arXiv subjects

P. Van Duppen

Publications and source records attributed to P. Van Duppen.

At least 37 records · Page 2Linked to original sources

arXiv2019

Shape staggering of mid-shell mercury isotopes from in-source laser spectroscopy compared with Density Functional Theory and Monte Carlo Shell Model calculations

Neutron-deficient $^{177-185}$Hg isotopes were studied using in-source laser resonance-ionization spectroscopy at the CERN-ISOLDE radioactive ion-beam facility, in an experiment combining different detection methods tailored to the studied isotopes. These include either alpha-decay tagging or Multi-reflection Time-of-Flight gating to identify the isotopes of interest. The endpoint of the odd-even nuclear shape staggering in mercury was observed directly by measuring for the first time the isotope shifts and hyperfine structures of $^{177-180}$Hg. Changes in the mean-square charge radii for all mentioned isotopes, magnetic dipole and electric quadrupole moments of the odd-A isotopes and arguments in favor of $I = 7/2$ spin assignment for $^{177,179}$Hg were deduced. Experimental results are compared with Density Functional Theory (DFT) and Monte-Carlo Shell Model (MCSM) calculations. DFT calculations with several Skyrme parameterizations predict a large jump in the charge radius around the neutron $N = 104$ mid shell, with an odd-even staggering pattern related to the coexistence of nearly-degenerate oblate and prolate minima. This near-degeneracy is highly sensitive to many aspects of the effective interaction, a fact that renders perfect agreement with experiment out of reach for current functionals. Despite this inherent diffculty, the SLy5s1 and a modified UNEDF1^{SO} parameterization predict a qualitatively correct staggering that is off by two neutron numbers. MCSM calculations of states with the experimental spins and parities show good agreement for both electromagnetic moments and the observed charge radii. A clear mechanism for the origin of shape staggering within this context is identified: a substantial change in occupancy of the proton $πh_{9/2}$ and neutron $νi_{13/2}$ orbitals.

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arXiv2018

$β^-$ decay study of the $^{66}$Mn - $^{66}$Fe - $^{66}$Co - $^{66}$Ni chain

Background: Shell evolution can impact the structure of the nuclei and lead to effects such as shape coexistence. The nuclei around $^{68}$Ni represent an excellent study case, however, spectroscopic information of the neutron-rich, $Z<28$ nuclei is limited. Purpose: The goal is to measure $γ$-ray transitions in $^{66}$Fe, $^{66}$Co and $^{66}$Ni populated in the $β^-$ decay of $^{66}$Mn, to determine absolute $β$-feedings and relative $γ$-decay probabilities and to compare the results with Monte Carlo Shell Model calculations in order to study the influence of the relevant single neutron and proton orbitals occupancies around $Z=28$ and $N=40$. Method: The low-energy structures of $^{65,66}$Fe, $^{66}$Co and $^{66}$Ni were studied in the $β^-$ decay of $^{66}$Mn produced at ISOLDE, CERN. The beam was purified by means of laser resonance ionization and mass separation. The $β$ and $γ$ events detected by three plastic scintillators and two MiniBall cluster germanium detectors, respectively, were correlated in time to build the low-energy excitation schemes and to determine the $β$-decay half-lives of the nuclei. Results: The relative small $β$-decay ground state feeding of $^{66}$Fe obtained in this work is at variant to the earlier studies. Spin and parity $1^+$ was assigned to the $^{66}$Co ground state based on the strong ground state feeding in the decay of $^{66}$Fe as well as in the decay of $^{66}$Co. Experimental log(ft) values, $γ$-ray deexcitation patterns and energies of excited states were compared to Monte Carlo Shell Model calculations. Based on this comparison, spin and parity assignments for the selected number of low-lying states in the $^{66}$Mn to $^{66}$Ni chain were proposed. Conclusions: The $β$-decay chain starting $^{66}$Mn towards $^{66}$Ni, crossing $N=40$, evolves from deformed nuclei to sphericity...

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arXiv2018

First Accurate Normalization of the $β$-delayed $α$ Decay of $^{16}$N and Implications for the $^{12}$C$(α,γ)^{16}$O Astrophysical Reaction Rate

The $^{12}\text{C}(α,γ){}^{16}\text{O}$ reaction plays a central role in astrophysics, but its cross section at energies relevant for astrophysical applications is only poorly constrained by laboratory data. The reduced $α$ width, $γ_{11}$, of the bound $1^-$ level in $^{16}$O is particularly important to determine the cross section. The magnitude of $γ_{11}$ is determined via sub-Coulomb $α$-transfer reactions or the $β$-delayed $α$ decay of $^{16}$N, but the latter approach is presently hampered by the lack of sufficiently precise data on the $β$-decay branching ratios. Here we report improved branching ratios for the bound $1^-$ level [$b_{β,11} = (5.02\pm 0.10)\times 10^{-2}$] and for $β$-delayed $α$ emission [$b_{βα} = (1.59\pm 0.06)\times 10^{-5}$]. Our value for $b_{βα}$ is 33% larger than previously held, leading to a substantial increase in $γ_{11}$. Our revised value for $γ_{11}$ is in good agreement with the value obtained in $α$-transfer studies and the weighted average of the two gives a robust and precise determination of $γ_{11}$, which provides significantly improved constraints on the $^{12}$C$(α,γ)$ cross section in the energy range relevant to hydrostatic He burning.

