arXiv subjects

Peng Lv

Publications and source records attributed to Peng Lv.

At least 19 recordsLinked to original sources

arXiv2025

Sub-5-fs compression and synchronization of relativistic electron bunches enabled by a high-gradient $\alpha$-magnet and low-jitter photoinjector

Generating high-brightness relativistic electron bunches with few-femtosecond duration, while simultaneously achieving few-fs synchronization with ultrafast lasers, remains an outstanding challenge at the frontier of accelerator physics and ultrafast science. In this Letter, we present the beam physics and experimental demonstration of a new method that, for the first time, enables simultaneous control of bunch duration and synchronization with few-fs precision. Timing stabilization is achieved using a tailored high-gradient $\alpha$-magnet that optimizes the correlation between time of flight and momentum, together with a photocathode RF gun designed to suppress the effect of RF-to-laser timing jitter. Compression is realized by manipulating the time-momentum correlation in phase space, primarily through space-charge effects. Sub-5-fs rms bunch duration and synchronization are demonstrated. This method establishes a new regime in electron bunch control, unlocking new capabilities for ultrafast beam physics and applications.

physics.acc-ph↗

arXiv2025

Enhanced Charge Transport in A-site Ordered Perovskite Derivatives A2A'Bi2I9 (A = Cs; A'= Ag, Cu): A First-Principles Study

Recent experiments have synthesized Cs2AgBi2I9 by partially substituting Cs+ with Ag+ at the A-site of Cs3Bi2I9, resulting in enhanced charge transport properties compared to Cs3Bi2I9. However, the atomic-scale mechanisms behind this enhancement remain unclear. In this work, we investigate the carrier transport mechanisms in Cs2A'Bi2I9 (A' = Ag, Cu) using first-principles calculations and Boltzmann transport calculations. Our results reveal that A-site ordered Cs2A'Bi2I9 exhibits carrier mobilities that are 3-4 times higher than those of Cs3Bi2I9 within the 100-500 K temperature range. We identify polar phonon scattering as the dominant mechanism limiting mobility. Furthermore, the enhanced out-of-plane carrier mobility in Cs2A'Bi2I9, particularly between 100 and 200K, leads to reduced mobility anisotropy. These improvements are mainly due to the shorter A'-I bond lengths and increased Ag+/Cu+ s-I p orbital coupling. Notably, substitution with Cu+ results in a further reduction in the band gap and enhanced hole mobility compared to Ag+ substitution in Cs3Bi2I9. Further analysis reveals that the significant increase in carrier mobility in Cs2A'Bi2I9 can be largely explained by the smaller carrier effective masses (m*) and weaker Fr\"ohlich coupling strengths ({\alpha}), resulting in a lower polar mass {\alpha}(m*/me), compared to Cs3Bi2I9. Our study provides valuable insights into the transport properties of Bi-based perovskite derivatives, paving the way for their future applications in optoelectronic devices.

cond-mat.mtrl-sci↗

arXiv2024

A Game-Theoretical Approach for Optimal Supervisory Control of Discrete Event Systems under Energy Constraints

In this paper, we investigate the problem of optimal supervisory control for the discrete event systems under energy constraints. We consider that the execution of events consumes energy and the energy can be replenished at specific reload states. When the energy level drops below zero, the system will be crashed. To capture the above scenario, we introduce a new model, called consumption discrete event system (cDES). Our objective is to find the minimal initial energy value and synthesize an optimal supervisor ensuring that the energy will never be exhausted. To solve this problem, we propose a game-theoretical approach by converting the cDES as a consumption two-player graph game (cTPG) and reformulate the optimal supervisory control problem in game theory. In particular, we demonstrate that the converted game can be decomposed into independent reachability games related to reload vertices, which can be solved by a fixed point iterative algorithm proposed in this paper. Through iteratively removing unsafe reload vertices and solving reachability games for the remaining reload vertices, a solution can be found.

