arXiv subjects

P. Van Duppen

Publications and source records attributed to P. Van Duppen.

At least 19 recordsLinked to original sources

arXiv2026

Exploring $α$- and $β$-decay-induced quenching of the $^{229}$Th nuclear-clock isomer in solid-state hosts

The radiative decay dynamics of an ensemble of $^{229\mathrm{m}}$Th nuclei embedded in CaF$_2$ and MgF$_2$ is investigated. The isomer is populated through $β$ decay of $^{229}$Ac following ion implantation, and its radiative decay is detected using vacuum-ultraviolet spectroscopy and measured as a function of time. This allows to identify and quantify the quenching of the radiative-decay signal induced by $α$ or $β$ radiation. The quenching probability density is determined in different CaF$_2$ crystals and in a MgF$_2$ crystal, revealing differences up to two orders of magnitude between the investigated samples and a strong dependence on the host material and defect densities. The results support a microscopic mechanism mediated by charge carriers in which electronic excitations created by the decay radiation are captured near Th defects, thereby favoring non-radiative decay channels.

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arXiv2026

Beta delayed neutron emission of $N=84$ $^{132}$Cd

Using the time-of-flight technique, we measured the beta-delayed neutron emission of $^{132}$Cd. From our large-scale shell model (LSSM) calculation using the N$^3$LO interaction [Z.Y. Xu et al., Phys. Rev. Lett. 131, 022501 (2023)], we suggest the decay is dominated by the transformation of a neutron in the $g_{7/2}$ orbital, deep below the Fermi surface, into a proton in the $g_{9/2}$ orbital. We compare the beta-decay half-lives and neutron branching ratios of nuclei with $Z<50$ and $N\geq82$ obtained with our LSSM with those of leading "global" models such as Finite-Range Droplet Model (FRDM). Our calculations match known half-lives and neutron branching ratios well and suggest that current leading models overestimate the yet-to-be-measured half-lives. Our model, backed by the $^{132}$Cd decay data presented here, offers robust predictive power for nuclei of astrophysical interest such as $r$-process waiting points.

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arXiv2025

An experimental setup for the study of gas-cell processes for the S$^3$-Low Energy Branch

We present an experimental setup dedicated to the study of in-gas ion processes and characterization of gas stopping cells for the Low Energy Branch of the Super Separator Spectrometer (S$^3$) at SPIRAL2-GANIL. The first application is the development of a new gas stopper with a neutralization mechanism designed for faster extraction of the radioactive ions. This development should enable in-gas-jet laser spectroscopy and other low-energy experiments with shorter lived radioactive isotopes. We discuss in detail the motivation and objectives of these developments and we present the results of simulations performed in the design phase, as well as the first experimental results.

physics.ins-det↗

arXiv2025

Study of thorium in hypersonic gas jets: Ionization potentials of Th and Th$^+$

Laser ionization spectroscopy was performed on both neutral and singly ionized $^{232}$Th with the aim of identifying the nuclear-clock isomer in the singly charged ionic state of $^{229}$Th. A search for an efficient laser ionization scheme of $^{232}$Th$^+$ was conducted in an argon-filled gas cell. This revealed a congested spectrum due to collisional quenching effects and the presence of several auto-ionizing states, one of which has a laser ionization efficiency of at least $1.2 \%$. Using a threshold approach, the second ionization potential was determined to be $12.300(9)\,$eV. The subsequent study on atomic $^{232}$Th validated the threshold approach. Conducting spectroscopy in a hypersonic gas jet, suppressed the gas-collision-induced quenching, revealing a Rydberg series that converges to the first ionization potential, determined to be $6.306879(14)\,$eV. The gas jet also cools down the thorium, allowing for high-resolution laser spectroscopy with a resolution of $240(30)\,$MHz. Using the Multiconfigurational Dirac-Hartree-Fock (MCDHF) method, the ionization potentials were computed, showing a relative difference of 0.06\% and 0.19\% between theory and our experimental values for the ionization potentials of Th and Th$^+$ respectively. Further calculations using a pseudo-relativistic Hartree-Fock method reveal strong mixing in the used intermediate state at $26113.27\,$cm$^{-1}$ of Th. A dedicated fast-extraction gas cell with $^{233}$U recoil sources was used to study $^{229}$Th$^+$ but no photo-ionization signal could be observed.