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arXiv2017

The SPEDE spectrometer

The electron spectrometer, SPEDE, has been developed and will be employed in conjunction with the Miniball spectrometer at the HIE-ISOLDE facility, CERN. SPEDE allows for direct measurement of internal conversion electrons emitted in-flight, without employing magnetic fields to transport or momentum filter the electrons. Together with the Miniball spectrometer, it enables simultaneous observation of γ rays and conversion electrons in Coulomb-excitation experiments using radioactive ion beams.

physics.ins-det↗

arXiv2016

Spectroscopy of 46Ar by the (t,p) two-neutron transfer reaction

States in the $N=28$ nucleus $^{46}$Ar have been studied by a two-neutron transfer reaction at REX-ISOLDE (CERN). A beam of radioactive $^{44}$ at an energy of 2.16~AMeV and a tritium loaded titanium target were used to populate $^{46}$ by the t($^{44}$,p) two-neutron transfer reaction. Protons emitted from the target were identified in the T-REX silicon detector array. The excitation energies of states in $^{46}$ have been reconstructed from the measured angles and energies of recoil protons. Angular distributions for three final states were measured and based on the shape of the differential cross section an excited state at 3695~keV has been identified as $J^π= 0^+$. The angular differential cross section for the population of different states are compared to calculations using a reaction model employing both sequential and direct transfer of two neutrons. Results are compared to shell model calculations using state-of-the-art effective interactions.

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arXiv2016

The structure of low-lying states in ${}^{140}$Sm studied by Coulomb excitation

The electromagnetic structure of $^{140}$Sm was studied in a low-energy Coulomb excitation experiment with a radioactive ion beam from the REX-ISOLDE facility at CERN. The $2^+$ and $4^+$ states of the ground-state band and a second $2^+$ state were populated by multi-step excitation. The analysis of the differential Coulomb excitation cross sections yielded reduced transition probabilities between all observed states and the spectroscopic quadrupole moment for the $2_1^+$ state. The experimental results are compared to large-scale shell model calculations and beyond-mean-field calculations based on the Gogny D1S interaction with a five-dimensional collective Hamiltonian formalism. Simpler geometric and algebraic models are also employed to interpret the experimental data. The results indicate that $^{140}$Sm shows considerable $γ$ softness, but in contrast to earlier speculation no signs of shape coexistence at low excitation energy. This work sheds more light on the onset of deformation and collectivity in this mass region.

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arXiv2016

Analysis methods of safe Coulomb-excitation experiments with radioactive ion beams using the gosia code

With the recent advances in radioactive ion beam technology, Coulomb excitation at safe energies becomes an important experimental tool in nuclear-structure physics. The usefulness of the technique to extract key information on the electromagnetic properties of nuclei has been demonstrated since the 1960's with stable beam and target combinations. New challenges present themselves when studying exotic nuclei with this technique, including dealing with low statistics or number of data points, absolute and relative normalisation of the measured cross sections and a lack of complimentary experimental data, such as excited-state lifetimes and branching ratios. This paper addresses some of these common issues and presents analysis techniques to extract transition strengths and quadrupole moments utilising the least-squares fit code, {\rmfamily \textsc{gosia}}.

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arXiv2015

Low-energy Coulomb excitation of $^{62}$Fe and $^{62}$Mn following in-beam decay of $^{62}$Mn

Sub-barrier Coulomb-excitation was performed on a mixed beam of $^{62}$Mn and $^{62}$Fe, following in-trap $β^{-}$ decay of $^{62}$Mn at REX-ISOLDE, CERN. The trapping and charge breeding times were varied in order to alter the composition of the beam, which was measured by means of an ionisation chamber at the zero-angle position of the Miniball array. A new transition was observed at 418~keV, which has been tentatively associated to a $(2^{+},3^{+})\rightarrow1^{+}_{g.s.}$ transition. This fixes the relative positions of the $β$-decaying $4^{+}$ and $1^{+}$ states in $^{62}$Mn for the first time. Population of the $2^{+}_{1}$ state was observed in $^{62}$Fe and the cross-section determined by normalisation to the $^{109}$Ag target excitation, confirming the $B(E2)$ value measured in recoil-distance lifetime experiments.