eess.SY↗

arXiv2024

Flexomagnetoelectric effect in Sr2IrO4 thin films

Symmetry engineering is explicitly effective to manipulate and even create phases and orderings in strongly correlated materials. Flexural stress is universally practical to break the space-inversion or time-reversal symmetry. Here, by introducing strain gradient in a centrosymmetric antiferromagnet Sr2IrO4, the space-inversion symmetry is broken accompanying a non-equivalent O p-Ir d orbital hybridization along z axis. Thus, emergent polar phase and out-of-plane magnetic moment have been simultaneously observed in these asymmetric Sr2IrO4 thin films, which both are absent in its ground state. Furthermore, upon the application of magnetic field, such polarization can be controlled by modifying the occupied d orbitals through spin-orbit interaction, giving rise to a flexomagnetoelectric effect. This work provides a general strategy to artificially design multiple symmetries and ferroic orderings in strongly correlated systems.

cond-mat.str-el↗

arXiv2023

Mapping electrostatic potential in electrolyte solution

Mapping the electrostatic potential (ESP) distribution around ions in electrolyte solution is crucial for the establishment of a microscopic understanding of electrolyte solution properties. For solutions in the bulk phase, it has not been possible to measure the ESP distribution on Angstrom scale. Here we show that liquid electron scattering experiment using state-of-the-art relativistic electron beam can be used to measure the Debye screening length of aqueous LiCl, KCl, and KI solutions across a wide range of concentrations. We observe that the Debye screening length is long-ranged at low concentration and short-ranged at high concentration, providing key insight into the decades-long debate over whether the impact of ions in water is long-ranged or short-ranged. In addition, we show that the measured ESP can be used to retrieve the non-local dielectric function of electrolyte solution, which can serve as a promising route to investigate the electrostatic origin of special ion effects. Our observations show that, interaction, as one of the two fundamental perspectives for understanding electrolyte solution, can provide much richer information than structure.

cond-mat.soft↗

arXiv2023

Ultra-high-density double-atom catalyst with spin moment as activity descriptor for oxygen reduction reaction

One of the great challenges facing atomically dispersed catalysts, including single-atom catalyst (SAC) and double-atom catalyst (DAC) is their ultra-low metal loading (typically less than 5 wt%), basically limiting the practical catalytic application, such as oxygen reduction reaction (ORR) crucial to hydrogen fuel cell and metal-air battery. Although some important progresses have been achieved on ultra-high-density (UHD) SACs, the reports on UHD-DACs with stable uniform dispersion is still lacking. Herein, based on the experimentally synthesized M2N6 motif (M = Sc-Zn), we theoretically demonstrated the existence of the UHD-DACs with the metal loading > 40 wt%, which were confirmed by systematic analysis of dynamic, thermal, mechanical, thermodynamic, and electrochemical stabilities. Furthermore, ORR activities of the UHD-DACs are comparable with or even better than those of the experimentally synthesized low-density (LD) counterparts, and the Fe2N6 and Co2N6 UHD-DACs locate at the peak of the activity volcano with ultra-low overpotentials of 0.31 and 0.33 V, respectively. Finally, spin magnetic moment of active center is found to be a catalytic descriptor for ORR on the DACs. Our work will stimulate the experimental exploration of the ultra-high-density DACs and provides the novel insight into the relationship between ORR activity of the DACs and their spin states.

cond-mat.mtrl-sci↗

arXiv2022

QCSH: a Full Quantum Computer Nuclear Shell-Model Package

Nucleus is a typical many-body quantum system. Full calculation of a nuclear system in a classical computer is far beyond the capacity of current classical computers. With fast development of hardware, the prospect of using quantum computers in nuclear physics is closing. Here, we report a full quantum package, QCSH, for solving nuclear shell-model in a quantum computer. QCSH uses the linear combination of unitaries formalism of quantum computing, and performs all calculations in a quantum computer. The complexities of qubit resource, number of basic gates of QCSH, are both polynomial to the nuclear size. QCSH can already provide meaningful results in the near term. As examples, the binding energies of twelve light nuclei, $^{2}$H, $^{3}$H, $^{3}$He, $^{4}$He, $^{6}$Li, $^{7}$Li, $^{12}$C, $^{14}$N, $^{16}$O, $^{17}$O, $^{23}$Na and $^{40}$Ca are calculated using QCSH in a classical quantum emulator. The binding energy of Deuteron has already been experimentally studied using QCSH on a superconducting quantum computing device. QCSH not only works in near-term quantum devices, but also in future large-scale quantum computers. With the development of quantum devices, nuclear system constitutes another promising area for demonstrating practical quantum advantage.