physics.atom-ph↗

arXiv2025

The 76Cu conundrum remains unsolved

Near the doubly-magic nucleus \nuc{Ni}{78} ($Z=28$, $N=50$), there has been a decades-long debate on the existence of a long-lived isomer in \nuc{Cu}{76}. A recent mass measurement claimed to have settled the debate, by measuring the energy of the isomer and shedding light on the structure of the nucleus. In this work, we present new, more accurate, and precise values of the half-lives of the isomeric and ground states in \nuc{Cu}{76}. Our findings suggest that both states have very similar half-lives, in the 600-700 ms range, in disagreement with the literature values, implying that they cannot be differentiated by their decay curves. These results raise more questions than they answer, reopening the debate and showing that the structures in \nuc{Cu}{76} are still not fully understood.

nucl-ex↗

arXiv2024

Revealing the nature of yrast states in neutron-rich polonium isotopes

Polonium isotopes having two protons above the shell closure at $Z=82$ show a wide variety of low-lying high-spin isomeric states across the whole chain. The structure of neutron-deficient isotopes up to $^{210}$Po ($N=126$) is well established as they are easily produced through various methods. However, there is not much information available for the neutron-rich counterparts for which only selective techniques can be used for their production. We report on the first fast-timing measurements of yrast states up to the 8$^+$ level in $^{214,216,218}$Po isotopes produced in the $β^-$ decay of $^{214,216,218}$Bi at ISOLDE, CERN. In particular, our new half-life value of 607(14) ps for the 8$_1^+$ state in $^{214}$Po is nearly 20 times shorter than the one available in literature and comparable with the newly measured half-lives of 409(16) and 628(25) ps for the corresponding 8$_1^+$ states in $^{216,218}$Po, respectively. The measured $B(E2;8_1^+ \to 6_1^+)$ transition probability values follow an increasing trend relative to isotope mass, reaching a maximum for $^{216}$Po. The increase contradicts the previous claims of isomerism for the $8^+$ yrast states in neutron-rich $^{214}$Po and beyond. Together with the other measured yrast transitions, the $B(E2)$ values provide a crucial test of the different theoretical approaches describing the underlying configurations of the yrast band. The new experimental results are compared to shell-model calculations using the KHPE and H208 effective interactions and their pairing modified versions, showing an increase in configuration mixing when moving towards the heavier isotopes.

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arXiv2024

Radiative Decay of the $^{229m}$Th Nuclear Clock Isomer in Different Host Materials

A comparative vacuum ultraviolet spectroscopy study conducted at ISOLDE-CERN of the radiative decay of the $^{229m}$Th nuclear clock isomer embedded in different host materials is reported. The ratio of the number of radiative decay photons and the number of $^{229m}$Th embedded are determined for single crystalline CaF$_2$, MgF$_2$, LiSrAlF$_6$, AlN, and amorphous SiO$_2$. For the latter two materials, no radiative decay signal was observed and an upper limit of the ratio is reported. The radiative decay wavelength was determined in LiSrAlF$_6$ and CaF$_2$, reducing its uncertainty by a factor of 2.5 relative to our previous measurement. This value is in agreement with the recently reported improved values from laser excitation.