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arXiv2015

Empirical description of beta-delayed fission partial half-lives

Background: The process of beta-delayed fission (bDF) provides a versatile tool to study low-energy fission in nuclei far away from the beta-stability line, especially for nuclei which do not fission spontaneously. Purpose: The aim of this paper is to investigate systematic trends in bDF partial half-lives. Method: A semi-phenomenological framework was developed to systematically account for the behavior of bDF partial half-lives. Results: The bDF partial half-life appears to exponentially depend on the difference between the Q value for beta decay of the parent nucleus and the fission-barrier energy of the daughter (after beta decay) product. Such dependence was found to arise naturally from some simple theoretical considerations. Conclusions: This systematic trend was confirmed for experimental bDF partial half-lives spanning over 7 orders of magnitudes when using fission barriers calculated from either the Thomas-Fermi or the liquid-drop fission model. The same dependence was also observed, although less pronounced, when comparing to fission barriers from the finite-range liquid-drop model or the Thomas-Fermi plus Strutinsky Integral method.

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arXiv2015

Collectivity in the light radon nuclei measured directly via Coulomb excitation

Background: Shape coexistence in heavy nuclei poses a strong challenge to state-of-the-art nuclear models, where several competing shape minima are found close to the ground state. A classic region for investigating this phenomenon is in the region around $Z=82$ and the neutron mid-shell at $N=104$. Purpose: Evidence for shape coexistence has been inferred from $α$-decay measurements, laser spectroscopy and in-beam measurements. While the latter allow the pattern of excited states and rotational band structures to be mapped out, a detailed understanding of shape coexistence can only come from measurements of electromagnetic matrix elements. Method: Secondary, radioactive ion beams of $^{202}$Rn and $^{204}$Rn were studied by means of low-energy Coulomb excitation at the REX-ISOLDE facility in CERN. Results: The electric-quadrupole ($E2$) matrix element connecting the ground state and first-excited $2^{+}_{1}$ state was extracted for both $^{202}$Rn and $^{204}$Rn, corresponding to ${B(E2;2^{+}_{1} \to 2^{+}_{1})=29^{+8}_{-8}}$ W.u. and $43^{+17}_{-12}$ W.u., respectively. Additionally, $E2$ matrix elements connecting the $2^{+}_{1}$ state with the $4^{+}_{1}$ and $2^{+}_{2}$ states were determined in $^{202}$Rn. No excited $0^{+}$ states were observed in the current data set, possibly due to a limited population of second-order processes at the currently-available beam energies. Conclusions: The results are discussed in terms of collectivity and the deformation of both nuclei studied is deduced to be weak, as expected from the low-lying level-energy schemes. Comparisons are also made to state-of-the-art beyond-mean-field model calculations and the magnitude of the transitional quadrupole moments are well reproduced.

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arXiv2014

On the Validity of the Geiger-Nuttall Alpha-Decay Law and its Microscopic Basis

The Geiger-Nuttall (GN) law relates the partial $α$-decay half-life with the energy of the escaping $α$ particle and contains for every isotopic chain two experimentally determined coefficients. The expression is supported by several phenomenological approaches, however its coefficients lack a fully microscopic basis. In this paper we will show that: 1) the empirical coefficients that appear in the GN law have a deep physical meaning and 2) the GN law is successful within the restricted experimental data sets available so far, but is not valid in general. We will show that, when the dependence of logarithm values of the $α$ formation probability on the neutron number is not linear or constant, the GN law is broken. For the $α$ decay of neutron-deficient nucleus $^{186}$Po, the difference between the experimental half-life and that predicted by the GN Law is as large as one order of magnitude.

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arXiv2014

Shape coexistence in neutron-deficient Hg isotopes studied via lifetime measurements in $^{184,186}$Hg and two-state mixing calculations

The neutron-deficient mercury isotopes, $^{184,186}$Hg, were studied with the Recoil Distance Doppler Shift (RDDS) method using the Gammasphere array and the Köln Plunger device. The Differential Decay Curve Method (DDCM) was employed to determine the lifetimes of the yrast states in $^{184,186}$Hg. An improvement on previously measured values of yrast states up to $8^{+}$ is presented as well as first values for the $9_{3}$ state in $^{184}$Hg and $10^{+}$ state in $^{186}$Hg. $B(E2)$ values are calculated and compared to a two-state mixing model which utilizes the variable moment of inertia (VMI) model, allowing for extraction of spin-dependent mixing strengths and amplitudes.