quant-ph↗

arXiv2021

Evidence for anisotropic spin-triplet Andreev reflection at the 2D van der Waals ferromagnet/superconductor interface

Fundamental symmetry breaking and relativistic spin-orbit coupling give rise to fascinating phenomena in quantum materials. Of particular interest are the interfaces between ferromagnets and common s-wave superconductors, where the emergent spin-orbit fields support elusive spin-triplet superconductivity, crucial for superconducting spintronics and topologically-protected Majorana bound states. Here, we report the observation of large magnetoresistances at the interface between a quasi-two-dimensional van der Waals ferromagnet Fe0.29TaS2 and a conventional s-wave superconductor NbN, which provides the possible experimental evidence for the spin triplet Andreev reflection and induced spin-triplet superconductivity at ferromagnet/superconductor interface arising from Rashba spin-orbit coupling. The temperature, voltage, and interfacial barrier dependences of the magnetoresistance further support the induced spin-triplet superconductivity and spin-triplet Andreev reflection. This discovery, together with the impressive advances in two-dimensional van der Waals ferromagnets, opens an important opportunity to design and probe superconducting interfaces with exotic properties.

cond-mat.supr-con↗

arXiv2020

Conductive Domain Walls in Non-Oxide Ferroelectrics Sn2P2S6

The conductive domain wall (CDW) is extensively investigated in ferroelectrics, which can be considered as a quasi-two-dimensional reconfigurable conducting channel embedded into an insulating material. Therefore, it is highly important for the application of ferroelectric nanoelectronics. Hitherto, most CDW investigations are restricted in oxides, and limited work has been reported in non-oxides to the contrary. Here, by successfully synthesizing the non-oxide ferroelectric Sn2P2S6 single crystal, we observed and confirmed the domain wall conductivity by using different scanning probe techniques which origins from the nature of inclined domain walls. Moreover, the domains separated by CDW also exhibit distinguishable electrical conductivity due to the interfacial polarization charge with opposite signs. The result provides a novel platform for understanding electrical conductivity behavior of the domains and domain walls in non-oxide ferroelectrics.

cond-mat.mtrl-sci↗

arXiv2020

Ferroelastic switching with van der Waals direction transformation in layered PdSe2 driven by uniaxial and shear strain

Uniaxial and biaxial strain approaches are usually implemented to switch the ferroelastic states, which play a key role in the application of the ferroics and shape memory materials. In this work, by using the first-principles calculations, we found not only uniaxial strain, but also shear strain can induce a novel ferroelastic switching, in which the van der Waals (vdW) layered direction rotates with the ferroelastic transition in layered bulk PdSe2. The shear strain induces ferroelastic switching with three times amplitude smaller than uniaxial strain. The novel three-states ferroelastic switching in layered PdSe2 also occurs under shear strain. Our result shows that the shear strain could be used as an effective approach for manipulating the functionalities of layered materials in potential device applications.

cond-mat.mtrl-sci↗

arXiv2019

Thickness-dependent in-plane polarization and structural phase transition in van der Waals Ferroelectric CuInP2S6

Van der Waals (vdW) layered materials have rather weaker interlayer bonding than the intra-layer bonding, therefore the exfoliation along the stacking direction enables the achievement of monolayer or few layers vdW materials with emerging novel physical properties and functionalities. The ferroelectricity in vdW materials recently attracts renewed interest for the potential use in high-density storage devices. As the thickness going thinner, the competition between the surface energy, depolarization field and interfacial chemical bonds may give rise to the modification of ferroelectricity and crystalline structure, which has limited investigations. In this work, combining the piezoresponse force microscope scanning, contact resonance imaging, we report the existence of the intrinsic in-plane polarization in vdW ferroelectrics CuInP2S6 (CIPS) single crystals, whereas below a critical thickness between 90-100 nm, the in-plane polarization disappears. The Young's modulus also shows an abrupt stiffness at the critical thickness. Based on the density functional theory calculations, we ascribe these behaviors to a structural phase transition from monoclinic to trigonal structure, which is further verified by transmission electron microscope technique. Taken together, these findings demonstrate the foundational importance of structural phase transition for enhancing the rich functionality and broad utility of vdW ferroelectrics.