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arXiv2023

Simultaneous $γ$-ray and electron spectroscopy of $^{182,184,186}$Hg isotopes

Background: The mercury isotopes around $N=104$ are a well-known example of nuclei exhibiting shape coexistence. Mixing of configurations can be studied by measuring the monopole strength $ρ^2(E0)$, however, currently the experimental information is scarce and lacks precision, especially for the $I^π\rightarrow I^π$ ($I \neq 0$) transitions. Purpose: The goals of this study were to increase the precision of the known branching ratios and internal conversion coefficients, to increase the amount of available information regarding excited states in $^{182,184,186}$Hg and to interpret the results in the framework of shape coexistence using different models. Method: The low-energy structures in $^{182,184,186}$Hg were populated in the $β$ decay of $^{182,184,186}$Tl, produced at ISOLDE and purified by laser ionization and mass separation. The $γ$-ray and internal conversion electron events were detected by five germanium clover detectors and a segmented silicon detector, respectively, and correlated in time to build decay schemes. Results: In total, 193, 178 and 156 transitions, including 144, 140 and 108 observed for the first time in a $β$-decay experiment, were assigned to $^{182,184,186}$Hg, respectively. Internal conversion coefficients were determined for 23 transitions, out of which 12 had an $E0$ component. Extracted branching ratios allowed the sign of the interference term in $^{182}$Hg as well as $ρ^2(E0;0^+_2\rightarrow 0^+_1)$ and $B(E2;0^+_2\rightarrow 2^+_1)$ in $^{184}$Hg to be determined. By means of electron-electron coincidences, the $0^+_3$ state was identified in $^{184}$Hg. The experimental results were qualitatively reproduced by five theoretical approaches, the IBM with configuration mixing with two different parametrizations, the General Bohr Hamiltonian, the BMF model and the SCCM model. However, a quantitative description is lacking.

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arXiv2023

133In: A Rosetta Stone for decays of r-process nuclei

The $β$ decays from both the ground state and a long-lived isomer of $^{133}$In were studied at the ISOLDE Decay Station (IDS). With a hybrid detection system sensitive to $β$, $γ$, and neutron spectroscopy, the comparative partial half-lives (logft) have been measured for all their dominant $β$-decay channels for the first time, including a low-energy Gamow-Teller transition and several First-Forbidden (FF) transitions. Uniquely for such a heavy neutron-rich nucleus, their $β$ decays selectively populate only a few isolated neutron unbound states in $^{133}$Sn. Precise energy and branching-ratio measurements of those resonances allow us to benchmark $β$-decay theories at an unprecedented level in this region of the nuclear chart. The results show good agreement with the newly developed large-scale shell model (LSSM) calculations. The experimental findings establish an archetype for the $β$ decay of neutron-rich nuclei southeast of $^{132}$Sn and will serve as a guide for future theoretical development aiming to describe accurately the key $β$ decays in the rapid-neutron capture (r-) process.

nucl-ex↗

arXiv2023

Beta-delayed neutron spectroscopy of $^{133}$In

The decay properties of $^{133}$In were studied in detail at the ISOLDE Decay Station (IDS). The implementation of the Resonance Ionization Laser Ion Source (RILIS) allowed separate measurements of its $9/2^+$ ground state ($^{133g}$In) and $1/2^-$ isomer ($^{133m}$In). With the use of $β$-delayed neutron and $γ$ spectroscopy, the decay strengths above the neutron separation energy were quantified in this neutron-rich nucleus for the first time. The allowed Gamow-Teller transition $9/2^+\rightarrow7/2^+$ was located at 5.92 MeV in the $^{133g}$In decay with a logft = 4.7(1). In addition, several neutron-unbound states were populated at lower excitation energies by the First-Forbidden decays of $^{133g,m}$In. We assigned spins and parities to those neutron-unbound states based on the $β$-decay selection rules, the logft values, and systematics.

