arXiv subjects

Patrick Huber

Publications and source records attributed to Patrick Huber.

At least 145 records · Page 8Linked to original sources

arXiv2015

Thermotropic Orientational Order of Discotic Liquid Crystals in Nanochannels: An Optical Polarimetry Study and a Landau-de Gennes Analysis

Optical polarimetry measurements of the orientational order of a discotic liquid crystal based on a pyrene derivative and confined in parallel-aligned nanochannels of monolithic mesoporous alumina, silica, and silicon as a function of temperature, channel radius (3 - 22 nm) and surface chemistry reveal a competition of radial and axial columnar order. The evolution of the orientational order parameter of the confined systems is continuous, in contrast to the discontinuous transition in the bulk. For channel radii larger than 10 nm we suggest several, alternative defect structures, which are compatible both with the optical experiments on the collective molecular orientation presented here and with a translational, radial columnar order reported in previous diffraction studies. For smaller channel radii our observations can semi-quantitatively be described by a Landau-de Gennes model with a nematic shell of radially ordered columns (affected by elastic splay deformations) that coexists with an orientationally disordered, isotropic core. For these structures, the cylindrical phase boundaries are predicted to move from the channel walls to the channel centres upon cooling, and vice-versa upon heating, in accord with the pronounced cooling/heating hystereses observed and the scaling behavior of the transition temperatures with channel diameter. The absence of experimental hints of a paranematic state is consistent with a biquadratic coupling of the splay deformations to the order parameter.

cond-mat.soft↗

arXiv2015

Protein Adsorption into Mesopores: A Combination of Electrostatic Interaction, Counterion Release and van der Waals Forces

Bovine heart cytochrome c has been immobilized into the mesoporous silica host material SBA-15 in both its native folded and urea-unfolded state. The comparison of the two folding states' behavior casts doubt on the commonly used explanation of cytochrome c adsorption, i.e. the electrostatic interaction model. A detailed investigation of the protein binding as a function of pH and ionic strength of the buffer solution reveals the complex nature of the protein-silica interaction. Electrostatic interaction, van der Waals forces and entropic contributions by counterion release each contribute to adsorption on the silica pore walls.

physics.bio-ph↗

arXiv2015

Soft matter in hard confinement: phase transition thermodynamics, structure, texture, diffusion and flow in nanoporous media - topical review

Spatial confinement in nanoporous media affects the structure, thermodynamics and mobility of molecular soft matter often markedly. This article reviews thermodynamic equilibrium phenomena, such as physisorption, capillary condensation, crystallisation, self-diffusion, and structural phase transitions as well as selected aspects of the emerging field of spatially confined, non-equilibrium physics, i.e. the rheology of liquids, capillarity-driven flow phenomena, and imbibition front broadening in nanoporous materials. The observations in the nanoscale systems are related to the corresponding bulk phenomenologies. The complexity of the confined molecular species is varied from simple building blocks, like noble gas atoms, normal alkanes and alcohols to liquid crystals, polymers, ionic liquids, proteins and water. Mostly, experiments with mesoporous solids of alumina, carbon, gold, silica, and silicon having pore diameters ranging from a few up to 50 nanometers are presented. The observed peculiarities of nanopore-confined condensed matter are also discussed with regard to applications. A particular emphasis is put on texture formation upon crystallisation in nanoporous media, a topic both of high fundamental interest and of increasing nanotechnological importance, e.g., for the synthesis of organic/inorganic hybrid materials by melt infiltration, the usage of nanoporous solids in crystal nucleation or in template-assisted electrochemical deposition of nano structures.

cond-mat.soft↗

arXiv2015

A Staged Muon Accelerator Facility For Neutrino and Collider Physics

Muon-based facilities offer unique potential to provide capabilities at both the Intensity Frontier with Neutrino Factories and the Energy Frontier with Muon Colliders. They rely on a novel technology with challenging parameters, for which the feasibility is currently being evaluated by the Muon Accelerator Program (MAP). A realistic scenario for a complementary series of staged facilities with increasing complexity and significant physics potential at each stage has been developed. It takes advantage of and leverages the capabilities already planned for Fermilab, especially the strategy for long-term improvement of the accelerator complex being initiated with the Proton Improvement Plan (PIP-II) and the Long Baseline Neutrino Facility (LBNF). Each stage is designed to provide an R&D platform to validate the technologies required for subsequent stages. The rationale and sequence of the staging process and the critical issues to be addressed at each stage, are presented.