cond-mat.mtrl-sci↗

arXiv2019

Spontaneous photo-generated carrier separation of SnO/BiOX (X=Cl, Br, I) bilayer under visible light irradiation for water splitting

Alloying in 2D materials plays a more and more important role due to wide range bandgap tunability and integrating the advantages of HER and OER. Here, the novel bilayers of SnO/BiOX (X= Cl, Br and I) bilayer are constructed to integrate the advantages of narrow bandgap and separating photo-generated carriers. The bandgap of the bilayers can be tuned from 1.09 to 1.84 eV, remarkably improving the utilization of solar energy. The large difference in effective masses and built-in electric field effectively hamper the fast recombination of photo-generated carries, which highly enhances the photocatalytic efficiency. Besides that, the type-II band alignment guarantee the two half reactions could occur at different surfaces. Moreover, the optical absorption (the strong transition between band edges and high joint density of states) and band-edge level further confirm the SnO/BiOX (X= Cl and Br) bilayer is a promising candidate for overall water-splitting.

cond-mat.mtrl-sci↗

arXiv2018

Quantum transport through three-dimensional topological insulator p-n junction under magnetic field

The 3D topological insulator (TI) PN junction under magnetic fields presents a novel transport property which is investigated both theoretically and numerically in this paper. Transport in this device can be tuned by the axial magnetic field. Specifically, the scattering coefficients between incoming and outgoing modes oscillate with axial magnetic flux at the harmonic form. In the condition of horizontal mirror symmetry, the initial phase of the harmonic oscillation is dependent on the parities of incoming and outgoing modes. This symmetry is broken when a vertical bias is applied which leads to a kinetic phase shift added to the initial phase. On the other hand, the amplitude of oscillation is suppressed by the surface disorder while it has no influence on the phase of oscillation. Furthermore, with the help of the vertical bias, a special (1,-2) 3D TI PN junction can be achieved, leading to a novel spin precession phenomenon.

cond-mat.mes-hall↗

arXiv2018

High Curie temperature half metallic 2D M2Se3 (M = Co, Ni, and Pd) monolayers with superior mechanical flexibility

Pursuing two-dimensional (2D) intrinsic ferromagnetism with high Curie temperature and great mechanical flexibility has attracted great interest in flexible spintronics. In the present work, we carried out a density functional theory (DFT) investigation on the 2D M2Se3 (M=Co, Ni and Pd) monolayers to understand their structural stabilities, electronic, magnetic and mechanical properties. Our results show that the Co2Se3 monolayer exhibits a fascinating half-metallic ferromagnetism with high Curie temperature (>700K). In addition, due to their unique buckling hinge-like structure, M2Se3 monolayers possess the large out-of-plane negative Poisson's ratio (NPR) and superior mechanical flexibility evidenced by their unusual critical strain two times greater than the well-known 2D materials. These findings imply that 2D M2Se3 family is the promising materials for the applications in the flexible and high-density spintronic nanodevices.

cond-mat.mtrl-sci↗

arXiv2018

Magnetic Flux Control of Chiral Majorana Edge Modes in Topological Superconductor

We study the transport of chiral Majorana edge modes (CMEMs) in a hybrid quantum anomalous Hall insulator-topological superconductor (QAHI-TSC) system in which the TSC region contains a Josephson junction and a cavity. The Josephson junction undergoes a topological transition when the magnetic flux through the cavity passes through half-integer multiples of magnetic flux quantum. For the trivial phase, the CMEMs transmit along the QAHI-TSC interface as without magnetic flux. However, for the nontrivial phase, a zero-energy Majorana state appears in the cavity, leading that a CMEM can resonantly tunnel through the Majorana state to a different CMEM. These findings may provide a feasible scheme to control the transport of CMEMs by using the magnetic flux and the transport pattern can be customized by setting the size of the TSC.

cond-mat.mes-hall↗

arXiv2018

Gate voltage controlled thermoelectric figure of merit in three-dimensional topological insulator nanowires