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arXiv2021

Charge radii, moments and masses of mercury isotopes across the N = 126 shell closure

Combining laser spectroscopy in a Versatile Arc Discharge and Laser Ion Source, with Penning-trap mass spectrometry at the CERN-ISOLDE facility, this work reports on mean-square charge radii of neutron-rich mercury isotopes across the $N = 126$ shell closure, the electromagnetic moments of $^{207}$Hg and more precise mass values of $^{206-208}$Hg. The odd-even staggering (OES) of the mean square charge radii and the kink at $N = 126$ are analyzed within the framework of covariant density functional theory (CDFT), with comparisons between different functionals to investigate the dependence of the results on the underlying single-particle structure. The observed features are defined predominantly in the particle-hole channel in CDFT, since both are present in the calculations without pairing. However, the magnitude of the kink is still affected by the occupation of the $1i_{11/2}$ and $2g_{9/2}$ orbitals with a dependence on the relative energies as well as pairing.

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arXiv2020

Laser spectroscopy of neutron-rich $^{207,208}$Hg isotopes: Illuminating the kink and odd-even staggering in charge radii across the $N=126$ shell closure

The mean-square charge radii of $^{207,208}$Hg ($Z=80, N=127,128$) have been studied for the first time and those of $^{202,203,206}$Hg ($N=122,123,126$) remeasured by the application of in-source resonance-ionization laser spectroscopy at ISOLDE (CERN). The characteristic \textit{kink} in the charge radii at the $N=126$ neutron shell closure has been revealed, providing the first information on its behavior below the $Z=82$ proton shell closure. A theoretical analysis has been performed within relativistic Hartree-Bogoliubov and non-relativistic Hartree-Fock-Bogoliubov approaches, considering both the new mercury results and existing lead data. Contrary to previous interpretations, it is demonstrated that both the kink at $N=126$ and the odd-even staggering (OES) in its vicinity can be described predominately at the mean-field level, and that pairing does not need to play a crucial role in their origin. A new OES mechanism is suggested, related to the staggering in the occupation of the different neutron orbitals in odd- and even-$A$ nuclei, facilitated by particle-vibration coupling for odd-$A$ nuclei.

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arXiv2020

Decay studies of the long-lived states in $^{186}$Tl

Decay spectroscopy of the long-lived states in $^{186}$Tl has been performed at the ISOLDE Decay Station at ISOLDE, CERN. The $α$ decay from the low-spin $(2^-)$ state in $^{186}$Tl was observed for the first time and a half-life of $3.4^{+0.5}_{-0.4}$ s was determined. Based on the $α$-decay energy, the relative positions of the long-lived states were fixed, with the $(2^-)$ state as the ground state, the $7^{(+)}$ state at 77(56)~keV and the $10^{(-)}$ state at 451(56) keV. The level scheme of the internal decay of the $^{186}$Tl($10^{(-)}$) state ($T_{1/2} = 3.40(9)$ s), which was known to decay solely through emission of 374 keV $γ$-ray transition, was extended and a lower-limit for the $β$-decay branching $b_β> 5.9(3)\%$ was determined. The extracted retardation factors for the $γ$ decay of the $10^{(-)}$ state were compared to the available data in neighboring odd-odd thallium isotopes indicating the importance of the $πd_{3/2}$ shell in the isomeric decay and significant structure differences between $^{184}$Tl and $^{186}$Tl.

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arXiv2020

Detailed spectroscopy of doubly magic $^{132}$Sn

The structure of the doubly magic $^{132}_{50}$Sn$_{82}$ has been investigated at the ISOLDE facility at CERN, populated both by the $β^-$decay of $^{132}$In and $β^-$-delayed neutron emission of $^{133}$In. The level scheme of $^{132}$Sn is greatly expanded with the addition of 68 $γ$-transitions and 17 levels observed for the first time in the $β$ decay. The information on the excited structure is completed by new $γ$-transitions and states populated in the $β$-n decay of $^{133}$In. Improved delayed neutron emission probabilities are obtained both for $^{132}$In and $^{133}$In. Level lifetimes are measured via the Advanced Time-Delayed $βγγ$(t) fast-timing method. An interpretation of the level structure is given based on the experimental findings and the particle-hole configurations arising from core excitations both from the \textit{N} = 82 and \textit{Z} = 50 shells, leading to positive and negative parity particle-hole multiplets. The experimental information provides new data to challenge the theoretical description of $^{132}$Sn.