physics.acc-ph↗

arXiv2014

The Case for Muon-based Neutrino Beams

For the foreseeable future, high energy physics accelerator capabilities in the US will be deployed to study the physics of the neutrino sector. In this context, it is useful to explore the sensitivities and limiting systematic effects of the planned neutrino oscillation program, so that we can evaluate the issues that must be addressed in order to ensure the success of these efforts. It is only in this way that we will ultimately be able to elucidate the fundamental physics processes involved. We conclude that success can only be guaranteed by, at some point in the future, being able to deploy muon accelerator capabilities. Such capabilities provide the only route to precision neutrino beams with which to study and mitigate, at the sub-percent level, the limiting systematic issues of future oscillation measurements. Thus this analysis argues strongly for maintaining a viable accelerator research program towards future muon accelerator capabilities.

hep-ex↗

arXiv2014

Combining dark matter detectors and electron-capture sources to hunt for new physics in the neutrino sector

In this letter we point out the possibility to study new physics in the neutrino sector using dark matter detectors based on liquid xenon. These are characterized by very good spatial resolution and extremely low thresholds for electron recoil energies. When combined with a radioactive $ν_e$ source, both features in combination allow for a very competitive sensitivity to neutrino magnetic moments and sterile neutrino oscillations. We find that, for realistic values of detector size and source strength, the bound on the neutrino magnetic moment can be improved by an order of magnitude with respect to the present value. Regarding sterile neutrino searches, we find that most of the gallium anomaly could be explored at the 95% confidence level just using shape information.

hep-ph↗

arXiv2014

Switchable Imbibition in Nanoporous Gold

Spontaneous imbibition enables the elegant propelling of nano-flows because of the dominance of capillarity at small length scales. The imbibition kinetics are, however, solely determined by the static geometry of the porous host, the capillarity, and the fluidity of the imbibed liquid. This makes active control particularly challenging. Here, we show for aqueous electrolyte imbibition in nanoporous gold that the fluid flow can be reversibly switched on and off through electric potential control of the solid-liquid interfacial tension, i.e. we can accelerate the imbibition front, stop it, and have it proceed at will. Simultaneous measurements of the mass flux and the electrical current allow us to document simple scaling laws for the imbibition kinetics, and to explore the charge flow dynamics in the metallic nanopores. Our findings demonstrate that the high electric conductivity along with the pathways for ionic and/or fluid transport render nanoporous elemental gold a versatile, accurately controllable electro-capillary pump and flow sensor for minute amounts of liquids with exceptionally low operating voltages.

physics.flu-dyn↗

arXiv2014

Paranematic-to-nematic ordering of a binary mixture of rod-like liquid crystals confined in cylindrical nanochannels

We explore the optical birefringence of the nematic binary mixtures 6CB$_{1-x}$7CB$_x$ ($0~\le~x~\le~1$) imbibed into parallel-aligned nanochannels of mesoporous alumina and silica membranes for channel radii of $3.4~\le~R~\le 21.0$ nm. The results are compared with the bulk behavior and analyzed with a Landau-de-Gennes model. Depending on the channel radius the nematic ordering in the cylindrical nanochannels evolves either discontinuously (subcritical regime, nematic ordering field $σ<1/2$) or continuously (overcritical regime, $σ>1/2$), but in both cases with a characteristic paranematic precursor behavior. The strength of the ordering field, imposed by the channel walls, and the magnitude of quenched disorder varies linearly with the mole fraction $x$ and scales inversely proportionally with $R$ for channel radii larger than 4 nm. The critical pore radius, $R_c$, separating a continuous from a discontinuous paranematic-to-nematic evolution, varies linearly with $x$ and differs negligibly between the silica and alumina membranes. We find no hints of preferred adsorption of one species at the channels walls. By contrast, a linear variation of the nematic-to-paranematic transition point $T_{\rm PN}$ and of the nematic ordering field $σ$ vs. $x$ suggest that the binary mixtures of cyanobiphenyls 6CB and 7CB keep their homogeneous bulk stoichiometry also in nanoconfinement, at least for channel diameters larger than $\sim$7 nm.

cond-mat.soft↗

arXiv2014

Neutrino-nucleus interaction models and their impact on oscillation analyses

In neutrino oscillation experiments, neutrino interactions at the detector are simulated using event generators which attempt to reflect our understanding of nuclear physics. We study the impact of different neutrino interactions and nuclear models on the determination of neutrino oscillation parameters. We use two independent neutrino event generators, GENIE and GiBUU, and apply them to a setup with a conventional neutrino beam aiming at a water Čerenkov detector, for which only the QE-like sample is selected. Subsequently, we perform a fit to the oscillation parameters in the $ν_μ$ disappearance channel.