The thermoelectric properties of the surface states in three-dimensional topological insulator nanowires are studied. The Seebeck coefficients $S_c$ and the dimensionless thermoelectrical figure of merit $ZT$ are obtained by using the tight-binding Hamiltonian combining with the nonequilibrium Green's function method. They are strongly dependent on the gate voltage and the longitudinal and perpendicular magnetic fields. By changing the gate voltage or magnetic fields, the values of $S_c$ and $ZT$ can be easily controlled. At the zero magnetic fields and zero gate voltage, or at the large perpendicular magnetic field and nonzero gate voltage, $ZT$ has the large value. Owing to the electron-hole symmetry, $S_c$ is an odd function of the Fermi energy while $ZT$ is an even function regardless of the magnetic fields. $S_c$ and $ZT$ show peaks when the quantized transmission coefficient jumps from one plateau to another. The highest peak appears while the Fermi energy is near the Dirac point. At the zero perpendicular magnetic field and zero gate voltage, the height of $n$th peak of $S_C$ is $\frac{k_B}{e}\texttt{ln}2/(|n|+1/2)$ and $\frac{k_B}{e}\texttt{ln}2/|n|$ for the longitudinal magnetic flux $\phi_{\parallel} = 0 $ and $\pi$, respectively. Finally, we also study the effect of disorder and find that $S_c$ and $ZT$ are robust against disorder. In particular, the large value of $ZT$ can survive even if at the strong disorder. These characteristics (that $ZT$ has the large value, is easily regulated, and is robust against the disorder) are very beneficial for the application of the thermoelectricity.

cond-mat.mes-hall↗

arXiv2018

Magnetoanisotropic spin-triplet Andreev reflection in ferromagnet-Ising superconductor junctions

We theoretically study the electronic transport through a ferromagnet-Ising superconductor junction. A tight-binding Hamiltonian describing the Ising superconductor is presented. Then by combing the non-equilibrium Green's function method, the expressions of Andreev reflection coefficient and conductance are obtained. A strong magnetoanisotropic spin-triplet Andreev reflection is shown, and the magnetoanisotropic period is $\pi$ instead of $2\pi$ as in the conventional magnetoanisotropic system. We demonstrate a significant increase of the spin-triplet Andreev reflection for the single-band Ising superconductor. Furthermore, the dependence of the Andreev reflection on the incident energy and incident angle are also investigated. A complete Andreev reflection can occur when the incident energy is equal to the superconductor gap, regardless of the Fermi energy (spin polarization) of the ferromagnet. For the suitable oblique incidence, the spin-triplet Andreev reflection can be strongly enhanced. In addition, the conductance spectroscopies of both zero bias and finite bias are studied, and the influence of gate voltage, exchange energy, and spin-orbit coupling on the conductance spectroscopy are discussed in detail. The conductance reveals a strong magnetoanisotropy with period $\pi$ as the Andreev reflection coefficient. When the magnetization direction is parallel to the junction plane, a large conductance peak always emerges at the superconductor gap. This work offers a comprehensive and systematic study of the spin-triplet Andreev reflection, and has underlying application of $\pi$-periodic spin valve in spintronics.

cond-mat.supr-con↗

arXiv2017

Ginzburg-Landau-type theory of non-polarized spin superconductivity

Since the concept of spin superconductor was proposed, all the related studies concentrate on spin-polarized case. Here, we generalize the study to spin-non-polarized case. The free energy of non-polarized spin superconductor is obtained, and the Ginzburg-Landau-type equations are derived by using the variational method. These Ginzburg-Landau-type equations can be reduced to the spin-polarized case when the spin direction is fixed. Moreover, the expressions of super linear and angular spin currents inside the superconductor are derived. We demonstrate that the electric field induced by super spin current is equal to the one induced by equivalent charge obtained from the second Ginzburg-Landau-type equation, which shows self-consistency of our theory. By applying these Ginzburg-Landau-type equations, the effect of electric field on the superconductor is also studied. These results will help us get a better understanding of the spin superconductor and the related topics such as Bose-Einstein condensate of magnons and spin superfluidity.

cond-mat.supr-con↗