2π$-pulses, results in a coherent superposition of vacuum, one and two photons, with the two-photon term exceeding the one-photon component, a state allowing phase super-resolving interferometry. Our results open new paths for optical quantum technologies with access to the photon-number degree-of-freedom.

quant-ph↗

arXiv2018

Accurate measurement of a 96% input coupling into a cavity using polarization tomography

Pillar microcavities are excellent light-matter interfaces providing an electromagnetic confinement in small mode volumes with high quality factors. They also allow the efficient injection and extraction of photons, into and from the cavity, with potentially near-unity input and output-coupling efficiencies. Optimizing the input and output coupling is essential, in particular, in the development of solid-state quantum networks where artificial atoms are manipulated with single incoming photons. Here we propose a technique to accurately measure input and output coupling efficiencies using polarization tomography of the light reflected by the cavity. We use the residual birefringence of pillar microcavities to distinguish the light coupled to the cavity from the uncoupled light: the former participates to rotating the polarization of the reflected beam, while the latter decreases the polarization purity. Applying this technique to a micropillar cavity, we measure a $53 \pm2 \% $ output coupling and a $96 \pm 1\%$ input coupling with unprecedented precision.

quant-ph↗

arXiv2017

Nanomechanical resonators based on adiabatic periodicity-breaking in a superlattice

We propose a novel acoustic cavity design where we confine a mechanical mode by adiabatically changing the acoustic properties of a GaAs/AlAs superlattice. By means of high resolution Raman scattering measurements, we experimentally demonstrate the presence of a confined acoustic mode at a resonance frequency around 350 GHz. We observe an excellent agreement between the experimental data and numerical simulations based on a photoelastic model. We demonstrate that the spatial profile of the confined mode can be tuned by changing the magnitude of the adiabatic deformation, leading to strong variations of its mechanical quality factor and Raman scattering cross section. The reported alternative confinement method could lead to the development of a novel generation of nanophononic and optomechanical systems.

cond-mat.mes-hall↗

arXiv2017

Optomechanical properties of GaAs/AlAs micropillar resonators operating in the 18 GHz range

Recent experiments demonstrated that GaAs-AlAs based micropillar cavities are promising systems for quantum optomechanics, allowing the simultaneous three-dimensional confinement of near-infrared photons and acoustic phonons in the 18-100 GHz range. Here, we investigate through numerical simulations the optomechanical properties of this new platform. We evidence how the Poisson's ratio and semiconductor-vacuum boundary conditions lead to very distinct features in the mechanical and optical three dimensional confinement. We find a strong dependence of the mechanical quality factor and strain distribution on the micropillar radius, in great contrast to what is predicted and observed in the optical domain. The derived optomechanical coupling constants g_0 reach ultra-large values in the 10^6 rad/s range.

cond-mat.mes-hall↗

arXiv2017

Overcomplete quantum tomography of a path-entangled two-photon state

Path-entangled N-photon states can be obtained through the coalescence of indistinguishable photons inside linear networks. They are key resources for quantum enhanced metrology, quantum imaging, as well as quantum computation based on quantum walks. However, the quantum tomography of path-entangled indistinguishable photons is still in its infancy as it requires multiple phase estimations increasing rapidly with N. Here, we propose and implement a method to measure the quantum tomography of path-entangled two-photon states. A two-photon state is generated through the Hong-Ou-Mandel interference of highly indistinguishable single photons emitted by a semiconductor quantum dot-cavity device. To access both the populations and the coherences of the path-encoded density matrix, we introduce an ancilla spatial mode and perform photon correlations as a function of a single phase in a split Mach-Zehnder interferometer. We discuss the accuracy of standard quantum tomography techniques and show that an overcomplete data set can reveal spatial coherences that could be otherwise hidden due to limited or noisy statistics. Finally, we extend our analysis to extract the truly indistinguishable part of the density matrix, which allows us to identify the main origin for the imperfect fidelity to the maximally entangled state.