hep-ph↗

arXiv2014

Antineutrino monitoring for the Iranian heavy water reactor

In this note we discuss the potential application of antineutrino monitoring to the Iranian heavy water reactor at Arak, the IR-40, as a non-proliferation measure. We demonstrate that an above ground detector positioned right outside the IR-40 reactor building could meet and in some cases significantly exceed the verification goals identified by IAEA for plutonium production or diversion from declared inventories. In addition to monitoring the reactor during operation, observing antineutrino emissions from long-lived fission products could also allow monitoring the reactor when it is shutdown. Antineutrino monitoring could also be used to distinguish different levels of fuel enrichment. Most importantly, these capabilities would not require a complete reactor operational history and could provide a means to re-establish continuity of knowledge in safeguards conclusions should this become necessary.

physics.ins-det↗

arXiv2014

Antineutrino reactor safeguards - a case study

Antineutrinos have been proposed as a means of reactor safeguards for more than 30 years and there has been impressive experimental progress in neutrino detection. In this paper we conduct, for the first time, a case study of the application of antineutrino safeguards to a real-world scenario - the North Korean nuclear crisis in 1994. We derive detection limits to a partial or full core discharge in 1989 based on actual IAEA safeguards access and find that two independent methods would have yielded positive evidence for a second core with very high confidence. To generalize our results, we provide detailed estimates for the sensitivity to the plutonium content of various types of reactors, including most types of plutonium production reactors, based on detailed reactor simulations. A key finding of this study is that a wide class of reactors with a thermal power of less than 0.1-1 GWth can be safeguarded achieving IAEA goals for quantitative sensitivity and timeliness with detectors right outside the reactor building. This type of safeguards does not rely on the continuity of knowledge and provides information about core inventory and power status in real-time.

physics.ins-det↗

arXiv2014

Quantifying the sensitivity of oscillation experiments to the neutrino mass ordering

Determining the type of the neutrino mass ordering (normal versus inverted) is one of the most important open questions in neutrino physics. In this paper we clarify the statistical interpretation of sensitivity calculations for this measurement. We employ standard frequentist methods of hypothesis testing in order to precisely define terms like the median sensitivity of an experiment. We consider a test statistic $T$ which in a certain limit will be normal distributed. We show that the median sensitivity in this limit is very close to standard sensitivities based on $Δχ^2$ values from a data set without statistical fluctuations, such as widely used in the literature. Furthermore, we perform an explicit Monte Carlo simulation of the INO, JUNO, LBNE, NOvA, and PINGU experiments in order to verify the validity of the Gaussian limit, and provide a comparison of the expected sensitivities for those experiments.

hep-ph↗

arXiv2013

Opportunities in Neutrino Theory -- a Snowmass White Paper

Neutrino masses are clear evidence for physics beyond the standard model and much more remains to be understood about the neutrino sector. We highlight some of the outstanding questions and research opportunities in neutrino theory. We show that most of these questions are directly connected to the very rich experimental program currently being pursued (or at least under serious consideration) in the United States and worldwide. Finally, we also comment on the state of the theoretical neutrino physics community in the U.S.

hep-ph↗

arXiv2013

Physics Performance of a Low-Luminosity Low Energy Neutrino Factory

We investigate the minimal performance, in terms of beam luminosity and detector size, of a neutrino factory to achieve a competitive physics reach for the determination of the mass hierarchy and the discovery of leptonic CP violation. We find that a low luminosity of $2\times 10^{20}$ useful muon decays per year and 5 GeV muon energy aimed at a 10 kton magnetized liquid argon detector placed at 1300 km from the source provides a good starting point. This result relies on $θ_{13}$ being large and assumes that the so-called platinum channel can be used effectively. We find that such a minimal facility would perform significantly better than phase I of the LBNE project and thus could constitute a reasonable step towards a full neutrino factory.

hep-ph↗

arXiv2013

Thermotropic nematic order upon nano-capillary filling

Optical birefringence and light absorption measurements reveal four regimes for the thermotropic behavior of a nematogen liquid (7CB) upon sequential filling of parallel-aligned capillaries of 12 nm diameter in a monolithic, mesoporous silica membrane. No molecular reorientation is observed for the first adsorbed monolayer. In the film-condensed state (up to 1 nm thickness) a weak, continuous paranematic-to-nematic (P-N) transition is found, which is shifted by 10 K below the discontinuous bulk transition at T_IN=305K. The capillary-condensed state exhibits a more pronounced, albeit still continuous P-N reordering, located 4 K below T_IN. This shift vanishes abruptly on complete filling of the capillaries, which we tentatively trace to a 10 MPa tensile pressure release associated with the disappearance of concave menisci in the confined liquid.