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arXiv2013

In-gas-cell laser ionization spectroscopy in the vicinity of 100Sn: Magnetic moments and mean-square charge radii of N=50-54 Ag

In-gas-cell laser ionization spectroscopy studies on the neutron deficient 97-101Ag isotopes have been performed with the LISOL setup. Magnetic dipole moments and mean-square charge radii have been determined for the first time with the exception of 101Ag, which was found in good agreement with previous experimental values. The reported results allow tentatively assigning the spin of 97,99Ag to 9/2 and confirming the presence of an isomeric state in these two isotopes, whose collapsed hyperfine structure suggests a spin of 1/2 . The effect of the N=50 shell closure is not only manifested in the magnetic moments but also in the evolution of the mean-square charge radii of the isotopes investigated, in accordance with the spherical droplet model predictions.

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arXiv2012

The in-gas-jet laser ion source: resonance ionization spectroscopy of radioactive atoms in supersonic gas jets

New approaches to perform efficient and selective step-wise Resonance Ionization Spectroscopy (RIS) of radioactive atoms in different types of supersonic gas jets are proposed. This novel application results in a major expansion of the In-Gas Laser Ionization and Spectroscopy (IGLIS) method developed at KU Leuven. Implementation of resonance ionization in the supersonic gas jet allows to increase the spectral resolution by one order of magnitude in comparison with the currently performed in-gas-cell ionization spectroscopy. Properties of supersonic beams, obtained from the de Laval-, the spike-, and the free jet nozzles that are important for the reduction of the spectral line broadening mechanisms in cold and low density environments are discussed. Requirements for the laser radiation and for the vacuum pumping system are also examined. Finally, first results of high-resolution spectroscopy in the supersonic free jet are presented for the 327.4 nm 3d^{10}4s^{2}S_{1/2} \rightarrow 3d^{10}4p^{2}P_{1/2} transition in the stable 63Cu isotope using an amplified single mode laser radiation.

physics.atom-ph↗

arXiv2010

Coulomb excitation of 73Ga

The B(E2; Ii -> If) values for transitions in 71Ga and 73Ga were deduced from a Coulomb excitation experiment at the safe energy of 2.95 MeV/nucleon using post-accelerated beams of 71,73Ga at the REX-ISOLDE on-line isotope mass separator facility. The emitted gamma rays were detected by the MINIBALL-detector array and B(E2; Ii->If) values were obtained from the yields normalized to the known strength of the 2+ -> 0+ transition in the 120Sn target. The comparison of these new results with the data of less neutron-rich gallium isotopes shows a shift of the E2 collectivity towards lower excitation energy when adding neutrons beyond N = 40. This supports conclusions from previous studies of the gallium isotopes which indicated a structural change in this isotopical chain between N = 40 and N = 42. Combined with recent measurements from collinear laser spectroscopy showing a 1/2- spin and parity for the ground state, the extracted results revealed evidence for a 1/2-; 3/2- doublet near the ground state in 73 31Ga42 differing by at most 0.8 keV in energy.

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arXiv2010

Discovery of the shape coexisting 0+ state in 32Mg by a two neutron transfer reaction

The Island of Inversion nucleus 32Mg has been studied by a (t,p) two neutron transfer reaction in inverse kinematics at REX-ISOLDE. The shape coexistent excited 0+ state in 32Mg has been identified by the characteristic angular distribution of the protons of the DeltaL = 0 transfer. The excitation energy of 1058 keV is much lower than predicted by any theoretical model. The low gamma-ray intensity observed for the decay of this 0+ state indicates a lifetime of more than 10 ns. Deduced spectroscopic amplitudes are compared with occupation numbers from shell model calculations.

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arXiv2010

Early onset of ground-state deformation in the neutron-deficient polonium isotopes

In-source resonant ionization laser spectroscopy of the even-$A$ polonium isotopes $^{192-210,216,218}$Po has been performed using the $6p^37s$ $^5S_2$ to $6p^37p$ $^5P_2$ ($λ=843.38$ nm) transition in the polonium atom (Po-I) at the CERN ISOLDE facility. The comparison of the measured isotope shifts in $^{200-210}$Po with a previous data set allows to test for the first time recent large-scale atomic calculations that are essential to extract the changes in the mean-square charge radius of the atomic nucleus. When going to lighter masses, a surprisingly large and early departure from sphericity is observed, which is only partly reproduced by Beyond Mean Field calculations.

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arXiv2010

Abrupt changes in alpha decay systematics as a manifestation of collective nuclear modes

An abrupt change in $α$ decay systematics around the N=126 neutron shell closure is discussed. It is explained as a sudden hindrance of the clustering of the nucleons that eventually form the $α$ particle. This is because the clustering induced by the pairing mode acting upon the four nucleons is inhibited if the configuration space does not allow a proper manifestation of the pairing collectivity.

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