quant-ph↗

arXiv2017

BosonSampling with single-photon Fock states from a bright solid-state source

A BosonSampling device is a quantum machine expected to perform tasks intractable for a classical computer, yet requiring minimal non-classical resources as compared to full-scale quantum computers. Photonic implementations to date employed sources based on inefficient processes that only simulate heralded single-photon statistics when strongly reducing emission probabilities. BosonSampling with only single-photon input has thus never been realised. Here, we report on a BosonSampling device operated with a bright solid-state source of single-photon Fock states with high photon-number purity: the emission from an efficient and deterministic quantum dot-micropillar system is demultiplexed into three partially-indistinguishable single-photons, with a single-photon purity $1{-}g^{(2)}(0)$ of $0.990{\pm}0.001$, interfering in a linear optics network. Our demultiplexed source is between one and two orders-of-magnitude more efficient than current heralded multi-photon sources based on spontaneous parametric downconversion, allowing us to complete the BosonSampling experiment faster than previous equivalent implementations.

quant-ph↗

arXiv2017

Tomography of optical polarization rotation induced by a quantum dot-cavity device

We introduce a tomography approach to describe the optical response of a cavity quantum electrodynamics device, beyond the semiclassical image of polarization rotation, by analyzing the polarization density matrix of the reflected photons in the Poincaré sphere. Applying this approach to an electrically-controlled quantum dot-cavity device, we show that a single resonantly-excited quantum dot induces a large optical polarization rotation by $20^\circ$ in latitude and longitude in the Poincaré sphere, with a polarization purity remaining above $84\%$. The quantum dot resonance fluorescence is shown to contribute to the polarization rotation via its coherent part, whereas its incoherent part contributes to degrading the polarization purity.

cond-mat.mes-hall↗

arXiv2016

Active demultiplexing of single-photons from a solid-state source

A scheme for active temporal-to-spatial demultiplexing of single-photons generated by a solid-state source is introduced. The scheme scales quasi-polynomially with photon number, providing a viable technological path for routing n photons in the one temporal stream from a single emitter to n different spatial modes. The active demultiplexing is demonstrated using a state-of-the-art photon source---a quantum-dot deterministically coupled to a micropillar cavity---and a custom-built demultiplexer---a network of electro-optically reconfigurable waveguides monolithically integrated in a lithium niobate chip. The measured demultiplexer performance can enable a six-photon rate three orders of magnitude higher than the equivalent heralded SPDC source, providing a platform for intermediate quantum computation protocols.

quant-ph↗

arXiv2016

Time-Resolved Cavity Nano-Optomechanics in the 20-100 GHz range

Applications of cavity optomechanics span from gravitational wave detection to the study of quantum motion states in mesoscopic mechanical systems. The engineering of resonators supporting strongly interacting mechanical and optical modes is central to these developments. However, current technological and experimental approaches limit the accessible mechanical frequencies to a few GHz, imposing hard constraints on quantum mechanical studies. Here we demonstrate the optical control of 20-100~GHz mechanical modes confined in the three dimensions within semiconductor nano-optomechanical pillar cavities. We use a time-resolved transient optical reflectivity technique and access both the energy spectrum and dynamics of the mechanical modes at the picosecond timescale. A strong increase of the optomechanical coupling upon reducing the pillar size is observed together with unprecedent room temperature Q-frequency products above $10^{14}$. The measurements also reveal sideband generation in the optomechanical response. Such resonators can naturally integrate quantum wells and quantum dots, enabling novel applications in cavity quantum electrodynamics and high frequency nanomechanics.

physics.optics↗

arXiv2016

A solid-state single-photon filter

A strong limitation of linear optical quantum computing is the probabilistic operation of two-quantum bit gates based on the coalescence of indistinguishable photons. A route to deterministic operation is to exploit the single-photon nonlinearity of an atomic transition. Through engineering of the atom-photon interaction, phase shifters, photon filters and photon- photon gates have been demonstrated with natural atoms. Proofs of concept have been reported with semiconductor quantum dots, yet limited by inefficient atom-photon interfaces and dephasing. Here we report on a highly efficient single-photon filter based on a large optical non-linearity at the single photon level, in a near-optimal quantum-dot cavity interface. When probed with coherent light wavepackets, the device shows a record nonlinearity threshold around $0.3 \pm 0.1$ incident photons. We demonstrate that directly reflected pulses consist of 80% single-photon Fock state and that the two- and three-photon components are strongly suppressed compared to the single-photon one.