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arXiv2020

The observation of vibrating pear shapes in radon nuclei: update

There is a large body of evidence that atomic nuclei can undergo octupole distortion and assume the shape of a pear. This phenomenon is important for measurements of electric-dipole moments of atoms, which would indicate CP violation and hence probe physics beyond the standard model of particle physics. Isotopes of both radon and radium have been identified as candidates for such measurements. Here, we have observed the low-lying quantum states in $^{224}$Rn and $^{226}$Rn by accelerating beams of these radioactive nuclei. We report here additional states not assigned in our 2019 publication. We show that radon isotopes undergo octupole vibrations but do not possess static pear-shapes in their ground states. We conclude that radon atoms provide less favourable conditions for the enhancement of a measurable atomic electric-dipole moment.

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arXiv2020

Evolution of Octupole Deformation in Radium Nuclei from Coulomb Excitation of Radioactive $^{222}$Ra and $^{228}$Ra Beams

There is sparse direct experimental evidence that atomic nuclei can exhibit stable pear shapes arising from strong octupole correlations. In order to investigate the nature of octupole collectivity in radium isotopes, electric octupole ($E3$) matrix elements have been determined for transitions in $^{222,228}$Ra nuclei using the method of sub-barrier, multi-step Coulomb excitation. Beams of the radioactive radium isotopes were provided by the HIE-ISOLDE facility at CERN. The observed pattern of $E$3 matrix elements for different nuclear transitions is explained by describing $^{222}$Ra as pear-shaped with stable octupole deformation, while $^{228}$Ra behaves like an octupole vibrator.

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arXiv2019

Normal and intruder configurations in $^{34}$Si populated in the $β^-$ decay of $^{34}$Mg and $^{34}$Al

The structure of $^{34}$Si was studied through $γ$ spectroscopy separately in the $β^-$ decays of $^{34}$Mg and $^{34}$Al at the ISOLDE facility of CERN. Different configurations in $^{34}$Si were populated independently from the two recently identified $β$-decaying states in $^{34}$Al having spin-parity assignments $J^π= 4^-$ dominated by the normal configuration $π(d_{5/2})^{-1} \otimes ν(f_{7/2})$ and $J^π= 1^+$ by the intruder configuration $π(d_{5/2})^{-1} \otimes ν(d_{3/2})^{-1}(f_{7/2})^{2}$. The paper reports on spectroscopic properties of $^{34}$Si such as an extended level scheme, spin and parity assignments based on log($ft$) values and $γ$-ray branching ratios, absolute $β$ feeding intensities and neutron emission probabilities. A total of 11 newly identified levels and 26 transitions were added to the previously known level scheme of $^{34}$Si. Large scale shell-model calculations using the {\sc sdpf-u-mix} interaction, able to treat higher order intruder configurations, are compared with the new results and conclusions are drawn concerning the predictive power of {\sc sdpf-u-mix}, the $N=20$ shell gap, the level of mixing between normal and intruder configurations for the 0$_1^+$, 0$_2^+$ and 2$_1^+$ states and the absence of triaxial deformation in $^{34}$Si.

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arXiv2019

An alternative approach to populate and study the $^{229}$Th nuclear clock isomer

A new approach to observe the radiative decay of the $^{229}$Th nuclear isomer, and to determine its energy and radiative lifetime, is presented. Situated at a uniquely low excitation energy, this nuclear state might be a key ingredient for the development of a nuclear clock, a nuclear laser and the search for time variations of the fundamental constants. The isomer's $γ$ decay towards the ground state will be studied with a high-resolution VUV spectrometer after its production by the $β$ decay of $^{229}$Ac. The novel production method presents a number of advantages asserting its competitive nature with respect to the commonly used $^{233}$U $α$-decay recoil source. In this paper, a feasibility analysis of this new concept, and an experimental investigation of its key ingredients, using a pure $^{229}$Ac ion beam produced at the ISOLDE radioactive beam facility, is reported.

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