cond-mat.soft↗

arXiv2012

Systematic uncertainties in long-baseline neutrino oscillations for large $θ_{13}$

We study the physics potential of future long-baseline neutrino oscillation experiments at large $θ_{13}$, focusing especially on systematic uncertainties. We discuss superbeams, \bbeams, and neutrino factories, and for the first time compare these experiments on an equal footing with respect to systematic errors. We explicitly simulate near detectors for all experiments, we use the same implementation of systematic uncertainties for all experiments, and we fully correlate the uncertainties among detectors, oscillation channels, and beam polarizations as appropriate. As our primary performance indicator, we use the achievable precision in the measurement of the CP violating phase $\deltacp$. We find that a neutrino factory is the only instrument that can measure $\deltacp$ with a precision similar to that of its quark sector counterpart. All neutrino beams operating at peak energies $\gtrsim 2$ GeV are quite robust with respect to systematic uncertainties, whereas especially \bbeams and \thk suffer from large cross section uncertainties in the quasi-elastic regime, combined with their inability to measure the appearance signal cross sections at the near detector. A noteworthy exception is the combination of a $γ=100$ \bbeam with an \spl-based superbeam, in which all relevant cross sections can be measured in a self-consistent way. This provides a performance, second only to the neutrino factory. For other superbeam experiments such as \lbno and the setups studied in the context of the \lbne reconfiguration effort, statistics turns out to be the bottleneck. In almost all cases, the near detector is not critical to control systematics since the combined fit of appearance and disappearance data already constrains the impact of systematics to be small provided that the three active flavor oscillation framework is valid.

hep-ph↗

arXiv2012

Influence of nano confinement on nematic liquid crystals

We explore the nematic ordering of the rod-like liquid crystals 5CB and 6CB, embedded into parallel-aligned nanochannels in mesoporous silicon and silica membranes as a function of mean channel radius (4.7<=R <=8.3 nm), and thus geometrical confinement strength, by optical birefringence measurements in the infrared region. The orientational order inside the nanochannels results in an excess birefringence, which is proportional to the nematic order parameter. It evolves continuously upon cooling with a precursor behavior, typical of a paranematic state at high temperatures. These observations are compared with the bulk behavior and analyzed within a phenomenological model. Such an approach indicates that the strength of the nematic ordering fields sigma is beyond a critical threshold sigma_c =1/2, that separates discontinuous from continuous paranematic-to-nematic behavior. In agreement with the predictions of the phenomenological approach a linear dependency of sigma on the inverse channel radius is found and we can infer therefrom the critical channel radii, R_c, separating continuous from discontinuous paranematic-to-isotropic behavior, for 5CB (12.1 nm) and 6CB (14.0 nm). Our analysis suggests that the tangential anchoring at the channel walls is of similar strength in mesoporous silicon and mesoporous silica membranes. A comparison with the bulk phase behavior reveals that the nematic order in nanoconfinement is significantly affected by channel wall roughness leading to a reduction of the effective nematic ordering.

cond-mat.soft↗

arXiv2012

Anomalous Front Broadening During Spontaneous Imbibition in a Matrix with Elongated Pores

During spontaneous imbibition a wetting liquid is drawn into a porous medium by capillary forces. In systems with comparable pore length and diameter, such as paper and sand, the front of the propagating liquid forms a continuous interface. Sections of this interface advance in a highly correlated manner due to an effective surface tension, which restricts front broadening. Here we investigate water imbibition in a nanoporous glass (Vycor) in which the pores are much longer than they are wide. In this case, no continuous liquid-vapor interface with coalesced menisci can form. Anomalously fast imbibition front roughening is experimentally observed by neutron imaging.We propose a theoretical pore network model, whose structural details are adapted to the microscopic pore structure of Vycor glass, and show that it displays the same large scale roughening characteristics as observed in the experiment. The model predicts that menisci movements are uncorrelated. This indicates that despite the connectivity of the network the smoothening effect of surface tension on the imbibition front roughening is negligible. These results suggest a new universality class of imbibition behavior which is expected to occur in any matrix with elongated, interconnected pores of random radii.

cond-mat.soft↗