quant-ph↗

arXiv2016

Scalable performance in solid-state single-photon sources

The desiderata for an ideal photon source are high brightness, high single-photon purity, and high indistinguishability. Defining brightness at the first collection lens, these properties have been simultaneously demonstrated with solid-state sources, however absolute source efficiencies remain close to the 1% level, and indistinguishability only demonstrated for photons emitted consecutively on the few nanosecond scale. Here we employ deterministic quantum dot-micropillar devices to demonstrate solid-state single-photon sources with scalable performance. In one device, an absolute brightness at the output of a single-mode fibre of 14% and purities of 97.1-99.0% are demonstrated. When non-resontantly excited, it emits a long stream of photons that exhibit indistinguishability up to 70%---above the classical limit of 50%---even after 33 consecutively emitted photons, a 400 ns separation between them. Resonant excitation in other devices results in near-optimal indistinguishability values: 96% at short timescales, remaining at 88% in timescales as large as 463 ns, after 39 emitted photons. The performance attained by our devices brings solid-state sources into a regime suitable for scalable implementations.

quant-ph↗

arXiv2015

Coherent control of a solid-state quantum bit with few-photon pulses

Single photons are the natural link between the nodes of a quantum network: they coherently propagate and interact with many types of quantum bits including natural and artificial atoms. Ideally, one atom should deterministically control the state of a photon and vice-versa. The interaction between free space photons and an atom is however intrinsically weak and many efforts have been dedicated to develop an efficient interface. Recently, it was shown that the propagation of light can be controlled by an atomic resonance coupled to a cavity or a single mode waveguide. Here we demonstrate that the state of a single artificial atom in a cavity can be efficiently controlled by a few-photon pulse. We study a quantum dot optimally coupled to an electrically-controlled cavity device, acting as a near optimal one-dimensional atom. By monitoring the exciton population through resonant fluorescence, we demonstrate Rabi oscillations with a $π$-pulse of only 3.8 photons on average. The probability to flip the exciton quantum bit with a single photon Fock state is calculated to reach 55% in the same device.

quant-ph↗

arXiv2015

Near optimal single photon sources in the solid state

Single-photons are key elements of many future quantum technologies, be it for the realisation of large-scale quantum communication networks for quantum simulation of chemical and physical processes or for connecting quantum memories in a quantum computer. Scaling quantum technologies will thus require efficient, on-demand, sources of highly indistinguishable single-photons. Semiconductor quantum dots inserted in photonic structures are ultrabright single photon sources, but the photon indistinguishability is limited by charge noise induced by nearby surfaces. The current state of the art for indistinguishability are parametric down conversion single-photon sources, but they intrinsically generate multiphoton events and hence must be operated at very low brightness to maintain high single photon purity. To date, no technology has proven to be capable of providing a source that simultaneously generates near-unity indistinguishability and pure single photons with high brightness. Here, we report on such devices made of quantum dots in electrically controlled cavity structures. We demonstrate on-demand, bright and ultra-pure single photon generation. Application of an electrical bias on deterministically fabricated devices is shown to fully cancel charge noise effects. Under resonant excitation, an indistinguishability of $0.9956\pm0.0045$ is evidenced with a $g^{2}(0)=0.0028\pm0.0012$. The photon extraction of $65%$ and measured brightness of $0.154\pm0.015$ make this source $20$ times brighter than any source of equal quality. This new generation of sources open the way to a new level of complexity and scalability in optical quantum manipulation.

quant-ph↗

arXiv2015

Cavity-Enhanced Two-Photon Interference using Remote Quantum Dot Sources

Quantum dots in cavities have been shown to be very bright sources of indistinguishable single photons. Yet the quantum interference between two bright quantum dot sources, a critical step for photon based quantum computation, has never been investigated. Here we report on such a measurement, taking advantage of a deterministic fabrication of the devices. We show that cavity quantum electrodynamics can efficiently improve the quantum interference between remote quantum dot sources: poorly indistinguishable photons can still interfere with good contrast with high quality photons emitted by a source in the strong Purcell regime. Our measurements and calculations show that cavity quantum electrodynamics is a powerful tool for interconnecting several devices.

cond-mat.mes-hall↗

arXiv2013

Dynamic nuclear polarization in InGaAs/GaAs and GaAs/AlGaAs quantum dots under non-resonant ultra-low power optical excitation

We study experimentally the dependence of dynamic nuclear spin polarization on the power of non-resonant optical excitation in two types of individual neutral semiconductor quantum dots: InGaAs/GaAs and GaAs/AlGaAs. We show that the mechanism of nuclear spin pumping via second order recombination of optically forbidden (''dark'') exciton states recently reported in InP/GaInP quantum dots [Phys. Rev. B 83, 125318 (2011)] is relevant for material systems considered in this work. In the InGaAs/GaAs dots this nuclear spin polarization mechanism is particularly pronounced, resulting in Overhauser shifts up to ~80 micro-eV achieved at optical excitation power ~1000 times smaller than the power required to saturate ground state excitons. The Overhauser shifts observed at low-power optical pumping in the interface GaAs/AlGaAs dots are generally found to be smaller (up to ~40 micro-eV). Furthermore in GaAs/AlGaAs we observe dot-to-dot variation and even sign reversal of the Overhauser shift which is attributed to dark-bright exciton mixing originating from electron-hole exchange interaction in dots with reduced symmetry. Nuclear spin polarization degrees reported in this work under ultra-low power optical pumping are comparable to those achieved by techniques such as resonant optical pumping or above-gap pumping with high power circularly polarized light. Dynamic nuclear polarization via second-order recombination of ''dark'' excitons may become a useful tool in single quantum dot applications, where manipulation of the nuclear spin environment or electron spin is required.

cond-mat.mes-hall↗

arXiv2013

An entangling quantum-logic gate operated with an ultrabright single photon-source

We demonstrate unambiguous entangling operation of a photonic quantum-logic gate driven by an ultrabright solid-state single-photon source. Indistinguishable single photons emitted by a single semiconductor quantum dot in a micropillar optical cavity are used as target and control qubits. For a source brightness of 0.56 collected photons-per-pulse, the measured truth table has an overlap with the ideal case of 68.4%, increasing to 73.0% for a source brightness of 0.17 photons- per-pulse. The gate is entangling: at a source brightness of 0.48, the Bell-state fidelity is above the entangling threshold of 50%, and reaches 71.0% for a source brightness of 0.15.

quant-ph↗

arXiv2012

Isotope sensitive measurement of the hole-nuclear spin interaction in quantum dots

Decoherence caused by nuclear field fluctuations is a fundamental obstacle to the realization of quantum information processing using single electron spins. Alternative proposals have been made to use spin qubits based on valence band holes having weaker hyperfine coupling. However, it was demonstrated recently both theoretically and experimentally that the hole hyperfine interaction is not negligible, although a consistent picture of the mechanism controlling the magnitude of the hole-nuclear coupling is still lacking. Here we address this problem by performing isotope selective measurement of the valence band hyperfine coupling in InGaAs/GaAs, InP/GaInP and GaAs/AlGaAs quantum dots. Contrary to existing models we find that the hole hyperfine constant along the growth direction of the structure (normalized by the electron hyperfine constant) has opposite signs for different isotopes and ranges from -15% to +15%. We attribute such changes in hole hyperfine constants to the competing positive contributions of p-symmetry atomic orbitals and the negative contributions of d-orbitals. Furthermore, we find that the d-symmetry contribution leads to a new mechanism for hole-nuclear spin flips which may play an important role in hole spin decoherence. In addition the measured hyperfine constants enable a fundamentally new approach for verification of the computed Bloch wavefunctions in the vicinity of nuclei in semiconductor nanostructures.

cond-mat.mes-hall↗